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1.
The purpose of this paper is to develop a methodology to evaluate the feasibility of using landfill gas (LFG) as a liquefied natural gas (LNG) fuel source for heavy-duty refuse trucks operating on landfills. Using LFG as a vehicle fuel can make the landfills more self-sustaining, reduce their dependence on fossil fuels, and reduce emissions and greenhouse gases. Acrion Technologies Inc. in association with Mack Trucks Inc. developed a technology to generate LNG from LFG using the CO2 WASH process. A successful application of this process was performed at the Eco Complex in Burlington County, PA. During this application two LNG refuse trucks were operated for 600 hr each using LNG produced from gases from the landfill. The methodology developed in this paper can evaluate the feasibility of three LFG options: doing nothing, electricity generation, and producing LNG to fuel refuse trucks. The methodology involved the modeling of several components: LFG generation, energy recovery processes, fleet operations, economic feasibility, and decision-making. The economic feasibility considers factors such as capital, maintenance, operational, and fuel costs, emissions and tax benefits, and the sale of products such as surplus LNG and food-grade carbon dioxide (CO2). Texas was used as a case study. The 96 landfills in Texas were prioritized and 17 landfills were identified that showed potential for converting LFG to LNG for use as a refuse truck fuel. The methodology was applied to a pilot landfill in El Paso, TX. The analysis showed that converting LFG to LNG to fuel refuse trucks proved to be the most feasible option and that the methodology can be applied for any landfill that considers this option.  相似文献   

2.
Landfill gas (LFG) management is one of the most important tasks for landfill operation and closure because of its impact in potential global warming. The aim of this work is to present a case history evaluating an LFG capture and treatment system for the present landfill facility in Córdoba, Argentina. The results may be relevant for many developing countries around the world where landfill gas is not being properly managed. The LFG generation is evaluated by modeling gas production applying the zero-order model, Landfill Gas Emissions Model (LandGEM; U.S. Environmental Protection Agency [EPA]), Scholl Canyon model, and triangular model. Variability in waste properties, weather, and landfill management conditions are analyzed in order to evaluate the feasibility of implementing different treatment systems. The results show the advantages of capturing and treating LFG in order to reduce the emissions of gases responsible for global warming and to determine the revenue rate needed for the project’s financial requirements. This particular project reduces by half the emission of equivalent tons of carbon dioxide (CO2) compared with the situation where there is no gas treatment. In addition, the study highlights the need for a change in the electricity prices if it is to be economically feasible to implement the project in the current Argentinean electrical market.

Implications: Methane has 21 times more greenhouse gas potential than carbon dioxide. Because of that, it is of great importance to adequately manage biogas emissions from landfills. In addition, it is environmentally convenient to use this product as an alternative energy source, since it prevents methane emissions while preventing fossil fuel consumption, minimizing carbon dioxide emissions. Performed analysis indicated that biogas capturing and energy generation implies 3 times less equivalent carbon dioxide emissions; however, a change in the Argentinean electrical market fees are required to guarantee the financial feasibility of the project.  相似文献   


3.
Dramatic increases in the development of oil and natural gas from shale formations will result in large quantities of drill cuttings, flowback water, and produced water. These organic-rich shale gas formations often contain elevated concentrations of naturally occurring radioactive materials (NORM), such as uranium, thorium, and radium. Production of oil and gas from these formations will also lead to the development of technologically enhanced NORM (TENORM) in production equipment. Disposal of these potentially radium-bearing materials in municipal solid waste (MSW) landfills could release radon to the atmosphere. Risk analyses of disposal of radium-bearing TENORM in MSW landfills sponsored by the Department of Energy did not consider the effect of landfill gas (LFG) generation or LFG control systems on radon emissions. Simulation of radon emissions from landfills with LFG generation indicates that LFG generation can significantly increase radon emissions relative to emissions without LFG generation, where the radon emissions are largely controlled by vapor-phase diffusion. Although the operation of LFG control systems at landfills with radon source materials can result in point-source atmospheric radon plumes, the LFG control systems tend to reduce overall radon emissions by reducing advective gas flow through the landfill surface, and increasing the radon residence time in the subsurface, thus allowing more time for radon to decay. In some of the disposal scenarios considered, the radon flux from the landfill and off-site atmospheric activities exceed levels that would be allowed for radon emissions from uranium mill tailings.

Implications: Increased development of hydrocarbons from organic-rich shale formations has raised public concern that wastes from these activities containing naturally occurring radioactive materials, particularly radium, may be disposed in municipal solid waste landfills and endanger public health by releasing radon to the atmosphere. This paper analyses the processes by which radon may be emitted from a landfill to the atmosphere. The analyses indicate that landfill gas generation can significantly increase radon emissions, but that the actual level of radon emissions depend on the place of the waste, construction of the landfill cover, and nature of the landfill gas control system.  相似文献   

4.
Mercury-bearing material has been placed in municipal landfills from a wide array of sources including fluorescent lights, batteries, electrical switches, thermometers, and general waste. Despite its known volatility, persistence, and toxicity in the environment, the fate of mercury in landfills has not been widely studied. The nature of landfills designed to reduce waste through generation of methane by anaerobic bacteria suggests the possibility that these systems might also serve as bioreactors for the production of methylated mercury compounds. The toxicity of such species mandates the need to determine if they are emitted in municipal landfill gas (LFG). In a previous study, we had measured levels of total gaseous mercury (TGM) in LFG in the μg/m3 range in two Florida landfills, and elevated levels of monomethyl mercury (MMM) were identified in LFG condensate, suggesting the possible existence of gaseous organic Hg compounds in LFG. In the current study, we measured TGM, Hg0, and methylated mercury compounds directly in LFG from another Florida landfill. Again, TGM was in the μg/m3 range, MMM was found in condensate, and this time we positively identified dimethyl mercury (DMM) in the LGF in the ng/m3 range. These results identify landfills as a possible anthropogenic source of DMM emissions to air, and may help explain the reports of MMM in continental rainfall.  相似文献   

5.
Well testing procedures, such as the Tier 3 methodology specified in the U.S. Code of Federal Regulations (CFR) Subtitle D, are commonly used for directly estimating landfill gas (LFG) emissions at municipal solid waste (MSW) landfills. Similar procedures are also used to estimate LFG generation rates for the design of LFG-to-energy projects. These methodologies assume that the LFG generation rate equals the extraction rate of a test gas well within its radius of influence (ROI). The ROI is defined as the distance from the extraction well at which the induced pressure drop is immeasurable by some standard of precision. Based on fluid dynamic principles, Tier 3 and similar methodologies are demonstrated to be incapable of providing reliable estimates of the LFG generation rate. These tests may either over- or underestimate the LFG generation rate depending on the precision with which the ROI is determined, but they will only coincidentally produce an estimate that accurately represents the actual LFG generation rate. Fluid dynamic principles dictate that the actual LFG generation rate can only be estimated if the pneumatic properties of the refuse and cover materials as well as the excess pressure in the refuse caused by LFG generation are known or can be estimated.  相似文献   

6.
ABSTRACT

Previous greenhouse gas studies comparing landfilling with combustion of municipal solid waste (MSW) are limited to examinations of the emissions weighted by their relative radiative activity. This paper adds another dimension by analyzing the atmospheric response to these emissions. The heart of the analysis is a time-dependent model using a perturbation analysis of the IS92a results of the Intergovernmental Panel on Climate Change (IPCC). Using as inputs the emissions from the two technologies, the model calculates atmospheric concentration histories. Scenarios for a landfill and a combustor envision each accepting 1000 Mg refuse/day for a 30-year operating period followed by a 70-year postclosure period. The baseline scenario examines the basic greenhouse impact of each technology. The other scenario adds active gas collection at the landfill and energy offset credits for avoided power plant carbon emissions. For both scenarios, CH4 and trace gases from the landfill persist in the atmosphere, and they are relatively potent at forcing IR heating. The combination of these features place the landfill much higher than previously expected on the greenhouse impact scale. For the baseline scenario, the time-integrated radiative forcing from landfilling is 115 times that of combustion, and this ratio is 45 for the second scenario.  相似文献   

7.
The surface emission of landfill gas (LFG) was studied to estimate the amount of LFG efflux from solid waste landfills using an air flux chamber. LFG efflux increased as atmospheric temperature increased during the day, and the same pattern for the surface emission was observed for the change of seasons. LFG efflux rate decreased from summer through winter. The average LFG efflux rates of winter, spring and summer were 0.1584, 0.3013 and 0.8597 m3 m−2 h−1 respectively. The total amount of surface emission was calculated based on the seasonal LFG efflux rate and the landfill surface area. From the estimates of LFG generation, it is expected that about 30% of the generated LFG may be released through the surface without extraction process. As forced extraction with a blower proceeded, the extraction well pressure decreased from 1100 to –100 mm H2O, and the LFG surface efflux decreased markedly above 80%. Thus, the utilization of LFG by forced extraction would be the good solution for global warming and air pollution by LFG.  相似文献   

8.
ABSTRACT

The increase in solid waste generation has been a major contributor to the amount of Greenhouse gases (GHGs) present in the atmosphere. To some extent, a great chunk of these GHGs in the atmosphere is from landfill. This study assesses two theoretical models (LandGEM and Afvalzorg models) to estimate the amount of landfill gas (LFG) emitted from Thohoyandou landfill site. Also, the LFGcost Web model was used to estimate the cost and benefits of the implementation of an LFG utilization technology. The Thohoyandou landfill started operations in the year 2005 and it is proposed to reach its peak at approximately in the year 2026. The LandGEM calculates the mass of landfill gas emission using methane generation capacity, mass of deposited waste, methane generation constant and methane generation rate. Meanwhile, the Afvalzorg model determines the LFG emissions using the Methane correction factor, yearly waste mass disposal, waste composition, Degradation Organic Carbon, methane generation rate constant, LFG recovery efficiency. The study findings indicate that the methane (CH4) and carbon dioxide (CO2) emitted from the landfill estimated from LandGEM will peak in the year 2026 with values of 3517 Mg/year and 9649 Mg/year, respectively. Results from the Afvalzorg model show that CH4 emission will peak in the year 2026 (3336 Mg/year). The LandGEM model showed that the total LFG, CH4 and CO2 emitted from the landfill between 2005 and 2040 are 293239.3 Mg/year, 78325.7 Mg/year and 214908.6 Mg/year, respectively. The simulation from the Afvalzorg model found that the CH4 emitted from the years 2005– 2040 is 74302 Mg/year. The implementation of an LFG utilization technology was economically feasible from consideration of the sales of electricity generated and Certified Emission Reductions (CER) (carbon credits).  相似文献   

9.
Abstract

Mercury-bearing material enters municipal landfills from a wide array of sources, including fluorescent lights, batteries, electrical switches, thermometers, and general waste; however, the fate of mercury (Hg) in landfills has not been widely studied. Using automated flux chambers and downwind atmospheric sampling, we quantified the primary pathways of Hg vapor releases to the atmosphere at six municipal landfill operations in Florida. These pathways included landfill gas (LFG) releases from active vent systems, passive emissions from landfill surface covers, and emissions from daily activities at each working face (WF). We spiked the WF at two sites with known Hg sources; these were readily detected downwind, and were used to test our emission modeling approaches. Gaseous elemental mercury (Hg0) was released to the atmosphere at readily detectable rates from all sources measured; rates ranged from ~1–10 ng m?2 hr?1 over aged landfill cover, from ~8–20 mg/hr from LFG flares (LFG included Hg0 at μg/m3 concentrations), and from ~200–400 mg/hr at the WF. These fluxes exceed our earlier published estimates. Attempts to identify specific Hg sources in excavated and sorted waste indicated few readily identifiable sources; because of effective mixing and diffusion of Hg0, the entire waste mass acts as a source. We estimate that atmospheric Hg releases from municipal landfill operations in the state of Florida are on the order of 10–50 kg/yr, substantially larger than our original estimates, but still a small fraction of current overall anthropogenic losses.  相似文献   

10.

The investigation of municipal solid waste (MSW) treatment in China is rare due to its sensitivity and difficulty in terms of access. We chose Beijing, the capital of China, as an example to identify the characteristics of MSW landfill treatments using a 2-month investigation with 20 participants. MSW landfill treatments account for nearly 70% of the annual MSW disposal in Beijing; the landfill processes are equipped with many kinds of technologies and consume a large amount of energy and produce a variety of contaminants. The cover method (the most obvious difference in landfill tamping) mainly includes high-density polyethylene (HDPE) geomembranes with loess and soil alone (i.e., loess or sandy soil). We investigated the actual conditions of landfills and collected data on leachate and landfill gas (LFG) emissions and energy consumption during 2009–2011. The results indicated that the cover method employed by landfills was related to treatment quantity, operation, and especially landfill location. Early large-scale landfills located in plains were covered with HDPE geomembranes, and newly built landfills covered with soil tended to be equipped with HDPE covers. Using HDPE cover also contributed greatly to LFG production due to its impermeability but had no remarkable effect on leachate yield reduction due to the dry climate in Beijing. The potential was reinforced by the potentials of decrement and reuse. The disposal method of LFG can be optimized, and the power generated by the LFG process can meet the landfill demand. The gray water recycled from the leachate could be used in the landfill process.

  相似文献   

11.
生活垃圾可持续化填埋   总被引:5,自引:0,他引:5  
通过对中国填埋场现状分析,提出了"可持续填理"的概念.认为生活垃圾填埋场将从单纯的最终处置场所演变为填埋与中转相结合的场所.填埋场的可持续发展也将从两方面得到体现:一为垃圾降解过程及其副产品处理中以能量形式得到利用,另一方面为稳定化后的垃圾及填埋场本身空间得到再一次的利用.  相似文献   

12.
Abstract

Idle emissions data from 19 medium heavy-duty diesel and gasoline trucks are presented in this paper. Emissions from these trucks were characterized using full-flow exhaust dilution as part of the Coordinating Research Council (CRC) Project E-55/59. Idle emissions data were not available from dedicated measurements, but were extracted from the continuous emissions data on the low-speed transient mode of the medium heavy-duty truck (MHDTLO) cycle. The four gasoline trucks produced very low oxides of nitrogen (NOx) and negligible particulate matter (PM) during idle. However, carbon monoxide (CO) and hydrocarbons (HCs) from these four trucks were approximately 285 and 153 g/hr on average, respectively. The gasoline trucks consumed substantially more fuel at an hourly rate (0.84 gal/hr) than their diesel counterparts (0.44 gal/hr) during idling. The diesel trucks, on the other hand, emitted higher NOx (79 g/hr) and comparatively higher PM (4.1 g/hr), on average, than the gasoline trucks (3.8 g/hr of NOx and 0.9 g/hr of PM, on average). Idle NOx emissions from diesel trucks were high for post-1992 model year engines, but no trends were observed for fuel consumption. Idle emissions and fuel consumption from the medium heavy-duty diesel trucks (MHDDTs) were marginally lower than those from the heavy heavy-duty diesel trucks (HHDDTs), previously reported in the literature.  相似文献   

13.
Abstract

The estimation of odor production and dispersion from landfill sites is a very complicated task because of the different chemical species that exist in biogas. To site a new landfill, it is necessary to know the distance that odors can travel around the landfill under atmospheric conditions that increase the concentration of pollutants. Although CH4 is an odorless gas, it can be used as an index to determine the dispersion of low-reactivity odorous species around a landfill site. Methane production rates, estimated by biogas production models, were used by an air dispersion model to determine the spatial distribution of CH4 around landfill sites. By utilizing dispersion models under extreme atmospheric conditions, a maximum CH4 concentration around the landfills was determined. Based on the ratio between CH4 and odorous chemical species, the spatial distribution of the concentration of an odorous species was determined for those species with low reactivity in the atmosphere. For odorous species with high reactivity in the atmosphere, a dispersion-reaction model must be used. In this way, the acceptable distance between new landfills and residential areas can be determined. The proposed methodology could be used as a design tool for those who are interested in landfill siting.  相似文献   

14.
One of the most significant environmental problems arising from landfills is the emission of methane into the atmosphere. In this study, methane emissions from a currently in-use Spanish landfill were modeled as well as being experimentally measured using a two-step method. The first step involved a qualitative walkover survey to detect where gases were being emitted on the surface of the landfill. The second stage comprised a quantitative analysis of these surface methane emissions at a selected number of points on the landfill surface using a specially designed flux chamber. The statistical analysis of the data obtained was based on the Sichel function and resulted in an average emission rate of 74.9 g·m?2·day?1, with 27.8 and 202.1 g·m?2·day?1 as the lower and upper limits of the 95% confidence interval, respectively. The total emission for the landfill, with an emitting surface of 335,000 m2, is 9.16 × 103 ton/yr. These values have been compared with those from three different models, with the model results being above the calculated mean emissions measured at the landfill, but below the upper confidence limit at 95%.

Implications: One of the main environmental problems arising from the presence of landfills is the emission of biogas (which mainly contains methane and carbon dioxide) into the atmosphere. Several experimental methods as well as models have been developed to quantify these emissions. In this work, the authors have compared the results obtained using experimental measurements with those provided by some local and international models using the default parameters proposed. The results obtained from the experimental method are in accordance with those provided by the models, although the models could be slightly overestimating these emissions.  相似文献   


15.

Background, aim and scope  

Landfill gas (LFG) tends to escape from the landfill surface even when LFG collecting systems are installed. Since LFG leaks are generally a noticeable percentage of the total production of LFG, the optimisation of the collection system is a fundamental step for both energy recovery and environmental impact mitigation. In this work, we suggest to take into account the results of direct measurements of gas fluxes at the air–cover interface to achieve this goal.  相似文献   

16.
Mercury-bearing material enters municipal landfills from a wide array of sources, including fluorescent lights, batteries, electrical switches, thermometers, and general waste; however, the fate of mercury (Hg) in landfills has not been widely studied. Using automated flux chambers and downwind atmospheric sampling, we quantified the primary pathways of Hg vapor releases to the atmosphere at six municipal landfill operations in Florida. These pathways included landfill gas (LFG) releases from active vent systems, passive emissions from landfill surface covers, and emissions from daily activities at each working face (WF). We spiked the WF at two sites with known Hg sources; these were readily detected downwind, and were used to test our emission modeling approaches. Gaseous elemental mercury (Hg(O)) was released to the atmosphere at readily detectable rates from all sources measured; rates ranged from approximately 1-10 ng m(-2) hr(-1) over aged landfill cover, from approximately 8-20 mg/hr from LFG flares (LFG included Hg(O) at microg/m3 concentrations), and from approximately 200-400 mg/hr at the WF. These fluxes exceed our earlier published estimates. Attempts to identify specific Hg sources in excavated and sorted waste indicated few readily identifiable sources; because of effective mixing and diffusion of Hg(O), the entire waste mass acts as a source. We estimate that atmospheric Hg releases from municipal landfill operations in the state of Florida are on the order of 10-50 kg/yr, substantially larger than our original estimates, but still a small fraction of current overall anthropogenic losses.  相似文献   

17.
A performance-based method for evaluating methane (CH4) oxidation as the best available control technology (BACT) for passive management of landfill gas (LFG) was applied at a municipal solid waste (MSW) landfill in central Washington, USA, to predict when conditions for functional stability with respect to LFG management would be expected. The permitted final cover design at the subject landfill is an all-soil evapotranspirative (ET) cover system. Using a model, a correlation between CH4 loading flux and oxidation was developed for the specific ET cover design. Under Washington’s regulations, a MSW landfill is functionally stable when it does not present a threat to human health or the environment (HHE) at the relevant point of exposure (POE), which was conservatively established as the cover surface. Approaches for modeling LFG migration and CH4 oxidation are discussed, along with comparisons between CH4 oxidation and biodegradation of non-CH4 organic compounds (NMOCs). The modeled oxidation capacity of the ET cover design is 15 g/m2/day under average climatic conditions at the site, with 100% oxidation expected on an annual average basis for fluxes up to 8 g/m2/day. This translates to a sitewide CH4 generation rate of about 260 m3/hr, which represents the functional stability target for allowing transition to cover oxidation as the BACT (subject to completion of a confirmation monitoring program). It is recognized that less than 100% oxidation might occur periodically if climate and/or cover conditions do not precisely match the model, but that residual emissions during such events would be de minimis in comparison with published limit values. Accordingly, it is also noted that nonzero net emissions may not represent a threat to HHE at a POE (i.e., a target flux between 8 and 15 g/m2/day might be appropriate for functional stability) depending on the site reuse plan and distance to potential receptors.

Implications: This study provides a scientifically defensible method for estimating when methane oxidation in landfill cover soils may represent the best available control technology for residual landfill gas (LFG) emissions. This should help operators and regulators agree on the process of safely eliminating active LFG controls in favor of passive control measures once LFG generation exhibits asymptotic trend behavior below the oxidation capacity of the soil. It also helps illustrate the potential benefits of evolving landfill designs to include all-soil vegetated evapotranspirative (ET) covers that meet sustainability objectives as well as regulatory performance objectives for infiltration control.  相似文献   


18.
Open dumping and landfilling are the prevalent solid waste disposal practices in Thailand. Surveys on the disposal sites revealed the presence of 95 landfills and 330 open dumps. Methane emission potential at these sites was estimated by three methods. Results of the Intergovernmental Panel on Climate Change (IPCC) method, Landfill Gas Emission model (LandGEM), and closed flux chamber technique were compared. The methane emission potential of 366 Gg/yr using the IPCC method was higher than the estimations of the LandGEM and closed flux chamber method of 115 Gg/yr and 103 Gg/yr, respectively. An understanding of the methane emission potential initiated the analysis of upgrading the open dumps into landfills, adding landfills to meet the future needs and utilization of landfill gases. Upgrading the open dumps to landfills increased the methane emission rates and their utilization potential. Approximately 20 additional landfills may be required to meet future demands. Landfill gas (LFG) utilization appears to be feasible in the large-scale landfills.  相似文献   

19.
An updated assessment of fine particle emissions from light- and heavy-duty vehicles is needed due to recent changes to the composition of gasoline and diesel fuel, more stringent emission standards applying to new vehicles sold in the 1990s, and the adoption of a new ambient air quality standard for fine particulate matter (PM2.5) in the United States. This paper reports the measurement of emissions from vehicles in a northern California roadway tunnel during summer 1997. Separate measurements were made of uphill traffic in two tunnel bores: one bore carried both light-duty vehicles and heavy-duty diesel trucks, and the second bore was reserved for light-duty vehicles. Ninety-eight percent of the light-duty vehicles were gasoline-powered. In the tunnel, heavy-duty diesel trucks emitted 24, 37, and 21 times more fine particle, black carbon, and sulfate mass per unit mass of fuel burned than light-duty vehicles. Heavy-duty diesel trucks also emitted 15–20 times the number of particles per unit mass of fuel burned compared to light-duty vehicles. Fine particle emissions from both vehicle classes were composed mostly of carbon; diesel-derived particulate matter contained more black carbon (51±11% of PM2.5 mass) than did light-duty fine particle emissions (33±4%). Sulfate comprised only 2% of total fine particle emissions for both vehicle classes. Sulfate emissions measured in this study for heavy-duty diesel trucks are significantly lower than values reported in earlier studies conducted before the introduction of low-sulfur diesel fuel. This study suggests that heavy-duty diesel vehicles in California are responsible for nearly half of oxides of nitrogen emissions and greater than three-quarters of exhaust fine particle emissions from on-road motor vehicles.  相似文献   

20.
ABSTRACT

This study models emissions quantities and neighboring exposure concentrations of six airborne pollutants, including PM10, PM2.5, crystalline silica, arsenic, uranium, and barium, which resulted from the disposal of Marcellus shale drill cuttings waste during the 2011–2017 period. Using these predicted exposures, this study evaluates current setback distances required in Pennsylvania from waste facilities. For potential residents living at the perimeter of the current setback distance, 274 m (900 ft), a waste disposal rate of 612.4 metric tons per day at landfills (the 99th percentile in record) does not result in exceedances of the exposure limits for any of the six investigated pollutants. However, the current setback distance can result in exceedance with respect to the 24-hr daily concentration standards for PM10 and PM2.5 established in the National Air Ambient Quality Standards (NAAQS), if daily waste disposal rate surpasses 900 metric tons per day. Dry depositions of barium-containing and uranium-containing particulate matter should not be a danger to public health based on these results. To investigate the air quality impacts of waste transportation and the potential for reductions, this article describes an optimization of landfill locations in Pennsylvania indicating the potential benefits in reduced environmental health hazard level possible by decreasing the distance traveled by waste disposal trucks. This strategy could reduce annual emissions of PM10 and PM2.5 by a mean of 64% and reduce the expected number of annual fatal accidents by nearly half, and should be considered a potential risk management goal in the long run. Therefore, policy to limit or encourage reduction of distances traveled by waste removal trucks and manage setback distances as a function of delivered waste quantities is merited.  相似文献   

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