The impact of electric passenger transport technology under an economy-wide climate policy in the United States: Carbon dioxide emissions,coal use,and carbon dioxide capture and storage

Plug-in hybrid electric vehicles (PHEVs) have the potential to be an economic means of reducing direct (or tailpipe) carbon dioxide (CO₂) emissions from the transportation sector. However, without a climate policy that places a limit on CO₂ emissions from the electric generation sector, the net impact of widespread deployment of PHEVs on overall U.S. CO₂ emissions is not as clear. A comprehensive analysis must consider jointly the transportation and electricity sectors, along with feedbacks to the rest of the energy system. In this paper, we use the Pacific Northwest National Laboratory's MiniCAM model to perform an integrated economic analysis of the penetration of PHEVs and the resulting impact on total U.S. CO₂ emissions. In MiniCAM, the deployment of PHEVs (or any technology) is determined based on its relative economics compared to all other methods of providing fuels and energy carriers to serve passenger transportation demands. Under the assumptions used in this analysis where PHEVs obtain 50–60% of the market for passenger automobiles and light-duty trucks, the ability to deploy PHEVs under the two climate policies modelled here results in over 400 million tons (MT) CO₂ per year of additional cost-effective emissions reductions from the U.S. economy by 2050. In addition to investments in nuclear and renewables, one of the key technology options for mitigating emissions in the electric sector is CO₂ capture and storage (CCS). The additional demand for geologic CO₂ storage created by the introduction of the PHEVs is relatively modest: approximately equal to the cumulative geologic CO₂ storage demanded by two to three large 1000 megawatt (MW) coal-fired power plants using CCS over a 50-year period. The introduction of PHEVs into the U.S. transportation sector, coupled with climate policies such as those examined here, could also reduce U.S. demand for oil by 20–30% by 2050 compared to today's levels.     

Assessment of a reclamation cover system for phosphogypsum stacks in Central Alberta, Canada

Phosphogypsum (PG), a byproduct of the phosphate fertilizer industry, was produced and stockpiled at the Agrium Fort Saskatchewan facility from 1965 to 1991. Upon decommissioning, the outer slopes of the PG stacks were reclaimed by applying 15 cm of topsoil and planting a non-native seed mix. Physical, chemical, and hydrologic evaluations of the cover system confirmed that plants were successfully growing in various soil capping depths and were often rooting more than 200 mm into the PG. Percolation past the substrate into PG during a typical storm event was low (< 10 mm), and runoff from the stacks was negligible. Runoff quality met most guidelines, but some parameters, including fluoride, were up to 18 times higher than provincial or federal guidelines for soil and water quality. However, the cover system, when applied appropriately, does meet basic reclamation objectives. The exceedances are found in areas where the cover system has been compromised by erosion or mixing or in areas where the cover system has not been fully applied, such as roads or the inner basin. In areas where the cover system has been applied successfully, basic reclamation requirements are met.     

Cumulative Industrial Activity Alters Lotic Fish Assemblages in Two Boreal Forest Watersheds of Alberta,Canada

We evaluated the cumulative effects of land use disturbance resulting from forest harvesting, and exploration and extraction of oil and gas resources on the occurrence and structure of stream fish assemblages in the Kakwa and Simonette watersheds in Alberta, Canada. Logistic regression models showed that the occurrence of numerically dominant species in both watersheds was related to two metrics defining industrial activity (i.e., percent disturbance and road density), in addition to stream wetted width, elevation, reach slope, and percent fines. Occurrences of bull trout, slimy sculpin, and white sucker were negatively related to percent disturbance and that of Arctic grayling, and mountain whitefish were positively related to percent disturbance and road density. Assessments of individual sites showed that 76% of the 74 and 46 test sites in the Kakwa and Simonette watersheds were possibly impaired or impaired. Impaired sites in the Kakwa Watershed supported lower densities of bull trout, mountain whitefish, and rainbow trout, but higher densities of Arctic grayling compared to appropriate reference sites. Impaired sites in the Simonette Watershed supported lower densities of bull trout, but higher densities of lake chub compared to reference sites. Our data suggest that current levels of land use disturbance alters the occurrence and structure of stream fish assemblages.     

“The Schweinrich structure”, a potential site for industrial scale CO2 storage and a test case for safety assessment in Germany

The identification of risks associated with the geological storage of CO₂ requires methods that can analyse and assess potential safety hazards. This paper evaluates how performance assessment can be used as a method for assessing the impact of CO₂ storage on health, safety and the environment (HSE) with particular respect to potential future aquifer storage in the anticlinal structure Schweinrich in Germany. The performance assessment was conducted under the CO2STORE European Fifth Framework project as one of the four cases on the aquifer storage of CO₂. It is known as the Schwarze Pumpe case study.Being a case study, it is restrictive from a feasibility study point of view—i.e., the extended identification of the key safety factors where an actual CO₂ storage project would be considered for the Schweinrich structure. The study is based on data currently available, gathered in prior surveys, and on the use of simplified models, with CO₂ leakage levels from natural analogues being the evaluation criteria. While the results should be interpreted as provisional, they point out clearly which additional data should be gathered in relation to the long-term storage performance in the event that the site warrants further investigation.     

Legal and regulatory challenges in the implementation of CO2 geological storage: An Alberta and Canadian perspective

Alberta is the province with the largest CO₂ emissions in Canada, with approximately two-thirds of emissions originating from large stationary sources. Due to the fortuitous association of large CO₂ sources with the storage capacity offered by the underlying Alberta basin, it is expected that large-scale CO₂ geological storage in Canada will occur in Alberta first, and both levels of governments are contemplating measures to facilitate implementation. A review of the current provincial and federal legislation and regulations presented in this paper indicates that the existing legal and regulatory regime is reasonably sufficient, with some modifications, to accommodate the active injection phase of CO₂ capture and storage (CCS) operations, and the early takers of this new technology. However, governments in Alberta and Canada, and likely everywhere, need to address several pressing issues dealing mainly with the CCS post-operational phase. These issues, reviewed in this paper from an Alberta and Canadian perspective, fall into several categories: jurisdictional, property (ownership), regulatory and liability. Because Alberta is a landlocked province, matters relating to CO₂ storage under the seabed will not be addressed here except when discussing matters of jurisdiction and CO₂ classification. Possible models for post-injection liability transfer to the state are also presented. Although this review is focused on western Canada conditions, the issues are broad enough to be of interest in other jurisdictions, which may also adopt parts of the legal and regulatory framework that is quite well developed in Alberta.     

Hazardous waste site identification using aerial photography: A pilot study in Burlington County,New Jersey,USA

The objective of the project was to identify all hazardous waste sites in Burlington County, New Jersey that could be detected on existing, medium-scale aerial photographs of the county. The complete set of over 1000 black- and-white stereopairs at a scale of 1:12,000 was carefully examined for initial identification of possible sites. All suspicious sites were examined again on color transparencies of the county at the same 1:12,000 scale. Out of the 1094 black- and-white photos, 250 required further checking on color transparencies using a zoom stereoscope. This examination resulted in a final identification of 67 sites, the locations of which were delineated on 1:24,000 USGS maps. The use of air photo interpretation techniques provided an effective procedure for identifying waste sites quickly as well as providing a useful demonstration program for county and state officials.     

How organizational motives and communications affect public trust in organizations: The case of carbon dioxide capture and storage

Preventing climate change is among the greatest environmental challenges facing the world today. Recently developed carbon dioxide capture and storage (CCS) technology is an important strategy to mitigate climate change. Public trust in organizations involved in CCS technology is important for successful implementation of this technology. This work adresses how inferred organizational motives and organizational communications affect public trust in these organizations. Study 1 (N = 264) showed that Dutch citizens generally have less trust in the industrial organizations than in the environmental NGOs involved in CCS. As predicted, inferred organizational motives (organization-serving motives versus public-serving motives) accounted for this difference. In Study 2 (N = 78) and Study 3 (N = 51) we used experimental designs. Both experiments showed that organizations that communicated arguments incongruent with inferred organizational motives instigated less trust than organizations that communicated arguments congruent with inferred organizational motives. Study 3 additionally showed that communicating an incongruent and a congruent argument together diminished the negative effects of the incongruent argument. In both Study 2 and Study 3 the effect of congruency on trust was mediated by perceived honesty of the organizations.     

CO2 storage and enhanced coalbed methane recovery: Reservoir characterization and fluid flow simulations of the Big George coal,Powder River Basin,Wyoming, USA

Coalbeds are an attractive geological environment for storage of carbon dioxide (CO₂) because CO₂ is retained in the coal as an adsorbed phase and the cost of injection can be offset by enhanced coalbed methane (ECBM) production. This paper presents the findings of a CO₂ storage feasibility study on coalbeds in the Wyodak-Anderson coal zone of the Powder River Basin, Wyoming, USA, using reservoir characterization and fluid flow simulations. A 3D numerical model of the Big George coal was constructed using geostatistical techniques, with values of cleat and matrix permeability and porosity constrained through history-matching of production data from coalbed methane (CBM) wells in the field area.Following history-matching, several ECBM and CO₂ storage scenarios were investigated: shrinkage and swelling of the coal was either allowed or disallowed, a horizontal hydraulic fracture was either placed at the injection well or removed from the model, the number of model layers was varied between 1 and 24, and the permeability and porosity fields were constructed to be either homogeneous or heterogeneous in accordance with geostatistical models of regional variability. All simulations assumed that the injected gas was 100% CO₂ and that the coalbed was overlain by an impermeable caprock. Depending on the scenario, the simulations predicted that after 13 years of CO₂ injection, the cumulative methane production would be enhanced by a factor of 1.5–5. Including coal matrix shrinkage and swelling in the model predicted swelling near the injection well, which resulted in a slight reduction (10%) in injection rate. However, including a horizontal hydraulic fracture in the model at the base of the injection well helped mitigate the negative effect of swelling on injection rate. It was also found that six model layers were needed to have sufficient resolution in the vertical direction to account for the buoyancy effects between the gas and resident water, and that capturing the heterogeneous nature of the coal permeability and porosity fields predicted lower estimates of the storage capacity of the Wyodak-Anderson coal zone.After noting that gravity and buoyancy were the major driving forces behind gas flow within the Big George coal, several leakage scenarios were also investigated, in an effort to better understand the interplay between diffusion and flow properties on the transport and storage of CO₂. The modeling predicted that the upward migration of gas due to the buoyancy effect was faster than the diffusion of CO₂ and therefore the gas rapidly rose to the top of the coalbed and migrated into overlying strata when an impermeable caprock was not included in the model.     

Fresh, stockpiled, and composted beef cattle feedlot manure: nutrient levels and mass balance estimates in Alberta and Manitoba

The fate of manure nutrients in beef cattle (Bos taurus) feedlots is influenced by handling treatment, yet few data are available in western Canada comparing traditional practices (fresh handling, stockpiling) with newer ones (composting). This study examined the influence of handling treatment (fresh, stockpiled, or composted) on nutrient levels and mass balance estimates of feedlot manure at Lethbridge, Alberta, and Brandon, Manitoba. Total carbon (TC) concentration of compost (161 kg Mg(-1)) was lower (P < 0.001) than stockpiled (248 kg Mg(-1)), which was in turn lower (P < 0.001) than fresh manure (314 kg Mg(-1)). Total nitrogen (TN) concentration was not affected by handling treatment while total phosphorus (TP) concentration increased with composting at Lethbridge. The percent inorganic nitrogen (PIN) was lower (P < 0.01) for compost (5.1%) than both fresh (24.7%) and stockpiled (28.9%) manure. Composting led to higher (P < 0.05) dry matter (DM) losses (39.8%) compared to stockpiling (22.5%) and higher (P < 0.05) total mass (water + DM) losses (65.6 vs. 35.2%). Carbon (C) losses were higher (P < 0.01) with composting (66.9% of initial) than with stockpiling (37.5%), as were nitrogen (N) losses (46.3 vs. 22.5%, P < 0.05). Composting allowed transport of two times as much P as fresh manure and 1.4 times as much P as stockpiled manure (P < 0.001) on an "as is" basis. Our study looked at one aspect of manure management (i.e., handling treatment effects on nutrient concentrations and mass balance estimates) and, as such, should be viewed as one component in the larger context of a life cycle assessment.     

华东地区碳源、碳汇和碳生产力研究

从碳源、碳汇和碳生产力的角度深入研究了华东地区6省1市2005-2011年之间低碳经济发展现状,采用变异系数和空间自相关等分析方法对该地区碳源、碳汇和碳生产力差异大小及其空间聚集特性进行了分析,以期为分析华东地区乃至全国低碳经济发展现状和趋势提供借鉴.     

Investigations on CO2 storage capacity in saline aquifers: Part 1. Dimensional analysis of flow processes and reservoir characteristics

The CO₂ storage capacity of geological reservoirs is of great interest for the selection of potential storage sites in carbon capture and storage (CCS) projects. A detailed analysis essentially requires a thorough understanding of the interaction of forces acting within the system. By defining characteristic quantities for length, time, pressure and velocity, the governing multiphase flow equations can be non-dimensionalised. This allows for the definition of physically sound dimensionless numbers, resembling the ratios of acting forces like viscous, capillary and gravitational forces. An analysis of the relation of forces in reservoirs with different parameter setups allows their intercomparison with respect to their CO₂ storage capacity potential. To back up the analysis, a comprehensive reservoir parameter database with more than 1200 reservoirs is analysed and statistical characteristics are derived. Effects of reservoir parameters like depth, temperature, absolute and relative permeability, as well as capillary pressure are investigated. It is shown that dimensionless numbers can be used to qualitatively order reservoirs with respect to the forces acting in the reservoir. Moreover, it is shown that the relative permeability relations together with the residual saturations have a great influence on the balance of forces.     

Carbon dioxide efflux from soil with poultry litter applications in conventional and conservation tillage systems in northern Alabama

Increased CO2 release from soils resulting from agricultural practices such as tillage has generated concerns about contributions to global warming. Maintaining current levels of soil C and/or sequestering additional C in soils are important mechanisms to reduce CO2 in the atmosphere through production agriculture. We conducted a study in northern Alabama from 2003 to 2006 to measure CO2 efflux and C storage in long-term tilled and non-tilled cotton (Gossypium hirsutum L.) plots receiving poultry litter or ammonium nitrate (AN). Treatments were established in 1996 on a Decatur silt loam (clayey, kaolinitic thermic, Typic Paleudults) and consisted of conventional-tillage (CT), mulch-tillage (MT), and no-tillage (NT) systems with winter rye [Secale cereale (L.)] cover cropping and AN and poultry litter (PL) as nitrogen sources. Cotton was planted in 2003, 2004, and 2006. Corn was planted in 2005 as a rotation crop using a no-till planter in all plots, and no fertilizer was applied. Poultry litter application resulted in higher CO2 emission from soil compared with AN application regardless of tillage system. In 2003 and 2006, CT (4.39 and 3.40 micromol m(-2) s(-1), respectively) and MT (4.17 and 3.39 micromol m(-2) s(-1), respectively) with PL at 100 kg N ha(-1) (100 PLN) recorded significantly higher CO2 efflux compared with NT with 100 PLN (2.84 and 2.47 micromol m(-2) s(-1), respectively). Total soil C at 0- to 15-cm depth was not affected by tillage but significantly increased with PL application and winter rye cover cropping. In general, cotton produced with NT conservation tillage in conjunction with PL and winter rye cover cropping reduced CO2 emissions and sequestered more soil C compared with control treatments.     

CO2 capture and storage from a bioethanol plant: Carbon and energy footprint and economic assessment

Biomass energy and carbon capture and storage (BECCS) can lead to a net removal of atmospheric CO₂. This paper investigates environmental and economic performances of CCS retrofit applied to two mid-sized refineries producing ethanol from sugar beets. Located in the Region Centre France, each refinery has two major CO₂ sources: fermentation and cogeneration units. “carbon and energy footprint” (CEF) and “discounted cash flow” (DCF) analyses show that such a project could be a good opportunity for CCS early deployment. CCS retrofit on fermentation only with natural gas fired cogeneration improves CEF of ethanol production and consumption by 60% without increasing much the non renewable energy consumption. CCS retrofit on fermentation and natural gas fired cogeneration is even more appealing by decreasing of 115% CO₂ emissions, while increasing non renewable energy consumption by 40%. DCF shows that significant project rates of return can be achieved for such small sources if both a stringent carbon policy and direct subsidies corresponding to 25% of necessary investment are assumed. We also underlined that transport and storage cost dilution can be realistically achieved by clustering emissions from various plants located in the same area. On a single plant basis, increasing ethanol production can also produce strong economies of scale.     

Environmental concentrations of agricultural herbicides in Saskatchewan, Canada: bromoxynil, dicamba, diclofop, MCPA, and trifluralin

Herbicides are the most commonly used group of agricultural pesticides on the Canadian Prairies and, in 1990, more than 20000 Mg of herbicides were applied in the provinces of Alberta, Saskatchewan, and Manitoba. The present paper reports on environmental concentrations of five herbicides currently used in the prairie region. The herbicides bromoxynil [3,5-dibromo-4-hydroxy-benzonitrile], dicamba [3,6-dichloro-o-anisic acid], diclofop [(RS)-2-[4-(2,4-dichlorophenoxy)-phenoxy]propanoic acid], MCPA [(4-chloro-2-methylphenoxy)acetic acid], and trifluralin [alpha,alpha,alpha-trifluoro-2,6-dinitro-N,N-isopropyl-p-toluidine] were measured in the atmosphere, bulk atmospheric deposits, surface film, and dugout (pond) water at two sites near Regina, Saskatchewan, during 1989 and 1990. All five herbicides were detected in air and surface film and all but trifluralin were detected in the bulk atmospheric deposits and dugout water. Trifluralin was most frequently detected in air (79% of samples) whereas bromoxynil was present in maximum concentration (4.2 ng m(-3)). MCPA was present in maximum levels in bulk atmospheric (wet plus dry) deposits (2350 ng m(-2) d(-1)), surface film (390 ng m(-2)), and dugout water (330 ng L(-1)), whereas dicamba was most frequently detected in surface film (47%) and dugout water (97%). The highest quantities of the herbicides tended to be present during or immediately after the time of regional application.     

CO2 transportation for carbon capture and storage: Sublimation of carbon dioxide from a dry ice bank

Climate change is being caused by greenhouse gases such as carbon dioxide (CO₂). Carbon capture and storage (CCS) is of interest to the scientific community as one way of achieving significant global reductions of atmospheric CO₂ emissions in the medium term. CO₂ would be captured from large stationary sources such as power plants and transported via pipelines under high pressure conditions to underground storage. If a downward leakage from a surface transportation system module occurs, the CO₂ would undergo a large temperature reduction and form a bank of “dry ice” on the ground surface; the sublimation of the gas from this bank represents an area source term for subsequent atmospheric dispersion, with an emission rate dependent on the energy balance at the bank surface. Gaseous CO₂ is denser than air and tends to remain close to the surface; it is an asphyxiant, a cerebral vasodilator and at high concentrations causes rapid circulatory insufficiency leading to coma and death. Hence a subliming bank of dry ice represents safety hazard. A model is presented for evaluating the energy balance and sublimation rate at the surface of a solid frozen CO₂ bank under different environmental conditions. The results suggest that subliming gas behaves as a proper dense gas (i.e. it remains close to the ground surface) only for low ambient wind speeds.     

Carbon isotope ratios in logged and unlogged boreal forests: Examination of the potential for determining wildlife habitat use

Due to assimilation of recycled CO₂ from litter decomposition and photosynthetic changes in carbon fractionation at low light levels, the foliage at the base of a forest is often more depleted in¹³C compared to that exposed to the atmosphere in either the canopy or in open clearings. This is referred to as the canopy effect. African research has indicated that these habitat differences in foliar ¹³C can be substantial enough to affect the carbon isotope ratios of resident fauna. Previous work documenting a 30-year chronology on moose teeth from Isle Royale National Park indicated a progressive depletion in¹³C and suggested that this could be due to forest regrowth following extensive burning. The present study examined the assumption implicit in this hypothesis that foliar ¹³C varies between open and closed boreal forest sites. I found a marginal canopy effect of 2 ¹³C difference between upper canopy and ground flora for a forest in northwestern Ontario and an average difference of 1.2 in under- and mid-story vegetation between closed forests and open clear-cuts. Because of these small differences, the utility of carbon isotope analysis in quantifying temporally integrated exploitation of deforested habitats will be low for northern boreal locations. In denser forests, such as those in the tropics or western North American where the canopy effect can be expected to be much greater, ¹³C analysis may still offer some promise for determining selection by wildlife of disturbed habitats.     

Carbon dioxide flux as affected by tillage and irrigation in soil converted from perennial forages to annual crops

Among greenhouse gases, carbon dioxide (CO(2)) is one of the most significant contributors to regional and global warming as well as climatic change. A field study was conducted to (i) determine the effect of soil characteristics resulting from changes in soil management practices on CO(2) flux from the soil surface to the atmosphere in transitional land from perennial forages to annual crops, and (ii) develop empirical relationships that predict CO(2) flux from soil temperature and soil water content. The CO(2) flux, soil temperature (T(s)), volumetric soil water content (theta(v)) were measured every 1-2 weeks in no-till (NT) and conventional till (CT) malt barley and undisturbed soil grass-alfalfa (UGA) systems in a Lihen sandy loam soil (sandy, mixed, frigid Entic Haplustoll) under irrigated and non-irrigated conditions in western North Dakota. Soil air-filled porosity (epsilon) was calculated from total soil porosity and theta(v) measurements. Significant differences in CO(2) fluxes between land management practices (irrigation and tillage) were observed on some measurement dates. Higher CO(2) fluxes were detected in CT plots than in NT and UGA treatments immediately after rainfall or irrigation. Soil CO(2) fluxes increased with increasing soil moisture (R(2)=0.15, P<0.01) while an exponential relationship was found between CO(2) emission and T(s) (R(2)=0.59). Using a stepwise regression analysis procedure, a significant multiple regression equation was developed between CO(2) flux and theta(v), T(s) (CO(2) [Formula: see text] ; R(2)=0.68, P0.01). Not surprisingly, soil temperature was a driving factor in the equation, which accounted for approximately 59% in variation of CO(2) flux. It was concluded that less intensive tillage, such as no-till or strip tillage, along with careful irrigation management will reduce soil CO(2) evolution from land being converted from perennial forages to annual crops.