The distribution and history of nuclear weapons related contamination in sediments from the Ob River, Siberia as determined by isotopic ratios of plutonium and neptunium

Isotopic ratios of Pu and Np measured in sediment cores from 5 locations in the Ob River drainage basin show clear evidence of input from sources other than global fallout (non-fallout sources). Historical contaminant records obtained by combining isotopic ratio information with chronological information indicate that non-fallout inputs are from several sources that have varied significantly over the past 50 years. Unique isotopic signatures observed in sediments from tributaries that drain areas containing known or suspected sources of non-fallout contamination are used to identify the source of materials in sediments collected at downstream locations. These data can lead to a better understanding of the transport behavior, fate, and relative importance of particle reactive, weapons related contaminants originating from the nuclear facilities Mayak. Tomsk-7, and Semipalitinsk, which lie within the drainage basin. From our work to date, we draw the following conclusions: (1) Persistent non-fallout contamination is observed in the Ob River above its confluence with the Irtysh River, indicating contamination from the Tomsk-7 facility. (2) Non-fallout contamination in the Tobol River above its confluence with the Irtysh River indicates contamination from the Mayak facility. (3) Non-fallout contamination in the Irtysh River above its confluence with the Tobol River indicates contamination from the Semipalitinsk weapons test site. (4) The occurrence of isotopic ratios in Ob Delta sediments that are similar to those observed in source tributaries suggests that contamination from at least two sources has been transported along the length of the river system. (5) Global fallout, a result of high-yield atmospheric weapons tests conducted by the FSU and USA primarily, is the dominant source of Pu and Np to the region; however, there have been brief periods when inputs from non-fallout sources exceeded those from global fallout.     

Distribution of Np and Pu in Swedish lichen samples (Cladonia stellaris) contaminated by atmospheric fallout

The activity concentrations of (237)Np and the two Pu isotopes, (239)Pu and (240)Pu, were determined in lichen samples (Cladonia stellaris) contaminated by fallout from atmospheric nuclear test explosions and the Chernobyl accident. The samples were collected at 18 locations in Sweden, from north to south, between 1986 and 1988 and analysed with high-resolution inductively coupled plasma mass spectrometry (HR-ICP-MS) and alpha spectrometry. Data on the activity ratios (238)Pu/(239+240)Pu and (134)Cs/(137)Cs measured previously were also included in this study for comparison. The (237)Np activity concentration ranged from 0.08 +/- 0.01 to 2.08 +/- 0.17 MBq kg(-1), depending on the location of the sampling site and time of collection. The (239+240)Pu activity concentration ranged from 0.09 +/- 0.01 to 4.09 +/- 0.15 Bq kg(-1), with the (240)Pu/(239)Pu atomic ratio ranging between 0.16 +/- 0.01 and 0.44 +/- 0.03, the higher ratios indicating a combination of weapons test fallout and Chernobyl fallout. The (237)Np/(239)Pu atomic ratios ranged between 0.06 +/- 0.01 and 0.42 +/- 0.04, the lower ratios indicating combination of weapons test fallout and Chernobyl fallout. At a well-defined sampling site at Lake Rogen (62.32 degrees N, 12.38 degrees E), additional lichen samples were collected between 1987 and 1998 to study the distribution of Np and Pu in different layers. The concentrations of the two elements follow each other quite well in the profile.     

Monitoring of radiation and radioactivity in the environment

This report lists the programs for monitoring radiation and radioactivity in the environment that are known to be in operation or to have been in operation recently. It is intended as a guide to be used when seeking information on the programs of other institutions. Sources of the data have been the literature and personal correspondence and discussions.The programs are divided into the categories of weapons test fallout, natural activity and environmental monitoring of releases from specific facilities. Where possible, the types of measurements being made are also listed. While the data are as up to date as possible the field is changing rapidly and there may be ommissions.     

A 10-year study of the 137Cs distribution in soil and a comparison of Cs soil inventory with precipitation-determined deposition

During a 10-year period, 1988-1998, surface soil samples have been collected at Blentarp in southern Sweden and analysed for 137Cs from the Chernobyl accident and from the nuclear weapons tests. The distance between the sampling plots on the different sampling occasions has been no more than 3 m. The results show that the depth distribution of 137Cs is very similar for each of the sampling occasions, indicating that the caesium migration at this site is very small. The total activity measured in the soil cores is in agreement with the calculated activity of 137Cs deposited at the site after nuclear weapons tests and the Chernobyl accident, based on air activity concentration and the amount of precipitation. The calculated deposition of 137Cs originating from the bomb tests amounts to 1.41 kBq m-2 for the period 1962-1986, which is in agreement with the activity of nuclear weapons fallout measured in the soil samples (1.60 kBq m-2 as a mean value of the first four years of sampling). The calculated activity of 137Cs of Chernobyl origin was 0.79 kBq m-2, which agrees well with the value of 0.79 kBq m-2 measured in the soil samples in 1988.     

Aquatic mosses as a monitoring tool for 137Cs contamination in streams and rivers-a field study from central southern Norway

Mosses are frequently used as biomonitors for trace element pollution in the aquatic environment. The purpose of this study was to assess their usefulness as a tool in monitoring and in regional surveys of radioactive contamination. Specimens of the aquatic mosses, Fontinalis antipyretica and F. dalecarlica, were transplanted from non-contaminated areas to streams and rivers in the Norwegian Jotunheimen Mountains and neighbouring lowland areas that had received radioactive fallout after the Chernobyl accident. Equilibrium concentrations of 137Cs in the exposed mosses were reached after a few weeks. Two series from 20 streams in 1994 and 1996 show linear correlations between activities in water and moss samples and biomagnification ratios of 10(4) - 10(5). We conclude that mosses are better suited for monitoring purposes than water samples, because they provide values integrated over weeks while the radioactivity in surface waters can be subject to rapid variations according to hydrological events. The activity concentrations in aquatic mosses can be easily measured with good precision even when aqueous concentrations are below the limit of detection. Use of aquatic mosses also reduces the logistic problems of transporting large volumes of water, especially in areas inaccessible by road.     

Artificial radioactivity in Cumbria: Summary of an assessment by measurement and modelling

At the Harwell laboratory, the distributions of the artificial radionuclides discharged by British Nuclear Fuels at Sellafield have been measured within Cumbria, with particular emphasis on the transfer between environmental media. The results of the measurements have been incorporated into a model of the Cumbrian environment.The object of this work is to estimate the radiological impact upon man by exploring the pathways leading to external irradiation, to inhalation and to the ingestion of foodstuffs.Distributions have been established for caesium-137, plutonium isotopes and americium-241. Transfer from sea to land, of actinide radioactivity discharged to the sea, occures on a very small scale. The relative contributions to deposition and airborne radioactivity from sea-to-land transfer, fallout from nuclear weapons testing and atmospheric releases from Sellafield are compared. The dose resulting from sea-to-land transfer of actinides to a resident of Seascale peaked in 1973 at less than 1% of the ICRP annual limit for the general public and should fall steadily up to the year 2000.     

An analysis of the environmental mobility of radiostrontium from weapons testing and Chernobyl in Finnish river catchments

The mobility of radiostrontium within the Arctic environment and surrounding area has been studied by analysing the mobility of 90Sr in river catchments that are within Finland. The environmental mobility of 90Sr deposited by both nuclear weapons testing and the Chernobyl accident has been investigated in five Finnish river catchments. Different models assessing the time-dependent mobility of 90Sr have been evaluated. No significant differences were found between the mobility of 90Sr from nuclear weapons tests and from the Chernobyl accident. Model parameters obtained by fitting to the measurements of the deposition and runoff rates of the nuclear weapons test fallout gave predictions which were consistent with the mid- and long-term contamination by the Chernobyl fallout. A comparison of 90Sr with 137Cs showed that they had similar mobility on deposition but, as time passed, the relative mobility of 90Sr increased with respect to 137Cs over a period of 5-8 years. Once the relative migration of 90Sr with respect to 137Cs reached equilibrium, its runoff rate was, on average, approximately an order of magnitude greater than 137Cs.     

Distribution of environmental Cesium-137 in tree rings

Environmental ¹³⁷Cs concentrations in tree rings grown since 1914 and 1929 were measured and compared with the record of ¹³⁷Cs deposition from weapons fallout. ¹³⁷Cs was found in tree rings formed prior to 1945 when the first nuclear weapon test was conducted. The radiocesium record in wood is not correlated with that of fallout deposition.     

南水北调工程及其生态安全：优先研究领域

南水北调工程的实施将大幅度增加黄河上游径流量，并同时减少长江尤其是其上游及汉江下游的径流量，从而导致两条主要河流及其支流的水环境改变。中线工程从汉江上游丹江口水库调水，库区上游90 000余km2内的非点源污染和1 300万人口的生活污水处理设施的缺乏对水质将产生重大影响;调水引起水文节律的改变从而对东线沿途的湖泊生态系统产生重大影响;黄淮海平原受水区可利用水量的增加也可能导致该地区的盐渍化。介绍了南水北调工程并讨论了其必要性，提出了工程对生物迁移的影响、水环境及水生态安全、水资源保护的流域生态系统管理和西部退化生态系统的恢复和重建等优先研究领域，并提出结合“中国生态系统研究网络”、“生态环境国家野外科学观测研究站”的建设和长期监测来保障工程生态安全的策略。     

Modelling the distribution of plutonium in the Pacific Ocean

An Oceanic General Circulation Model (OGCM) including a plutonium scavenging model as well as an advection-diffusion model has been developed for modelling the distribution of plutonium in the Pacific Ocean. Calculated 239, 240Pu water profile concentrations and 239, 240Pu inventories in water and sediment of the Pacific Ocean have showed a reasonable agreement with the experimental results. The presence of local fallout plutonium in central North Pacific waters has been confirmed. The observed 240Pu/239Pu mass ratios confirm that plutonium originating from local fallout from nuclear weapons tests carried out at Bikini and Enewetak Atolls is more rapidly removed from surface waters to deeper waters than plutonium originating from global fallout. The developed OGCM can be used for modelling the dispersion of other non-conservative tracers in the ocean as well.     

国内外大型水电工程生态环境监测与保护

简要介绍了世界银行对水电工程的环境政策,概述了埃及阿斯旺、巴西伊泰普、中国的二滩和三峡等四个世界著名水电站的长期环境监测计划和减少负面影响的对策。水电工程对周边环境会产生正面或负面影响,对大型水坝的负面影响作了集中的阐述。埃及的阿斯旺高坝建于20世纪60年代, 当时人们对生态环境影响问题还没有引起重视。长期的生态环境监测结果表明,一些环境影响比如河床侵蚀等实际上被过分夸大,而另外一些,如对传统的制砖业带来的影响又被忽视;巴西的伊泰普水坝在兴建过程中注意了采取措施减少负面影响,如在库周地区植树造林,兴建生物屏障,建立自然保护区,实施动物救护等;中国的二滩水电站由世界银行贷款兴建,并执行了世界银行的环境政策来降低负面影响;这些大型水电工程兴建中的经验给在建的三峡工程提供了有益的借鉴,一系列的环境保护措施正在实施,世界上最大的生态环境监测网络已在三峡库区及相关地区建成。     

Concentration of radionuclides in hydrosphere affected by Temelín Nuclear Power Plant in Czech Republic

The paper presents results of a long-term field study of the possible impact of Temelín NPP on the Vltava and Elbe Rivers. The study was divided into 2 stages: before and after the operation of the NPP. The main goal of the investigation before the operation (1989–2000) was to determine the background levels of radionuclides resulting from the tests of nuclear weapons and the Chernobyl accident for different components of the environment. The paper discusses also the risk of a river radioactive contamination due to the tritium discharges in wastewater from Temelín NPP. During the operation period of 2001–2006, the results of the monitoring did not detect any impact of Temelín NPP on the concentrations of activation and fission products in the hydrosphere, apart from tritium. The annual average tritium concentrations in the Vltava River correspond with the previously calculated predictions for the conditions of the average and minimum guaranteed flows. The maximum concentration of tritium of 26.6 Bq/l in Vltava River at Prague was observed after dry period in 2003.     

Vertical migration studies of 137Cs from nuclear weapons fallout and the Chernobyl accident

The vertical migration of (137)Cs originating from nuclear weapons fallout (NWF) and the Chernobyl accident has been studied at 33 sampling sites in western Sweden. An attempt to describe the present depth distribution with a solution to the convection-diffusion equation (CDE) with a pulse-like fallout event as the initial condition was made. A sum of two CDEs describing the NWF and Chernobyl debris was fitted to the actual depth profiles measured by soil sampling. The fitted depth profiles were used to correct in situ measurements for the actual depth distribution, showing good agreement with the accumulated activities in soil samples. As expected, the vertical migration was very slow and most caesium was still present in the upper soil layers. The ranges of the apparent convection velocity, v, and apparent diffusion coefficient, D, were between 0 and 0.35 cm/year and 0.06 and 2.63 cm(2)/year, respectively.     

阿斯旺高坝的生态环境问题

:通过对阿斯旺高坝和尼罗河的实际考察和生态环境监测数据的分析 ,介绍了埃及政府相关管理部门的官员和专家对阿斯旺工程的看法 ,对阿斯旺高坝及其生态环境问题进行了评述。认为阿斯旺工程是一个成功的工程 ,它对埃及发挥的巨大影响和积极作用是有目共睹的。它对生态环境的不利影响 ,确被很多批评者盲目地夸大了 ,其中也包含有政治因素。中国在修建水利工程时 ,要对环境的影响作出客观、科学的评价 ,并采取措施把不利影响减少到最小。阿斯旺高坝运行近 30年 ,在生态环境监测方面积累了丰富的数据 ,这些成果和结论对三峡工程具有直接的借鉴和参考价值。     

The radiological impact of the Chernobyl debris compared with that from nuclear weapons fallout

Our basic knowledge of the radiological impact of fallout from nuclear accidents is based on the experience gained from the study of nuclear weapons fallout. Radioecologically, the most important radionuclides generated by the Chernobyl accident were ¹³⁷Cs, ¹³⁴Cs, ¹³¹I and, to a lesser degree, ⁹⁰Sr. These nuclides are well known from global fallout, although in different relative amounts to those observed in the Chernobyl debris. Another important difference between the fallout from Chernobyl and that from nuclear weapon tests is that their seasonal and geographical distributions were quite dissimilar. A number of examples show how these differences influenced transfer factors and thus population doses. Special emphasis is paid to the contamination of milk and cereal products.Furthermore, it is shown how the composition of the Chernobyl debris changed with distance from Chernobyl, due to the differences in volatility of the various radionuclides involved. Finally, the paper compares the dose equivalents received from unit releases (1 P Bq ¹³⁷Cs) of global fallout and of Chernobyl accident debris.     

A new general dynamic model predicting radionuclide concentrations and fluxes in coastal areas from readily accessible driving variables

This paper presents a general, process-based dynamic model for coastal areas for radionuclides (metals, organics and nutrients) from both single pulse fallout and continuous deposition. The model gives radionuclide concentrations in water (total, dissolved and particulate phases and concentrations in sediments and fish) for entire defined coastal areas. The model gives monthly variations. It accounts for inflow from tributaries, direct fallout to the coastal area, internal fluxes (sedimentation, resuspension, diffusion, burial, mixing and biouptake and retention in fish) and fluxes to and from the sea outside the defined coastal area and/or adjacent coastal areas. The fluxes of water and substances between the sea and the coastal area are differentiated into three categories of coast types: (i) areas where the water exchange is regulated by tidal effects; (ii) open coastal areas where the water exchange is regulated by coastal currents; and (iii) semi-enclosed archipelago coasts. The coastal model gives the fluxes to and from the following four abiotic compartments: surface water, deep water, ET areas (i.e., areas where fine sediment erosion and transport processes dominate the bottom dynamic conditions and resuspension appears) and A-areas (i.e., areas of continuous fine sediment accumulation). Criteria to define the boundaries for the given coastal area towards the sea, and to define whether a coastal area is open or closed are given in operational terms. The model is simple to apply since all driving variables may be readily accessed from maps and standard monitoring programs. The driving variables are: latitude, catchment area, mean annual precipitation, fallout and month of fallout and parameters expressing coastal size and form as determined from, e.g., digitized bathymetric maps using a GIS program. Selected results: the predictions of radionuclide concentrations in water and fish largely depend on two factors, the concentration in the sea outside the given coastal area and/or adjacent coastal areas and the ecological half-life of the radionuclide in the sea. Uncertainties in these factors generally dominate all other uncertainties, e.g., concerning the surface water retention time, the settling velocity of the particulate fraction, the distribution coefficient regulating the fluxes in dissolved and particulate phases, the catchment area influences and the factors regulating biouptake and excretion of the radionuclide in fish. This means that the conditions in the sea are of paramount importance for the conditions in the coastal area, even for relatively enclosed coastal areas. This coastal model may be regarded as a tool for testing working hypotheses on the relative roles of different processes in different coastal areas. Such information is essential for getting realistic expectations of various remedial measures, such as coastal dredging discussed in this work.     

三峡水库库首水温监测及初步分析

水温是评价水库水生态系统影响的重要水质参数之一,为研究三峡水库库首水温分布状况,于2011年在距三峡大坝约为35 km处,对三峡水库建成后各个运行期库首水温进行了详细监测。研究发现：在已确定的三峡工程常规调度运行方式下, 12~4月库首底部形成明显的低温区域,3月表层和底部水温之差为全年的最大值208℃,最大温度梯度为0156。5月底部低温区迅速减弱,表层和底部水温之差小于10℃。6~9月期间,低温区一直处于减弱的趋势,水体垂向掺混逐渐增强,库首水温垂向分布基本均匀一致。但进入10月后,由于上游来流水温较低,水体由于密度较大而潜入底部对低温区域起到了加强的作用,致使表底层温差达到146℃。根据2012年3~5月对三峡水库库首茅坪断面水温监测数据可知,在横向断面上,水温几乎没有差别。在分析三峡水库库首水温空间分布时,可以近似认为其横向水温分布基本一致。为研究三峡大坝的建成对河道水温的改变以及坝前是否存在水温分层现象提供依据和参考     

Distribution and flux of 238Pu, 239,240Pu, 241Am, 137Cs and 210Pb to high arctic lakes in the Thule district (Greenland)

Environmental samples (soil, sediment and lake water) in the Thule area (NW Greenland) have been studied to assess the contamination of radionuclides originating from a nuclear weapons accident (the Thule accident in 1968). Four lakes were chosen at different distances from the point of impact with the Thule air base community situated in between. The sedimentation rates in the lakes varied from 0.4 mm a(-1) (5 mg cm(-2) a(-1)) to 1.6 mm a(-1) (82 mg cm(-2) a(-1)). With these sedimentation rates, it is not possible to resolve the (239,240)Pu global fallout peak from a possible (239,240)Pu "accident" peak in the sediment depth profiles. However, the (239,240)Pu/(137)Cs and the (238)Pu/(239,240)Pu ratios agreed well with global fallout ratios, indicating that plutonium originating from the accident had not reached these lakes. This also indicates that the Thule air base community has probably only been exposed to radionuclides from the accident to a very limited extent. A limited study showed that (210)Pb could not be used as a normalizing nuclide to explain the transport of transuranic elements from the catchment area to the lake, i.e. (210)Pb has a different transport mechanism from that of the transuranic elements studied in this investigation.     

水利工程对长江河口生态环境的影响

我国对长江水资源的开发利用．如在干流和支流上已建和在建的许多大大小小的水利工程．特别是规模宏伟的三峡大坝建设和南水北调工程．将显著改变长江的水、沙动态，改变营养物质的输移特征，不仅直接影响下游河道的水文、水环境条件．而且对远离工程的河口生态环境也将产生显著和潜在的影响。分析了由于上游蓄水和引水造成的河流径流量减少、季节分配变化而对水体营养物质输移能力和水体自净能力的影响，以及因上游来水来沙量减少对河口生态环境和生物多样性的影响。水文因素是沼泽湿地和滨海湿地形成和发育的重要环境因素。上游建坝蓄水以后．洪水的消除或洪泛次数减少削弱了河流与湿地之间的联系，造成湿地逐渐萎缩，甚至大面积丧失，生物食物链中断，生物多样性和生产力下降。人海径流量减少将造成海水沿河上溯，盐水入侵河道，并污染地下水，滩地土壤发生盐渍化。河流携带泥沙能力下降，将导致三角洲从淤积型向侵蚀型转化，海岸线蚀退。水利工程对河口生态环境的影响是长期的、缓慢的、潜在的和极其复杂的，并且往往是上游各水利工程的叠加作用。因此在工程建设前后研究分析河口生态环境可能或已经遭受的影响，对生态环境的变化进行长期的跟踪、监测和评价，可为今后水利工程建设和生态环境保护提供理论依据和研究基础。     

三峡水库蓄水对香溪河水环境的影响及对策研究

通过监测论证三峡建库后形成香溪河回水库湾水环境条件改变特征,评价表明水质由轻污染至重污染趋势发展。确定库湾周边的工业、生活污染点源、磷矿面源是构成水污染的主要负荷。指出溶解氧沿河道下游沿程逐渐减小,复氧系数降低,是引起水质恶化,破坏库湾生态平衡的主要因素。磷浓度过高将引起三峡水库局部水域富营养化,预测了总磷浓度沿程变化趋势。针对已发生和潜在的水环境污染问题,提出了加强流域非点源污染的管理、实施总量控制、建立污染源在线监测系统、立项建设污染治理工程、开展河湖水域接触氧化直接净化技术的科研究和实践、制定《三峡库区水污染防治法》地方法规、正确处理资源开发与环境保护协调发展的关系、走可持续发展道路等项防治对策与建议。