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1.
The concentration of water-soluble organic nitrogen (WSON) in precipitation has been measured at seven sites across the United Kingdom, over a period of 1–2 years, using protocols developed in a pilot study. Samples were collected over 1–2 weeks in continuously open funnels made of stainless steel, draining to a glass bottle, and were preserved during and after collection by the addition of thymol. After chemical analysis, samples were excluded from the long-term average if they showed signs of contamination (significant concentrations of K+ or PO4 3?). Two methods of measuring total dissolved N were used, persulphate oxidation and high-temperature chemiluminescence. The latter generally gave the larger values, and has been used to asses the organic component of dissolved N. The long-term data set confirms the original results from the pilot study—organic N contributes between 24 and 40% to the total annual wet deposition of dissolved N across the United Kingdom. The fraction of WSON was greatest at western sites, and was strongly correlated with ammonium concentrations. However, the seasonal pattern across all sites showed a late spring maximum for ammonium and nitrate, but a late summer maximum for WSON. The magnitude of the contribution of WSON to wet-deposited N has implications for the setting and assessment of critical loads for N deposition. 相似文献
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Impact of Land Use on Soluble Organic Nitrogen in Soil 总被引:5,自引:0,他引:5
Victoria B. Willett James J. Green Andrew J. Macdonald John A. Baddeley Georg Cadisch Steven M. J. Francis Keith W. T. Goulding Gary Saunders Elizabeth A. Stockdale Christine A. Watson David L. Jones 《Water, Air, & Soil Pollution: Focus》2004,4(6):53-60
Although it has been hypothesized that soluble organic nitrogen (SON) plays a central role in regulating productivity in some terrestrial ecosystems, the factors controlling the size of the SON pool in soil remain poorly understood. Therefore our principal aim in this work was to assess the impact of seven different land use systems (rough and managed grassland, deciduous and coniferous woodland, heathland, wetland and tilled land) on the size of the SON and inorganic N (NO
3
–
, NH
4
+
) pools in the surface soil layer (0–15 cm). After extraction with deionised water, we found that in most cases the size of the water extractable organic N (WEON) pool was similar in size to the inorganic N pool. In contrast, the KCl extractable organic N (KClEON) pool constituted the dominant form of soluble N in soils under all land uses, perhaps indicating that significant amounts were held on the soil exchange phase. In contrast to inorganic N, which varied significantly with land use, the size of the KClEON and WEON pool was similar for all land uses with the exception of KClEON in tilled land, where significantly lower amounts were observed. We conclude that SON constitutes an important soil N pool in a broad range of land uses, and that its role in microbial N assimilation, plant nutrition and ecosystem responses to atmospheric N deposition warrants further attention.
SAFRD, University of Newcastle, Newcastle-upon-Tyne, NE1 7RU, U.K. 相似文献
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兼氧技术应用于有机污泥的处理 总被引:4,自引:0,他引:4
应用兼氧技术处理有机污泥,对处理过程中挥发性脂肪酸的生成、N元素的变化、兼氧微生物的种群进行了检测,结果表明,有机污泥经过24h兼氧反应后,污泥中的有机物得到降解,酸化反应生成了质量浓度的2531mg/L的乙酸;系统中NH3-N含量略有上升;兼氧反应过程中的微生物以异养型的产酸细菌为优势菌种。污泥被水解酸化后回流到废水处理系统,系统基本无剩余污泥排放。 相似文献
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Tim Chatterton Stephen Dorling Andrew Lovett Michael Stephenson 《Water, Air, & Soil Pollution: Focus》2002,2(5-6):173-187
This study uses a combination of data from U.K. monitoringstations and from modelling undertaken with the U.K.Meteorological Office's NAME Model to investigate therelative influences of primary and secondary particulateson total PM10 levels at sites in the United Kingdom. Co-located PM10 and sulphate aerosol measurementsindicate that sulphate has a disproportionately largeinfluence on the variation of PM10 levels incomparison to its contribution to their total mass.Comparisons of measured PM10 at urban centre, roadsideand rural sites suggest that local primary sources havevery little influence on daily mean levels. NAME has beenused to model both primary particles and sulphate aerosolfrom sources across the whole of Europe. The discrepanciesbetween modelled and observed PM10 suggest that coarseparticles, such as windblown dust and resuspended roaddust,may comprise a very large, if not dominant, proportion ofobserved PM10 levels. The apparently minor role ofprimary particles (especially locally-sourced ones) raisesa number of issues regarding the suitability of current U.K.and European legislation to addressing the particle problem. 相似文献
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Philip A. Meyers 《Water, Air, & Soil Pollution: Focus》2006,6(5-6):453-463
The isotopic and molecular compositions of organic matter buried in lake sediments provide information that helps to reconstruct
past environmental conditions and to assess impacts of humans on local ecosystems. This overview of sedimentary records from
the North American Great Lakes region describes examples of applications of organic geochemistry to paleolimnological reconstructions.
These lakes experienced a succession of human-induced environmental changes that started after completion of the Erie Canal
in 1825. Agricultural deforestation in the mid-nineteenth century released soil nutrients that increased algal productivity
and caused an associated increase in algal biomarkers in sediment records. Eutrophication that accompanied magnified delivery
of municipal nutrients to the lakes in the 1960s and 1970s created excursions to less negative δ13C values in sediment organic matter. Increased organic carbon mass accumulation rates mirror the isotopic evidence of eutrophication
in the Great Lakes. 相似文献
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Hall Jane Reynolds Brian Langan Simon Hornung Mike Kennedy Fiona Aherne Julian 《Water, Air, & Soil Pollution: Focus》2001,1(1-2):43-56
The Simple Mass Balance (SMB)equation has been developed and used as one ofthe principal methods for calculating criticalloads of acidity for forest ecosystems. Criticalloads have formed the basis for informing policyrelated to the control and abatement of emissionsof acidifying pollutants. The SMB equationrelies on a variety of assumptions and dataderived from a variety of sources. Each of thesecomponent constituents has a potential source oferror depending on the method(s) used for theirderivation and the value(s) assigned. The resultis the possibility of generating a range ofcritical load values for a single ecosystem. This paper summarises the SMB equation, examinesthe uncertainties in deriving input values andreviews other works on the key assumptions. 相似文献
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自来水厂常规净水工艺除有机污染物效果的监测 总被引:1,自引:0,他引:1
采用GC-MS/COMP技术对宁波梅林水厂姚江水源水及各净水工序出水中的有机污染物进行了监测,结果表明,姚江水中主要有机污染物为苯系物、多环芳烃、染料及中间体等,水厂现有的常规净水工艺对上述有机污染物的去除率较低。 相似文献
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The atmospheric deposition of reactive nitrogen on turf grassland in Tsukuba, central Japan, was investigated from July 2003
to December 2004. The target components were ammonium, nitrate, and nitrite ions for wet deposition and gaseous ammonia, nitric
and nitrous acids, and particulate ammonium, nitrate, and nitrite for dry deposition. Organic nitrogen was also evaluated
by subtracting the amount of inorganic nitrogen from total nitrogen. A wet-only sampler and filter holders were used to collect
precipitation and the atmospheric components, respectively. An inferential method was applied to calculate the dry deposition
velocity of gases and particles, which involved the effects of surface wetness and ammonia volatilization through stomata
on the dry deposition velocity. The mean fraction of the monthly wet to total deposition was different among chemical species;
37, 77, and 1% for ammoniacal, nitrate-, and nitrite-nitrogen, respectively. The annual deposition of inorganic nitrogen in
2004 was 47 and 48 mmol m−2 yr−1 for wet and dry deposition, respectively; 51% of atmospheric deposition was contributed by dry deposition. The annual wet
deposition in 2004 was 20, 27, and 0.07 mmol m−2 yr−1, and the annual dry deposition in 2004 was 35, 7.4, and 5.4 mmol m−2 yr−1 for ammoniacal, nitrate-, and nitrite-nitrogen, respectively. Ammoniacal nitrogen was the most important reactive nitrogen
because of its remarkable contribution to both wet and dry deposition. The median ratio of the organic nitrogen concentration
to total nitrogen was 9.8, 17, and 15% for precipitation, gases, and particles, respectively. 相似文献