Environmental Science and Pollution Research - According to the “fetal origin of disease” hypothesis, air pollution exposure in pregnancy may play an important role in stimulating the... 相似文献
Recent calculations of carbon dioxide (CO2) emissions have faced challenges because data consist of only partial information, which is called “incomplete information.” According to the emission factor method, energy consumption and CO2 emission factors with incomplete information may lead to unmatched multiplication between themselves, which affects accuracy and increases uncertainties in emission results. To address a specific case of incomplete information that has not been fully explored, we studied the effects of incomplete condition information on the estimates of CO2 emissions from liquefied natural gas (LNG) in China. Based on Chinese LNG sampling data, we obtained the specific-country CO2 emission factor for LNG in China and calculated the corresponding CO2 emissions. By applying hypothesis testing, regression analysis, variance analysis, or Monte Carlo (MC) simulations, the effects of incomplete information on the uncertainty of CO2 emission calculations in three cases were analyzed. The results indicate that calorific values have more than a 9.8% impact on CO2 emission factors and CO2 emissions with incomplete sample information. Regarding incomplete statistical information, the impact of statistical temperature on CO2 emissions exceeds 5.5%. Regarding incomplete sample and statistical information, sample and statistical temperatures can individually increase estimate biases by more than 5.2%. Significantly, the impacts of sample temperature and statistical temperature may offset each other. Therefore, the incomplete condition information is quite important and cannot be ignored in the estimation of CO2 emissions from LNG and international fair comparison.
Biochar (BC) and activated carbon (AC) were both produced from corn straw. Biochar-supported zerovalent iron (BC-ZVI) and activated carbon-supported zerovalent iron (AC-ZVI) were synthesized and applied for Se(IV)/Se(VI) removal. The sorption capacity of BC-ZVI for Se(IV) and Se(VI) was reported at 62.52 and 35.39 mg g?1, higher than that of AC-ZVI (56.02 and 33.24 mg g?1), respectively, due to its higher iron content and more positive charges. The spectroscopic analyses showed that Se(IV)/Se(VI) were reduced to Se(0)/Se(-II) of less toxicity and solubility. The effects of various factors such as pH, ionic strength, co-existing cations and anions, and natural organic matter (NOM) were also investigated. Ionic strength showed no significant effect on Se(IV)/Se(VI) removal, but pH was critical. The presence of NO3? and SO42? did not cause obvious inhibition to the removal, while PO43? inhibited the sorption capacity of BC-ZVI and AC-ZVI for Se(IV)/Se(VI) significantly. Common cations (K+, Ca2+, and Mg2+) were found to slightly enhance the removal, while NOM significantly decreased the sorption capacity of BC-ZVI and AC-ZVI for Se(IV)/Se(VI). Besides, NOM showed stronger inhibition effect on AC-ZVI than that on BC-ZVI. These results indicated that BC-ZVI, compared with AC-ZVI, could be a promising sorbent to remove Se(IV)/Se(VI) due to its low cost and high efficiency.
Environmental Science and Pollution Research - Ectomycorrhizal fungi can enhance the tolerance of plants to heavy metal stress by reducing the accumulation of heavy metals in the aerial parts of... 相似文献
In this study, m-xylene biodegradation was examined in bacteria-water mixed solution and biotrickling filter (BTF) systems amended with the nonionic surfactant Tween 80. The mixed bacteria were obtained from the activated sludge of a coking plant through a multisubstrate acclimatization process. High-throughput sequencing analysis revealed that Rhodanobacter sp. was the dominant species among the mixed bacteria. In the bacteria-water mixed solution, the bacterial density increased with increasing Tween 80 concentration. Hence, Tween 80 could be utilized as substrate by the mixed bacteria. Tween 80, with concentrations of 50–100 mg L?1, could enhance the bioavailability of m-xylene and consequently improve the degradation efficiency of m-xylene. However, further increasing the initial concentration of Tween 80 would decrease the degradation efficiency of m-xylene. At concentrations exceeding 100 mg L?1, Tween 80 was preferentially degraded by the mixed bacteria over m-xylene. In BTF systems, when the m-xylene inlet concentration was 1200 mg m?3 and the empty bed residence time was 20 sec, the removal efficiency and elimination capacity of BTF1 with Tween 80 addition were at most 20% and 24% higher than those of BTF2 without Tween 80 addition. Overall, the integrated application of the mixed bacteria and surfactant was demonstrated to be a highly effective strategy for m-xylene waste gas treatment.Implications: The integrated application of mixed bacteria and surfactant was demonstrated to be a promising approach for the highly efficient removal of m-xylene. Surfactant can activate mixed bacteria to degrade m-xylene by increasing its bioavailability. Besides, surfactant can be utilized as carbon source by the mixed bacteria so that the growth of mixed bacteria can be promoted. It is expected that the integrated application of both technologies will become more common in future chemical industry. 相似文献