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1.
A three-dimensional Joint frequency distribution (3DJFD) map of Florida is developed based upon wind rose data available for 10 cities. This map may be used in conjunction with the analytic polar coordinate Gaussian Plume Model or conventional dispersion models to calculate the approximate incremental pollution concentration contours associated with an emission source at any site in Florida. Possible means of generalizing the work to other geographic regions, to stack height altitudes, and to incorporate time dependence are discussed.  相似文献   

2.
Abstract

This paper evaluates the application of dispersion models to estimate near-field pollutant concentrations in two case studies. The Industrial Source Complex Short-Term Model (ISCST3) was evaluated with hexavalent chromium measurements collected within 100 m of two facilities in Barrio Logan, San Diego, CA. ISCST3 provided reasonable estimates for higher pollutant concentrations but underestimated lower concentrations. To understand the observed distribution of concentrations in Barrio Logan, a recently conducted tracer experiment was analyzed. The tracer, sulfur hexafluoride, was released at ambient temperature from an urban facility at the University of California at Riverside, and concentrations were measured within 20 m of the source. Modeling results indicated that Industrial Source Complex–Plume Rise Model Enhancement and American Meteorological Society/U.S. Environmental Protection Agency Regulatory Model–Plume Rise Model Enhancement overestimated high concentrations and underestimated low concentrations. A diagnostic study with a simple Gaussian dispersion model that incorporated site-specific meteorology was used to evaluate model results. This study found that incorporating lateral meandering for nonbuoyant urban plumes in Gaussian dispersion models could improve concentration estimates even when downwash is not considered. Incorporating a meandering component in ISCST3 resulted in improvements in estimating hexavalent chromium concentrations in Barrio Logan. Credible near-source concentration estimates depend on accurate characterization of emissions, onsite micrometeorology, and a method to account for lateral meandering in the near field.  相似文献   

3.
ABSTRACT

A new Gaussian dispersion model, the Plume Rise Model Enhancements (PRIME), has been developed for plume rise and building downwash. PRIME considers the position of the stack relative to the building, streamline deflection near the building, and vertical wind speed shear and velocity deficit effects on plume rise. Within the wake created by a sharp-edged, rectangular building, PRIME explicitly calculates fields of turbulence intensity, wind speed, and streamline slope, which gradually decay to ambient values downwind of the building. The plume trajectory within these modified fields is estimated using a numerical plume rise model. A probability density function and an eddy diffusivity scheme are used for dispersion in the wake. A cavity module calculates the fraction of plume mass captured by and recirculated within the near wake. The captured plume is re-emitted to the far wake as a volume source and added to the uncaptured primary plume contribution to obtain the far wake concentrations.

The modeling procedures currently recommended by the U.S. Environmental Protection Agency (EPA), using SCREEN and the Industrial Source Complex model (ISC), do not include these features. PRIME also avoids the discontinuities resulting from the different downwash modules within the current models and the reported overpredictions during light-wind speed, stable conditions. PRIME is intended for use in regulatory models. It was evaluated using data from a power plant measurement program, a tracer field study for a combustion turbine, and several wind-tunnel studies. PRIME performed as well as or better than ISC/SCREEN for nearly all of the comparisons.  相似文献   

4.
A new Gaussian dispersion model, the Plume Rise Model Enhancements (PRIME), has been developed for plume rise and building downwash. PRIME considers the position of the stack relative to the building, streamline deflection near the building, and vertical wind speed shear and velocity deficit effects on plume rise. Within the wake created by a sharp-edged, rectangular building, PRIME explicitly calculates fields of turbulence intensity, wind speed, and streamline slope, which gradually decay to ambient values downwind of the building. The plume trajectory within these modified fields is estimated using a numerical plume rise model. A probability density function and an eddy diffusivity scheme are used for dispersion in the wake. A cavity module calculates the fraction of plume mass captured by and recirculated within the near wake. The captured plume is re-emitted to the far wake as a volume source and added to the uncaptured primary plume contribution to obtain the far wake concentrations. The modeling procedures currently recommended by the U.S. Environmental Protection Agency (EPA), using SCREEN and the Industrial Source Complex model (ISC), do not include these features. PRIME also avoids the discontinuities resulting from the different downwash modules within the current models and the reported overpredictions during light-wind speed, stable conditions. PRIME is intended for use in regulatory models. It was evaluated using data from a power plant measurement program, a tracer field study for a combustion turbine, and several wind-tunnel studies. PRIME performed as well as or better than ISC/SCREEN for nearly all of the comparisons.  相似文献   

5.
A data set for studying transport and dispersion in complex terrain was collected at the Westvaco Corporation's Luke Mill, located in the Potomac River valley in western Maryland. Meteorological analyses indicate very strong channeling of winds and the presence of strong inversions and wind shears in a shallow layer at the height of the surrounding mountaintops (300 m above the valley floor). Wind velocities observed near the valley floor are unrepresentative of wind velocities at plume height. Observed turbulence intensities at plume height are about twice as large as those observed over flat terrain. Standard stability classification schemes generally underestimate plume dispersion at this site. When high 3-h and 24-h average SO2 concentrations are observed, winds are usually light and an inversion is present. These instances of relatively high concentrations are often associated with periods when the wind shifts direction 180° from up-valley to down-valley or vice versa, and the nearly stagnant polluted air mass blows against the mountainsides.A dispersion model was developed that is Gaussian in form but uses observed meteorological data to the maximum extent possible. For example, observed turbulence intensities at plume height are used to estimate dispersion. Plume impaction on terrain is calculated if the plume height is below a critical height dependent on the Hill Froude number. Evaluation of the model with the full 2-y data set shows that it can estimate the second highest 3-h and 24-h average concentrations (of regulatory significance) with a mean bias of less than 7%.  相似文献   

6.
The only documentation on the building downwash algorithm in AERMOD (American Meteorological Society/U.S. Environmental Protection Agency Regulatory Model), referred to as PRIME (Plume Rise Model Enhancements), is found in the 2000 A&WMA journal article by Schulman, Strimaitis and Scire. Recent field and wind tunnel studies have shown that AERMOD can overpredict concentrations by factors of 2 to 8 for certain building configurations. While a wind tunnel equivalent building dimension study (EBD) can be conducted to approximately correct the overprediction bias, past field and wind tunnel studies indicate that there are notable flaws in the PRIME building downwash theory. A detailed review of the theory supported by CFD (Computational Fluid Dynamics) and wind tunnel simulations of flow over simple rectangular buildings revealed the following serious theoretical flaws: enhanced turbulence in the building wake starting at the wrong longitudinal location; constant enhanced turbulence extending up to the wake height; constant initial enhanced turbulence in the building wake (does not vary with roughness or stability); discontinuities in the streamline calculations; and no method to account for streamlined or porous structures.

Implications: This paper documents theoretical and other problems in PRIME along with CFD simulations and wind tunnel observations that support these findings. Although AERMOD/PRIME may provide accurate and unbiased estimates (within a factor of 2) for some building configurations, a major review and update is needed so that accurate estimates can be obtained for other building configurations where significant overpredictions or underpredictions are common due to downwash effects. This will ensure that regulatory evaluations subject to dispersion modeling requirements can be based on an accurate model. Thus, it is imperative that the downwash theory in PRIME is corrected to improve model performance and ensure that the model better represents reality.  相似文献   


7.
Assimilating concentration data into an atmospheric transport and dispersion model can provide information to improve downwind concentration forecasts. The forecast model is typically a one-way coupled set of equations: the meteorological equations impact the concentration, but the concentration does not generally affect the meteorological field. Thus, indirect methods of using concentration data to influence the meteorological variables are required. The problem studied here involves a simple wind field forcing Gaussian dispersion. Two methods of assimilating concentration data to infer the wind direction are demonstrated. The first method is Lagrangian in nature and treats the puff as an entity using feature extraction coupled with nudging. The second method is an Eulerian field approach akin to traditional variational approaches, but minimizes the error by using a genetic algorithm (GA) to directly optimize the match between observations and predictions. Both methods show success at inferring the wind field. The GA-variational method, however, is more accurate but requires more computational time. Dynamic assimilation of a continuous release modeled by a Gaussian plume is also demonstrated using the genetic algorithm approach.  相似文献   

8.
The performance of a CRSTER equivalent Gaussian plume model (CEQM) is examined using data from the EPRI Plume Model Validation study at the Klncaid, Illinois site. Four-way comparisons are made on the ordered statistics or the cumulative frequency distribution (CFD) of maximum hourly observed and predicted concentrations. Using the uniform random distribution and the lognormal random distribution as simple predictive schemes without any physical context, it Is found that the CEQM predicts a concentration CFD which matches the observed CFD significantly closer than the CFD predicted by the uniform random distribution. The two-parameter lognormal random distribution predicts the concentration CFD better than the CEQM over all concentration ranges; however, the CEQM fits the upper range of the concentration distribution better than the lognormal random distribution,, despite the fact that the predictions are generated using dispersion conditions entirely different from those of the observations. The nature of this ergodicity of distribution is probed by exercising CEQM using randomized input based on the observed frequency distributions of the Input parameters instead of feeding the hour-by-hour model input matched by time into CEQM as is customarily done. The exercise of the model by uncoupling the time linkage in model Input has no systematic effect on the predicted cumulative frequency distribution of concentrations. Only at the highest concentration range (99.5% or higher) do the two sets of predictions begin to diverge.  相似文献   

9.
Air quality models are typically used to predict the fate and transport of air emissions from industrial sources to comply with federal and state regulatory requirements and environmental standards, as well as to determine pollution control requirements. For many years, the U.S. Environmental Protection Agency (EPA) widely used the Industrial Source Complex (ISC) model because of its broad applicability to multiple source types. Recently, EPA adopted a new rule that replaces ISC with AERMOD, a state-of-the-practice air dispersion model, in many air quality impact assessments. This study compared the two models as well as their enhanced versions that incorporate the Plume Rise Model Enhancements (PRIME) algorithm. PRIME takes into account the effects of building downwash on plume dispersion. The comparison used actual point, area, and volume sources located on two separate facilities in conjunction with site-specific terrain and meteorological data. The modeled maximum total period average ground-level air concentrations were used to calculate potential health effects for human receptors. The results show that the switch from ISC to AERMOD and the incorporation of the PRIME algorithm tend to generate lower concentration estimates at the point of maximum ground-level concentration. However, the magnitude of difference varies from insignificant to significant depending on the types of the sources and the site-specific conditions. The differences in human health effects, predicted using results from the two models, mirror the concentrations predicted by the models.  相似文献   

10.
As of December 2006, the American Meteorological Society/U.S. Environmental Protection Agency (EPA) Regulatory Model with Plume Rise Model Enhancements (AERMOD-PRIME; hereafter AERMOD) replaced the Industrial Source Complex Short Term Version 3 (ISCST3) as the EPA-preferred regulatory model. The change from ISCST3 to AERMOD will affect Prevention of Significant Deterioration (PSD) increment consumption as well as permit compliance in states where regulatory agencies limit property line concentrations using modeling analysis. Because of differences in model formulation and the treatment of terrain features, one cannot predict a priori whether ISCST3 or AERMOD will predict higher or lower pollutant concentrations downwind of a source. The objectives of this paper were to determine the sensitivity of AERMOD to various inputs and compare the highest downwind concentrations from a ground-level area source (GLAS) predicted by AERMOD to those predicted by ISCST3. Concentrations predicted using ISCST3 were sensitive to changes in wind speed, temperature, solar radiation (as it affects stability class), and mixing heights below 160 m. Surface roughness also affected downwind concentrations predicted by ISCST3. AERMOD was sensitive to changes in albedo, surface roughness, wind speed, temperature, and cloud cover. Bowen ratio did not affect the results from AERMOD. These results demonstrate AERMOD's sensitivity to small changes in wind speed and surface roughness. When AERMOD is used to determine property line concentrations, small changes in these variables may affect the distance within which concentration limits are exceeded by several hundred meters.  相似文献   

11.
Abstract

Certain widely used wind rose programs and air dispersion models use an overly simple data-transfer algorithm that induces a directional bias in their output products. The purpose of this paper is to provide a revised algorithm that corrects the directional bias that occurs from the aliasing that occurs when the sector widths used to report wind direction data are on the same order of magnitude, but not equal, to the sector widths used in the wind direction summaries. The directional bias issue arises when output products in 16 direction sectors (22.5° each) are produced from wind direction data reported in terms of 36 sectors (10° each). The result directional bias affects the results of simulations of air and surface concentrations using widely applied air dispersion models. Datasets or models with the directional bias discussed here give consistent positive biases (~30%) for cardinal direction sectors (north, south, east, and west) and consistent negative biases for all of the other sectors (around [?10%). Data summary and air dispersion programs providing outputs in direction sectors that do not match the observational sectors need to be checked for this bias. A revised data-transfer algorithm is provided that corrects the directional bias that can occur in transferring wind direction data between different sector widths.  相似文献   

12.
A Gaussian plume model was modified to simulate the dispersion of non-reactive air pollutants under non-homogeneous wind conditions through a multi-puff approach. It was applied to the city of Lisbon and evaluated by comparison with measured sulphur dioxide data, showing a reasonable skill to estimate the transport and dispersion of pollutants under complex wind field and different atmospheric conditions. The modelling results were integrated with observed data, based on correlation functions determined from historical values, to obtain the improved analytical results by using optimal interpolation. A significant improvement over the predictions by the Gaussian puff model alone was achieved.  相似文献   

13.
This paper evaluates the application of dispersion models to estimate near-field pollutant concentrations in two case studies. The Industrial Source Complex Short-Term Model (ISCST3) was evaluated with hexavalent chromium measurements collected within 100 m of two facilities in Barrio Logan, San Diego, CA. ISCST3 provided reasonable estimates for higher pollutant concentrations but underestimated lower concentrations. To understand the observed distribution of concentrations in Barrio Logan, a recently conducted tracer experiment was analyzed. The tracer, sulfur hexafluoride, was released at ambient temperature from an urban facility at the University of California at Riverside, and concentrations were measured within 20 m of the source. Modeling results indicated that Industrial Source Complex-Plume Rise Model Enhancement and American Meteorological Society/U.S. Environmental Protection Agency Regulatory Model-Plume Rise Model Enhancement overestimated high concentrations and underestimated low concentrations. A diagnostic study with a simple Gaussian dispersion model that incorporated site-specific meteorology was used to evaluate model results. This study found that incorporating lateral meandering for nonbuoyant urban plumes in Gaussian dispersion models could improve concentration estimates even when downwash is not considered. Incorporating a meandering component in ISCST3 resulted in improvements in estimating hexavalent chromium concentrations in Barrio Logan. Credible near-source concentration estimates depend on accurate characterization of emissions, onsite micrometeorology, and a method to account for lateral meandering in the near field.  相似文献   

14.
The prediction of spatial variation of the concentration of a pollutant governed by various sources and sinks is a complex problem. Gaussian air pollutant dispersion models such as AERMOD of the United States Environmental Protection Agency (USEPA) can be used for this purpose. AERMOD requires steady and horizontally homogeneous hourly surface and upper air meteorological observations. However, observations with such frequency are not easily available for most locations in India. To overcome this limitation, the planetary boundary layer and surface layer parameters required by AERMOD were computed using the Weather Research and Forecasting (WRF) Model (version 2.1.1) developed by the National Center for Atmospheric Research (NCAR). We have developed a preprocessor for offline coupling of WRF with AERMOD. Using this system, the dispersion of respirable particulate matter (RSPM/PM10) over Pune, India has been simulated. Data from the emissions inventory development and field-monitoring campaign (13–17 April 2005) conducted under the Pune Air Quality Management Program of the Ministry of Environment and Forests (MoEF), India and USEPA, have been used to drive and validate AERMOD. Comparison between the simulated and observed temperature and wind fields shows that WRF is capable of generating reliable meteorological inputs for AERMOD. The comparison of observed and simulated concentrations of PM10 shows that the model generally underestimates the concentrations over the city. However, data from this single case study would not be sufficient to conclude on suitability of regionally averaged meteorological parameters for driving Gaussian models like AERMOD and additional simulations with different WRF parameterizations along with an improved pollutant source data will be required for enhancing the reliability of the WRF–AERMOD modeling system.  相似文献   

15.
AERCOARE is a meteorological data preprocessor for the American Meteorological Society and U.S Environmental Protection Agency (EPA) Regulatory Model (AERMOD). AERCOARE includes algorithms developed during the Coupled-Ocean Atmosphere Response Experiment (COARE) to predict surface energy fluxes and stability from routine overwater measurements. The COARE algorithm is described and the implementation in AERCOARE is presented. Model performance for the combined AERCOARE-AERMOD modeling approach was evaluated against tracer measurements from four overwater field studies. Relatively better model performance was found when lateral turbulence measurements were available and when several key input variables to AERMOD were constrained. Namely, requiring the mixed layer height to be greater than 25 m and not allowing the Monin Obukhov length to be less than 5 m improved model performance in low wind speed stable conditions. Several options for low wind speed dispersion in AERMOD also affected the model performance results. Model performance for the combined AERCOARE-AERMOD modeling approach was found to be comparable to the current EPA regulatory Offshore Coastal Model (OCD) for the same tracer studies. AERCOARE-AERMOD predictions were also compared to simulations using the California Puff-Advection Model (CALPUFF) that also includes the COARE algorithm. Many model performance measures were found to be similar, but CALPUFF had significantly less scatter and better performance for one of the four field studies. For many offshore regulatory applications, the combined AERCOARE-AERMOD modeling approach was found to be a viable alternative to OCD the currently recommended model.

Implications: A new meteorological preprocessor called AERCOARE was developed for offshore source dispersion modeling using the U.S. Environmental Protection Agency (EPA) regulatory model AERMOD. The combined AERCOARE-AERMOD modeling approach allows stakeholders to use the same dispersion model for both offshore and onshore applications. This approach could replace current regulatory practices involving two completely different modeling systems. As improvements and features are added to the dispersion model component, AERMOD, such techniques can now also be applied to offshore air quality permitting.  相似文献   


16.
Certain widely used wind rose programs and air dispersion models use an overly simple data-transfer algorithm that induces a directional bias in their output products. The purpose of this paper is to provide a revised algorithm that corrects the directional bias that occurs from the aliasing that occurs when the sector widths used to report wind direction data are on the same order of magnitude, but not equal, to the sector widths used in the wind direction summaries. The directional bias issue arises when output products in 16 direction sectors (22.5 degrees each) are produced from wind direction data reported in terms of 36 sectors (10 degrees each). The result directional bias affects the results of simulations of air and surface concentrations using widely applied air dispersion models. Datasets or models with the directional bias discussed here give consistent positive biases (approximately 30%) for cardinal direction sectors (north, south, east, and west) and consistent negative biases for all of the other sectors (around -10%). Data summary and air dispersion programs providing outputs in direction sectors that do not match the observational sectors need to be checked for this bias. A revised data-transfer algorithm is provided that corrects the directional bias that can occur in transferring wind direction data between different sector widths.  相似文献   

17.
Source term estimation algorithms compute unknown atmospheric transport and dispersion modeling variables from concentration observations made by sensors in the field. Insufficient spatial and temporal resolution in the meteorological data as well as inherent uncertainty in the wind field data make source term estimation and the prediction of subsequent transport and dispersion extremely difficult. This work addresses the question: how many sensors are necessary in order to successfully estimate the source term and meteorological variables required for atmospheric transport and dispersion modeling?The source term estimation system presented here uses a robust optimization technique – a genetic algorithm (GA) – to find the combination of source location, source height, source strength, surface wind direction, surface wind speed, and time of release that produces a concentration field that best matches the sensor observations. The approach is validated using the Gaussian puff as the dispersion model in identical twin numerical experiments. The limits of the system are tested by incorporating additive and multiplicative noise into the synthetic data. The minimum requirements for data quantity and quality are determined by an extensive grid sensitivity analysis. Finally, a metric is developed for quantifying the minimum number of sensors necessary to accurately estimate the source term and to obtain the relevant wind information.  相似文献   

18.
Two field experiments, one at Kincaid, IL, in flat terrain, the other at Bull Run, TN, in rolling terrain, were conducted under the auspices of the Electric Power Research Institute's (EPRI) Plume Model Validation and Development program. Simultaneous observations were made of ground-level SF6 concentrations; plume cross-sections using light detection and ranging (lidar); turbulence; and routine meteorology at the surface and aloft. Due to terrain influences, surface wind-speeds at the Bull Run site were significantly lower than those at the Kincaid site, whereas thermal winds at Kincaid were generally larger than at Bull Run. At both sites, a reduction in turbulent intensity and an increase in atmospheric stability with height correlate with a substantial decrease in the rate of vertical plume dispersion. SF6 ground-level concentration (GLC) patterns over distances of 1–50 km from the source were categorized by shape. The GLC patterns at Bull Run were frequently ‘blobby’, when significant GLCs occurred over an azimuth angle exceeding 90°, whereas patterns at Kincaid were generally coherent and nearly elliptical. Plume behavior was examined for 154 h during which both GLCs of SF6 tracer and lidar cross-sections of the plume were of good quality. Results show that plume looping was rare at Kincaid, but occurred substantially more often at Bull Run (3%: 14%), with the reverse true for meandering (11%: 14%). Inversions that trapped plume material occurred much more often at Kincaid that at Bull Run (11%: <1%). Correlation of cross-wind concentration distributions of the plume aloft with those cross-wind SF6 concentrations distributions at the ground were poor at both sites.  相似文献   

19.
The evaluation of the high percentiles of concentration distributions is required by most national air quality guidelines, as well as the EU directives. However, it is problematic to compute such high percentiles in stable, low wind speed or calm conditions. This study utilizes the results of a previous measurement campaign near a major road at Elimäki in southern Finland in 1995, a campaign specifically designed for model evaluation purposes. In this study, numerical simulations were performed with a Gaussian finite line source dispersion model CAR-FMI and a Lagrangian dispersion model GRAL, and model predictions were compared with the field measurements. In comparison with corresponding results presented previously in the literature, the agreement of measured and predicted data sets was good for both models considered, as measured using various statistical parameters. For instance, considering all NOx data (N=587), the so-called index of agreement values varied from 0.76 to 0.87 and from 0.81 to 1.00 for the CAR-FMI and GRAL models, respectively. The CAR-FMI model tends to slightly overestimate the NOx concentrations (fractional bias FB=+14%), while the GRAL model has a tendency to underestimate NOx concentrations (FB=−16%). The GRAL model provides special treatment to account for enhanced horizontal dispersion in low wind speed conditions; while such adjustments have not been included in the CAR-FMI model. This type of Lagrangian model therefore predicts lower concentrations, in conditions of low wind speeds and stable stratification, in comparison with a standard Lagrangian model. In low wind speed conditions the meandering of the flow can be quite significant, leading to enhanced horizontal dispersion. We also analyzed the difference between the model predictions and measured data in terms of the wind speed and direction. The performance of the CAR-FMI model deteriorated as the wind direction approached a direction parallel to the road, and for the lowest wind speeds. However, the performance of the GRAL model varied less with wind speed and direction; the model simulated better the cases of low wind speed and those with the wind nearly parallel to the road.  相似文献   

20.
ABSTRACT

It is important to develop a general model to accurately simulate the air pollution in urban street areas. In this paper, the Operational Street Pollution Model (OSPM) initially developed in Denmark is tested with measured data from a relatively wide and open street in Beijing. Major factors influencing the dispersion, such as emission factors, stationary source emissions, and solar radiation, are analyzed. Results show that the model can reflect the basic dispersion pattern in the street but gives systematically higher concentrations. After modifications to estimate street-level wind speed in the model, performance is obviously improved.  相似文献   

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