A study of daily and seasonal variations of radon concentrations in underground buildings

A study of daily and seasonal variations of radon concentrations in underground buildings in major cities of China was carried out. According to the data from the Model 1027 continuous monitor, radon concentrations in the underground buildings changed through two cycles each day. The first cycle was from 12:00 to 0:00 and the highest or lowest value, depending on location, was at about 19:00. The second cycle had a little change. Based on the data from solid state nuclear detectors (SSNTDs), it was concluded that the radon concentrations in underground buildings in winter were lower than in summer, which was opposite to that above the ground level. Similar to that above the ground level, the radon concentrations in spring were close to the year-round average radon concentrations.     

Exposure to radon in the Gadime Cave, Kosovo

Air radon concentration was measured in summer and winter at 11 points along the tourist guided route in the Gadime Cave in Kosovo using alpha scintillation cells and etched track detectors. At two points in summer, values higher than 1700Bqm(-3) were observed; they otherwise were in the range 400-1000Bqm(-3). Values were lower in winter. The effective dose received by a person during a 90min visit is 3.7muSv in summer and 2.5muSv in winter. For a tourist guide the annual effective dose is less than 3.5mSv.     

An approach to assessing the probability of unsatisfactory radon in air-conditioned offices of Hong Kong

In order to maintain an acceptable Indoor Air Quality (IAQ), policies, strategies and guidelines have been developed worldwide and exposure concentrations of the indoor radon have been specified. Mapping indoor radon levels for a region could be done with intensive measurements on a large number of samples. To obtain the most accurate estimate of the levels with the uncertainties specified, a statistical model has been developed in this study to predict the fractions of samples in a region having an average radon level above the action levels of 150Bqm(-3) and 200Bqm(-3). The model was based on a transformation of the variation from a small sample set of data to a population geometric distribution via an estimator, known as the 'sample correction factor'. Using a dataset from a cross-sectional measurement of indoor radon levels in 216 Hong Kong offices, where the mean was 37.2Bqm(-3) and the 68% range was from 17.3Bqm(-3) to 80.3Bqm(-3), the 'sample correction factor' was evaluated and tested by the Monte-Carlo simulations. The model estimates of the fractions above the indoor radon action levels 150Bqm(-3) and 200Bqm(-3) (1.2-7.7% and 0.4-4.1% for a sample size of 20, 2.8-5.1% and 0.8-2.4% for a sample size of 60) were demonstrated to be consistent with those determined from the dataset (3.5% and 1.4%). With the 'sample correction factor' thus quantified, it will be possible to provide the required data for the policymakers making appropriate decisions on resources and manpower management.     

Indoor radon levels and influencing factors in houses of Patras,Greece

Measurements of indoor radon concentrations were performed in 28 low-rise houses and 30 apartments in Patras area from December 1996 to November 1997, using nuclear track detectors. The investigation was focused on the effects of season and floor number, as well as on the existence of a basement in low-rise houses on indoor radon levels. It was found that the differences in mean radon concentrations between adjacent seasons, in a number of 61 selected sampling sites distributed in 28 houses, were statistically significant. As expected, a maximum was found in winter and a minimum in summer. The differences in mean radon concentration on different floors of the same houses were also statistically significant and followed a linear decrease from underground to 2nd floor. In addition, indoor radon concentrations in the ground floor were found to be influenced by the existence or not of a basement. The average annual radon concentration was found to be 41 Bq m(-3) for the houses, 28 Bq m(-3) for the apartments and 38 Bq m(-3) for all the dwellings. These values lead to an average effective dose equivalent of 1.1, 0.7 and 0.9 mSv y(-1), respectively. Residents living on the underground in low-rise houses, during winter, where the average effective dose equivalent is 2.1 mSv y(-1), attain the higher risk.     

Comparative studies of health hazard from radon (Rn-222) in two selected lithologic formations in the Suwałki region (in Poland)

The aim of this work was to make a comparison of indoor radon concentrations in dwellings and in soil air in the area of two geological formations in the Suwa?ki region (Poland). The mean arithmetic airborne concentration was found to be the highest (301 Bq m (-3)) in the basements of buildings in the gravel and sand areas, whereas in the boulder clay areas it reached 587 Bq m (-3). Out of 54 measurements of radon concentrations performed at the ground floor, in eight cases concentrations were found to exceed 200 Bq m (-3) - permissible radon level in new-built houses in Poland and in three cases these values were even higher than 400 Bq m (-3). The highest radon levels were noted in houses with earthen basement floors and with direct entrance from the basement to rooms or kitchens. The mean arithmetic radon concentration in the soil air in the sandy and gravel formations was 39.7 kBq m (-3) and in clay formation it was 26.5 kBq m (-3). Higher radon levels were also found in the water obtained from household wells reaching 8367 Bq m (-3) as compared with tap water (2690 Bqm (-3)). The mean indoor concentration for the whole area under study was found to be 169.4 Bq m (-3), which is higher than the mean value for Poland (49.1 Bq m (-3)) by a factor of 3.5.     

High natural radiation exposure in radon spa areas: a detailed field investigation in Niska Banja (Balkan region)

The measurement campaigns have been done in the rural community of Niska Banja, a spa town located in southern Serbia, to evaluate population exposure to natural radioactivity. After a screening survey in 200 houses, annual radon and thoron concentrations were measured in 34 houses, and in 2004 a detailed investigation was carried out at six houses with elevated indoor radon concentrations. The paper presents the results of these detailed measurements. The complementary techniques were applied to determine radon and thoron concentrations in indoor air, in soil gas, radon exhalation from soil, soil permeability, and indoor and outdoor gamma doses. Soil and water samples were collected and analysed in the laboratory. Indoor radon and thoron concentrations were found to be more than 1kBqm(-3) and 200Bqm(-3), respectively. Extremely high concentrations of soil-gas radon (>2000kBqm(-3)) and radon exhalation rates (1.5mBqm(-2)s(-1)) were observed. These results will be utilised to set up the methodology for a more systematic investigation.     

Measurements of summer radon and its progeny concentrations along with environmental gamma dose rates in Taiwan

The concentrations of 222Rn (radon) and its progeny with surrounding environmental gamma-dose rates were measured simultaneously inside and outside of buildings at 10 locations around Taipei and Hualien in Taiwan. For summer radon in Taiwan, indoor concentrations were estimated to be about 20 Bq m(-3) with about 90 nSv h- of environmental gamma, and outdoors, about 10 Bq m(-3) with about 70 nSv h(-1). The equilibrium factors were calculated to be 0.2-0.3 indoors and 0.3-0.4 outdoors. Indoor radon concentration had a weak positive correlation with gamma-dose rate. Since there is a possibility that high radon concentrations exist indoors during the cool season in Taiwan because of extremely low ventilation rates in the dwellings, a winter survey in January through February will be needed for future estimation of the annual effective dose.     

Seasonal changes in radon concentrations in buildings in the region of northeastern Poland

In this study, seasonal observations of radon concentration changes inside buildings carried out in the northeastern region of Poland is presented. One-year measurements of radon concentrations were performed in chosen buildings. The integral method of Cr-39 trace detectors in diffusive chambers was used. Mean values of radon concentrations were determined in monthly, 2-, 3-, 6-month, and annual observations. The fraction of a mean annual concentration of the value obtained in a shorter observation was calculated. Monthly concentration values were from about 0.2 to 14.9 of the annual mean. All buildings revealed seasonal fluctuation of radon concentration. Negative correlation of indoor radon concentration in the buildings and the mean temperature outside was observed in most examined buildings. The lowest coefficient range, determining which part of the annual mean value would be obtained in the 6-month observation, was gained for exposure begun in April or October.     

Variations in the concentration of radon in parts of the Ogof Ffynnon Ddu system, Penwyllt, South Wales and estimates of doses to recreational cavers.

A new winter and summer investigation of radon concentrations in parts of the Ogof Ffynnon Ddu system at Penwyllt, South Wales, has been carried out using 100 environmental National Radiological Protection Board track etch detectors. Fifty detectors were installed in the system in December 1998 and again in August 1999 for a period of a month. The data obtained confirm that the system has moderately high radon concentrations with a system mean of 2318 Bq m(-3) in winter and 2844 Bq m(-3) in summer. Traverse means have a summer high of 3094 Bq m(-3) for OFDI to Cwm Dwr and a winter low of 1946 Bq m(-3). The extremely high concentrations approaching 20,000 Bq m(-3), reported previously from the system (Hyland, 1995), have not been reproduced. The data show that the airflow directions at the entrances are not what might have been predicted. Air appears to be largely continuously emerging from the lowest entrance but, at the higher entrances, conversely to the predictions, in winter air enters and in summer appears to be coming out or is variable. Internally, there are sites that in winter have very low radon concentrations that can only be explained by the ingress of fresh air. These are not matched in the summer experiment, again indicating that ingress of fresh air to some parts of the system is very variable. The data illustrate the complexity of airflow within a multi-entrance system but behind these variations several mean concentrations can be obtained from which an approximation of the dose likely to be received can be calculated. Using the maximum mean concentration obtained, 3094 Bq m(-3), and using the latest dose conversion, a 10 h underground trip in the Ogof Ffynnon Ddu system yields a calculated dose of 0.12 mSv. Given that the recommended limit for a member of the public is 1 mSv, this dose would be reached after about 80 h of caving in the system.     

Long period study of outdoor radon concentration in Milan and correlation between its temporal variations and dispersion properties of atmosphere

The results of a survey of outdoor radon concentrations in Milan are reported. Measurements were performed hourly over a continuous four year period from January 1997 to December 2000. Radon concentration was obtained by two means: both direct measurement of radon; and measurement of its decay products. The average daily pattern of radon concentration featured a minimum in the late afternoon and a maximum in the early hours of the morning. A seasonal pattern with higher concentrations in winter than in summer (from around 15 Bq m(-3) in winter to around 5 Bq m(-3) in summer) was also observed. Similar average annual values of around 10 Bq m(-3) were obtained. The annual effective outdoor radon dose was found to be 0.12 mSv. The variation from minimum in the afternoon to maximum the following morning was found to be a good indicator of the height of the nocturnal mixing layer. The variation between maximum and minimum levels on the same day is an index of the maximum height of the mixing layer. Furthermore, our long term measurements of radon have permitted us to examine the dispersion characteristics of the atmosphere over Milan, and to establish the frequency of conditions unfavourable to the dispersion of atmospheric pollutants.     

Radon concentration in hospital buildings erected during the last 40 years in Białystok, Poland

The aim of the study was to compare radon concentrations in neighbouring hospital buildings which were constructed in different years during the period 1963-2000 and are located in areas with similar radon potential. The value of arithmetic mean (AM) radon concentration in soil gas amounted to 14,464 Bq m(-3). In a hospital built 40 years ago, the AM radon concentration in the cellar was 38.4+/-36.7 Bq m(-3) and on higher levels it was 17.1+/-10.3 Bq m(-3). In a hospital built 16 years ago, these values equaled 45.5+/-47.2 Bq m(-3) and 20.4+/-12.5 Bq m(-3), respectively. In the newest hospital, built three years ago, radon concentration (AM) in a cellar was 32.3+/-27.4 Bq m(-3) and the respective value on higher levels amounted to 20.4+/-12.6 Bq m(-3). When comparing radon concentrations in the cellars, no statistically significant differences were found. Similarly, no statistically significant differences were observed between radon concentrations measured on higher levels in investigated hospital buildings.     

Radon levels in Cyprus

Radon levels in atmospheric and aquatic systems in Cyprus have recently been measured using the radon monitor Alpha Guard. Indoor and outdoor radon levels were obtained in situ, whereas analysis of radon concentrations in water was performed using tap and ground water samples collected from several areas of the island. The average value for outdoor and indoor radon concentration is 11+/-10 and 7+/-6 Bq m(-3), respectively, and for tap and ground water 0.4 Bq l(-1) and 1.4 Bq l(-1), respectively. From these data the annual dose equivalent of airborne radon to the Cypriot population is about 0.19 mSv y(-1), which is quite low compared to the total dose equivalent of natural and man-made ionising radiation in Cyprus. Radon levels in aquatic systems are relatively low due to an exhaustive utilisation of ground water resources and also to the increased input of desalinated sea water in the water distribution network and eventually into the ground water reservoirs.     

Measurements of indoor radon concentrations in the Santiago de Compostela area

Galician soils are among those with the highest (222)Rn exhalation rates in Spain. A year-round study of the indoor (222)Rn concentration in buildings in the Santiago de Compostela area (Galicia, Northwest of Spain) was performed. The study is based on systematic samplings with active charcoal canisters, following a modified EPA 520/5-87-005 protocol. These measurements were complemented by others obtained using etched track dosimeters. Each data set follows a log-normal distribution, with a geometric mean of (253+/-3)Bqm(-3) for charcoal canisters and (285+/-2.5)Bqm(-3) for etched track detectors. After correcting for the different measuring conditions, the mean value of both methods differed by only 2%. A careful analysis of the seasonal dependence of our measurements did not reveal any significant seasonal variations in the (222)Rn concentration. Parallel to these measurements, different meteorological parameters were recorded, which revealed a direct correlation between the indoor radon concentration and the outdoor temperature derivative with respect to time.     

Spatiotemporal variation of radon and carbon dioxide concentrations in an underground quarry: coupled processes of natural ventilation, barometric pumping and internal mixing

Radon-222 and carbon dioxide concentrations have been measured during several years at several points in the atmosphere of an underground limestone quarry located at a depth of 18 m in Vincennes, near Paris, France. Both concentrations showed a seasonal cycle. Radon concentration varied from 1200 to 2000 Bq m⁻³ in summer to about 800-1400 Bq m⁻³ in winter, indicating winter ventilation rates varying from 0.6 to 2.5 × 10⁻⁶ s⁻¹. Carbon dioxide concentration varied from 0.9 to 1.0% in summer, to about 0.1-0.3% in winter. Radon concentration can be corrected for natural ventilation using temperature measurements. The obtained model also accounts for the measured seasonal variation of carbon dioxide. After correction, radon concentrations still exhibit significant temporal variation, mostly associated with the variation of atmospheric pressure, with coupling coefficients varying from −7 to −26 Bq m⁻³ hPa⁻¹. This variation can be accounted for using a barometric pumping model, coupled with natural ventilation in winter, and including internal mixing as well. After correction, radon concentrations exhibit residual temporal variation, poorly correlated between different points, with standard deviations varying from 3 to 6%. This study shows that temporal variation of radon concentrations in underground cavities can be understood to a satisfactory level of detail using non-linear and time-dependent modelling. It is important to understand the temporal variation of radon concentrations and the limitations in their modelling to monitor the properties of natural or artificial underground settings, and to be able to assess the existence of new processes, for example associated with the preparatory phases of volcanic eruptions or earthquakes.     

The practical use of electrets in a public health radon remediation campaign

As part of a long-term assessment of domestic radon in Northamptonshire, England, a batch of 50 commercially available electrets was deployed for nearly 1,000 exposures, individual exposure periods ranging from one to eight weeks. Responsivity was comparable with that of recently-calibrated Durridge RAD-7 continuously-monitoring equipment. Voltage history analysis indicated mean voltage decay during manufacturers' QA assessment of 0.059+/-0.026 Vday(-1), increasing to 0.114+/-0.073 Vday(-1) during storage to first use and to 0.204+/-0.49 Vday(-1) during inter-deployment storage. At a representative elevated radon concentration of 500 Bqm(-3), the resulting perturbation is 3% over a 7-day deployment; at the typical mean Northamptonshire level of 80 Bqm(-3) it approaches 22%. Each electret can be used for up to 25 measurements, which makes the technology attractive for organisational use. It is not suited for deployment by individual householders.     

Radon gas distribution in natural gas processing facilities and workplace air environment

Evaluation was made of the distribution of radon gas and radiation exposure rates in the four main natural gas treatment facilities in Syria. The results showed that radiation exposure rates at contact of all equipment were within the natural levels (0.09-0.1 microSvh(-1)) except for the reflex pumps where a dose rate value of 3 microSvh(-1) was recorded. Radon concentrations in Syrian natural gas varied between 15.4 Bq m(-3) and 1141 Bq m(-3); natural gas associated with oil production was found to contain higher concentrations than the non-associated natural gas. In addition, radon concentrations were higher in the central processing facilities than the wellheads; these high levels are due to pressurizing and concentrating processes that enhance radon gas and its decay products. Moreover, the lowest 222Rn concentration was in the natural gas fraction used for producing sulfur; a value of 80 Bq m(-3) was observed. On the other hand, maximum radon gas and its decay product concentrations in workplace air environments were found to be relatively high in the gas analysis laboratories; a value of 458 Bq m(-3) was observed. However, all reported levels in the workplaces in the four main stations were below the action level set by IAEA for chronic exposure situations involving radon, which is 1000 Bq m(-3).     

Evaluation of indoor radon measurements in Hungary

The RAD Laboratory measured annual means of radon activity concentrations in 15 277 first-floor rooms of dwellings and in 325 rooms on upper floors in Hungary (1994-2004). The original purpose of the survey was to find radon-prone area in Hungary. The maximum measured value was 5800 Bq m(-3), while the minimum was 10 Bq m(-3). Due to geological diversity and different structures of buildings, the data set of first-floor rooms did not follow the lognormal distribution. Therefore, strata were chosen so that the measured data fitted the lognormal distribution. The numbers of dwellings above a given radon level were determined in each stratum. The national distribution was then taken as the sum of the individual distributions of all strata. This distribution was not lognormal. The parameters of the best fitting lognormal distribution were GM = 58 Bq m(-3), GSD = 2.2. The weighted averages of strata values GM = 62 Bq m(-3), GSD=2.1 were obtained corresponding to 92% of Hungarian dwellings.     

Seasonal variations of aerosol residence time in the lower atmospheric boundary layer

During a one year period, from Jan. 2002 up to Dec. 2002, approximately 130 air samples were analyzed to determine the atmospheric air activity concentrations of short- and long-lived (222Rn) decay products 214Pb and 210Pb. The samples were taken by using a single-filter technique and gamma-spectrometry was applied to determine the activity concentrations. A seasonal fluctuation in the concentration of 214Pb and 210Pb in surface air was observed. The activity concentrations of both radionuclides were observed to be relatively higher during the winter/autumn season than in spring/summer season. The mean activity concentration of 214Pb and 210Pb within the whole year was found to be 1.4+/-0.27 Bq m(-3) and 1.2+/-0.15 mBq m(-3), respectively. Different 210Pb:214Pb activity ratios during the year varied between 1.78 x 10(-4) and 1.6 x 10(-3) with a mean value of 8.9 x 10(-4) +/- 7.6 x 10(-5). From the ratio between the activity concentrations of the radon decay products 214Pb and 210Pb a mean residence time (MRT) of aerosol particles in the atmosphere of about 10.5+/-0.91 d could be estimated. The seasonal variation pattern shows relatively higher values of MRT in spring/summer season than in winter/autumn season. The MRT data together with relative humidity (RH), air temperature (T) and wind speed (WS), were used for a comprehensive regression analysis of its seasonal variation in the atmospheric air.     

Radon-222 signatures of natural ventilation regimes in an underground quarry

Radon-222 activity concentration has been monitored since 1999 in an underground limestone quarry located in Vincennes, near Paris, France. It is homogeneous in summer, with an average value of 1700 Bq m(-3), and varies from 730 to 1450 Bq m(-3) in winter, indicating natural ventilation with a rate ranging from 0.5 to 2.4 x 10(-6) s(-1) (0.04-0.22 day(-1)). This hypothesis is supported by measurements in the vertical access pit where, in winter, a turbulent air current produces a stable radon profile, smoothly decreasing from 700 Bq m(-3) at 20 m depth to 300 Bq m(-3) at surface. In summer, a thermal stratification is maintained in the pit, but the radon-222 concentration jumps repeatedly between 100 and 2000 Bq m(-3). These jumps are due to atmospheric pressure pumping, which induces ventilation in the quarry at a rate of about 0.1 x 10(-6) s(-1) (0.009 day(-1)). Radon-222 monitoring thus provides a dynamical characterisation of ventilation regimes, which is important for the assessment of the long-term evolution of underground systems.     

The distribution of radon in tunnels with different geological characteristics in China

In China, as the economy is developing and the population is expanding, some underground buildings have been used as supermarkets, restaurants and entertainment places. Tunnels in mountains are one type of underground building, and the radon (²²²Rn) level in tunnels is an important issue. Radon levels in different type tunnels appear to differ, and relatively higher levels of ²²²Rn are associated with particular types of bedrock. The ²²²Rn levels in tunnels in five different geological characteristics were analyzed. Those built in granite had the highest ²²²Rn levels with a geometric mean (GM) of 280 Bq m⁻³, while those built in limestone (GM: 100 Bq m⁻³) and andesitic porphyry (GM: 96 Bq m⁻³) were lower. The sequence of ²²²Rn concentrations was: granite > tuff > quartz sandstone > limestone > andesitic porphyry, and the ²²²Rn in granite was statistically significantly higher than in limestone and andesitic porphyry. Tunnels built in granite, tuff, quartz sandstone, limestone tended to have higher ²²²Rn concentrations in summer than in winter, while the reverse tendency was true in andesitic porphyry tunnels. Only the difference in limestone was statistically significant.