田湾核电站周边土壤及植物中137Cs含量调查及人群内辐射风险评价

为了调查田湾核电站运行后土壤环境中核素137Cs放射性水平的变化及评估其对当地居民的健康风险,采用现场采样测定的方法,分析了田湾核电站装料2年后周边土壤及植物中137Cs的放射性水平,并与运行前的本底调查结果进行了比较,同时利用放射性核素对人群内辐射风险评价模型结合田湾地区居民饮食情况对人群辐射风险进行了评估.结果表明,核电站运行2年后周边土壤中137Cs的放射性水平与运行前相比总体上没有明显变化,但个别村镇点位的137Cs放射性水平升高;核电站周边植物中137Cs的放射性水平均远低于我国相关国家标准(GB14882-1994)和运行前的本底值;田湾地区高公岛居民核素137Cs的年总摄入量为18.62Bq·a-1,远低于我国国标成人限值(GB14882-1994).通过摄入137Cs引起的人群内辐射总致癌风险较低,为1.51×10-7a-1,其中超过50%的风险来源于摄入鱼类海产品.     

农业生态系统中同位素示踪技术及发展趋势

在土壤侵蚀研究中，^137Cs、^210Pb和^7Be示踪技术已得到广泛应用，^210Pb主要用在沉积速率的测定及沉积年代的示踪研究上，^137Cs特别适用于大面积的水土流失普查和土壤侵蚀普查，^7Be用于短期内土壤侵蚀研究。在土壤肥效和植物营养元素研究中，常用^13C、^32P和^15N及其化合物示踪定量评价土壤养分，追踪植物对养分的吸收、运转、分配和代谢过程。在环境污染方面，用重金属如Pb、Hg、Cd、Zn等元素的同位素判别污染物质来源，研究污染历史和污染元素在土-水-气-植物中的迁移转化以及在动物有机体内的迁移累积。文章综述了同位素示踪技术在上述方面的应用现状和发展趋势。     

核素示踪法研究农耕地土壤侵蚀的定量模型及其评价

应用137Cs示踪技术估算农耕地土壤侵蚀量的定量模型主要有两类径流小区上建立的经验关系式及各种理论模型.文章主要对各种主要模型作了简要介绍,并对各种模型的优点、局限性进行了比较和评价;指出今后在模型的建立和应用中注意的问题.     

利用~(137)Cs示踪技术与土壤化学物质研究滇池流域土壤侵蚀

核素示踪技术研究作为一种新的土壤侵蚀研究方法,已经在土壤侵蚀研究中获得了极大应用,并在土壤侵蚀的沉积、侵蚀、运移研究上取得许多成果.采用放射性核素作为土壤示踪剂,可以很好的进行流域尺度的范围研究,且可靠性比较高,省时省力.云贵高原在处于我国的西南地区,是我国南方水土流失严重的地区之一.该地区缺乏较长时间的资料积累,仅通过短时间的测定,无法准确估算中长期(约50 a)的平均土壤侵蚀速率.文章应用137Cs示踪技术,并结合土壤有机碳、全氮等土壤化学物质,首次研究了云南省滇池流域土壤侵蚀的强度分异规律.1)山坡不同部位的土壤侵蚀速率大小顺序是:坡中部>坡下部>坡上部,坡位是影响土壤侵蚀的重要因素.2)土壤利用方式上看,非耕地(林地和撂荒地)的侵蚀速率小于耕地的侵蚀速率.同一种土地利用方式下,由于耕作措施与耕作方法的差异,也会直接影响到土壤侵蚀的速率大小.3)从土壤侵蚀模数来看,区域整体上属于轻度侵蚀.土壤平均侵蚀速率为1280.2 t·km-2·a-1,其中耕地的平均土壤侵蚀速率为1672.8 t·km-2·a-1,非耕地土壤平均侵蚀模数为1161.2 t·km-2·a-1.4)虽然是轻度侵蚀,但是随着土壤侵蚀的进行,土壤有机碳、氮等的流失,造成土地退化较为严重,这给当地的生态环境带来直接的危害:滇池土壤淤积,土壤中的有机质、化肥等物质也直接随土壤流入滇池,会导致水体富营养化和水质变差.     

核素~(137)Cs在北太平洋典型生物体内的分布与富集

为了解日本福岛核泄漏对北太平洋公海渔场海洋生物的危害程度及影响状况,2011—2012年连续两年在北太平公海渔场采集典型生物样品,采用γ谱仪进行检测,发现所采样品均含有放射性核素~(137)Cs。同时运用分类和分组织器官等处理方法,进行对照分析。结果显示,(1)2011年,~(137)Cs在鲨鱼(Mustelus griseus)体内的分布最高,高达1.16Bq·kg~(-1),最低是日本海的太平洋褶柔鱼(Todarodes pacificus),仅为0.05 Bq·kg~(-1)。2012年整体上所有海洋生物体内的~(137)Cs质量活度降低了1个数量级,~(137)Cs最高质量活度出现在蜞鳅(Coryphaena hippurus)体内,达0.04 Bq·kg~(-1),最低也是日本海的太平洋褶柔鱼,仅为0.001 Bq·kg~(-1)。(2)2011年中不同胴长组巴特柔鱼(Ommastrephes bartramii)的~(137)Cs质量活度最高的是250~300mm,达到了0.73 Bq·kg~(-1)。2012年中~(137)Cs质量活度最高的胴长组是200~250 mm,达0.034 Bq·kg~(-1)。(3)从两年巴特柔鱼的不同组织部位的质量活度分布情况来看,内脏聚集的核素~(137)Cs质量活度最高,其他3个部位(头部、躯干和鳍部)明显偏低。(4)通过两年的营养级分析,~(137)Cs核素质量活度初步呈倒金字塔分布。所测得的生物体中的核素质量活度水平均未超过中国食品放射性核素质量活度的限制水平与通用水平。初步了解了核泄漏对北太平洋公海主要渔场核辐射的影响,以期为海洋放射性深入研究提供基础资料。     

137 Cs在我国滨海核电周边海洋生物的富集及生态风险研究

铯-137(~(137)Cs)是滨海核电站液态流出物中主要人工放射性核素和重要监控指标之一,易被水生生物累积,有关核电周边海域内海洋生物的核素富集状况备受关注。通过分析海洋生物富集放射性~(137)Cs的方式、生物富集系数的种群特征、人工放射性核素在生物体内的辐射剂量率状况,结果显示:1)滨海核电周边海域内~(137)Cs的放射性水平较低; 2)海洋生物对于~(137)Cs的富集未呈现显著的种群规律; 3)目前对放射性铯的富集能力较高的生物主要是底栖生物; 4)核电厂周边海域内海洋生物通常未达到可导致电离辐射损伤的辐射剂量率水平。随着滨海核电在我国的大力发展,对能够快速反映环境放射性状况的指示生物的筛选、生物放射性质量安全及其生态健康风险需进一步关注。     

川中丘陵区紫色土坡耕地土壤侵蚀特征

利用137Cs示踪方法与耕作侵蚀模型评价了川中丘陵区紫色土坡耕地土壤侵蚀速率,并通过比较分析方法探讨了2种典型坡耕地-短陡坡与缓长坡耕地-土壤侵蚀特征差异。结果表明,短陡坡耕地土壤侵蚀速率高达52.6 t.hm-2.a-1,是缓长坡耕地土壤侵蚀速率（26.7 t.hm-2.a-1）的2倍。耕作侵蚀是短陡坡耕地的主要侵蚀过程,它整体性搬运土壤,其对土壤总侵蚀的贡献高达74%。水蚀是缓长坡耕地的主要侵蚀过程,其分选性搬运土壤,对土壤总侵蚀的贡献为55%。短陡坡耕地与缓长坡耕地土壤侵蚀速率均沿着向下坡方向逐渐降低,但短陡坡耕地土壤侵蚀速率下降梯度明显高于缓长坡耕地。耕作侵蚀导致两种坡耕地的坡顶土壤损失最为严重。因此,川中丘陵区的耕作侵蚀风险应该引起重视。     

黄土高原植被破坏与重建过程中土壤侵蚀强度变化

运用137Cs示踪方法,通过采集不同利用方式的坡面土壤,研究了黄土高原典型丘陵区流域植被破坏与重建过程中土壤侵蚀强度的变化情况.研究结果表明:植被破坏耕垦后使137Cs遭受了大量流失,坡耕地耕垦时间越长,土壤侵蚀愈严重;植被恢复重建有效地减轻了侵蚀强度;通过比较刺槐林、果园及封禁自然恢复的撂荒地三种植被建造方式的土壤侵蚀模数,发现以封禁自然恢复的撂荒地土壤保持效果最好,其次是刺槐林,最差的是果园,其原因与果园的管理方式有关.立地条件不同的同种植被建造方式.土壤侵蚀强度差异较大,表现为峁坡阳坡此槐林地侵蚀模数远远大于谷坡阴坡刺槐林地.根据退耕时间不同的坡地土壤侵蚀强度的变化及流域土地利用类型的变化等方面对燕沟流域土壤侵蚀变化趋势作了进一步预测.     

南渡江流域降雨侵蚀力时空分布与变化趋势研究

降雨侵蚀力是表征降雨侵蚀强度的重要指标,对研究区域水土流失潜在风险以及土壤侵蚀模型预测具有重要意义。为分析南渡江流域降雨侵蚀力时空变化趋势,基于日降雨侵蚀力模型,利用流域及其周边13个气象站1971—2020年逐日降雨数据,采用Mann-Kendall非参数趋势/突变检验、小波分析和反距离加权插值等方法在不同时空尺度上对降雨侵蚀力进行研究,从而确定降雨侵蚀力的时间和空间变化趋势。结果表明,南渡江流域1971—2020年年均降雨侵蚀力范围为11 841.33～23 692.14 MJ·mm·hm^-2·h^-1,均值为16 497.67 MJ·mm·hm^-2·h^-1,年际变化整体呈现波动上升趋势,年降雨侵蚀力存在周期性变化,未发生显著性突变;降雨侵蚀力年内分布集中在7—9月,因此需加强期间水土流失防治工作。季节的年际变化除春季降雨侵蚀力呈现下降趋势外,夏季、秋季和冬季均呈上升趋势;降雨侵蚀力空间分布呈现从南向北逐渐降低的趋势,各气象站变异系数范围为0.24～0.43,由北向南逐步递减,具有较高的区域变异性...     

遥感水文耦合模型的研究进展

遥感水文的耦合模型在目前生态环境领域,特别是在水资源的应用和管理中其作用日益重要,具有大流域尺度上快速应用、实时动态监测等优点。结合国内外近年来取得的研究成果,文章综述了遥感水文耦合模型的研究进展。首先介绍了遥感技术在水文学中的应用,讨论了它的分类发展概况,接着介绍了几种主要的遥感水文耦合模型及其应用实例,包括SCS(SoilConservationServices)模型、SiB2(SimpleBiosphereModelversion2)简化生物圈模型、SRM(SnowmeltRunoffModel)融雪径流模型以及SWAT(SoilandWaterAssessmentTool)模型,最后展望了遥感水文耦合模型未来的发展趋势,指出尺度问题上的时空变异性仍是其发展的关键,与GIS(Geographicinformationsystem)及其他空间技术的相结合是其未来发展的重要方向,从而为水文学、水资源的预测评价等研究提供参考。     

水土流失的定量遥感及其应用研究进展

简要介绍了水土流失定量遥感的概念，阐述了它的四项基本要求，报道了它的应用研究进展，并为尽快实现中国水土流失定量遥感提出了若干建议。     

雅鲁藏布江源区土壤侵蚀特征

以雅鲁藏布江源区所在的马泉河流域为研究区域,运用遥感和G IS技术对土壤侵蚀及其空间分布的地貌特征进行研究,结果表明:轻度及其以上强度土壤侵蚀面积为18 933.33 km2,占源区面积的71.86%;冻融侵蚀是土壤侵蚀的主要形式,占源区面积的82.53%;风力侵蚀占5.33%,集中分布在河谷宽谷段;水力侵蚀面积所占比例较小,以微度侵蚀为主。土壤侵蚀的地理分布规律受海拔高度的影响较大,垂直分异明显,主要发生在坡度等级较低、地势较平坦的地区。轻度以上冻融侵蚀主要分布在海拔4 600~5 200 m,且有20%以上集中在0°~5°坡地;风力侵蚀主要分布在海拔4 600~5 600 m、0°~25°坡地。极强烈风力侵蚀以西南坡向最大,南、西、东南坡和平地分布较少。强烈风力侵蚀以平地所占比例最大,东北和西2个坡向次之。坡向对冻融侵蚀影响较小。     

Retention of 137cesium in acid sulphate soils of South Central Thailand

Adsorption and desorption of ¹³⁷Cs by acid sulphate soils from the Nakhon Nayok province, South Central Plain of Thailand located near the Ongkarak Nuclear Research Center (ONRC) were investigated using a batch equilibration technique. The influence of added limestone (12 and 18 tons ha^?1) on ¹³⁷Cs adsorption–desorption was studied. Based on Freundlich isotherms, both adsorption and desorption of ¹³⁷Cs were nonlinear. A large portion (98.26–99.97%) of added ¹³⁷Cs (3.7?×?10³?7.03?×?10⁵ Bq l^?1) was sorbed by the soils with or without added lime. The higher lime treatments, however, favoured stronger adsorption of ¹³⁷Cs as compared with soil with no lime, which was supported by higher K _ads values. The addition of lime, the cation exchange capacity and pH of the soil increased and hence favoured the stronger adsorption of ¹³⁷Cs. Acid sulphate soils with a high clay content, medium to high organic matter, high CEC, and predominant clay types consisting of a mixture of illite, kaolinite, and montmorillonite were the main soil factors contributing to the high ¹³⁷Cs adsorption capacity. Competing cations such as NH₄ ⁺, K⁺, Na⁺, Ca²⁺, and Mg²⁺ had little influence on ¹³⁷Cs adsorption as compared with liming, where a significant positive correlation between K _ads and soil pH was observed. The ¹³⁷Cs adsorption–desorption characteristics of the acid sulphate soils studied exhibited a very strong irreversible sorption pattern. Only a small portion (0.09–0.58%) of ¹³⁷Cs adsorbed at the highest added initial ¹³⁷Cs concentration was desorbed by four successive soil extractions. Results clearly demonstrated that Nakhon Nayok province acid sulphate soils have a high ¹³⁷Cs adsorption capacity, which limits the ¹³⁷Cs bioavailability.     

Soil erosion hazard evaluation—An integrated use of remote sensing,GIS and statistical approaches with biophysical parameters towards management strategies

Soil erosion hazard maps can be an essential tool in erosion prone areas as they explain and display the distribution of hazards and areas likely to be affected to different magnitudes. Therefore, it is very useful to planners and policy makers initiating remedial measures and for prioritizing areas. In this study, a numerical model was developed for soil erosion hazard assessment, in which Z-score analysis was combined with a geographical information system (GIS) to compute a synthetic soil erosion hazard index (SEHI). For this model, nine factors which have notable impact on soil erosion were selected. To generate the selected factors remote sensing, analytical hierarchy process (AHP) and GIS techniques along with spatial models were applied. To standardize all of the factors and establish the factor weights, the AHP method was adopted. For Z-score analysis with selected standardized factors, the Integrated Land and Water Information System (ILWIS) software was used and nine individual layers with Z-scores were prepared. Afterwards, the layers were integrated with their factor weights by means of a weighted linear combination to derive a SEHI value for each pixel. To classify the discrete SEHI map to represent a meaningful regionalization of soil erosion hazard, the equal distance cluster principle was used and graded into four levels of hazard; very high, high, moderate and low. The results depicted that in general, a moderate hazardous condition of soil erosion was found in the study area and the proposed approach was also able to identify the areas under high and very high hazards that require urgent intervention on a priority basis. Based on this study, comprehensive erosion hazard management strategies were anticipated for the efficient management of present and future erosion disaster in the area.     

红壤丘陵区LAI与土壤侵蚀分布特征的关系

叶面积指数(LAI)是常用的一个用于描述植被覆盖的方面指数,土壤侵蚀的分布又与植被的覆盖状况息息相关,这就意味着LAI与土壤侵蚀有一定的相关性,目前有关这二者的相关性研究还鲜有文献报道。基于这此,本研究首先利用2000年的遥感影像(TM)解释出该年度的土壤侵蚀强度图,再利用该遥感影像通过图像的代数运算得出该地区的NDVI栅格图,通过实测该县不同典型植被条件的LAI值,得出实测的LAI与图像NDVI值之间的函数关系式,由图像的代数运算把NDVI图转换成LAI图,即实现了遥感图像的实测LAI纠正。在GIS软件的帮助下,通过将LAI栅格图与土壤侵蚀强度图的空间叠加分析,得到不同LAI条件下的土壤侵蚀分布。结果表明,LAI与土壤侵蚀的分布表现为:大致以LAI=2为分界线,当LAI<2时,土壤侵蚀并未随LAI的增加而迅速减少,LAI>2时,土壤侵蚀的分布随植被指数的增加而减少,当LAI=2左右时,土壤侵蚀的面积最大。这种情况对于轻度、中度及强度土壤侵蚀的影响是类似的,都呈类正态分布的曲线形式,但在曲线的两侧土壤侵蚀类型是有本质区别的,在曲线的左侧土壤侵蚀类型的分布是中度和强度为主,而在曲线右侧则以轻度为主。表明LAI这个指标与土壤侵蚀有很好的相关性,可以用于土壤侵蚀方面的相关研究工作。     

基于遥感与GIS的土壤侵蚀强度快速估测方法

针对土壤侵蚀问题,提出了一种基于遥感数据、气象数据、土壤数据的区域土壤侵蚀快速估测方法。首先,通过对土壤侵蚀问题形成原因和影响因素的分析,确定土壤侵蚀敏感性因子;其次,利用遥感(RS)、GIS技术提取土壤侵蚀敏感性因子信息;然后,在GIS系统支持下,运用主成分分析方法,进行土壤侵蚀强度分级;以北京密云水库周边区域为例,进行了土壤侵蚀估测方法的应用,并对该区域的土壤侵蚀空间特征进行分析。研究结果表明:(1)区域土壤侵蚀快速估测方法与实际情况有较好的一致性;(2)密云水库周边地区土壤侵蚀以微度和轻度侵蚀为主,所占面积比例为67.51%,中度以上侵蚀仅占面积的1.46%;(3)土壤侵蚀受坡度、地貌影响明显,中度侵蚀主要发生在低山、丘陵区以耕地为主的土地利用上以及坡度在大于25°的阳坡地带。     

Cäsium-137 in Böden saarländischer Waldökosysteme

Scopes and main features

In order to explain the behaviour of the artificial radioisotope¹³⁷Cs towards landscape resources in the Saar-Lor-Lux-Region, the cross-border region between southwestern Germany/ Saarland, France/Lorraine and Luxembourg, regional distribution as well as downward translocation and depth functions of¹³⁷Cs in the main soil substrates of forest ecosystems in the Saarland were investigated.

Results

The study shows that the highest¹³⁷Cs activities are found in the north of the Saarland, whereas the south and south-eastern regions show distinctly lower concentrations of¹³⁷Cs. Migration rates range between 0.25 cm/a and 1.0 cm/a. On an average, the highest migration rates were found in the clayey-silty substrates of the lime stone areas in theMuschelkalk regions (Middle Triassic) (0.66 cm/a), followed by the loamy substrates of Lower Permian clastic sediments (Unterrotliegendes) (0.53 cm/a) and the sandy substrates of theBuntsandstein areas (Lower Triassic sandstone) (0.41 cm/a). 90 to 95% of the¹³⁷Cs activities in the clay-poor soils of the Unterrotliegendes and the Buntsandstein were traced in the upper 10 cm of the humus topsoil. The substrates of the lime stone areas (Muschelkalk), in contrast to this, reveal a¹³⁷Cs activity of only 70–76% at the same depth.

Conclusions

Due to the fact that the primary and secondary pores of the soil pore system, in their function as translocation pathways, decrease with increasing soil depth, a significant reduction in the migration rates of¹³⁷Cs can be expected with increasing soil depth. On the other hand, the maximal migration depth of 40 cm found in shallow soils on jointed parent material, as well as on sites with high groundwater tables, implies a possible contamination of near-surface groundwater.

Future outlook

Based on the results of this study, a permanent monitoring of¹³⁷Cs was added to the long-term Soil Monitoring Program run by the Federal Administrative Office of Environment of the Saarland (Landesamt für Umweltschutz des Saarlandes)     

High immobilization of soil cesium using ball milling with nano-metallic Ca/CaO/NaH2PO4: implications for the remediation of radioactive soils

This report shows that cesium can be immobilized in soils with an efficiency of 96.4% by ball milling with nano-metallic Ca/PO₄. In Japan, the major concern on ¹³⁷Cs deposition and soil contamination due to the emission from the Fukushima Daiichi nuclear power plant showed up after a massive quake on March 11, 2011. The accident rated 7, the highest possible on the international nuclear event scale, released 160 petabecquerels (PBq) of iodine ¹³¹I and 15 PBq of ¹³⁷Cs according to the Japanese Nuclear and Industrial Safety Agency. Both ¹³⁷Cs and ¹³¹I radioactive nuclides are increasing cancer risk. Nonetheless, ¹³⁷Cs, with a half-life of about 30 years compared with 8 days for ¹³¹I, is a major threat for agriculture and stock farming and, in turn, human life for decades. Therefore, in Japan, the ¹³⁷Cs fixation and immobilization in contaminated soil is the most important problem, which should be solved by suitable technologies. Ball milling treatment is a promising treatment for the remediation of cesium-contaminated soil in dry conditions. Here, we studied the effect, factors and mechanisms of soil Cs immobilization by ball milling with the addition of nano-metallic Ca/CaO/NaH₂PO₄, termed “nano-metallic Ca/PO₄.” We used scanning electron microscopy combined with electron dispersive spectroscopy (SEM/EDS) and X-ray diffraction. Results show that immobilization efficiency increases from 56.4% in the absence of treatment to 89.9, 91.5, and 97.7 when the soil is ball-milled for 30, 60 and 120 min, respectively. The addition of nano-metallic Ca/PO₄ increased the immobilization efficiency to about 96.4% and decreased the ball milling time. SEM/EDS analysis allows us to observe that the amount of Cs decreased on soil particle surface. Use of nano-metallic Ca/PO₄ over a short milling time also decreases Cs leaching. Therefore, ball milling with nano-metallic Ca/PO₄ treatment may be potentially applicable for the remediation of radioactive Cs-contaminated soil in dry conditions.