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1.
Radon is a radioactive gas, abundant in granitic areas, such as in the city of Porto at the north-east of Portugal. This gas is a recognized carcinogenic agent, being appointed by the World Health Organization as the leading cause of lung cancer after smoking. The aim of this preliminary survey was to determine indoor radon concentrations in public primary schools, to analyse the main factors influencing their indoor concentration levels and to estimate the effective dose in students and teachers in primary schools. Radon concentrations were measured in 45 classrooms from 13 public primary schools located in Porto, using CR-39 passive radon detectors for about 2-month period. In all schools, radon concentrations ranged from 56 to 889 Bq/m3 (mean = 197 Bq/m3). The results showed that the limit of 100 Bq/m3 established by WHO IAQ guidelines was exceeded in 92 % of the measurements, as well as 8 % of the measurements exceeded the limit of 400 Bq/m3 established by the national legislation. Moreover, the mean annual effective dose was calculated as 1.25 mSv/y (ranging between 0.58 and 3.07 mSv/y), which is below the action level (3–10 mSv). The considerable variability of radon concentration observed between and within floors indicates a need to monitor concentrations in several rooms for each floor. A single radon detector for each room can be used, provided that the measurement error is considerably lower than variability of radon concentration between rooms. The results of the present survey will provide useful baseline data for adopting safety measures and dealing effectively with radiation emergencies. In particular, radon remediation techniques should be used in buildings located in the highest radon risk areas of Portugal. The results obtained in the current study concerning radon levels and their variations will be useful to optimize the design of future research surveys.  相似文献   

2.
The main objective of this study is to assess the health hazard due to the indoor radon. Measurement studies have been carried out in 56 dwellings belonging to 14 residential areas in Alexandria city, Egypt. Results are obtained using the LR-115 (Type II) alpha track detector in “closed-can” geometry. The dosimeters were installed in bedroom, living room, and the kitchens of each house. For intercomparison purpose, dosimeters are installed in basements, ground floor, and first floor. Measured indoor radon concentrations were found to vary from 15 to 132 Bq m?3. The average radon concentrations in living room, bedrooms, and kitchen in basements were found to vary from to be 39 ± 10, 63 ± 15 and 81 ± 25 Bq m?3, respectively. In living room, bedrooms, and kitchen, on ground floor, the average radon concentrations were found to be 35 ± 9, 44 ± 6 and 56 ± 10 Bq m?3, whereas on first floor, the average values are 29 ± 8, 34 ± 7 and 45 ± 8 Bq m?3, respectively. The overall mean radon concentration in all surveyed districts has been found to be 44 ± 16 Bq m?3. The mean annual estimated effective dose received by the residents of the studied area is estimated to be 0.75 mSv. The obtained results are compared with the indoor radon levels prescribed by the International Commission on Radiation Protection and are found to be less than the action level recommended.  相似文献   

3.
A screening survey has been carried out to determine activity concentrations of radon (222Rn) in drinking water and indoor air in various locations in Kenya. The concentration of 222Rn in water was measured using a liquid scintillation counter (LSC). Three different passive integrating devices were used in the measurements of 222Rn in air. In the short-term measurements, radon is absorbed in activated charcoal and the analyses were carried out using either LSC or gamma ray spectrometry. The long-term measurements were carried out using solid-state nuclear track detectors (SSNTD). The mean and maximum values of 222Rn concentrations in water are 37 and 410 Bq L–1 and 100 and 1160 Bq m–3, respectively, in air. The highest values were obtained from groundwater sources and in the basements of buildings. When these values are compared with the internationally recommended reference levels, there are indications of existence of radon problems in some of the water sources and the dwellings tested in this survey.  相似文献   

4.
Because detrimental effects of exposure to lead (Pb) on human health have been observed, we previously investigated concentrations of Pb in water supplies and blood of adult residents of Riyadh, Saudi Arabia. The objectives of the present study were to: (1) examine seasonal rates of deposition of Pb in dust in several areas of Riyadh city, (2) measure concentrations of Pb in both outdoor and indoor dust, (3) compare concentrations of Pb in dust in Riyadh with those reported for other cities, and (4) quantify Pb in blood of children living in Riyadh. Mean, monthly deposition of PB in outdoor dust was 4.7 × 101 ± 3.6 tons km?2, with a mean Pb concentration of 2.4 × 102 ± 4.4 × 101 μg/g. Mean, monthly deposition of Pb in indoor dust was 2.7 ± 0.70 tons km?2, with a mean concentration of 2.9 × 101 ± 1.5 × 101 μg Pb/g. There was a significant (P < 0.01) correlation between concentrations of Pb in outdoor and indoor dust. There was no correlation between concentrations of Pb in indoor dust and that in blood of children of Riyadh, whereas there was a weakly significant (P < 0.05) correlation between concentrations of Pb in outdoor dust and that in blood of children. The mean (±SD) concentration of Pb in blood of children in Riyadh was 5.2 ± 1.7, with a range of 1.7–1.6 × 101 μg/dl. Concentrations of Pb in blood of 17.8 % of children in Riyadh were greater than 10 μg/dl, which is the CDC’s level of concern.  相似文献   

5.
Radon has been determined in soil, groundwater, and air in Mexico, both indoors and outdoors, as part of geophysical studies and to estimate effective doses as a result of radon exposure. Detection of radon has mainly been performed with solid-state nuclear track detectors (SSNTD) and, occasionally, with active detection devices based on silicon detectors or ionization chambers. The liquid scintillation technique, also, has been used for determination of radon in groundwater. The adjusted geometric mean indoor radon concentration (74 Bq m−3) in urban developments, for example Mexico City, is higher than the worldwide median concentration of radon in dwellings. In some regions, particularly hilly regions of Mexico where air pollution is high, radon concentrations are higher than action levels and the effective dose for the general population has increased. Higher soil radon levels have been found in the uranium mining areas in the northern part of the country. Groundwater radon levels are, in general, low. Soil-air radon contributing to indoor atmospheres and air pollution is the main source of increased exposure of the population.  相似文献   

6.
Recently, the problem of indoor particulate matter pollution has received much attention. An increasing number of epidemiological studies show that the concentration of atmospheric particulate matter has a significant effect on human health, even at very low concentrations. Most of these investigations have relied upon outdoor particle concentrations as surrogates of human exposures. However, considering that the concentration distribution of the indoor particulate matter is largely dependent on the extent to which these particles penetrate the building and on the degree of suspension in the indoor air, human exposures to particles of outdoor origin may not be equal to outdoor particle concentration levels. Therefore, it is critical to understand the relationship between the particle concentrations found outdoors and those found in indoor micro-environments. In this study, experiments were conducted using a naturally ventilated office located in Qingdao, China. The indoor and outdoor particle concentrations were measured at the same time using an optical counter with four size ranges. The particle size distribution ranged from 0.3 to 2.5 μm, and the experimental period was from April to September, 2016. Based on the experimental data, the dynamic and mass balance model based on time was used to estimate the penetration rate and deposition rate at air exchange rates of 0.03–0.25 h?1. The values of the penetration rate and deposition velocity of indoor particles were determined to range from 0.45 to 0.82 h?1 and 1.71 to 2.82 m/h, respectively. In addition, the particulate pollution exposure in the indoor environment was analyzed to estimate the exposure hazard from indoor particulate matter pollution, which is important for human exposure to particles and associated health effects. The conclusions from this study can serve to provide a better understanding the dynamics and behaviors of airborne particle entering into buildings. And they will also highlight effective methods to reduce exposure to particles in office buildings.  相似文献   

7.

Concentrations of radon (222Rn) and thoron (220Rn) were measured in the air of different marble factories by using a nuclear track technique. The influence of the marble dust nature and ventilation on radon and thoron concentrations was investigated. It was observed that measured radon and thoron concentration ranged from 310 to 903 Bq m−3 and 6 to 48 Bq m−3, respectively. In addition, alpha-activities due to the unattached and attached fractions of 218Po and 214Po radon short-lived progeny were evaluated in the marble factories studied. Committed equivalent doses due to the attached and unattached fractions of 218Po and 214Po nuclei were evaluated in the lung tissues of marble factory workers. The dependence of the resulting committed equivalent dose on the concentration of the attached and unattached fractions of the 218Po and 214Po radionuclides and mass of the tissue was investigated. The resulting annual committed effective doses to the lung of marble factory workers due to the attached and unattached fractions of the 218Po and 214Po radionuclides were calculated. The obtained results show that about 80% of the global committed effective doses received by workers in the studied marble factories are due to the attached fraction of the 218Po and 214Po radon short-lived daughters from the inhalation of polluted air. Male workers spending 8 h per day (2080 h per year) in a marble factory receive a maximum dose of 34.46 mSv y−1 which is higher than the (3–10 mSv y−1) dose limit interval given by the ICRP. Good agreement was found between data obtained for the average effective dose gotten by using this method and the UNSCEAR and ICRP conversion dose coefficients.

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8.
Hydrothermal areas are potentially hazardous to humans as volcanic gases such as radon (222Rn) are continuously released from soil diffuse degassing. Exposure to radon is estimated to be the second leading cause of lung cancer, but little is known about radon health-associated risks in hydrothermal regions. This cross-sectional study was designed to evaluate the DNA damage in the buccal epithelial cells of individuals chronically exposed to indoor radon in a volcanic area (Furnas volcano, Azores, Portugal) with a hydrothermal system. Buccal epithelial cells were collected from 33 individuals inhabiting the hydrothermal area (Ribeira Quente village) and from 49 individuals inhabiting a non-hydrothermal area (Ponta Delgada city). Indoor radon was measured with Ramon 2.2 detectors. Chromosome damage was measured by micronucleus cytome assay, and RAPD-PCR was used as a complementary tool to evaluate DNA damage, using three 10-mer primers (D11, F1 and F12). Indoor radon concentration correlated positively with the frequency of micronucleated cells (r s = 0.325, p = 0.003). Exposure to radon is a risk factor for the occurrence micronucleated cells in the inhabitants of the hydrothermal area (RR = 1.71; 95% CI, 1.2–2.4; p = 0.003). One RAPD-PCR primer (F12) produced differences in the banding pattern, a fact that can indicate its potential for detecting radon-induced specific genomic alterations. The observed association between chronic exposure to indoor radon and the occurrence of chromosome damage in human oral epithelial cells evidences the usefulness of biological surveillance to assess mutations involved in pre-carcinogenesis in hydrothermal areas, reinforcing the need for further studies with human populations living in these areas.  相似文献   

9.
In this study, indoor and outdoor radon (222Rn) surveys were carried out in the summer and winter seasons in homes of one hundred lung cancer patients in the year 2013–2014. The aim was to investigate the relationship between radon and cancer patients. Lung cancer patients completed a questionnaire concerning their living environment, various physical parameters and living habits. Pearson correlation and t tests revealed no meaningful results between radon concentrations, on one hand, and environmental and personal living habits, on the other hand. Consequently, the BEIR VI model was adapted and 222Rn exposure was estimated to be responsible for about 12% of the lung cancer incidences in the winter season and around 5% in the summer season in the Rize Province. However, due to the limited number of data and numerous parameters that could lead to lung cancer, the estimations done with the model should be taken very lightly. The annual effective doses due to inhalation of indoor and outdoor 222Rn were estimated to be, respectively, 1.43 and 0.94 mSv y?1. The indoor and outdoor annual effective doses were, respectively, close and below the world annual effective dose (1.3 mSv y?1). At the district level, the indoor annual effective dose equivalent in the ?yidere district was 4.52 mSv y?1, which was 3.5 times greater than the world average. The number of patients in the majority of the houses in this district was more than one.  相似文献   

10.
Indoor radon has been recognized as one of the health hazards for mankind. Common building materials used for construction of houses, which are considered as one of the major sources of this gas in indoor environment, have been studied for exhalation rate of radon. Non-nuclear industries, such as coal fired power plants or fertilizer production facilities, generate large amounts of waste gypsum as by-products. Compared to other building materials waste gypsum from fertilizer production facilities (phosphogypsum) shows increased rates of radon exhalation. In the present, investigation solid state alpha track detectors, CR-39 plastic detectors, were used to measure the indoor radon concentration and the radon exhalation rates from some building materials used in Egypt. The indoor radon concentration and the radon exhalation rate ranges were found to be 24–55 Bq m−3 and 11–223 mBq m−2 h−1, respectively. The effective dose equivalent range for the indoor was found 0.6–1.4 mSv y−1. The equilibrium factor between radon and its daughters increased with the increase of relative humidity.  相似文献   

11.
In this study, we collected particles with aerodynamic diameter ?2.5 μm (PM2.5) from three different public indoor places (a supermarket, a commercial office, and a university dining hall) in Jinan, a medium-sized city located in northern China. Water-soluble inorganic ions of PM2.5 and particle size distributions were also measured. Both indoor and outdoor PM2.5 levels (102.3–143.8 μg·m?3 and 160.2–301.3 μg·m?3, respectively) were substantially higher than the value recommended by the World Health Organization (25 μg·m?3), and outdoor sources were found to be the major contributors to indoor pollutants. Diurnal particle number size distributions were different, while the maximum volume concentrations all appeared to be approximately 300 nm in the three indoor locations. Concentrations of indoor and outdoor PM2.5 were shown to exhibit the same variation trends for the supermarket and dining hall. For the office, PM2.5 concentrations during nighttime were observed to decrease sharply. Among others, SO 4 2? , NH 4 + and NO 3 ? were found to be the dominant water-soluble ions of both indoor and outdoor particles. Concentrations of NO 3 ? in the supermarket and office during the daytime were observed to decrease sharply, which might be attributed to the fact that the indoor temperature was much higher than the outdoor temperature. In addition, domestic activities such as cleaning, water usage, cooking, and smoking also played roles in degraded indoor air quality. However, the results obtained here might be negatively impacted by the small number of samples and short sampling durations.  相似文献   

12.
Radium-226 is a significant source of radon-222 which enters buildings through soil, construction materials or water supply. When cigarette smoke is present, the radon daughters attach to smoke particles. Thus, the alpha radiation to a smoker’s lungs from the natural radon daughters is increased because of smoking. To investigate whether the cigarette tobacco itself is a potential source of indoor radon, the α potential energy exposure level contents of radon (222Rn, 3.82d) and Thoron (220Rn, 55.60s) were measured in 10 different cigarette tobacco samples using CR-39 solid-state nuclear track detectors (SSNTDs). The results showed that the 222, 220Rn concentrations in these samples ranged from 128 to 266 and 49 to 148 Bqm−3, respectively. The radon concentrations emerged from all investigated samples were significantly higher than the background level. Also, the annual equivalent doses from the samples were determined. The mean values of the equivalent dose were 3.51 (0.89) and 1.44 (0.08) mSvy−1, respectively. Measurement of the average indoor radon concentrations in 20 café rooms was, significantly, higher than 20 smoking-free residential houses. The result refers to the dual (chemical and radioactive) effect of smoking as a risk factor for lung cancer.  相似文献   

13.
Despite the widespread use of benzotriazoles as corrosion inhibitors in many household goods, studies on the occurrence of these compounds in indoor air are scarce. In this study, five benzotriazole derivatives were measured in 83 indoor air samples collected from various locations in Albany, New York, USA. Benzotriazoles were found in a majority of the indoor air samples, and the concentrations of their sum in bulk (vapor plus particulate phases) indoor air ranged from below the method limit of quantification to 492 ng·m?3 (geometric mean: 5.8 ng·m?3). The highest geometric mean concentration was found in air samples collected in parking garages (155 ng·m?3), followed by barbershops (13.6), public places (11.5), auto repair shops (5.2), automobiles (4.5), homes (4.5), offices (3.7), and laboratories (2.8). Inhalation exposure to benzotriazoles was calculated on the basis of the measured geometric mean concentrations and air inhalation rate. The highest exposure dose was found for teenagers, with a geometric mean inhalation exposure dose of 79 ng·day?1. The body-weight normalized exposure dose, however, was the highest for infants, at 3.2 ng·(kg bw)?1·day?1.  相似文献   

14.
In this work, phthalic acid esters (PAEs): dimethyl phthalate (DMP), diethyl phthalate (DEP), di-n-butyl phthalate, benzyl butyl phthalate, bis(2-ethylhexyl) phthalate, and di-n-octyl phthalate in indoor dust (used as passive sampler) were investigated. The settled dust samples were collected from thirteen indoor environments from Palermo city. A fast and simple method using Soxhlet and GC–MS analysis has been optimized to identify and quantify the phthalates. Total phthalates concentrations in indoor dusts ranged from 269 to 4,831 mg/kg d.w. (d.w. = dry weight). The data show a linear correlation between total PAEs concentration and a single compound content, with the exclusion of the two most volatile components (DMP and DEP) that are present in appreciable amounts only in two samples. These results suggest that most of the PAEs identified in the samples of settled dust originate from the same type of material. This evidence indicates that, in a specific indoor environment, generally is not present only one compound but a mixture having over time comparable percentages of PAEs. Consequently, for routine analyses of a specific indoor environment, only a smaller number of compounds could be determined to value the contamination of that environment. We also note differences in phthalate concentrations between buildings from different construction periods; the total concentration of PAEs was higher in ancient homes compared to those constructed later. This is due to a trend to reduce or remove certain hazardous compounds from building materials and consumer goods. A linear correlation between total PAEs concentration and age of the building was observed (R = 0.71).  相似文献   

15.
The highly populated Indian regions are currently in a phase of rapid economic growth resulting in high emissions of carbonaceous aerosols. This leads to poor air quality and impact on climate. The chemical composition of carbonaceous aerosols has rarely been studied in industrial areas of India. Here, we investigated carbonaceous aerosols in particulate matter (PM) monthly in the industrial area of Delhi in 2011. The concentrations of organic C and elemental C in PM10 fraction were analyzed. Results show a clear seasonal variability of organic and elemental C. PM10 ranged 95.9–453.5 μg m?3, organic C ranged 28.8–159.4 μg m?3, and elemental C ranged 7.5–44.0 μg m?3; those values were higher than reported values. Organic and elemental C were correlated with each other in pre-monsoon and winter seasons, implying the existence of similar emission sources such as coal combustion, biomass burning and vehicular exhaust. The annual average contribution of total carbonaceous aerosols in PM10 was estimated as 62 %.  相似文献   

16.
In this investigation, the concentrations of particles in ambient air, gaseous elemental mercury (GEM), and particulate-bound mercury (Hg(p)) in total suspended particulates (TSP) as well as dry deposition at a (Traffic) sampling site at Hung-kuang were studied during the day and night in 2012. The results reveal that the mean concentrations of TSP in ambient air, GEM, and Hg(p) were 69.72 μg/m3, 3.17, and 0.024 ng/m3, respectively, at the Hung-kuang (Traffic) sampling site during daytime sampling periods. The results also reveal that the mean rates of dry deposition of particles from ambient air and Hg(p) were 145.20 μg/m2 min and 0.022 ng/m2 min, respectively, at the Hung-kuang (Traffic) sampling site during the daytime sampling period. The mean concentrations of TSP in ambient air, GEM, and Hg(p) were 60.56 μg/m3, 2.74, and 0.018 ng/m3, respectively, at the Hung-kuang (Traffic) sampling site during the nighttime sampling period. The mean rates of dry deposition of particles and Hg(p) from ambient air were 132.58 μg/m2 min and 0.016 ng/m2 min, respectively, at the Hung-kuang (Traffic) sampling site during the nighttime sampling period.  相似文献   

17.
To assess the exposure doses of PM2.5 and to investigate its chemical components for the subpopulation (i.e., school children and industrial downwind residents), simultaneous sampling of indoor and outdoor PM2.5 was conducted at an elementary school close to traffic arteries and a residence located in the downwind area of a steel plant in metropolitan Guangzhou in 2010. Chemical components, i.e., organic carbon, elemental carbon and 6 water soluble ions were analyzed in PM2.5. A survey was also conducted to investigate the time-activity patterns of the school children and the industrial downwind residents. Indoor and outdoor PM2.5 were 63.2 ± 20.1 and (76.7 ± 35.8) μg/m3 at the school, and 118.8 ± 44.7 and 125.7 ± 57.1 μg/m3 in the community, respectively. Indoor PM2.5 was found to be highly related to outdoor sources, and stationary sources were the significant contributors to PM2.5 at both sites. The daily average doses of PM2.5 for the school children at the school (D children) and the industrial downwind residents in the community (D residents) were (7.6 ± 1.9) and (36.1 ± 36.8) μg/kg-day, respectively. The daily average doses of particulate organic mass and SO4 2? were the two most abundant chemical components in PM2.5. PM2.5 exposure for the school children was contributed by indoor and outdoor environments by 48.8 and 51.2 %, respectively; for the industrial downwind residents, the contributions were 66.0 and 34.0 %, respectively. Age and body weight were significantly and negatively correlated with D children, while age, body weight and education level were significantly and negatively correlated with D residents; gender was not a significant factor at both cases.  相似文献   

18.
The concentrations and flux of CO2, 222Radon (Rn), and gaseous elemental mercury (Hg) in soil gas were investigated based on the field measurements in June 2010 at ten sites along the seismic rupture zones produced by the May 12, 2008, Wenchuan M s 8.0 earthquake in order to assess the environmental impact of degassing of CO2, Rn and Hg. Soil gas concentrations of 344 sampling points were obtained. Seventy measurements of CO2, Rn and Hg flux by the static accumulation chamber method were performed. The results of risk assessment of CO2, Rn and Hg concentration in soil gas showed that (1) the concentration of CO2 in the epicenter of Wenchuan M s 8.0 earthquake and north end of seismic ruptures had low risk of asphyxia; (2) the concentrations of Rn in the north segment of seismic ruptures had high levels of radon, Maximum was up to level 4, according to Chinese code (GB 50325-2001); (3) the average geoaccumulation index I geo of soil Hg denoted the lack of soil contamination, and maximum values classified the soil gas as moderately to strongly polluted in the epicenter. The investigation of soil gas CO2, Rn and Hg degassing rate indicated that (1) the CO2 in soil gas was characterized by a mean \(\updelta^{13}C_{CO2}\) of ?20.4 ‰ and by a mean CO2 flux of 88.1 g m?2 day?1, which were in the range of the typical values for biologic CO2 degassing. The maximum of soil CO2 flux reached values of 399 g m?2 day?1 in the epicenter; (2) the soil Rn had higher exhalation in the north segment of seismic ruptures, the maximum reached value of 1976 m Bq m?2 s?1; (3) the soil Hg flux was lower, ranging from ?2.5 to 18.7 n g m?2 h?1 and increased from south to north. The mean flux over the all profiles was 4.2 n g m?2 h?1. The total output of CO2 and Hg degassing estimated along seismic ruptures for a survey area of 18.17 km2 were approximately 0.57 Mt year?1 and 688.19 g year?1. It is recommended that land-use planners should incorporate soil gas and/or gas flux measurements in the environmental assessment of areas of possible risk. A survey of all houses along seismic ruptures is advised as structural measures to prevent the ingress of soil gases, including CO2 and Rn, were needed in some houses.  相似文献   

19.
From September 2011 to February 2012, ambient air particulate and particulate-bound mercury [Hg(p)] concentrations were measured, together with dry deposition using a cold vapor atomic fluorescence spectrometry (CVAFS) analyser, at two characteristic sampling sites in central Taiwan. Results from the sampling site at Westin Park indicated that the lowest particulate dry deposition and lowest average particulate concentrations in total suspended particles (TSP) occurred in September (29.70±7.47 μ g m?2×min) and February (34.38±13.60 ng m?3), respectively. Moreover, results from the Gung-Ming junior high school (airport) site, showed that the highest average particulate dry deposition and average highest particulate concentrations in TSP occurred in February (156.76±30.36 μ g m?2×min) and January (125.49±9.51 ng m?3), respectively, during the winter. The Dragon Steel Plant and Han-Shian Aerospace Industrial Development Corporation were both nearby. These factors led to the high Hg(p) concentrations at Taichung Airport (TA) compared with Westin Park. Local large suspended particulates from heavy traffic were the main reason for the high average Hg(p) deposition at Westin Park compared with TA in this study.  相似文献   

20.
Radon in soil gas and its relationship with some major faults of SW England   总被引:3,自引:0,他引:3  
The south-west of England was designated by the National Radiological Protection Board (NRPB) as the first ‘Radon Affected Area’, as over 1% of the housing stock is estimated to have an indoor radon concentration in excess of the 200 Bq m−3 Action Level. The situation is even worse for houses situated above uraniferous granite intrusions, where over 30% are thought to be above the Action Level. The aim of this study is to investigate the relationship between the level of radon in soil gas and the local geology. Particularly high radon levels were measured along major fault zones. This could be explained by: increased rate of migration of the radon due to the permeable fault, the presence of radium or radon-bearing ground water within the fault, or secondary uranium mineralisation. Seasonal variations are also considered.  相似文献   

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