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M. Yamada Y. Iwasaka A. Matsuki D. Trochkine Y. S. Kim D. Zhang T. Nagatani G.-Y. Shi M. Nagatani H. Nakata Z. Shen B. Chen G. Li 《Water, Air, & Soil Pollution: Focus》2005,5(3-6):231-250
Free tropospheric aerosol particles were collected using a balloon-borne particle impactor in August of 2002 and March of
2003 at Dunhuang in northwestern China (40°00′N, 94°30′E), and the morphology and elemental composition of the aerosol particles
were analyzed in order to understand the mixing state of coarse dust particles (diameter >1 μm) over the desert areas in the
Asian continent in spring. Electron microscopic experiments on the particles revealed that dust particles were major constituents
of coarse mode particles in the free troposphere over the Taklamakan Desert in spring and summer.
Si-rich or Ca-rich particles are major components of dust particles collected in the free troposphere over dunhuang and the
values of [number of Ca-rich particles]/[number of Si-rich particles] differs markedly between spring and summer, being about
0.3 in the spring of 2003 and about 1.0 in the summer of 2002 at heights 3–5 km above sea level. It is likely that the condition
of the ground surface and the strength of vertical mixing in source areas of Asian dust are potential factors causing the
difference in the chemical types of dust particles.
Comparison of the elemental compositions of these particles with those of particles collected over Japan strongly suggests
that these particles were chemically modified during their long-range transport in the free troposphere. Analysis of wind
systems shows that both the predominating westerly wind in the free troposphere and the surface wind strongly controlled by
the geographical structure of the Tarim Basin are important in the long-range transport of KOSA particles originating in the
Taklamakan Desert. 相似文献