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1.
The main objective of this work was to quantify and characterize the major indoor air contaminants present in different stages of a municipal WWTP, including microorganisms (bacteria and fungi), carbon dioxide, carbon monoxide, hydrogen sulfide ammonia, formaldehyde, and volatile organic compounds (VOCs). In general, the total bacteria concentration was found to vary from 60 to >52,560 colony-forming units (CFU)/m3, and the total fungi concentration ranged from 369 to 14,068 CFU/m3. Generally, Gram-positive bacteria were observed in higher number than Gram-negative bacteria. CO2 concentration ranged from 251 to 9,710 ppm, and CO concentration was either not detected or presented a level of 1 ppm. H2S concentration ranged from 0.1 to 6.0 ppm. NH3 concentration was <2 ppm in most samples. Formaldehyde was <0.01 ppm at all sampling sites. The total VOC concentration ranged from 36 to 1,724 μg/m3. Among the VOCs, toluene presented the highest concentration. Results point to indoor/outdoor ratios higher than one. In general, the highest levels of airborne contaminants were detected at the primary treatment (SEDIPAC 3D), secondary sedimentation, and sludge dehydration. At most sampling sites, the concentrations of airborne contaminants were below the occupational exposure limits (OELs) for all the campaigns. However, a few contaminants were above OELs in some sampling sites.  相似文献   

2.
The aims of the present study were to determine the levels of bioaerosols including airborne culturable bacteria (total suspended bacteria, Gram-positive bacteria, Staphylococcus, Staphylococcus aureus, methicillin-resistant S. aureus (MRSA), and Gram-negative bacteria), fungi, endotoxin, and viruses (influenza A, influenza B, respiratory syncytial virus types A/B, parainfluenza virus types 1/2/3, metapnemovirus, and adenovirus) and their seasonal variations in indoor air of residential apartments. Of the total suspended bacteria cultured in an indoor environment, Staphylococcus was dominant and occupied 49.0 to 61.3 % of indoor air. Among Staphylococcus, S. aureus were detected in 100 % of households' indoor air ranging from 4 to 140 CFU/m3, and 66 % of households were positive for MRSA ranging from 2 to 80 CFU/m3. Staphylococcus and S. aureus concentrations correlated with indoor temperature (adjusted β: 0.4440 and 0.403, p?<?0.0001). Among respiratory viruses, adenovirus was detected in 14 (14 %) samples and influenza A virus was detected in 3 (3 %) samples regarding the indoor air of apartments. Adenovirus concentrations were generally higher in winter (mean concentration was 2,106 copies/m3) than in spring (mean concentration was 173 copies/m3), with concentrations ranging between 12 and 560 copies/m3. Also, a strong negative correlation between adenovirus concentrations and relative humidity in indoor air was observed (r?=??0.808, p?<?0.01). Furthermore, temperature also negatively correlated with adenovirus concentrations (r?=??0.559, p?<?0.05).  相似文献   

3.
This study was designed to evaluate the measuring range and lowest limit of detection of Bacillus endospores in the ambient room air when the Sartorius MD8 sampler, and two different culture methods for bacterial enumeration were used. Different concentrations of bioaerosol were generated inside the test chamber filled with either the high-efficiency particulate air (HEPA)-filtered air or with the ambient room air. The detection of endospores in the HEPA-filtered air was achievable: (1) when they were aerosolized at a concentration above 7.56?×?103 CFU/m3 and analyzed with spread plate method, and (2) when they were aerosolized at a concentration above 4.00?×?102 CFU/m3 and analyzed with pour plate method. The detection of endospores in the ambient room air was possible: (1) when they were aerosolized at a concentration above 9.1?×?103 CFU/m3 and analyzed with spread plate method, and (2) when they were aerosolized at a concentration above 5.6?×?102 CFU/m3 and analyzed with pour plate method. The microorganisms present in the ambient room air interfere with precise quantification of Bacillus endospores when their concentration is relatively low. The results of this study may be helpful in critical assessment of the results obtained from monitoring the air for bacterial endospores.  相似文献   

4.
A novel and robust method for the simultaneous determination of lead, cadmium, arsenic, and nickel in atmospheric particulate matter by multi-element electrothermal atomic absorption spectrometry was developed, using zirconium–iridium coating as permanent modifier (140 μg Zr and 4 μg Ir). After 300 atomization cycles, it was necessary to add 2 μg of Ir. Due to the varying concentrations of Pb in atmospheric particulate matter, lead was monitored at two wavelengths, at the less sensitive line of 261.4 nm for high concentration samples (>20 μg?L?1) or at 283.3 nm for the low concentration samples. Matrix-matched calibration had to be performed for quantitative recoveries (96–102 %). Following this approach, the four elements were determined in atmospheric particulate matter samples from an industrial area near the city of Athens in two different time periods (cold–warm) with limits of detection of 5.5 ng?m?3 for Pb at 261.4 nm and 0.29 ng?m?3 at 283.3 nm, 0.019 ng?m?3 for Cd, 0.14 ng?m?3 for As, and 0.22 ng?m?3 for Ni. Lead, Cd, and As levels were very low, whereas Ni content was at comparable levels with other areas worldwide.  相似文献   

5.
Airborne bacteria emissions from oxidation ditch with rotating aeration brushes were investigated in a municipal wastewater treatment plant in Beijing, China. Microbial samples were collected at different distances from the rotating brushes, different heights above the water surface, and different operation state over a 3-month period (April, May, and June) in order to estimate the seasonal variation and site-related distribution characteristics of the microorganisms present. The concentration of bacterial aerosol was analyzed by culture methods, while their dominant species, genetic structure and diversity were assayed using bio-molecular tools. Results showed that total microbial concentrations were highest in June and lowest in April. The mechanical rotation caused remarkable variation in concentration and diversity of culturable airborne bacteria before and after the rotating brushes. The highest concentration was observed near the rotating brushes (931?±?129–3,952?±?730 CFU/m3), with concentration decreasing as distance and height increased. Bacterial community polymerase chain reaction and denaturing gradient gel electrophoresis indicated that diversity decreased gradually with increasing height above the water surface but remained relatively constant at the same height. All dominant bacteria identified by DNA sequence analysis belonged to Firmicutes. Pathogenic species such as Moraxella nonliquefaciens and Flavobacterium odoratum were isolated from the bioaerosols. Due to the serious health risks involved, exposure of sewage workers to airborne microorganisms caused by brush aerators should be monitored and controlled.  相似文献   

6.
Delhi is one of the most polluted cities in the world. The generation of aerosols in the lower atmosphere of the city is mainly due to a large amount of natural dust advection and sizable anthropogenic activities. The compositions of organic compounds in aerosols are highly variable in this region and need to be investigated thoroughly. Twenty-four-hour sampling to assess concentrations of n-alkanes (ng/m3) in PM10 was carried out during January 2015 to June 2015 at Indira Gandhi Delhi Technical University for Women (IGDTUW) Campus, Delhi, India. The total average concentration of n-alkanes, 243.7 ± 5.5 ng/m3, along with the diagnostic tools has been calculated. The values of CPI1, CPI2, and CPI3 for the whole range of n-alkanes series, petrogenic n-alkanes, and biogenic n-alkanes were 1.00, 1.02, and 1.04, respectively, and C max were at C25 and C27. Diagnostic indices and curves indicated that the dominant inputs of n-alkanes are from petrogenic emissions, with lower contribution from biogenic emissions. Significant seasonal variations were observed in average concentrations of n-alkanes, which is comparatively higher in winter (187.4 ± 4.3 ng/m3) than during the summer season (56.3 ± 1.1 ng/m3).  相似文献   

7.
The soils at a factory for manufacturing pentachlorophenol were heavily contaminated by polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs). In order to verify the contributions of dry and wet deposition of PCDD/Fs from the ambient air, the concentration of PCDD/Fs in ambient air and soil were measured, the partition of particle- and gas-phases of atmospheric PCDD/Fs was calculated, and the annual fluxes of total dry and wet PCDD/F depositions were modeled. Average atmospheric PCDD/F concentration was 1.24 ng Nm???3 (or 0.0397 ng I-TEQ Nm???3). Moreover, over 92.8% of total PCDD/Fs were in the particle phase, and the dominant species were high chlorinated congeners. The total PCDD/F fluxes of dry and wet deposition were 119.5 ng m???2 year???1 (1.34 ng I-TEQ m???2 year???1) and 82.0 ng m???2 year???1 (1.07 ng I-TEQ m???2 year???1), respectively. By scenario simulation, the total fluxes of dry and wet PCDD/F depositions were 87.1 and 68.6 ng I-TEQ, respectively. However, the estimated PCDD/F contents in the contaminated soil were 839.9 ?? g I-TEQ. Hence, the contributions of total depositions of atmospheric PCDD/F were only 0.02%. The results indicated that the major sources of PCDD/F for the contaminated soil could be attributed to the pentachlorophenol manufacturing process.  相似文献   

8.
An investigation to find out presence of particulate matter in Marikana, a mining area in Rustenburg town, South Africa, was carried out in the months of August and November of 2008. Samples were collected for measurements of particulate matter (PM) of particle diameters of PM10, PM2.5, and PM1. After gravimetric analysis of daily measurements, it was found that PM10 concentration values ranged between 3 and 9 ??g/m3, PM2.5 concentration values ranged between 16 and 26 ??g/m3, and PM1 concentration values ranged between 14 and 18 ??g/m3 for the month of August 2008. For the month of November, it was found that PM10 concentration values ranged between 2 and 8 ??g/m3, PM2.5 concentration values ranged between 0 and 5 ??g/m3, and PM1 concentration values ranged between 4 and 15 ??g/m3. This study was undertaken as preliminary work having in mind that mining activities could be emitting high levels of particulate matter in the atmosphere which might be degrading the quality of the air. It was observed, however, that the daily particulate matter especially of PM10 emitted were quite low when compared to laid down International Air Quality Standards. The standards did not give guidelines for particulate matter of diameter 2.5 ??m. It was concluded that particulate matter came from three major sources: platinum mining, domestic biomass burning, and traffic emissions due to fuel burning.  相似文献   

9.
Indoor air quality in health care facilities is a major public health concern, particularly for immunocompromised patients who may be exposed to microbiological contaminants such as molds, mycotoxins, endotoxins, and (1,3)-ß-D-glucans. Over 2 years, bioaerosols were collected on a monthly basis in a cancer treatment center (Centre F. Baclesse, Normandy, France), characterized from areas where there was no any particular air treatment. Results showed the complexity of mycoflora in bioaerosols with more than 100 fungal species identified. A list of major strains in hospital environments could be put forward due to the frequency, the concentration level, and/or the capacity to produce mycotoxins in vitro: Aspergillus fumigatus, Aspergillus melleus, Aspergillus niger, Aspergillus versicolor, Cladosporium herbarum, Purpureocillium lilacinum, and Penicillium brevicompactum. The mean levels of viable airborne fungal particles were less than 30.530 CFU per m3 of air and were correlated to the total number of 0.30 to 20 μm particles. Seasonal variations were observed with fungal particle peaks during the summer and autumn. Statistical analysis showed that airborne fungal particle levels depended on the relative humidity level which could be a useful indicator of fungal contamination. Finally, the exposure to airborne mycotoxins was very low (only 3 positive samples), and no mutagenic activity was found in bioaerosols. Nevertheless, some fungal strains such as Aspergillus versicolor or Penicillium brevicompactum showed toxigenic potential in vitro.  相似文献   

10.
Airborne lead levels were assessed in nine workshops, three each from battery, electronic repair, and welding sources within the Kumasi Metropolis in Ghana. Samples were collected at 0, 2.5, and 5.0 m away from the emission source at the workshops during working hours and another at 5.0 m during break hours. Airborne lead particulates were collected and analyzed using the filter membrane technique and flame atomic absorption spectrophotometry, respectively. There were significant differences (p ≤ 0.05) among the air lead levels from the workshops. Workshop 3b produced the highest significant values of air lead concentrations of 2,820.31 ± 53.89, 2,406.74 ± 71.87, 754.55 ± 72.52, and 549.01 ± 67.30 μg/m3 at distances of 0, 2.5, 5.0, and 5.0 m (break-time measurement), respectively, while workshop 1w significantly produced the lowest air lead concentration values of 261.06 ± 21.60, 190.92 ± 36.90, 86.43 ± 16.26, and 61.05 ± 3.88 μg/m3 at distances of 0, 2.5, 5.0, and 5.0 m (break-time measurement), respectively. The air lead levels reduced with distance from emission source at the workshops. At all the distances of measurement at working hours, the airborne lead levels were higher than the World Health Organization standard of 50 μg/m3 and exceeded the threshold limit values of 100 to 150 μg/m3 recommended in most jurisdictions. Workers and people in the immediate environs were exposed to air lead levels that were too high by most international standards, thus posing a serious threat to their health.  相似文献   

11.
In this study, we measured the mercury concentration in 27 different fish species with high commercial value. Samples were taken from a region characterized by the diversity of aquatic environments. Mercury concentration in marine fish species varied from 30.4 to 216 ng g???1, while in estuarine species, it varied from 12.4 to 60.3 ng g???1. Compared to mercury concentration in marine species, none of the specimens from estuarine environment has reached a mercury concentration of 100 ng g???1. However, mercury concentrations in species from the freshwater Patos lagoon are remarkably higher (15.3 to 462 ng g???1) than those from the estuarine or marine region. Even though mercury concentrations in these fish species did not exceed the maximum level (500 ng g???1) allowed by WHO for human consumption, they represent the main food source for sea birds and mammals coming from South Pole during their migration period.  相似文献   

12.
Airborne particulates (PM10) from four different areas within Agra city (a semi-arid region) were collected using respirable dust samplers during the winter season (Nov. 2005–Feb 2006) and were then extracted with methylene chloride using an automated Soxhlet Extraction System (Soxtherm®). The extracts were analyzed for 17 target polycyclic aromatic hydrocarbons (PAHs) and the heterocycle carbazole. The average concentration of total PAH (TPAH) ranged from 8.04 to 97.93 ng m???3. The industrial site had the highest TPAH concentration followed by the residential, roadside, and agricultural sites. Indeno(1,2,3-cd)pyrene, benzo(g,h,i)perylene, and benzo(b)fluoranthene were the predominant compounds found in the samples collected from all of the sites. The average B(a)P-equivalent exposure, calculated by using toxic equivalent factors derived from literature and the USEPA, was approximately 7.6 ng m???3. Source identification using factor analysis identified prominent three, four, four, and four probable factors at industrial, residential, roadside, and agricultural sites, respectively.  相似文献   

13.
A dense monitoring network is vital for the reliable assessment of PM10 in different parts of an urban area. In this study, a new idea is employed for the re-construction of the 20 shut-down PM10 monitoring stations of Berlin. It endeavours to find the non-linear relationship between the hourly PM10 concentration of both the still operating and the shut-down PM10 monitoring stations by using a fuzzy modelling technique, called modified active learning method (MALM). In addition, the simulations were performed by using not only raw PM10 databases but also log-transformed PM10 databases for skewness reduction. According to the results of hourly PM10 simulation (root mean square error about 13.0 μg/m3, correlation coefficient 0.88), the shut-down stations have been appropriately simulated and the idea of dense monitoring network development by the re-construction of the shut-down stations was realised. The results of simulations using raw and log-transformed databases showed that data transformation has no significant effect on the performance of MALM in the simulation of shut-down PM10 stations. By the combination of the 11 still operating stations and the 20 re-constructed stations, a dense monitoring network was generated for Berlin and was utilised for the calculation of the reliable monthly and mean annual PM10 concentration for five different PM10 zones in Berlin (the suburban-background, urban-background, urban-traffic, rural-background and suburban-traffic areas). The results showed that the mean annual concentration of PM10 at the five zones increased by about 13.0% in 2014 (26.3 μg/m3) in comparison with 2013 (23.3 μg/m3). Furthermore, the mean annual concentration of PM10 in the traffic lanes of the suburban (2013 25.0 μg/m3, 2014 26.9 μg/m3) and urban (2013 27.7 μg/m3, 2014 31.3 μg/m3) areas is about 14 and 20% higher than the PM10 concentration of suburban-background (2013 21.3 μg/m3, 2014 24.5 μg/m3) and urban-background (2013 23.0 μg/m3, 2014 26.1 μg/m3) areas, respectively.  相似文献   

14.
We assessed the incidence of faecal-indicator bacteria in Tyume River over a 12-month period between August 2010 and July 2011. Total coliforms, faecal coliforms and enterococci were determined by the membrane filtration method. Total coliforms were detected in counts ranging from 2.1?×?102 to 3.4?×?104?CFU/100 ml. Faecal coliform counts ranged from 1?×?102 to 1.6?×?104?CFU/100 ml while enterococci counts were in the range of 3.3?×?101 to 5.1?×?103?CFU/100 ml. Indicator bacteria counts increased from upstream to downstream sampling sites. Counts of indicator bacteria at all sites were significantly affected by seasonal changes. The bacteriological qualities of the river water were poor, exceeding the guideline of 200 CFU/100 ml and 33 CFU/100 ml for faecal coliforms and enterococci, respectively, for recreational water. Faecal coliform counts also exceeded the 1,000 CFU/100 ml guideline for water used in fresh produce irrigation. Microbial source tracking results showed that faecal pollution was predominantly of human origin during spring at all sampling sites. During other seasons, human faecal pollution was largely confined to midstream and downstream sampling sites. Generally, the presence of faecal-indicator bacteria in the river water samples suggests faecal pollution of this freshwater resource, raising the possibility of the presence of pathogenic microorganisms in the water and a threat to public health.  相似文献   

15.
The metal concentrations of As, Be, Cr, Hg, Mn, and Ni in ambient air were measured at four sites in Japan from October 1997 to March 2006. The mean metal concentration data measured from the four sites (K1, K2, M, and Y) are found on the order of Mn > Cr–Ni > As > Hg > Be. The concentrations of Mn with the highest mean value were fairly variable across four sites such as 45.9 ± 42.8 (K1), 25.6 ± 19.4 (K2), 22.5 ± 19.7 (M), and 25.4 ± 19.8 ng m???3 (Y). In contrast, the concentrations of Be with the lowest mean value were less variable across four sites with means of 0.03 to 0.04 ng m???3. Inspection of the seasonal patterns indicates the peak occurrence of most metals during spring, although relative dominance during winter is seen at the most polluted area (K1). Evaluation of long-term patterns indicates that the noticeably high values of metals in the early stage of study reduced gradually across the years, although the metal concentration levels in most areas were affected significantly by anthropogenic activities. However, efforts to control pollution levels seemed to gradually contribute to a decrease in metal concentration levels of all study sites through the years.  相似文献   

16.
We characterize the monthly variation in (1 → 3)-β-d-glucan concentration measured over the course of 1 year, and we evaluate the characteristics of size selection using a two-stage cyclone sampler. The (1 → 3)-β-d-glucan concentrations were measured in four bio-related laboratories. A total of 156 samples were collected using a new two-stage cyclone sampler. Analysis of (1 → 3)-β-d-glucan was performed using the kinetic Limulus amebocyte lysate assay. The study showed that airborne (1 → 3)-β-d-glucan concentrations were significantly higher in laboratory D (mean ± SD 1,105?±?1,893 pg/m3) and in the spring (5,458 pg/m3). The highest concentration of (1 → 3)-β-d-glucan occurred in the spring, particularly in May.  相似文献   

17.
In this work, a numerical model is proposed to estimate air concentration of released airborne radioactive contaminants 131I and 137Cs. A Gaussian dispersion model is used to assess the atmospheric dispersion of radioactive contaminants released continuously from a nuclear power plant as a result of an accident. The model uses various input parameters such as source height, release rate, stability class, wind speed, and wind direction. The validation of the model was carried out by comparing its predicted values with published experimental data. The model was extensively tested by simulating several accidental situations. The main conclusion drawn from these tests is that for large downwind distances from the release point, the contaminant concentrations predicted by the model diverge drastically from measured data, while for short distances, the predicted values generally agree quite well with experimental data. The obtained activity concentrations range from 1.57?×?102 to 6.43?×?103 Bq/m3 for 131I and from 3.18?×?10?2 to 9.72?×?102 Bq/m3 for 137Cs. The estimated standard deviation coefficients values range of 7.2 to 6847.7 m, and the maximum absolute error predicted by the model for these parameters was less than 5%.  相似文献   

18.
The HOBAS aeration system was tested to compare changes in environmental and bacteriological parameters in ponds growing Penaeus monodon during a single production cycle. The stocking density in the aerated pond was doubled to 12 post-larvae (PL) m???2 in contrast to the non-aerated pond with 6 (PL) m???2. Microbial abundance in the ponds ranged between 105???6 cells ml???1. Among the physiological groups of bacteria enumerated, the heterotrophs dominated with an abundance of 104 CFU ml???1. Of the nitrogen and sulfur cycle bacteria, the nitrifiers flourished in the aerated pond and could maintain ammonia-N concentration within permissible levels. Bacterial activity also maintained sulfide concentrations at <?0.03 mg l???1. Non-aerated conditions promoted denitrification maintaining nitrate concentration between 0.32 and 0.98 μM NO3 ???-N l???1. However, a marked increase in ammonium content was observed in the non-aerated pond at the end of the culture period. Thus in high-density ponds, the aerators served to stimulate bacterial growth and activity which consequently maintained the quality of the water to match that of low-density ponds. Accordingly, these aerators could be effectively used to sustain higher yields. The effluent from the aerated pond is less likely to alter the redox balance of the receiving waters.  相似文献   

19.
Polycyclic aromatic hydrocarbons (PAHs) are organic pollutants derived from pyrolysis and pyrosynthesis processes. Industrial activity, motor vehicle emission, and domestic combustion are the main sources of PAHs in the urban atmosphere. In this work, samples collected during the day and night in the urban area of Sarajevo are analyzed separately for gaseous and particle-bound PAHs; the possible origin of PAHs at the receptor site was suggested using different methods applied to the solid phase and to the total PAHs (gaseous + particulate phase). Finally, the risk level in Sarajevo associated to the carcinogenic character of the studied PAHs has been assessed. The result of this study suggests that (a) the total PAH concentrations were higher than those reported in other European cities; (b) the PAH daytime concentrations are higher than nocturnal concentrations: the sum of the PAH day/night ratios is 1.52 (gas) and 1.45 (particle phase); (c) stationary combustion and traffic were suggested to be the main sources of PAHs; (d) the average particle-bound benzo(a)pyrene (BaP) concentration (5.4 ng/m3) is higher than EU target annual value (1 ng/m3); and (e) PAH cancer risk exceeds the carcinogenic benchmark level recommended by the EPA mainly due to BaP during both the day and night periods.  相似文献   

20.
The relationship between indoor and outdoor particulate air pollution was investigated at an urban background site on the Payambar Azam Campus of Mazandaran University of Medical Sciences in Sari, Northern Iran. The concentration of particulate matter sized with a diameter less than 1 μm (PM1.0), 2.5 μm (PM2.5), and 10 μm (PM10) was evaluated at 5 outdoor and 12 indoor locations. Indoor sites included classrooms, corridors, and office sites in four university buildings. Outdoor PM concentrations were characterized at five locations around the university campus. Indoor and outdoor PM measurements (1-min resolution) were conducted in parallel during weekday mornings and afternoons. No difference found between indoor PM10 (50.1 ± 32.1 μg/m3) and outdoor PM10 concentrations (46.5 ± 26.0 μg/m3), indoor PM2.5 (22.6 ± 17.4 μg/m3) and outdoor PM2.5 concentration (22.2 ± 15.4 μg/m3), or indoor PM1.0 (14.5 ± 13.4 μg/m3) and outdoor mean PM1.0 concentrations (14.2 ± 12.3 μg/m3). Despite these similar concentrations, no correlations were found between outdoor and indoor PM levels. The present findings are not only of importance for the potential health effects of particulate air pollution on people who spend their daytime over a period of several hours in closed and confined spaces located at a university campus but also can inform regulatory about the improvement of indoor air quality, especially in developing countries.  相似文献   

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