A statistical evaluation of the geogenic controls on indoor radon concentrations and radon risk

ANOVA is used to show that approximately 25% of the total variation of indoor radon concentrations in England and Wales can be explained by the mapped bedrock and superficial geology. The proportion of the total variation explained by geology is higher (up to 37%) in areas where there is strong contrast between the radon potential of sedimentary geological units and lower (14%) where the influence of confounding geological controls, such as uranium mineralisation, cut across mapped geological boundaries. When indoor radon measurements are grouped by geology and 1-km squares of the national grid, the cumulative percentage of the variation between and within mapped geological units is shown to be 34-40%. The proportion of the variation that can be attributed to mapped geological units increases with the level of detail of the digital geological data. This study confirms the importance of radon maps that show the variation of indoor radon concentrations both between and within mapped geological boundaries.     

Regional geology and radon variability in buildings

Radon concentrations in dwellings vary by more than two orders of magnitude. Predicting where and when concentrations are likely to be high requires studying the variability of the contributors to radon in buildings. Among common sources, geological factors (water supply and substrate) are the most variable, whereas building materials are much less variable. Ventillation variation among houses is generally responsible for radon variations comparable to those introduced by building materials, but it is more significant at lower ventilation rates. In some regions with relatively high proportions of houses with elevated radon concentrations, mappable geological factors are associated with most cases of high radon concentrations. However, a priori identification of rock types likely to be implicated is likely to be successful in only a few cases.     

Atmospheric radon in Hong Kong

For the first time in Hong Kong, atmospheric radon concentration was continuously monitored between November 2007 and October 2008. This paper presents the results obtained during the 12-month period. The annual mean atmospheric radon concentration in Hong Kong was found to be 9.3 Bq m⁻³ which was close to the level at neighbouring places like Guangdong and Taiwan. An estimation of the dose arising from atmospheric radon to the Hong Kong population was made. The meteorological effects on the variation of atmospheric radon concentration were discussed. It was found that the origin of the airmass and stability of the local atmosphere played vital roles in the seasonal and diurnal variations respectively, whereas precipitation caused abrupt changes in rainy days. An attempt was also made to find out the contribution of atmospheric radon to the ambient gamma dose rate.     

Mapping of the geogenic radon potential in France to improve radon risk management: methodology and first application to region Bourgogne

In order to improve regulatory tools for radon risk management in France, a harmonised methodology to derive a single map of the geogenic radon potential has been developed. This approach consists of determining the capacity of the geological units to produce radon and to facilitate its transfer to the atmosphere, based on the interpretation of existing geological data. This approach is firstly based on a classification of the geological units according to their uranium (U) content, to create a radon source potential map. This initial map is then improved by taking into account the main additional parameters, such as fault lines, which control the preferential pathways of radon through the ground and which can increase the radon levels in soils. The implementation of this methodology to the whole French territory is currently in progress. We present here the results obtained in one region (Bourgogne, Massif Central) which displays significant variations of the geogenic radon potential. The map obtained leads to a more precise zoning than the scale of the existing map of radon priority areas currently based solely on administrative boundaries.     

Geophysical methods in radon risk studies

The results of the studies presented in the paper have shown that in the Upper Silesian Region in Poland, radon indoor concentration levels depend first of all on the geological structure of the subsurface layers. The essential factors influencing radon migration ability are the mining-induced transformations of a rock mass. In some cases, significant variations of radon potential have been found at sites featuring similar geological structures and experiencing comparable mining effects. To find out the causes of these variations, studies involving geophysical methods such as electrical resistivity profiling (PE) and electrical resisitivity sounding (VES) were used. These studies have shown that the measurements made using the electrical resistivity method can be helpful in evaluating radon potential of both the tectonically disturbed areas and the mining-transformed ones.     

Search for radon sources in buildings--kindergartens

In ten high radon level kindergartens, radon sources were sought by applying a combination of several radon measuring techniques: etched track detectors to obtain average indoor air radon concentration, continuous devices to record radon concentration and see its diurnal variation, and alpha scintillation cells to determine radon concentration in the air entering a room from cracks, holes and sinks in the floor and from under-floor channels. In three cases, a strong local radon source was identified while, in the others, the bad quality of the basic concrete slab was responsible for the high indoor radon concentration.     

Groundwater radon measurements in the Mt. Etna area

Radon levels were measured in 119 groundwater samples collected throughout the active volcanic area of Mt. Etna by means of a portable Lucas-type scintillation chamber. The measured activity values range from 1.8 to 52.7 Bq l(-1). About 40% of the samples exceed the maximum contaminant level of 11 Bq l(-1) proposed by the USEPA in 1991. The highest radon levels are measured in the eastern sector of the volcano, which is the seismically most active zone of the volcano. On the contrary the south-western sector, which is both seismically active and a site of intense magmatic degassing, display lower radon levels. This is probably due to the formation of a free gas phase (oversaturation of CO(2)) that strips the radon from the water. Comparison of the data gathered at Mt. Etna with those of other areas indicates that (222)Rn activity in groundwater is positively correlated with both the content of parent elements in the aquifer rocks and the temperature of the geothermal systems that interacts with the sampled aquifers.     

Exposure to radon in the Gadime Cave, Kosovo

Air radon concentration was measured in summer and winter at 11 points along the tourist guided route in the Gadime Cave in Kosovo using alpha scintillation cells and etched track detectors. At two points in summer, values higher than 1700Bqm(-3) were observed; they otherwise were in the range 400-1000Bqm(-3). Values were lower in winter. The effective dose received by a person during a 90min visit is 3.7muSv in summer and 2.5muSv in winter. For a tourist guide the annual effective dose is less than 3.5mSv.     

A critical evaluation of the cost-effectiveness of radon protection methods in new homes in a radon Affected Area of England

In the UK, building new homes in areas prone to radon gas is currently subject to regulations that require installation of radon-proof membranes. These membranes are not, however, the only way to protect residents of new homes against radon's potential to cause lung cancer. Alternative regulatory regimes can be constructed that would achieve the same end.The purpose of this paper is to examine the cost-effectiveness of four alternative regimes and so determine if building regulations for new homes could be altered to protect residents from the effects of radon more cost-effectively than at present. In addressing this question, the paper also contributes to the wider debate on how best to reduce the effect on public health of exposure to radon.The measure of cost-effectiveness used, cost per quality-adjusted life-year gained, is determined from radon test results obtained in properties in Brixworth, England, UK, a radon Affected Area. Confidence intervals for the cost-effectiveness estimates are also derived using bootstrap techniques.The central estimates of cost-effectiveness range from £2870 per quality-adjusted life-year gained for the most cost-effective of the alternative regimes to £6182 for the current regime. These results suggest that alternative regimes may be more cost-effective in tackling the radon problem. A definitive assessment of the most suitable to adopt will require extensive negotiation between government departments, the construction industry, and other interested parties to ensure acceptance of any new regime. The paper offers suggestions for future research that should help in the process of identifying the key features of a new regulatory approach.     

Indoor radon levels in Greek schools

Radon and gamma dose rate measurements were performed in 512 schools in 8 of the 13 regions of Greece. The distribution of radon concentration was well described by a lognormal distribution. Most (86%) of the radon concentrations were between 60 and 250 Bq m⁻³ with a most probable value of 135 Bq m⁻³. The arithmetic and geometric means of the radon concentration are 149 Bq m⁻³ and 126 Bq m⁻³ respectively. The maximum measured radon gas concentration was 958 Bq m⁻³. As expected, no correlation between radon gas concentration and indoor gamma dose rate was observed. However, if only mean values for each region are considered, a linear correlation between radon gas concentration and gamma dose rate is apparent. Despite the fact that the results of radon concentration in schools cannot be applied directly for the estimation of radon concentration in homes, the results of the present survey indicate that it is desirable to perform an extended survey of indoor radon in homes for at least one region in Northern Greece.     

Air filtration and radon daughter levels

The authors investigate the effect of filtration and aerosol loading of the air on the level of short-lived air-borne daughter products of radon. By the use of a combination of filtration and aerosol loading, it is possible to shift the partitioning of the radon daughters in the room between the states: airborne, plated-out on the walls, and trapped by filters; the airborne fraction will shift between being attached to aerosol particles and existing as molecular-sized clusters. When the air filtered the equilibrium factor decreases with increasing filtration rate. At high aerosol concentrations the decrease can be explained solely as an effect of the filter removing the daughter products from the air passing through it. As the aerosol production and concentration is lowered, the decrease in equilibrium factor becomes larger. This is caused by an increase in the unattached fraction of the airborne activity and hence in the wall-deposited fraction of the total activity. At a given radon concentration, the dose delivered to a certain portion of the respiratory tract depends not only upon the equilibrium factor but also upon the fraction of, especially, ₈₄²¹⁸Po in the unattached state. It is further demonstrated that, according to the dose model of Harley and Pasternak, the dose to the basal cells of the epithelium of the bronchii will in general decrease with increasing filtration rate and increase with decreasing aerosol concentration.     

Dose estimation and radon action level problems due to nanosize radon progeny aerosols in underground manganese ore mine

One of the essential parameters influencing of the dose conversion factor is the ratio of unattached short-lived radon progeny. This may differ from the value identified for indoor conditions when considering special workplaces such as mines. Inevitably, application of the dose conversion factors used in surface workplaces considerably reduces the reliability of dose estimation in the case of mines.This paper surveyed the concentration of radon and its short-lived radon progeny and identified the unattached fraction of short-lived radon progeny. As well equilibrium factor during the month of August was calculated simultaneously at two extraction faces in a manganese ore mine.During working hours the average radon concentrations were 220 Bq m⁻³ and 530 Bq m⁻³ at Faces 1 and 2; the average short-lived progeny concentration was 90 Bq m⁻³ and 190 Bq m⁻³, the average equilibrium factors were 0.46 and 0.36, and the average unattached fractions were 0.21 and 0.17, respectively. The calculated dose conversion factor was between 9 and 27 mSv WLM⁻¹, but higher values could also be possible.     

Investigations on indoor radon in Austria, Part 1: Seasonality of indoor radon concentration

In general, indoor radon concentration is subject to seasonal variability. The reasons are to be found (1) in meteorological influence on the transport properties of soil, e.g. through temperature, frozen soil layers and soil water saturation; and (2) in living habits, e.g. the tendency to open windows in summer and keep them closed in winter, which in general leads to higher accumulation of geogenic Rn in closed rooms in winter. If one wants to standardize indoor Rn measurements originally performed at different times of the year, e.g. in order to make them comparable, some correction transform as a function of measurement time which accounts for these effects must be estimated. In this paper, the seasonality of indoor Rn concentration measured in Austria is investigated as a function of other factors that influence indoor Rn. Indoor radon concentration is clearly shown to have seasonal variability, with higher Rn levels in winter. However, it is complicated to quantify the effect because, as a consequence of the history of an Rn survey, the measurement season maybe correlated to geological regions, which may introduce a bias in the estimate of the seasonality amplitude.     

Determination of uranium and radon in potable water samples

In this work, potable water samples collected from boreholes of the Migdonia valley, located NE of the city of Thessaloniki, were analyzed for the determination of uranium (238U) and radon (222Rn) concentrations. The objective of the present work is to examine if there is any correlation between radon and uranium concentrations in the water samples. For the determination of traces of uranium in water samples, an analytical technique was developed based on the selective adsorption of uranium on the chelating resin, SRAFION NMRR, and the in situ determination of the retained uranium by instrumental neutron activation analysis (INAA). By the described procedure, it was possible to determine uranium amounts in the range of microg/l. For measuring radon in water, a liquid scintillation counting system, using the Packard protocol was employed. The measured 222Rn activity concentrations are from background level up to 160 Bq l (-1).     

Evaluation of indoor radon measurements in Hungary

The RAD Laboratory measured annual means of radon activity concentrations in 15 277 first-floor rooms of dwellings and in 325 rooms on upper floors in Hungary (1994-2004). The original purpose of the survey was to find radon-prone area in Hungary. The maximum measured value was 5800 Bq m(-3), while the minimum was 10 Bq m(-3). Due to geological diversity and different structures of buildings, the data set of first-floor rooms did not follow the lognormal distribution. Therefore, strata were chosen so that the measured data fitted the lognormal distribution. The numbers of dwellings above a given radon level were determined in each stratum. The national distribution was then taken as the sum of the individual distributions of all strata. This distribution was not lognormal. The parameters of the best fitting lognormal distribution were GM = 58 Bq m(-3), GSD = 2.2. The weighted averages of strata values GM = 62 Bq m(-3), GSD=2.1 were obtained corresponding to 92% of Hungarian dwellings.     

The cost effectiveness of radon reduction programmes in domestic housing in England and Wales: The impact of improved radon mapping and housing trends

In the UK, excessive levels of radon gas have been detected in domestic housing. Areas where 1% of existing homes were found to be over the Action Level of 200 Bq · m^− 3 were declared to be Radon Affected Areas. Building Regulations have been introduced which require that, for areas where between 3% and 10% of existing houses are above the Action Level, new homes should be built with basic radon protection using a membrane, and that, where 10% or more of existing homes exceed this level, new homes should be built with full radon protection.Initially these affected areas followed administrative boundaries, known as Counties. However, with increasing numbers of measurements of radon levels in domestic homes recorded in the national database, these areas have been successively refined into smaller units – 5 km grid squares in 1999, down to 1 km grid squares in 2007.One result is the identification of small areas with raised radon levels within regions where previously no problem had been identified. In addition, some parts of areas that were previously considered radon affected are now considered low, or no, risk. Our analysis suggests that the net result of improved mapping is to increase the number of affected houses. Further, the process is more complex for local builders, and inspectors, who need to work out whether radon protection in new homes is appropriate.Our group has assessed the cost-effectiveness of radon remediation programmes, and has applied this analysis to consider the cost-effectiveness of providing radon protection in both new and existing homes. This includes modelling the potential failure rate of membranes, and whether testing radon levels in new homes is appropriate. The analysis concludes that it is more cost effective to provide targeted radon protection in high radon areas, although this introduces more complexity.The paper also considers the trend in housing to a greater proportion of apartments, the regional variations in types of housing and the decreasing average number of occupants in each dwelling, and concludes that data and methods are now available to respond to the health risks of radon at a local level, in keeping with a general initiative to prioritise responses to health and social welfare issues at a more local level.     

九龙江流域河水溶解态碳的时空变化

为了研究九龙江流域河流中溶解碳变化规律,分别于2017年7月与2018年1月对九龙江河水溶解无机碳（DIC）与溶解有机碳（DOC）进行了分析。丰水季河水DIC浓度为7.50~49.04 mg/L,平均值为22.12 mg/L,枯水季DIC浓度为8.84~84.91 mg/L,平均浓度41.17 mg/L,丰水季河水中的DOC浓度为0.54~2.89 mg/L,平均值为1.04 mg/L,枯水季河水中DOC浓度变化在1.34~3.56 mg/L之间,平均值为2.34 mg/L,据此计算了九龙江河水DOC、DIC的入海通量。研究结果表明九龙江河水中溶解碳具有显著的时空变化特征,通过与中国其他河流溶解碳数据对比,解释了碳酸盐岩的风化、气候变化、河流中浮游植物以及人类活动对九龙江河流溶解碳浓度的影响。     

99Tc in seawater in the West Spitsbergen Current and adjacent areas

99Tc levels were measured in seawater samples collected between 2000 and 2002 in the West Spitsbergen Current (WSC) and along the western coast of Svalbard or Spitzbergen and compared with available oceanographic 3-D modelling results for the late 1990s. Additional data from related regions are also presented in order to support the data interpretation. The seawater in the Arctic fjord Kongsfjorden on the western coast of Svalbard is influenced by the WSC, as shown by the 99Tc levels in surface water. By means of the WSC, 99Tc reaches the Eastern Fram Strait, where one branch of the WSC turns west into the East Greenland Current (EGC), and another branch continues northwards into the Arctic Ocean. Surface seawater collected in the central part of the WSC during a cruise on board the R/V "Polarstern" in the summer of 2000, showed higher levels of (99)Tc than samples measured in Kongsfjorden in the spring of 2000. However, all levels measured in surface water are of the same order of magnitude. Data from sampling of deeper water in the WSC and EGC provide information pertaining to the lateral distribution of 99Tc. In all vertical profiling surveys (conducted in spring and summer), the highest levels of 99Tc were found in surface water. Comparison with oceanographic 3-D modelling indicates both significant seasonal variations in the lateral stratification of the WSC and variations with depth over shorter vertical distances. This information can be applied in sampling strategies, environmental monitoring, long-range transport of pollutants and physical oceanography.     

Measurements of indoor radon concentrations in the Santiago de Compostela area

Galician soils are among those with the highest (222)Rn exhalation rates in Spain. A year-round study of the indoor (222)Rn concentration in buildings in the Santiago de Compostela area (Galicia, Northwest of Spain) was performed. The study is based on systematic samplings with active charcoal canisters, following a modified EPA 520/5-87-005 protocol. These measurements were complemented by others obtained using etched track dosimeters. Each data set follows a log-normal distribution, with a geometric mean of (253+/-3)Bqm(-3) for charcoal canisters and (285+/-2.5)Bqm(-3) for etched track detectors. After correcting for the different measuring conditions, the mean value of both methods differed by only 2%. A careful analysis of the seasonal dependence of our measurements did not reveal any significant seasonal variations in the (222)Rn concentration. Parallel to these measurements, different meteorological parameters were recorded, which revealed a direct correlation between the indoor radon concentration and the outdoor temperature derivative with respect to time.     

Resolving the radon problem in Clinton, New Jersey, houses

Significantly elevated radon concentrations were found in several adjacent houses in Clinton, New Jersey. The United States Environmental Protection Agency screened 56 of the houses and selected 10 for demonstration of radon-reduction techniques. Each of the 10 houses received an intensive radon diagnostic evaluation before a house-specific radon reduction plan was developed. Depressurization effects caused by temperature differentials and the operation of mechanical equipment were quantified. Before and after radon reduction plans were implemented, radon concentrations were determined by charcoal canisters and continuous radon monitors. A variety of sealing and subslab depressurization techniques were applied to the 10 houses. Radon concentrations were reduced by over 95% in all 10 houses. The cost of applying radon reduction techniques ranged from $1500 to $8500 per house. House construction characteristics were described which contributed to the high cost of radon reduction. In summary, the 10-house radon reduction demonstration in Clinton, New Jersey was successful in showing homeowners with similar house types some effective ways of reducing radon concentrations.