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1.
Soil respiration rates of a clay-loam textured Acrisol under different uses (Atlantic forest, manioc, horticulture and pasture) from Rio de Janeiro State were measured. The relationship between carbon dioxide (CO2) emissions and soil physico-chemical properties were investigated. Rates of CO2 emission of two sites (Atlantic forest and horticulture) were also evaluated in different seasons in 1997 and 1998. In the forest site, monthly means of measured respiration rates showed good correlation with soil temperature in the range 19.6–24.1°C (r2 = 0.89). In the horticulture site, no change was observed with soil moisture alone, in the range 3.0–13.2 wt%. In the horticulture soil, even when the surface soil was very dry, respiration rates increased in the hot, wetter summer but remained higher than the mean flux from forest soil. The CO2 emission flux of the Acrisol under different use showed good correlation with soil temperature (r2 = 0.72) and moisture (r2 = 0.61).  相似文献   

2.
This paper summarized the study carried out in Krakow, Poland in 1975-76 on the estimated local air pollution as measured by carbon isotopes and total sulphur measurement in plants. Good correlation was found between δ14C value and the total sulphur (measured by radionuclide excited X-ray fluorescence) in beech leaves collected in the late summer, indicating the common source of both pollutants. Sampling and measurement of σ13C in atmospheric CO2 has shown that σ3C can be used as a pollution indicator only in the winter period when no fluctuations exist ddue to plant respiration. A method of CO2 sampling using molecular sieve proved to be feasible for instantaneous sampling with no isotope fractionation. The highest pollution by fossil CO2 was measured in winter (12.8% excess. During spring and summer the average contribution of fossil CO2 was 4.5 to 5.6%.  相似文献   

3.
This study was performed to investigate the concentration of PM10 and PM2.5 inside trains and platforms on subway lines 1, 2, 4 and 5 in Seoul, KOREA. PM10, PM2.5, carbon dioxide (CO2) and carbon monoxide (CO) were monitored using real-time monitoring instruments in the afternoons (between 13:00 and 16:00). The concentrations of PM10 and PM2.5 inside trains were significantly higher than those measured on platforms and in ambient air reported by the Korea Ministry of Environment (Korea MOE). This study found that PM10 levels inside subway lines 1, 2 and 4 exceeded the Korea indoor air quality (Korea IAQ) standard of 150 μg/m3. The average percentage that exceeded the PM10 standard was 83.3% on line 1, 37.9% on line 2 and 63.1% on line 4, respectively. PM2.5 concentration ranged from 77.7 μg/m3 to 158.2 μg/m3, which were found to be much higher than the ambient air PM2.5 standard promulgated by United States Environmental Protection Agency (US-EPA) (24 h arithmetic mean: 65 μg/m3). The reason for interior PM10 and PM2.5 being higher than those on platforms is due to subway trains in Korea not having mechanical ventilation systems to supply fresh air inside the train. This assumption was supported by the CO2 concentration results monitored in tube of subway that ranged from 1153 ppm to 3377 ppm. The percentage of PM2.5 in PM10 was 86.2% on platforms, 81.7% inside trains, 80.2% underground and 90.2% at ground track. These results indicated that fine particles (PM2.5) accounted for most of PM10 and polluted subway air. GLM statistical analysis indicated that two factors related to monitoring locations (underground and ground or inside trains and on platforms) significantly influence PM10 (p < 0.001, R2 = 0.230) and PM2.5 concentrations (p < 0.001, R2 = 0.172). Correlation analysis indicated that PM10, PM2.5, CO2 and CO were significantly correlated at p < 0.01 although correlation coefficients were different. The highest coefficient was 0.884 for the relationship between PM10 and PM2.5.  相似文献   

4.
Determined the contribution of root derived CO2 efflux to total CO2 efflux (including root and non-root derived CO2 efflux) is import to grope the mechanism of CO2 efflux, however, becaused of ‘rhizoshere priming effect’ (RPE), it is difficult to achieve in practice. In this study, we attempted to estimate the RPE via comparing basal soil respiration (Rb) achieved by two different methods namely, y-intercept regression and direct bare plot approach in an arid cotton field, central Asia. On the basis of the y-intercept of linear regressions between below-ground respiration (BGR) and root biomass, Rb was indirectly calculated. Comparing with the first approach, the second approach involved direct measurements of soil respiration from bare plots. Rb estimated by y-intercept method contained the component of RPE whereas direct bare plot did not. We found that RPE showed a phenological trend with highest value in flowering stage at 0.145 g CO2 m–2 h–1 and lowest at budding stage (0.007 g CO2 m–2 s–1), even after the data had been corrected for the influence of soil temperature. We concluded that RPE needed to be considered when Rb was estimated by y-intercept approach.  相似文献   

5.
The south east basin of France shelters deep CO2 reservoirs often studied with the aim of better constraining geological CO2 storage operations. Here we present new soil gas data, completing an existing dataset (CO2, 222Rn, 4He), together with mineralogical and physical characterisations of soil columns, in an attempt to better understand the spatial distribution of gas concentrations in the soils and to rule on the sealed character of the CO2 reservoir at present time.Anomalous gas concentrations were found but did not appear to be clearly related to geological structures that may drain deep gases up to the surface, implying a dominant influence of near surface processes as indicated by carbon isotope ratios. Coarse grained, quartz-rich soils favoured the existence of high CO2 concentrations. Fine grained clayey soils preferentially favoured the existence of 222Rn but not CO2. Soil formations did not act as barriers preventing gas migrations in soils, either due to water content or due to mineralogical composition. No abundant leakage from the Montmiral reservoir can be highlighted by the measurements, even near the exploitation well. As good correlation between CO2 and 222Rn concentrations still exist, it is suggested that 222Rn migration is also CO2 dependent in non-leaking areas - diffusion dominated systems.  相似文献   

6.
Economic Analysis of CO2 Emission Trends in China   总被引:1,自引:0,他引:1  
Climate change is one of hot spots all around the world. China, the second biggest CO2 emitter, is facing increasingly severe pressure to reduce CO2 emission. The article first describes Kaya Identity and its policy implications. Second, it uses the modified Kaya Identity and makes decomposition without residues on CO2 emission during the period 1971-2005. Taking into account the changes of macroeconomic background, it conducts a detailed analysis in terms of CO2 emission trend from 4th Five Year Plan through 10th Five Year Plan. The decomposition results indicate that economic development and increase in population are major driving forces, and that improvement in energy efficiency contributes to the reduction of CO2 emission, and that decarbonization in primary energy structure is also an important strategic choice. Finally, the article stresses that in CO2 order to realize the binding target of 20% reduction in GDP energy intensity during the 11th Five Year Plan, China should speed up the readjustment of the industrial structure and energetically develop the energy-efficient technologies and clean fuel technology, which will effectively promote the country to reduce CO2 emission and contribute to the mitigation of climate change.  相似文献   

7.
Oxidation of hydrocarbon in asphalt binder leads to the production of carbon dioxide (CO2) during the production of hot mix asphalt. The objective of this laboratory study was to investigate the effects of the asphalt additive Sasobit®, asphalt content and mixing/placement temperature on CO2 emissions from binder with laboratory measurements. The isolated effects of Sasobit on asphalt absorption into the aggregate were also looked at. Temperature was found to be the only statistically significant factor on emissions. This would suggest that warm mix asphalt technology, which employs the use of Sasobit in asphalt mixtures, is a very effective way of lowering the industry's CO2 emission impact, both directly and by the use of less energy for heating. This work predicts that greater than 30% reduction of CO2 emissions is possible with typically used levels of Sasobit.  相似文献   

8.
The study was conducted to assess the potential of Norwegian agricultural ecosystems to sequester carbon (C) based on the data from some long-term agronomic and land use experiments. The total emission of CO2 in Norway in 1998 was 41.4 million metric ton (MMT), of which agriculture contributed only 0.157 MMT, or <0.4% of the total emissions. With regards to methane (CH4) and nitrous oxide (N2O) gases, however, agricultural activities contributed 32.5% and 51.3% of their respective emissions in Norway. The soil organic carbon (SOC) losses associated with accelerated soil erosion in Norway are estimated at 0.475 MMTC yr–1. Land use changes and soil/crop management practices with potential for SOC sequestration include conservation tillage methods, judicious use of fertilizers and manures, use of crop residues, diverse crop rotations, and erosion control measures. The potential for SOC sequestration is 0.146 MMTC yr–1 for adopting conservation tillage, 0.011–0.035 MMTC yr–1 for crop residue management, 0.026 MMTC yr–1 for judicious use of mineral fertilizer, 0.016–0.135 MMTC yr–1 for manure application, and 0.036 MMTC yr–1 for adopting crop rotations. The overall potential of these practices for SOC sequestration ranges from 0.591 to 1.022 MMTC yr–1 with an average value of 0.806 MMTC yr–1. Of the total potential, 59% is due to adoption of erosion control measures, 5.8% to restoration of peat lands, 21% to conversion to conservation tillage and residue management, and 14% to adoption of improved cropping systems. Enhancing SOC sequestration and improving soil quality, through adoption of judicious land use and improved system of soil and crop management, are prudent strategies for sustainable management of soil, water and environment resources.Readers should send their comments on this paper to: bhaskarn ath@aol.com within 3 months of publication of this issue.  相似文献   

9.
Global atmospheric CO2 concentration has increased since the beginning of reliable monitoring in 1958 at a mean rate of about 0.9 ppm CO2/yr. Now, atmospheric CO2 concentration is at 330 ppm. From about 1860 up to 1974, man's intervention in the global carbon cycle caused a likely increase of 76.6 × 1015 gC, corresponding to 36 ppm CO2 in the atmosphere, if a preindustrial content of 294 ppm CO2 or 625.3 × 1015 g C is adopted to be valid. A further rise of atmospheric CO2 seems to be inevitable and probably will be responsible for a climatic warming in the next several decades; therefore, a global examination of carbon reservoirs and carbon fluxes has been undertaken to determine their storage capacity for excess carbon which orginated mainly from burning fossil fuels and from land clearing. During 1860–1974 about 136 × 1015 g C have ben emitted into the atmosphere by fossil fuel combustion and cement production. At present, the emission rate is about 5 × 1015 g C/yr. The worldwide examination of carbon release, primarily by deforestation and soil cultivation since 1860, is estimated to be about 120 × 1015 g C. The net transfer of carbon to the atmosphere owing to man's interference with the biosphere is now believed to be about 2.4 × 1015 g C/yr. An oceanic uptake of roughly 179 × 1015 g C since 1860 is open to discussion. According to the chemical buffering of sea surface water only about 35.5 × 1015 g C could have been absorbed. It is argued, however, that oceanic circulations might have been more effective in removing atmospheric excess carbon of anthropogenic origin.  相似文献   

10.
The air quality in a newly built preschool was investigated in a longitudinal study. Typical air contaminants emanating from building materials were determined, their variation over time (0–18 months) was measured, and the influence of the ventilation system (81%–91% recirculation of return air) on contaminant concentrations was studied. Volatile organic compounds were sampled by adsorption on porous polymer, analysed by a GC/FID system, and identified by MS. A spatial build-up in concentration (ppb or μg/m3 levels) is evident for all the organic compounds, as well as for CO2, from the outdoor air, through the ventilation system, and through the rooms to the exhaust air. The longitudinal comparison over time shows that all the organic compounds decline in concentration mainly within the first 6 months of occupancy: 1-butanol 4–14 times, toluene and pentanal + hexanal 2–4 times, while formaldehyde remained at a constant low level of 90 ppb (110 μg/m3). It is difficult to believe that the problems of poor air quality in 100 preschools in Stockholm are caused by the organic compounds alone unless interactions occur. A preschool building needs to be gassed off during the first 6 months after its construction with no recirculation of return air allowed (outdoor air rate approx 4–5 ach). During at least 1–2 additional years, it is desired that the recirculation rate of return air is restricted, perhaps to 50%.  相似文献   

11.
This study investigates the contribution of radon (222Rn)-bearing water to indoor 222Rn in thermal baths. The 222Rn concentrations in air were monitored in the bathroom and the bedroom. Particulate matter (PM, both PM10 and PM2.5) and carbon dioxide (CO2) were also monitored with portable analyzers. The bathrooms were supplied with hot spring water containing 66-260 kBq m−3 of 222Rn. The results show that the spray of hot spring water from the bath spouts is the dominant mechanism by which 222Rn is released into the air of the bathroom, and then it diffuses into the bedroom. Average 222Rn level was 110-410% higher in the bedrooms and 510-1200% higher in the bathrooms compared to the corresponding average levels when there was no use of hot spring water. The indoor 222Rn levels were influenced by the 222Rn concentrations in the hot spring water and the bathing times. The average 222Rn transfer coefficients from water to air were 6.2 × 10−4-4.1 × 10−3. The 24-h average levels of CO2 and PM10 in the hotel rooms were 89% and 22% higher than the present Indoor Air Quality (IAQ) standard of China. The main particle pollutant in the hotel rooms was PM2.5. Radon and PM10 levels in some hotel rooms were at much higher concentrations than guideline levels, and thus the potential health risks to tourists and especially to the hotel workers should be of great concern, and measures should be taken to lower inhalation exposure to these air pollutants.  相似文献   

12.
An incubation experiment was performed to study the effect of sewage sludge on microbial respiration and nutrient mineralization in a sandy soil as an indication of its effects on soil biological properties and nutrient transformation. Sewage sludge was amended with a sandy soil at 0, 25, 50, 150 and 350 g kg−1 fresh weight. An increase in the sludge amendment rate caused an increase in both pH and electrical conductivity (EC). However, pH decreased while EC increased and then decreased along the incubation time. Nevertheless salinity and heavy metal contents of the soil sludge mixture were all within the safety guidelines. Soluble NH4+, NO32− and PO32− increased after amending the soil with sewage sludge, but increasing the application rate to 350 g kg−1 of sludge decreased the N and P mineralization efficiency and created an adverse effect on nitrification. The daily CO2 evolution pattern was the same in all treatments that CO2 evolution increased initially and then decreased till the end of the incubation period. All the treatments had peak CO2 evolution at day 7, except for the soil amended with 350 g kg−1 of sludge which had peak CO2 evolution at day 2. Similarly, the percentage of C-mineralization decreased with an increase in sludge amendment rate. The present experiment indicated that an application rate of 50–150 g kg−1 sludge for sandy soil would have the optimal beneficial effect on the soil in terms of microbial activity and nutrient transformation.  相似文献   

13.
The influence of long-term exposure of model plantations at elevated atmospheric CO2 (550 ppm) on soil respiration under natural conditions has been studied using an automated Free-Air CO2 Enrichment (FACE) system at the Hokkaido University, Japan. In the course of the experiment, an attempt has been made to simulate the effect of forthcoming climate change on the process of CO2 emission from different soil types.  相似文献   

14.
The Pechelbronn oilfield (Rhine Graben, France), where mining activity ended in the 1960s, has been used for waste disposal for twenty years. Since the wastes are varied, work is underway to identify the discharged materials and their derivatives, as well as to locate and quantify potential discharge sites. Two major goals were assigned to the present work. The first was to identify or refine the location of hidden structures that could facilitate gas emanation up to the surface, by studying soil gas concentrations (mainly 222Rn, CO2, CH4 and helium) and carbon isotope ratios in the CO2 phase. The second was devoted to examining, from a health and safety viewpoint, if the use of the oilfield as a waste disposal site might have led to enhanced or modified gas emanation throughout the area.It appeared that CO2 and 222Rn evolution in the whole area were similar, except near some of the faults and fractures that are known through surface mapping and underground observations. These 222Rn and CO2 anomalies made it possible to highlight more emissive zones that are either related to main faults or to secondary fractures acting as migration pathways. In that sense, the CO2 phase can be used to evaluate 222Rn activities distant from tectonic structures but can lead to erroneous evaluations near to gas migration pathways. Dumping of wastes, as well as oil residues, did not appear to have a strong influence on soil gaseous species and emanation. Similarly, enhanced gas migration due to underground galleries and exploitation wells has not been established. Carbon isotope ratios suggested a balance of biological phenomena, despite the high CO2 contents reached. Other monitored gaseous species (N2, Ar, H2 and alkanes), when detected, always showed amounts close to those found subsurface and/or in atmospheric gases.  相似文献   

15.
This research was the first long-term attempt to concurrently measure and identify major sources of both PM10 and PM2.5 in Bangkok Metropolitan Region (BMR). Ambient PM10 and PM2.5 were evaluated at four monitoring stations and analyzed for elemental compositions, water-soluble ions, and total carbon during February 2002–January 2003. Fifteen chemical elements, four water-soluble ions, and total carbon were analyzed to assist major source identification by a receptor model approach, known as chemical mass balance. PM10 and PM2.5 were significantly different (p < 0.05) at all sites and 24 h averages were high at traffic location while two separated residential sites were similar. Seasonal difference of PM10 and PM2.5 concentrations was distinct between dry and wet seasons. Major source of PM10 at the traffic site indicated that automobile emissions and biomass burning-related sources contributed approximately 33% each. Automobiles contributed approximately 39 and 22% of PM10 mass at two residential sites while biomass burning contributed about 36 and 28%. PM10 from re-suspended soil and cooking sources accounted for 10 to 15% at a residential site. Major sources of PM2.5 at traffic site were automobile and biomass burning, contributing approximately 32 and 26%, respectively. Biomass burning was the major source of PM2.5 mass concentrations at residential sites. Meat cooking also accounted for 31% of PM2.5 mass at a low impact site. Automobile, biomass burning, and road dust were less significant, contributed 10, 6, and 5%, respectively. Major sources identification at some location had difficulty to achieve performance criteria due to limited source profiles. Improved in characterize other sources profiles will help local authority to better air quality.  相似文献   

16.
The effects of probable climate change—an increase in atmospheric CO2(by two times), air temperature, precipitation—on CO2exchange and temperature dependence of net photosynthesis in the larch and Siberian stone pine undergrowth formed in the light larch forests of West Siberia were studied in chambers with an artificial climate. The change of the aforementioned ecological factors caused an increase in the temperature optima of photosynthesis and the range of optimum temperatures (in the case of Siberian stone pine, to a slightly greater degree). Therefore, the ranges of both species may broaden, and the Siberian stone pine can expand to the north, displacing larch tree stands.  相似文献   

17.
We estimated carbon dioxide (CO2) and methane (CH4) emissions by diffusion, ebullition, and degassing in turbines from a semi-arid hydropower reservoir in northeastern Brazil. Sampling sites were allocated within the littoral and deeper waters of one embayment, the main-stream, and at turbines. Annual carbon emissions were estimated at 2.3?×?105?±?7.45?×?104 t C year?1, or in CO2-equivalents (CO2-eq) at 1.33?×?106?±?4.5?×?105 t CO2-eq year?1. Diffusion across the water surface was the main pathway accounting for 96% of total carbon emissions. Ebullition was limited to littoral areas. A slight accumulation of CO2, but not of CH4, in bottom waters close to the turbines inlet led to degassing emissions about 8?×?103 t C year?1. Emissions in littoral areas were higher than in main-stream and contribute to 40% of the total carbon. Carbon (C) emissions per electricity generated, at 60% of installed capacity, is 0.05 t C-CO2-eq MWh?1. The ratio increases to 0.09 t C-CO2 MWh?1, equating 80% of the emissions from natural gas and 40% of diesel or coal power plants. Retention time and benthic metabolism were identified as main drivers for carbon emissions in littoral areas, while water column mixing and rapid water flow are important factors preventing CH4 accumulation and loss by degassing. Our results indicate that Itaparica Reservoir, located in the semi-arid region of Northeastern Brazil, acts as a source of GHGs. Management measurements are needed to prevent emissions to raise in the future.  相似文献   

18.
The Syabru-Bensi hydrothermal zone, Langtang region (Nepal), is characterized by high radon-222 and CO2 discharge. Seasonal variations of gas fluxes were studied on a reference transect in a newly discovered gas discharge zone. Radon-222 and CO2 fluxes were measured with the accumulation chamber technique, coupled with the scintillation flask method for radon. In the reference transect, fluxes reach exceptional mean values, as high as 8700 ± 1500 g m−2 d−1 for CO2 and 3400 ± 100 × 10−3 Bq m−2 s−1 for radon. Gases fluxes were measured in September 2007 during the monsoon and during the dry winter season, in December 2007 to January 2008 and in December 2008 to January 2009. Contrary to expectations, radon and its carrier gas fluxes were similar during both seasons. The integrated flux along this transect was approximately the same for radon, with a small increase of 11 ± 4% during the wet season, whereas it was reduced by 38 ± 5% during the monsoon for CO2. In order to account for the persistence of the high gas emissions during monsoon, watering experiments have been performed at selected radon measurement points. After watering, radon flux decreased within 5 min by a factor of 2–7 depending on the point. Subsequently, it returned to its original value, firstly, by an initial partial recovery within 3–4 h, followed by a slow relaxation, lasting around 10 h and possibly superimposed by diurnal variations. Monsoon, in this part of the Himalayas, proceeds generally by brutal rainfall events separated by two- or three-day lapses. Thus, the recovery ability shown in the watering experiments accounts for the observed long-term persistence of gas discharge. This persistence is an important asset for long-term monitoring, for example to study possible temporal variations associated with stress accumulation and release.  相似文献   

19.
Carbon dioxide exchange was studied in the photosynthetic apparatus of Siberian spruce (Picea obovata Ledeb.), Siberian larch (Larix sibirica Ledeb.), and weeping birch (Betula pendula Roth.) in a mature spruce forest. Parameters of CO2 balance in different weather were characterized quantitatively on the basis of daily measurements of CO2 exchange in needles and leaves of woody plants. The percent ratios of the components of carbon balance in needles and leaves of woody plants depending on daily photosynthetic fixation of carbon were determined. In summer, trees consumed 210 kg CO2/ha (57 kg C/ha) in variable weather and 117 kg CO2/ha (32 kg C/ha) in cloudy weather. Species specificity of CO2 consumption was revealed, and the effects of environmental factors on the assimilatory activity of trees were determined.  相似文献   

20.
Establishing positive and urgent targets for CO2 reduction and emission peak, and promoting energy conservation and energy structure adjustment are among the strategies to address global climate change and CO2 emissions reduction. They are also means to break through the constraints of domestic resources and environment, and internal needs, to achieve sustainable development. Generally speaking, a country's CO2 emission peak appears after achieving urbanization and industrialization. By then, connotative economic growth will appear, GDP will grow slowly, energy consumption elasticity will decrease, and energy consumption growth will slow down – dependent mainly on new and renewable energies. Fossil fuel consumption will not increase further. When CO2 emission reaches its peak, the annual reduction rate of CO2 intensity of GDP is greater than GDP annual growth rate; and the annual reduction rate of CO2 intensity of energy use is greater than the annual growth rate of energy consumption. Therefore, three important approaches to promotion of CO2 emission peak can be concluded: maintaining reasonable control of GDP growth, strengthening energy conservation to significantly reduce the GDP energy intensity, and optimizing the energy mix to reduce the CO2 intensity of energy use. By around 2030, China will basically have completed its rapid development phase of industrialization and urbanization. Connotative economic growth will appear with the acceleration of industrial structure adjustment. The target of GDP energy intensity will still be to maintain an average annual reduction of 3% or higher. The proportion of non-fossil fuels will reach 20–25%, and the aim will be to maintain an average annual growth rate of 6–8%. The total annual energy demand growth of 1.5% will be satisfied by the newly increased supply of non-fossil fuels. The annual decline in CO2 intensity of GDP will reach 4.5% or higher, which is compatible with an average annual GDP growth rate of approximately 4.5% in order to reach CO2 emission peak. This corresponds to the level of China's potential economic growth. Achieving CO2 emission peak will not impose a rigid constraint on economic development, but rather promote economic development and accelerate the transformation of green, low-carbon development. The CO2 emission peak can be controlled with a cap of 11 billion tons, which means that CO2 emission will increase by less than 50% compared with 2010. The per capita emission peak will be controlled at a level of less than 8 tons, which is lower than the 9.5 tons in the EU and Japan and much lower than the 20 tons in the US, future economic and social development faces many uncertainties in achieving the CO2 emission peak discussed above. It depends on current and future strategies and policies, as well as the pace and strength of economic transformation, innovation, and new energy technologies. If the economic transformation pattern fails to meet expectations, the time required to reach CO2 emission peak would be delayed and the peak level would be higher than expected. Therefore, we need to coordinate thoughts and ideas and deploy these in advance; to highlight the strategic position of low-carbon development and its priorities; to enact mid- to long-term energy development strategies; and to establish and improve a system of laws, regulations, and policies as well as an implementation mechanism for green, low-carbon development. Oriented by positive and urgent CO2 reduction and peak targets, the government would form a reversed mechanism to promote economic transformation and embark on the path of green, low-carbon development as soon as possible.  相似文献   

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