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Comprehensive surveys conducted at 5-yr intervals were used to estimate sulfur dioxide (SO,) and nitrogen oxides (NO.) emissions from U.S. pulp and paper mills for 1980, 1985, 1990, 1995, 2000, and 2005. Over the 25-yr period, paper production increased by 50%, whereas total SO, emissions declined by 60% to 340,000 short tons (t) and total NO, emissions decreased approximately 15% to 230,000 t. The downward emission trends resulted from a combination of factors, including reductions in oil and coal use, steadily declining fuel sulfur content, lower pulp and paper production in recent years, increased use of flue gas desulfurization systems on boilers, growing use of combustion modifications and add-on control systems to reduce boiler and gas turbine NO, emissions, and improvements in kraft recovery furnace operations.  相似文献   

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Since 1972, at the University of Hohenheim in Stuttgart, Germany, airborne particulate matter (PM12 and then PM10) was continuously collected on filters and analyzed for environmentally relevant elements by X-ray fluorescence analysis. The resulting long-term time series are suitable for the investigation of trends and of seasonal variation. For the period 1972-2005, monthly and annual concentration mean values of 13 elements (Br, Ca, Cr, Cu, Fe, K, Mn, Ni, Pb, S, Ti, V, and Zn) in the air are presented. Trend curves were fitted and the mean yearly variation of the concentration for these elements was calculated and represented graphically. All trend curves show a diminution of the air pollution during this period, but to different extents. Mean trends in percent per year were calculated for each element both for the entire investigation period and for three data subsets of 10-11 years. Possible explanations are discussed in detail.  相似文献   

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Trends in vehicular emissions in China's mega cities from 1995 to 2005   总被引:1,自引:0,他引:1  
Multiyear inventories of vehicular emissions in Beijing, Shanghai and Guangzhou from 1995 through 2005 have been developed in this paper to study the vehicle emissions trends in China's mega cities during the past decade. The results show that the vehicular emissions of CO, HC, NOx and PM10 have begun to slow their growth rates and perhaps even to decline in recent years due to the implementation of measures to control vehicular emissions in these cities. However, vehicular CO2 emissions have substantially increased and still continue to grow due to little fuel economy improvement. Passenger cars and large vehicles (including heavy duty trucks and buses) are the major sources of vehicular CO2 and CO emissions while large vehicles were responsible for nearly 70% and 80% of the vehicular NOx and PM10 emissions in these mega cities. Motorcycles are also important contributors to vehicular emissions in Guangzhou and Shanghai.  相似文献   

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Multi-year inventories of vehicular emissions at a high spatial resolution of 40 km×40 km were established in China using the GIS methodology for the period 1980–2005, based on provincial statistical data from yearbooks regarding vehicles and roads, and on the emission factors for each vehicle category in each province calculated by COPERT III program. Results showed that the emissions of CH4, CO, CO2, NMVOC, NOx, PM10, and SO2 increased from 5, 1066, 19 893, 169, 174, 26, and 16 thousand tons in 1980 to 377, 36 197, 674 629, 5911, 4539, 983, and 484 thousand tons in 2005 at an annual average rate of 19%, 15%, 15%, 15%, 14%, 16%, and 15%, respectively. Statistical analysis of vehicular emissions and GDP showed that they were well positively correlated, which revealed that increase of pollutant emissions has been accompanying the growth of GDP. Spatial distribution of pollutant emissions was rather unbalanced: over three-quarters of the total emissions concentrated in developed regions of China's southeastern, northern and central areas covering only 35.2% of China's territory, while the remaining emissions were distributed over the southwestern, northwestern and northeastern regions covering as much as 64.8% of the territory. In 2005, the Beijing–Tianjin–Hebei region, the Yangtze River Delta, and the Pearl River Delta covering only 2.3%, 2.2%, and 1.9%, respectively, of the territory, generated about 10%, 19%, and 12%, respectively, of the total emissions. Since 1990, motorcycles have been the major contributors to the CH4, CO, NMVOC, and PM10 emissions, due to the large population. Heavy-duty vans were the major contributors to the NOx and SO2 emissions because of high emission factors. Passenger cars contributed about one third of the emissions of each pollutant. Contributions of vehicle categories to emissions varied from province to province, due to the diversity of vehicle compositions among provinces.  相似文献   

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