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To apply PET depolymerization in supercritical methanol to commercial recycling, the benefits of supercritical methanol usage in PET depolymerization was investigated from the viewpoint of the reaction rate and energy demands. PET was depolymerized in a batch reactor at 573 K in supercritical methanol under 14.7 MPa and in vapor methanol under 0.98 MPa in our previous work. The main products of both reactions were the PET monomers of dimethyl terephthalate (DMT) and ethylene glycol (EG). The rate of PET depolymerization in supercritical methanol was faster than that of PET depolymerization in vapor methanol. This indicates supercritical fluid is beneficial in reducing reaction time without the use of a catalyst. We depicted the simple process flow of PET depolymerization in supercritical methanol and in vapor methanol, and by simulation evaluated the total heat demand of each process. In this simulation, bis-hydroxyethyl terephthalate (BHET) was used as a model component of PET. The total heat demand of PET depolymerization in supercritical methanol was 2.35 x 10(6)kJ/kmol Produced-DMT. That of PET depolymerization in vapor methanol was 2.84 x 10(6)kJ/kmol Produced-DMT. The smaller total heat demand of PET depolymerization in supercritical methanol clearly reveals the advantage of using supercritical fluid in terms of energy savings. 相似文献
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There are size-related differences in the use of feeding habitats (planktonic or benthic; oceanic or neritic) by adult female loggerhead sea turtles (Caretta caretta) within Japanese populations. We thus hypothesized that the differences may be reflected in their remigration and growth patterns, and investigated the relationships between body size and remigration intervals, growth rates, and remigration percentages, for female loggerheads nesting on a Japanese beach between 1991 and 2001. Although remigration intervals, growth rates, and remigration percentages were not significantly different among females, there were trends for longer remigration intervals and lower remigration percentages in smaller females. All females grew little. Considering these results along with previous findings, we speculated on the life-history strategy of female Japanese loggerheads.Communicated by T. Ikeda, Hakodate 相似文献
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A method for regional-scale material flow and decoupling analysis: A demonstration case study of Aichi prefecture, Japan 总被引:6,自引:0,他引:6
Junzo Tachibana Keiko Hirota Naohiro Goto Koichi Fujie 《Resources, Conservation and Recycling》2008,52(12):1382-1390
We have developed a method to analyse the annual material flow in a prefecture and have calculated environmental indicators for a prefecture. Material flow analysis (MFA) is important to clarify the structure of a regional society and obtain environmental indicators for a circular society. However, MFA has not advanced in local governments because of few local statistics. We have developed a method to analyse the annual material flow in Aichi prefecture from 1980 to 2000 using an input–output (I–O) table and statistics of Aichi. We have verified the accuracy of this method by comparing its results for 2000 which calculated on the basis of official I–O table for 1995 with the I–O table data for 2000; the correlation coefficient obtained in this case is greater than 0.95. Moreover, by performing MFA, we have estimated the resource consumption and decoupling indicator of each industry in Aichi prefecture from 1980 to 2000. We could obtain more detailed and accurate environmental indicators by using our method. From these results, we could estimate the progress of Aichi prefecture towards a circular society. 相似文献
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Wahyudiono Mitsuru Sasaki Motonobu Goto 《Journal of Material Cycles and Waste Management》2011,13(1):68-79
The conversion of biomass waste into resources as a recycling process is receiving increased interest due to the perceived
need for a sustainable global carbon cycle and environmental considerations. Several treatment processes are being developed.
Hydrothermal treatment is one of the most effective approaches, because water at high temperatures and high pressures behaves
as a reaction medium with remarkable properties. In this work, the reaction behavior of guaiacol as a biomass model compound
was studied in subcritical water at 483–563 K and in supercritical water at 653–673 K using a batch reactor. Guaiacol can
be considered representative of the aromatic ring structures present in lignin, a major component of woody biomass. The chemical
species formed in aqueous products were identified by gas chromatography/mass spectrometry and quantified using high-performance
liquid chromatography. The effect of pressure and reaction time on the conversion process of guaiacol is discussed. The results
obtained indicate that this method has potential for efficient organic waste conversion. 相似文献