Indoor air pollution and public policy

In recent years, scientist have come to realize that contaminated air inside buildings is a major route of human exposure to certain air pollutants. While scientific interest in the problem continues to grow, efforts to measure indoor pollution concentrations, define exposure levels, and estimate health risks remain in their infancy. Within this arena, policymakers must deal with the question of how best to protect public health and safety in the face of incomplete and often contradictory information. In the past, official response to environmental pollution has traditionally taken the form of “control by regulation.” However, creation of a regulatory framework for indoor air quality poses special policy issues that suggest the need to explore alternative modes of intervention. Ambient outdoor air is a public good, in the sense that enjoyment by one individual in no way detracts from use or enjoyment by others. Indoor air, on the other hand, is not a public good, especially in private residences. Costs and benefits of maintaining adequate indoor air quality are internalized within households, suggesting the possibility of a private demand for clean indoor air. Promulgation of indoor air quality standards and other regulations must confront the fact that individuals are already making decisions about their own air quality. Regulations might or might not improve these decisions. Development of effective and reasonable policy requires an appreciation of the scope for private action and consideration of the likelihood that public intervention will foster improved private choices. Among the logical and relatively inexpensive modes of intervention are public information programs, development of simple warning devices, and product testing and labeling.     

Olfactory and chemical characterization of indoor air. Towards a psychophysical model for air quality

The relationship between the odor strength of total air samples and the odor strengths of the constituents was investigated in three field experiments in an office building and a new preschool. The odor strength was scaled by magnitude estimation according to a master scale principle which results in comparable values for the total and the constituent odors. Between 60 and 120 chemical components were detected by GC/FID in the indoor air samples (N = 66). Most (81%) of the detected components in an air sample were odorous, even though most of them were of the low concentrations. By a method of pattern analysis, chemical as well as odor patterns of indoor air were found to be characteristics of different buildings. From the odor patterns (POG), the “odor print” of the outdoor air associated with the buildings was also recognized in the indoor air. Thus, the “odor print” of an air sample is different from its “chemical print”. A model was found that predicts the overall odor strength of an air sample from the number of FID-detected components most frequently reported to have a strong odor.     

Low-infiltration housing in Rochester, New York: A study of air-exchange rates and indoor air quality

A sample of 58 occupied homes in Rochester, NY, most of which incorporated special builder-designed weatherization components, were studied to assess (1) the effectiveness of construction techniques designed to reduce air leakage; (2) the indoor air quality and air-exchange rates in selected airtight houses, and (3) the impact on indoor air quality of mechanical ventilation systems employing air-to-air heat exchangers. The “specific leakage area” was measured in each house using the fan pressurization technique. Houses built with polyethylene vapor barriers and joint-sealing were as a group 50% tighter than a similar group of houses without such components. Mechanical ventilation systems with air-to-air heat exchangers were installed in nine relatively airtight houses, some of which had gas stoves and/or tobacco smoking occupants. Air-exchange rates and indoor concentrations of radon (Rn), formaldehyde (HCHO), nitrogen dioxide (NO₂), and humidity were measured in each house for 1-week periods with and without mechanical ventilation. More detailed measurements, including concentrations of carbon monoxide and inhalable particulates, were made in two of these houses by a mobile laboratory. In all nine houses, air-exchange rates were relatively low (0.2–0.5 ach) without mechanical ventilation, and yet indoor concentrations of Rn, HCHO, and NO₂ were below existing guidelines. Mechanical ventilation systems were effective in further reducing indoor contaminant concentrations. We conclude that when contaminant source strengths are low, acceptable indoor air quality can be compatible with low air-exchange rates.     

A study of effects of ambient urban air pollution using personal samplers; a preliminary report

Air pollution has been associated with an increased incidence of respiratory disease. However, significant differences may exist between air pollution levels measured at conventional fixed monitoring stations and actual levels inhaled by a subject. Furthermore, studies of effects of air pollution might best be done using asthmatics as study subjects, since they have irritable airways. This is a preliminary report of a study using a control and asthmatic group in which effects of air pollution are assessed by sympton and medication diaries and simple pulmonary function tests. Air pollution exposure is measured using a small portable sampler for particulates, SO₂ and NO₂; these samplers are carried by the subject (“personal”) and are situated inside and outside the home. Levels obtained are compared to data obtained from the same type of sampler located at a fixed monitoring station. Preliminary analysis of the data shows that the levels of pollutants are low and there are significant differences between the four air pollution measurements, with weak correlations among the various measurements. In this preliminary report, change in pulmonary function during the day correlates only with personal NO₂ measurements. This suggests the need for estimating air pollution exposure using “personal” samplers, when investigating health effects.     

Guidelines for Nordic building regulations regarding indoor air quality

A subcommittee of the Nordic Committee for Building Codes has released guidelines for building regulations regarding indoor air quality, especially concerning ventilation. The main features of the guidelines, such as acceptable outdoor air quality for ventilation and minimum outdoor air flows for dwellings and offices, are presented and discussed. Mechanical ventilation is, in principle, required in all buildings including dwellings, due to the requirement of a minimum outdoor air change of 0.5 h⁻¹ and the normal highly airtight nature of new buildings. The guidelines are a basis for designing energy-efficient buildings while maintaining an indoor air quality which provides acceptable comfort and does not impair health.     

Interactions between diesel emissions and gaseous copollutants in photochemical air pollution: Some health implications

A complete assessment of the health effects of diesel emissions must take into account the possible chemical transformations (and associated biological impacts) of particulate organic matter (POM) due to reactions with the many gaseous copollutants which have now been unambiguously demonstrated to be present in atmospheres burdened by photochemical air pollution. These copollutants include the “trace” species, nitric (HNO₃) and nitrous (HONO) acids, the nitrate radical (NO₃), formaldehyde (H₂CO) and formic acid (HCOOH), as well as the criteria pollutants, ozone (O₃) and nitrogen dioxide (NO₂). Techniques for establishing the atmospheric concentrations of the trace pollutants (and their spatial and temporal variations) are briefly described, and we present results of investigations into the reactions of polycyclic aromatic hydrocarbons (PAH) coated on filters and exposed to ambient concentrations of O₃ and NO₂. Environmental health implications of these results are discussed and include the potential for sampling “artifacts” and their possible effects on the correlation (or lack thereof) between ambient PAH levels and urban lung cancer rates, as well as the problems associated with understanding the appropriate POM “dose” to be employed in animal testing and assessments of impacts on human health.     

Efficient ventilation in office rooms

Results from a two-box model for calculation of tracer gas concentrations in rooms are given and consequences of different definitions of “ventilation efficiency” are discussed. Results from three different series of experiments are presented. The first two series were dilution experiments; examples of the results are given and discussed. The third series of tests was performed with one person working at a desk in the test room. Above the person;s head, a tracer gas (N₂O) was injected into the convection plume, with as low momentum as possible. Starting with zero concentration, a test continued until steady-state conditions were established for the concentration levels in the different parts of the room. The tests included simulation of summer, autumn/spring, and winter daytime conditions. The results indicate a tendency towards lower tracer gas concentrations in the “breathing zone” when the supply air (typical flow rate equivalent to two air changes per hour) is brought into the room at a low level as compared to a high level close to the ceiling. The exhaust air terminal device in all tests was situated high in the “corridor” wall.     

Volatile organic compounds in indoor environment and photocatalytic oxidation: state of the art

Volatile organic compounds (VOCs) are the major pollutants in indoor air, which significantly impact indoor air quality and thus influencing human health. A long-term exposure to VOCs will be detrimental to human health causing sick building syndrome (SBS). Photocatalytic oxidation of VOCs is a cost-effective technology for VOCs removal compared with adsorption, biofiltration, or thermal catalysis. In this paper, we review the current exposure level of VOCs in various indoor environment and state of the art technology for photocatalytic oxidation of VOCs from indoor air. The concentrations and emission rates of commonly occurring VOCs in indoor air are presented. The effective catalyst systems, under UV and visible light, are discussed and the kinetics of photocatalytic oxidation is also presented.     

Suspended particulate matter in dwellings — the impact of tobacco smoking

The indoor concentration of suspended particulate matter (SPM) was measured in forty-four retrofitted and tight dwellings, which had electric cooking and were central heated and where the basic ventilation rate in median amounted 0.23 air changes per hour as measured with a tracer dilution method. The indoor concentration of SPM was in median 230 μg/m³ with a strong correlation to the tobacco consumption (r_s=0.716), but with no correlation to the frequency of airing or the basic ventilation rate. Tobacco smoking seems to be the main indoor source of SPM in contemporary dwellings. The importance of these findings is underlined by epidemiologic studies on passive smoking and health. Air quality standards for the ambient air are based on certain risk groups such as infants, children, persons with chronic obstructive lung disorders, and indoor air standards should be based on the same concepts of health protection.     

Methods for control of indoor air quality

This report presents results of a review of available methods for control of environmental hazards applied to indoor air pollutants. Indoor air pollution originates from transport of ambient outdoor air contaminants into occupied spaces by natural infiltration ventilation, or by mechanical ventilation using outdoor makeup air, plus contributions from indoor emission sources. When air exchange with the external ambient environment is reduced to conserve energy, contributions from indoor emission sources may dominate indoor air pollutant levels. This paper identifies alternative methods available to control indoor air pollutant exposures. The performance characteristics of ventilation systems and of air cleaning devices used in mixed modes for ventilation of occupied spaces are described. Models for predicting effectiveness of several alternative modes are reviewed, with field trial validation results cited where available. Results of previous confined-space studies are briefly reviewed as points of departure for consideration of necessary air quality, ventilation, and air cleaning. Understanding of indoor air contaminant generation and controls is aided by examination of earlier studies of indoor air quality, using modern perspectives on occupational environmental health and hygiene.     

Impact of climate change on the domestic indoor environment and associated health risks in the UK

There is growing evidence that projected climate change has the potential to significantly affect public health. In the UK, much of this impact is likely to arise by amplifying existing risks related to heat exposure, flooding, and chemical and biological contamination in buildings. Identifying the health effects of climate change on the indoor environment, and risks and opportunities related to climate change adaptation and mitigation, can help protect public health.We explored a range of health risks in the domestic indoor environment related to climate change, as well as the potential health benefits and unintended harmful effects of climate change mitigation and adaptation policies in the UK housing sector. We reviewed relevant scientific literature, focusing on housing-related health effects in the UK likely to arise through either direct or indirect mechanisms of climate change or mitigation and adaptation measures in the built environment. We considered the following categories of effect: (i) indoor temperatures, (ii) indoor air quality, (iii) indoor allergens and infections, and (iv) flood damage and water contamination.Climate change may exacerbate health risks and inequalities across these categories and in a variety of ways, if adequate adaptation measures are not taken. Certain changes to the indoor environment can affect indoor air quality or promote the growth and propagation of pathogenic organisms. Measures aimed at reducing greenhouse gas emissions have the potential for ancillary public health benefits including reductions in health burdens related heat and cold, indoor exposure to air pollution derived from outdoor sources, and mould growth. However, increasing airtightness of dwellings in pursuit of energy efficiency could also have negative effects by increasing concentrations of pollutants (such as PM_2.5, CO and radon) derived from indoor or ground sources, and biological contamination. These effects can largely be ameliorated by mechanical ventilation with heat recovery (MVHR) and air filtration, where such solution is feasible and when the system is properly installed, operated and maintained. Groups at high risk of these adverse health effects include the elderly (especially those living on their own), individuals with pre-existing illnesses, people living in overcrowded accommodation, and the socioeconomically deprived.A better understanding of how current and emerging building infrastructure design, construction, and materials may affect health in the context of climate change and mitigation and adaptation measures is needed in the UK and other high income countries. Long-term, energy efficient building design interventions, ensuring adequate ventilation, need to be promoted.     

Air pollution control policy in the Federal Republic of Germany as a strategy for dealing with environmental risks

The paper describes criteria for the development of energy systems, with emphasis on “environmental compatibility.” It outlines the main objectives underlying political and regulatory action in the Federal Republic of Germany to ensure this compatibility through the management of environmental risks. The air pollution control policy in the Federal Republic of Germany is presented as a strategy for risk management, focusing on its philosophy and on the recent ordinances concerning air pollution control in large firing (combustion) installations.     

Physical characterization of diesel exhaust particles in exposure chambers

Since the deposition of particulate in the respiratory system is strongly influenced by particle size, a correct assessment of this parameter is important for any inhalation experiment studying the potential health effects of air pollutants. Measuring the distribution of particles according to their aerodynamic diameter and mechanical mobility diameter is crucial in analyzing the deposition of submicron particles in the lower respiratory system. Cascade impactor measurements of diluted diesel exhaust in 12.6 m³ animal exposure chambers in the GMR Biomedical Science Department showed that the mass median aerodynamic diameter of the aerosol was 0.2 μm with 88% of the mass in particles smaller than 1 μm. Diffusion battery measurements showed that the mass median mechanical mobility diameter was about 0.11 μm. Transmission electron micrographs of particles deposited on chamber surfaces revealed both agglomerates and nearly spherical particles. The particles in these chambers are similar in size and shape to diesel particles described elsewhere. The flux of diesel particles to food surfaces was measured. Calculations of the expected daily dose by inhalation and by feeding showed that the “worst case” dose by feeding was only about one-tenth the dose by breathing.     

The effect of air control systems on the indoor distributions of viable particles

We have investigated the filtering effects of three types of air control systems of enclosed structures on viable particles in the ambient air. Aspergillus fumigatus and other thermophilic organisms were used as monitors for viable particles. The indoor concentrations of viable particles were found to be affected by building design and the use of conventional mechanical air systems. Viable particles of approximately 4.0 μm and greater in aerodynamic diameter were filtered from the air while respirable size particles less than 4.0 μm were not filtered as well. There was evidence of growth of viable particles within the mechanical air systems. Conventional air control systems may not be adequate for the control of viable particle contamination of the indoor environment without modifications and proper maintenance.     

Chemical dusts, vapours, and fumes causing asthma

Allergic respiratory disease due to common allergens of organic origin is wwell known. Less familiar, but of increasing importance, are chemicals of organic and inorganic nature, met as dusts, vapours, and fumes. Their relevance is shown in occupational respiratory allergic disorders. Confirmation is given by “real life,” simulated, occupational-type provocation tests. Controlled exposure with minute amounts for brief periods, thus closely simulating allergic sensitivity, can precisely identify etiological causes in often complex exposures. The capacity of these widely different agents in different forms to elicit the different patterns of asthmatic reactions, is a pointed example of their potential role, as well as the role of chemical agents in general. The introduction into indoor environments of such materials demands consideration of their possible allergenic ffects and of the need to recognise the various forms of allergic respiratory reaction they may cause.     

Pilot field study: Carbon monoxide exposure monitoring in the general population

A pilot field study was conducted with nine members of the general public to measure carbon monoxide exposure using personal monitors. The principal study objectives were to design and evaluate the research protocol and the instrumentation performance for application to the conduct of a large-scale personal monitoring program. Integrated carbon monoxide exposure was monitored and recorded according to type of activity such as “commuting” or “at work” for approximately 45 days by each subject. All subjects except one were able to handle both the equipment and data recording requirements with no significant problems. Actual data recording responsibilities consumed less than 10 min daily. The data consisted of 355 person-days each over 6-h duration, and weekdays only, from which 8-h average personal exposure levels could be computed. The 9 ppm (μL/L) ambient air quality standard was exceeded on 22 person-days. Elevated carbon monoxide concentrations during the commuting activity were frequently associated with the exceedences.     

Detection of fluorotelomer alcohols in indoor environments and their relevance for human exposure

Fluorotelomer alcohols (FTOH) are important precursors of perfluorinated carboxylic acids (PFCA). These neutral and volatile compounds are frequently found in indoor air and may contribute to the overall human exposure to per- and polyfluorinated alkyl substances (PFAS). In this study air samples of ten workplace environments and a car interior were analysed. In addition, extracts and emissions from selected outdoor textiles were analysed in order to establish their potential contribution to the indoor levels of the above-mentioned compounds.Concentrations of FTOHs measured in air ranged from 0.15 to 46.8, 0.25 to 286, and 0.11 to 57.5 ng/m³ for 6:2, 8:2 and 10:2 FTOHs, respectively. The highest concentrations in air were identified in shops selling outdoor clothing, indicating outdoor textiles to be a relevant source of FTOH in indoor workplace environments. Total amounts of FTOH in materials of outdoor textiles accounted for < 0.8–7.6, 12.1–180.9 and 4.65–105.7 μg/dm² for 6:2, 8:2 and 10:2 FTOHs, respectively. Emission from selected textiles revealed emission rates of up to 494 ng/h.The measured data show that a) FTOHs are present in indoor textiles (e.g. carpets), b) they are released at ambient temperatures and c) indoor air of shops selling outdoor textiles contains the highest levels of FTOH. Exposure of humans to perfluorooctanoic acid (PFOA) through absorption of FTOH and subsequent degradation is discussed on the basis of indoor air levels. Calculation of indoor air-related exposure using the median of the measured air levels revealed that exposure is on the same order of magnitude as the recently reported dietary intakes for a background-exposed population. On the basis of the 95th percentile, indoor air exposure to PFOA was estimated to exceed dietary exposure. However, indoor air-related intakes of FTOH are far below the tolerable daily intake (TDI) of PFOA, indicating that there is no risk to health, even when assuming an unrealistic complete degradation of FTOH into PFOA.     

Two-year follow-up study of nonregulatory recommendations for better air quality in indoor ice arenas

A standardized questionnaire was used in a two-year follow-up study to test the effectiveness of non-regulatory recommendations to improve indoor air quality of 103 ice arenas in Finland. In addition, the performance of a state-of-the-art emission control technology (ECT) on propane-fueled resurfacers was evaluated by measuring the one-week average nitrogen dioxide (NO₂) concentration in a small sample of arenas. The number of retrofitted ECT on propane-fueled resurfacers increased from 6 to 37 (8% to 37% of ice arenas) and the number of electric resurfacers from 7 to 9 (both 9% of arenas) in 1994–1996. At the same time, the prevalence of inadequate ventilation increased among the most susceptible small arenas (volume <30 000 m³) from 11 (31%) to 19 (38%). Combustion-powered resurfacers (88%) and inadequate ventilation (24%) were prevalent also among the 17 new arenas built in 1994–1996. ECT resurfacers significantly decreased the mean indoor NO₂ concentration of eleven arenas from 650 μg/m³ to 147 μg/m³. Thus, retrofitting resurfacers with ECT seems to be a feasible mitigation option to improve indoor air quality in ice arenas, but the ultimate solution is an electric ice resurfacer. Non-regulatory recommendations seem to be partially effective in abatement against the air quality problems, but additional regulatory measures are needed for full compliance in all arenas.     

Improving the efficiency of free-jet scrubbers

A free-jet scrubber is an innovative gas cleaner in which the primary liquid/gas contacting takes place in the turbulent mixing zone emanating from a jet nozzle. The first such devices, powered by supersonic steam or air ejectors, were exceptionally effective cleaners but were criticized as being high-energy users. A great reduction in the energy consumption of free-jet scrubbers has been accomplished in the last four years, a feat which may seem in contradiction to the “contacting power rule.” An explanation of what is happening in these devices must take into account the effectiveness with which energy and water are utilized. thereby leading one to a somewhat circular definition of “effective contacting power.” The theoretical implication of this analysis is primarily to remind us that there are many paths between two states and some are more energy efficient than others. The practical value is that such analysis generates information which aids in choosing between several design options, a direct benefit of the various free-jet configurations.