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1.
The vertical distribution of 137Cs activity in peat soil profiles and 137Cs activity concentration in plants of various species was studied in samples collected at two sites on a raised bog in central Sweden. One site (open bog) was in an area with no trees and only a few sparsely growing plant species, while the other (low pine) was less than 100 m from the open bog site and had slowly growing Scots pine, a field layer dominated by some ericaceous plants and ground well-covered by plants. The plant samples were collected in 2004–2007 and were compared with samples collected in 1989 from the same open bog and low pine sites. Ground deposition of 137Cs in 2005 was similar at both sites, 23?000 Bq m−2. In the open bog peat profile it seems to be an upward transport of caesium since a clear peak of 137Cs activity was found in the uppermost 1–4 cm of Sphagnum layers, whereas at the low pine site 137Cs was mainly found in deeper (10–12 cm) layers. The migration rate was 0.57 cm yr−1 at the open bog site and the migration centre of 137Cs was at a depth of 10.7, while the rate at the low pine site was 0.78 cm yr−1 and the migration centre was at 14.9 cm. Heather (Calluna vulgaris) was the plant species with the highest 137Cs activity concentrations at both sites, 43.5 k Bq−1 DM in 1989 decreasing to 20.4 in 2004–2007 on open bog and 22.3 k Bq kg−1 DM in 1989 decreasing to 11.2 k Bq−1 DM by the period 2004–2007 on the low pine site. 137Cs transfer factors in plants varied between 0.88 and 1.35 on the open bog and between 0.48 and 0.69 m2 kg−1 DM at the low pine site.  相似文献   

2.
Following the Chernobyl accident, 137Cs contamination levels of wild boar in some districts of Southern Germany are still exceeding thousands of Bq kg−1. While the long term 137Cs concentration in forest plants, mushrooms, and roe deer meat has decreased significantly, for wild boar it has remained constant during the last decade. Between 1998 and 2008, we analysed the muscle meat of 656 wild boars shot in the district (“Landkreis”) Ravensburg. The 137Cs activity concentration showed considerable variability from less than 5 up to 8266 Bq kg−1 and it followed a seasonal pattern, which is attributed to changes in dietary habits, fodder availability, meteorological conditions and specific behaviour of 137Cs in wild boar organism. Tag values for wild boars from the district Ravensburg varied from 0.008 to 0.062 m2 kg−1 during 2000–2008.  相似文献   

3.
The 7Be wet deposition has been intensively investigated in a semiarid region at San Luis Province, Argentina. From November 2006 to May 2008, the 7Be content in rainwater was determined in 58 individual rain events, randomly comprising more than 50% of all individual precipitations at the sampling period. 7Be activity concentration in rainwater ranged from 0.7 ± 0.3 Bq l−1 to 3.2 ± 0.7 Bq l−1, with a mean value of 1.7 Bq l−1 (sd = 0.53 Bq l−1). No relationship was found between 7Be content in rainwater and (a) rainfall amount, (b) precipitation intensity and (c) elapsed time between events. 7Be ground deposition was found to be well correlated with rainfall amount (R = 0.92). For the precipitation events considered, the 7Be depositional fluxes ranged from 1.1 to 120 Bq m−2, with a mean value of 32.7 Bq m−2 (sd = 29.9 Bq m−2). The annual depositional flux was estimated at 1140 ± 120 Bq m−2 y−1. Assuming the same monthly deposition pattern and that the 7Be content in soil decreases only through radioactive decay, the seasonal variation of 7Be areal activity density in soil was estimated. Results of this investigation may contribute to a valuable characterization of 7Be input in the explored semiarid ecosystem and its potential use as tracer of environmental processes.  相似文献   

4.
Sediment deposits are the ultimate sink for anthropogenic radionuclides entering the marine environment. The major sources of anthropogenic radionuclides to the Barents Sea are fallout from nuclear weapons tests, long range transport from other seas, and river and non-point freshwater supplies. In this study we investigated activity concentrations, ratios, and inventories of the anthropogenic radionuclides, 137Cs, 238Pu, 239,240Pu in dated sediment cores collected along a north-south transect in the northwestern Barents Sea. The data were used to evaluate the influence of different sources on the derived spatial and temporal patterns of anthropogenic radionuclides in seafloor sediment deposits. Activity concentrations of 137Cs ranged from <0.1 Bq/kg to 10.5 Bq/kg while 239,240Pu ranged from <0.01 Bq/kg to 2.74 Bq/kg and 238Pu activity concentrations ranged from <0.01 Bq/kg to 0.22 Bq/kg. Total inventories of 137Cs ranged from 29.5 ± 1.5 Bq/m2 to 152.7 ± 5.6 Bq/m2 and for 239,240Pu inventories (6 sediment layers only) ranged from 9.5 ± 0.3 Bq/m2 to 29.7 ± 0.4 Bq/m2. Source contributions varied among stations and between the investigated radionuclides. The 238Pu/239,240Pu ratios up to 0.18 indicate discharges from nuclear fuel reprocessing plants as a main contributor of plutonium. Based on 238Pu/239,240Pu ratio, it was calculated that up to 19-27% of plutonium is supplied from sources other than atmospheric global fallout. Taking into account Atlantic current flow trajectories and that both activity concentrations and inventories of plutonium negatively correlate with latitude, Sellafield is a major source for the Barents Sea. Concentrations and inventories of 137Cs correlate positively with latitude and negatively with distance from the Svalbard archipelago. The 137Cs concentrations are highest in an area of intensive melting of sea ice formed along the Siberian coast. Thus, sea ice and supplies from Svalbard may be important source of 137Cs to the Barents Sea seafloor.  相似文献   

5.
Several medicinal plants used in Italy were analysed to determine natural and artificial radioactivity in those parts (leaves, fruits, seeds, roots, peduncles, flowers, barks, berries, thallus) used generally as remedies. The radionuclides were determined by alpha (238U, 210Po) and gamma (214Pb-Bi, 210Pb, 40K and 137Cs) spectrometry. 238U ranged between <0.1 and 7.32 Bq kgdry−1; 210Po between <0.1 and 30.3 Bq kgdry−1; 214Pb-214Bi between <0.3 and 16.6 Bq kgdry−1; 210Pb between <3 and 58.3 Bq kgdry−1; 40K between 66.2 and 3582.0 Bq kgdry−1; 137Cs between <0.3 and 10.7 Bq kgdry−1. The percentage of 210Po extraction in infusion and decoction was also determined; the arithmetical mean value of percentage of 210Po extraction resulted 20.7 ± 7.5.  相似文献   

6.
Radon and gamma radiation level measurements were carried out inside the La Carolina mine, one of the oldest gold mining camps of southern South America, which is open for touristic visits nowadays. CR-39 track-etch detectors and thermoluminescent dosimeters of natural CaF2 and LiF TLD-100 were exposed at 14 points along the mine tunnels in order to estimate the mean 222Rn concentration and the ambient dose equivalent during the summer season (November 2008 to February 2009). The values for the 222Rn concentration at each monitoring site ranged from 1.8 ± 0.1 kBq m−3 to 6.0 ± 0.5 kBq m−3, with a mean value of 4.8 kBq m−3, indicating that these measurements exceed in about three times the upper action level recommended by ICRP for workplaces. The correlations between radon and gamma radiation levels inside the mine were also investigated. Effective doses due to 222Rn and gamma rays inside the mine were determined, resulting in negligible values to tourists. Considering the effective dose to the mine tourist guides, values exceeding 20 mSv of internal contribution to the effective doses can be reached, depending on the number of working hours inside the mine.  相似文献   

7.
Indoor radon distribution of subway stations in a Korean major city   总被引:1,自引:0,他引:1  
The overall survey on indoor radon concentration was conducted at all subway stations in a major city, Daejeon in the central part of Korea. It was quarterly performed from September 2007 to August 2008. The annual arithmetic mean of indoor radon concentration of all the stations was 34.1 ± 14.7 Bq m−3, and the range of values was from 9.4 to 98.2 Bq m−3. The radon concentrations in groundwater (average 31.0 ± 0.8 Bq m−3) were not significantly high in most stations, but the concentration (177.9 ± 2.3 Bq L−1) of one station was over the level of 148 Bq L−1 in drinking water proposed by U.S. EPA. Based on indoor survey results, the approximate average of the annual effective dose by radon inhalation to the employees and passengers were 0.24 mSv y−1, and 0.02 mSv y−1, respectively. Although the effective dose based on the UNSCEAR report was potentially estimated, for more accurate assessment, the additional survey on the influence by indoor radon will be necessary.  相似文献   

8.
This paper describes a quantitative radioactivity analysis method especially suitable for environmental samples with low-level activity. The method, consisting of a multi-group approximation based on total absorption and Compton spectra of gamma rays, is coherently formalized and a computer algorithm thereof designed to analyze low-level activity NaI(Tl) gamma ray spectra of environmental samples. Milk powder from 1988 was used as the example case. Included is a special analysis on the uncertainty estimation. Gamma sensitiveness is defined and numerically evaluated. The results reproduced the calibration data well, attesting to the reliability of the method. The special analysis shows that the uncertainty of the assessed activity is tied to that of the calibration activity data. More than 77% of measured 1461-keV photons of 40K were counted in the range of clearly lower energies. Pile-up of single line photons (137Cs) looks negligible compared to that of a two-line cascade (134Cs). The detection limit varies with radionuclide and spectrum region and is related to the gamma sensitiveness of the detection system. The best detection limit always lies in a spectrum region holding a line of the radionuclide and the highest sensitiveness. The most radioactive milk powder sample showed a activity concentration of 21 ± 1 Bq g−1for 137Cs, 323 ± 13 Bq g−1 for 40K and no 134Cs.  相似文献   

9.
Radioactive markers are useful in dating lead deposition patterns from industrialization in peat archive. Peat cores were collected in an ombrotrophic peat bog in the Great Hinggan Mountains in Northeast China in September 2008 and dated using 210Pb and 137Cs radiometric techniques. The mosses in both cores were examined systematically for dry bulk density, water and ash content. Lead also was measured using atomic emission spectroscopy with inductively coupled plasma (ICP-AES). Both patterned peat profiles were preserved well without evident anthropogenic disturbance. Unsupported 210Pb and 137Cs decreased with the depth in both of the two sample cores. The 210Pb chronologies were established using the constant rate of supply model (CRS) and are in good agreement with the 137Cs time marker. Recent atmospheric 210Pb flux in Great Hinggan Mountains peat bog was estimated to be 337 Bq m−2 y−1, which is consistent with published data for the region. Lead deposition rate in this region was also derived from these two peat cores and ranged from 24.6 to 55.8 mg m−2 y−1 with a range of Pb concentration of 14-262 μg g−1. The Pb deposition patterns were consistent with increasing industrialization over the last 135-170 y, with a peak of production and coal burning in the last 50 y in Northeast China. This work presents a first estimation of atmospheric Pb deposition rate in peatlands in China and suggests an increasing trend of environmental pollution due to anthropogenic contaminants in the atmosphere. More attention should be paid to current local pollution problems, and society should take actions to seek a balance between economic development and environmental protection.  相似文献   

10.
The aim of this work is to determine the radioactivity concentration of 226Ra, 232Th and 40K in sub-surface (0-5 cm) soil samples collected from Awanda, Bikoué, Ngombas in the southwestern region of Cameroon, to assess their contribution to the external dose exposure relative to the United Nation Scientific Committee on Effects of Atomic Radiation (UNSCEAR) data. An HPGe p-type detector coupled to a multichannel analyzer was used to perform measurements and data processing. The activity concentrations of 226Ra varied from 0.06 ± 0.01 to 0.27 ± 0.02 kBq kg−1 with a mean value of 0.13 ± 0.01 kBq kg−1 wet weight. The activity concentrations of 232Th varied from 0.10 ± 0.01 to 0.70 ± 0.05 kBq kg−1 with a mean value of 0.39 ± 0.03 kBq kg−1 wet weight, and 40K concentrations varied from 0.37 ± 0.02 to 1.53 ± 0.11 kBq kg−1 with a mean value of 0.85 ± 0.07 kBq kg−1 wet weight, respectively. The mean value of outdoor annual effective doses were estimated to be 0.48 mSv y−1, 0.39 mSv y−1 and 0.38 mSv y−1 from Ngombas, Awanda and Bikoué, respectively. The studied areas can be said to have a high background radiation level.  相似文献   

11.
Natural background gamma radiation and radioactivity concentrations were investigated from 2003 to 2005 in Kinta District, Perak, Malaysia. Sample locations were distant from any ‘amang’ processing plants. The external gamma dose rates ranged from 39 to 1039 nGy h−1. The mean external gamma dose rate was 222 ± 191 nGy h−1. Small areas of relatively enhanced activity were located having external gamma dose rates of up to 1039 ± 104 nGy h−1. The activity concentrations of 238U, 232Th and 40K were analyzed by using a high-resolution co-axial HPGe detector system. The activity concentration ranges were 12–426 Bq kg−1 for 238U, 19–1377 Bq kg−1 for 232Th and <19–2204 Bq kg−1 for 40 K. Based on the radioactivity levels determined, the gamma-absorbed dose rates in air at 1 m above the ground were calculated. The calculated dose rates and measured dose rates had a good correlation coefficient, R of 0.94. To evaluate the radiological hazard of the natural radioactivity, the radium equivalent activity, the gamma-absorbed dose rate and the mean population weighted dose rate were calculated. An isodose map for the Kinta District was also produced.  相似文献   

12.
Radon exhalation from building materials for decorative use   总被引:2,自引:0,他引:2  
Long-term exposure to radon increases the risk of developing lung cancer. There is considerable public concern about radon exhalation from building materials and the contribution to indoor radon levels. To address this concern, radon exhalation rates were determined for 53 different samples of drywall, tile and granite available on the Canadian market for interior home decoration. The radon exhalation rates ranged from non-detectable to 312 Bq m−2 d−1. Slate tiles and granite slabs had relatively higher radon exhalation rates than other decorative materials, such as ceramic or porcelain tiles. The average radon exhalation rates were 30 Bq m−2 d−1 for slate tiles and 42 Bq m−2 d−1 for granite slabs of various types and origins. Analysis showed that even if an entire floor was covered with a material having a radon exhalation rate of 300 Bq m−2 d−1, it would contribute only 18 Bq m−3 to a tightly sealed house with an air exchange rate of 0.3 per hour. Generally speaking, building materials used in home decoration make no significant contribution to indoor radon for a house with adequate air exchange.  相似文献   

13.
The evaluation and assessment of monitoring data generated over a period of 1983-2007 (25 years) of a nuclear facility is presented. Time trends of particulate radioactivity, correlation between 137Cs in discharge canal seawater and station discharged activity and correlation of 137Cs, 60Co, and 131I in marine species such as sponge and Nerita (gastropod) and corresponding discharged activity are discussed. The concentration of 137Cs and 131I in seawater versus biota are discussed. A good correlation between 137Cs in seawater and 137Cs in liquid waste discharged was observed (R2 = 0.8, p < 0.001). Similarly, correlation was good for Nerita and discharged concentration of 137Cs, 131I and 60Co (R2 = 0.55-0.73 and p < 0.001). The measurements over the years indicated that there is no accumulation of radionuclides in either the terrestrial or aquatic environments. The mean 137Cs decreased from the pre-operational levels: 7.0-3.6 Bq kg−1 in soil, 0.91-0.016 Bq L−1 in milk and 0.28-0.036 Bq kg−1 in vegetation. Similarly, the mean 90Sr in these matrixes decreased from 3.9 to 0.26 Bq kg−1; 0.37-0.011 Bq L−1 and 0.34-0.022 Bq kg−1 respectively. Cesium-137 of about 700 μBq m−3 was measured in the air filter disks during 1986 and there was a decrease of three orders of magnitude in concentration over the 25 years. The evaluation of environmental data indicated that the radionuclide concentrations and potential impacts, in terms of effective dose to the members of public, have significantly reduced since 1969.  相似文献   

14.
Concentrations of the natural radionuclides 238U, 226Ra, 232Th and 40K have been measured by γ-ray spectrometry in 796 topsoil samples from the Pearl River Delta Zone (PRDZ) of Guangdong, China. The mean concentrations for 238U, 226Ra, 232Th and 40K were found to be 140 ± 37 Bq kg−1, 134 ± 41 Bq kg−1, 187 ± 80 Bq kg−1 and 680 ± 203 Bq kg−1 dry mass, respectively. These values were all higher than the mean values in soil for China and the world. Outdoor air-absorbed dose rates, calculated from activity concentrations of 226Ra, 232Th and 40K, ranged from 86 to 237 nGy h−1, with a mean value of 165 ± 46 nGy h−1. The corresponding annual outdoor effective dose rate per person was estimated to be between 0.11 and 0.29 mSv y−1, with a mean value of 0.20 ± 0.06 mSv y−1, which was also higher than the world mean value of 0.07 mSv y−1. The radium equivalent activity (Raeq) and the external hazard index (Ir) resulted from the natural radionuclides in soil, were also calculated and found to vary from 230 to 676 Bq kg−1 and from 0.6 to 1.8, respectively. The Raeq and the Ir in all the investigated regions were up to 75% higher than the set limits of 370 Bq kg−1 and 1.0, respectively.  相似文献   

15.
Radioiodine (131I) in air and rainwater as high as 497 μBq m−3 and 0.7 Bq L−1, respectively, as well as 137Cs and 134Cs in air as high as 145 μBq m−3 and 126 μBq m−3, respectively were recorded in Thessaloniki, Northern Greece (40°38′N, 22°58′E) from March 24, 2011 through April 09, 2011, after a nuclear accident occurred at Fukushima, Japan (37°45′N, 140°28′E) on March 11, 2011.  相似文献   

16.
The activity of 210Po and 210Pb was determined in mussels of the same size (3.5-4.0 cm shell length) sampled monthly over a 17-month period at the Atlantic coast of Portugal. Average radionuclide concentration values in mussels were 759 ± 277 Bq kg−1 for 210Po (range 460-1470 Bq kg−1 dry weight), and 45 ± 19 Bq kg−1 for 210Pb (range 23-96 Bq kg−1 dry weight). Environmental parameters and mussel biometric parameters were monitored during the same period. Although there was no seasonal variation of radionuclide concentrations in sea water during the study period, the concentration of radionuclide activity in mussels varied seasonally displaying peaks of high concentrations in winter and low concentrations in summer. Analysis of radionuclide data in relation to the physiological Condition Index of mussels revealed that 210Po and 210Pb activities in the mussel (average activity per individual) remained nearly constant during the investigation period, while mussel body weight fluctuated due to fat storage/expenditure in the soft tissues. Similar variation of radionuclide concentrations was observed in mussels transplanted from the sea coast into the Tejo Estuary. However, under estuarine environmental conditions and with higher food availability throughout the year, transplanted mussel Condition Index was higher than in coastal mussels and average radionuclide concentrations were 210 ± 75 Bq kg−1 (dry weight) for 210Po and 10 ± 4 Bq kg−1 (dry weight) for 210Pb, therefore lower than in coastal mussels with similar shell length. It is concluded that the apparent seasonal fluctuation and inter-site difference of radionuclide concentrations were mostly caused by mussel body weight fluctuation and not by radionuclide body burden fluctuation. This interpretation can be extended to the apparent seasonal fluctuation in concentrations of lipophilic and lipophobic contaminants in mussels, and provides an explanation for occasional high concentrations of 210Po and man-made contaminants measured in mussels far from pollution sources.  相似文献   

17.
A shallow-land radioactive waste repository operated in boggy forest environment from 1963 to 1989. During the operation period, a considerable amount of technogenic radionuclides, in solidified state, was disposed into the vault established in the geological structure at the depth of up to 3 m. Environmental monitoring activities started after the closure of the repository in 1989. Recent investigations revealed transfer of radiocarbon and plutonium to the groundwater in the prevailing flow direction. Activity concentration of 239,240Pu in non-filtered fraction of the groundwater from observation well no. 4 determined by alpha-spectrometry was 6.4 × 10−5 Bq l−1 in 2005, and 3.2 × 10−4 Bq l−1 in 2006. Further analysis of colloid-facilitated transport of plutonium is planned. Variation of 14C activity concentration in the same well was monitored in 2006. It varied from 0.2 ± 0.1 Bq l−1 in October to 2.8 ± 0.6 Bq l−1 in June and July. Results imply further research into radiocarbon transfer to atmosphere and selected plant species.  相似文献   

18.
Natural radioactive materials under certain conditions can reach hazardous radiological levels. So, it becomes necessary to study the natural radioactivity levels in soil to assess the dose for the population in order to know the health risks and to have a baseline for future changes in the environmental radioactivity due to human activities. The natural radionuclide (226Ra, 232Th, and 40K) contents in soil were determined for 26 locations around the Upper Siwaliks of Kala Amb, Nahan and Morni Hills, Northern India, using high-resolution gamma-ray spectrometric analysis. It was observed that the concentration of natural radionuclides viz., 226Ra, 232Th and 40K, in the soil varies from 28.3 ± 0.5 to 81.0 ± 1.7 Bq kg−1, 61.2 ± 1.3 to 140.3 ± 2.6 Bq kg−1 and 363.4 ± 4.9 to 1002.2 ± 11.2 Bq kg−1 respectively. The total absorbed dose rate calculated from activity concentration of 226Ra, 232Th and 40K ranged from 71.1 to 162.0 nGy h−1. The radium equivalent (Req) and the external hazard index (Hex), which resulted from the natural radionuclides in soil, were also calculated and found to vary from 149.4 to 351.8 Bq kg−1and from 0.40 to 0.95 respectively. These values in Upper Siwaliks area were compared with that from the adjoining areas of Punjab. The radium equivalent activities in all the soil samples were lower than the limit (370 Bq kg−1) set in the Organization for Economic Cooperation and Development (OECD) report and the dose equivalent was within the safe limit of 1 mSv y−1.  相似文献   

19.
In the framework of a 222Rn screening campaign that was carried out in 58 public secondary schools in Galicia (NW Spain), the largest radon-prone area in the Iberian Peninsula, a positive correlation between indoor 222Rn concentration and outdoor gamma exposure rate was obtained. A new approach to the data acquisition in screening surveys was tested, improving the performances of this type of study and gathering useful data for future remedial actions. Using short-period detectors (charcoal canisters) firstly, in order to detect places showing 222Rn concentrations over 400 Bq m−3, the number of locations to be measured with long-period detectors (etched track detectors) is reduced. In this screening campaign, 34% of the schools surveyed presented at least one site exceeding the 400 Bq m−3 recommended action level established by the EU, and 15% had at least one site with 222Rn values over 800 Bq m−3. The maximum value recorded was 2084 ± 63 Bq m−3. These results are discussed and compared with data obtained in schools of several countries with similar geology. Seven schools were also studied for seasonal variations of 222Rn activity concentration. The results were not conclusive, and no significant correlation between season and 222Rn concentration was established. Finally, a continuous 222Rn concentration monitor was placed in the secondary school exhibiting a mean value of the 222Rn concentration very close to 400 Bq m−3. Maximum 222Rn concentration values were found to occur at times when the school was unoccupied.  相似文献   

20.
Twenty-one years after the Chernobyl accident, lichen and moss samples were collected from the Ordu province, which was already chosen for a related study some years ago. It was observed that 137Cs activity concentration ranged from 31 to 469 Bq kg−1 in the moss and from 132 to 1508 Bq kg−1 in the lichen samples. The decrease of the activity concentrations in the present measurements (2007) relative to those in 1997 (over a period of 10 y) indicated ecological half-lives between 1.8 and 10.4 y for the moss and between 2.1 and 13.7 y for the lichen samples. It was observed that 137Cs was still eminent in the area studied. Moreover, 40K activity concentrations and K element concentrations were measured and their relationships were discussed.  相似文献   

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