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101.
Lability of drinking water treatment residuals (WTR) immobilized phosphorus: aging and pH effects 总被引:3,自引:0,他引:3
Time constraints associated with conducting long-term (>20 yr) field experiments to test the stability of drinking water treatment residuals (WTR) sorbed phosphorus (P) inhibit improved understanding of the fate of sorbed P in soils when important soil properties (e.g., pH) change. We used artificially aged samples to evaluate aging and pH effects on lability of WTR-immobilized P. Artificial aging was achieved through incubation at elevated temperatures (46 or 70 degrees C) for 4.5 yr, and through repeated wetting and drying for 2 yr. Using a modified isotopic ((32)P) dilution technique, coupled with a stepwise acidification procedure, we monitored changes in labile P concentrations over time. This technique enabled evaluation of the effect of pH on the lability of WTR-immobilized P. Within the pH range of 4 to 7, WTR amendment, coupled with artificial aging, ultimately reduced labile P concentrations by > or = 75% relative to the control (no-WTR) samples. Soil samples with different physicochemical properties from two 7.5-yr-old, one-time WTR-amended field sites were utilized to validate the trends observed with the artificially aged samples. Despite the differences in physicochemical properties among the three (two field-aged and one artificially aged) soil samples, similar trends of aging and pH effects on lability of WTR-immobilized P were observed. Labile P concentrations of the WTR-amended field-aged samples of the two sites decreased 6 mo after WTR amendment and the reduction persisted for 7.5 yr, ultimately resulting in > or = 70% reduction, compared to the control plots. We conclude that WTR application is capable of reducing labile P concentration in P-impacted soils, doing so for a long time, and that within the commonly encountered range of pH values for agricultural soils WTR-immobilized P should be stable. 相似文献
102.
Sand-sized particles (>63 microm) in whole storm water samples collected from urban runoff have the potential to produce data with substantial bias and/or poor precision both during sample splitting and laboratory analysis. New techniques were evaluated in an effort to overcome some of the limitations associated with sample splitting and analyzing whole storm water samples containing sand-sized particles. Wet-sieving separates sand-sized particles from a whole storm water sample. Once separated, both the sieved solids and the remaining aqueous (water suspension of particles less than 63 microm) samples were analyzed for total recoverable metals using a modification of USEPA Method 200.7. The modified version digests the entire sample, rather than an aliquot, of the sample. Using a total recoverable acid digestion on the entire contents of the sieved solid and aqueous samples improved the accuracy of the derived sediment-associated constituent concentrations. Concentration values of sieved solid and aqueous samples can later be summed to determine an event mean concentration. 相似文献
103.
Cost-efficient sample designs for collection of ground data and accurate mapping of variables are required to monitor natural
resources and environmental and ecological systems. In this study, a sample design and mapping method was developed by integrating
stratification, model updating, and cokriging with Landsat Thematic Mapper (TM) imagery. This method is based on the spatial
autocorrelation of variables and the spatial cross-correlation among them. It can lead to sample designs with variable grid
spacing, where sampling distances between plots vary depending on spatial variability of the variables from location to location.
This has potential cost-efficiencies in terms of sample design and mapping. This method is also applicable for mapping in
the case in which no ground data can be collected in some parts of a study area because of the high cost. The method was validated
in a case study in which a ground and vegetation cover factor was sampled and mapped for monitoring soil erosion. The results
showed that when the sample obtained with three strata using the developed method was used for sampling and mapping the cover
factor, the sampling cost was greatly decreased, although the error of the map was slightly increased compared to that without
stratification; that is, the sample cost-efficiency quantified by the product of cost and error was greatly increased. The
increase of cost-efficiency was more obvious when the cover factor values of the plots within the no-significant-change stratum
were updated by a model developed using the previous observations instead of remeasuring them in the field. 相似文献
104.
George William Kajjumb Rachael E. Bokot Matias Attene-Ramos Erica J. Marti 《环境科学学报(英文版)》2022,34(7):295-304
In the race to deliver clean water to communities through potable water reuse, disinfection and water quality assessment are and will continue to be fundamental factors. There are over 700 disinfection byproducts (DBPs) in water; evaluating each compound is practically impossible and very time consuming. A bioanalytical approach could be an answer to this challenge. In this work, the response of four major classes of DBPs toward mitochondrial membrane potential (ΔΨm) and cytoplasmic adenosine triphosphate (C-ATP) was investigated with human carcinoma (HepG2) cells. Within 90 min of cell exposure, only the haloacetic acid (HAA) mixture caused a cytotoxic response as measured by C-ATP. All four groups (haloacetonitriles (HANs), trihalomethanes (THMs), nitrosamines (NOAs), and HAAs) responded well to ΔΨm, R2 > 0.70. Based on the half-maximum concentration that evoked a 50% response in ΔΨm, the response gradient was HANs >> HAAs ∼ THM > NOAs. The inhibition of the ΔΨm by HANs is driven by dibromoacetonitrile (DBAN), while dichloroacetonitrile (DCAN) did not cause a significant change in the ΔΨm at less than 2000 µM. A mixture of HANs exhibited an antagonistic behavior on the ΔΨm compared to individual compounds. If water samples are concentrated to increase HAN concentrations, especially DBAN, then ΔΨm could be used as a biomonitoring tool for DBP toxicity. 相似文献
105.
Excessive exploitation of and skewed access to dwindling water resources raise serious water justice concerns. Environmental justice movements and related literature have raised critical questions regarding the unequal distribution of the costs and benefits of a development paradigm that is founded on excessive exploitation and appropriation of natural resources. This paper explores the growing relevance of a water justice framework that addresses both the social and ecological aspects of water use and appropriation, with reference to a four-decade long water conflict over the Chaliyar River in Kerala, South India. It highlights how ecosystem degradation and denial of justice go hand in hand. The paper argues that the framing and articulation of the conflict in a partisan manner led to the glossing over of certain critical features, thus preventing a full view of water injustices. It also failed to inform subsequent policies and practices in this regard. 相似文献
106.
107.
Zoning and applying Limits of Acceptable Change (LAC) are two promising strategies for managing tourism in Marine Protected
Areas (MPAs). Typically, these management strategies require the collection and integration of ecological and socioeconomic
data. This problem is illustrated by a case study of Koh Chang National Marine Park, Thailand. Biophysical surveys assessed
coral communities in the MPA to derive indices of reef diversity and vulnerability. Social surveys assessed visitor perceptions
and satisfaction with conditions encountered on snorkelling tours. Notably, increased coral mortality caused a significant
decrease in visitor satisfaction. The two studies were integrated to prescribe zoning and “Limits of Acceptable Change” (LAC).
As a biophysical indicator, the data suggest a LAC value of 0.35 for the coral mortality index. As a social indicator, the
data suggest that a significant fraction of visitors would find a LAC value of under 30 snorkellers per site as acceptable.
The draft zoning plan prescribed four different types of zones: (I) a Conservation Zone with no access apart from monitoring
or research; (II) Tourism Zones with high tourism intensities at less vulnerable reefs; (III) Ecotourism zones with a social
LAC standard of <30 snorkellers per site, and (IV) General Use Zones to meet local artisanal fishery needs. This study illustrates
how ecological and socioeconomic field studies in MPAs can be integrated to craft zoning plans addressing multiple objectives. 相似文献
108.
Marvin E. Miller George C. Holzworth 《Journal of the Air & Waste Management Association (1995)》2013,63(1):46-50
An urban diffusion model, which does not require the use of an electronic computer, is presented. The main simplifying assumptions are that continuous pollutant sources are uniformly distributed over the urban area and vertical diffusion occurs until the effluent from each line source reaches the top of the mixing layer, after which the effluent is uniformly distributed through the mixing layer. After the appropriate vertical diffusion coefficient is specified, the calculated concentration is a function of source strength, linear dimension of the metropolis, mixing depth, and wind speed. The calculated concentration is interpreted either as a representative maximum concentration or, through integration, as the average concentration over the metropolitan area. When a representative pollutant concentration is known, the model may be used to determine the apparent “uniform” source strength. 相似文献
109.
Gregory F. Mclsaac Matthew B. Short George Groschen Paul Terrio 《Journal of the American Water Resources Association》2004,40(2):443-459
ABSTRACT: Long term data on surface water quality can sometimes be assembled by combining data collected by different agencies at different times and assuming that between agency differences in data quality are insignificant. The objective of this paper was to assess the quality of riverine nitrate (NO3) concentrations in Illinois measured and reported by four agencies from 1967 to 1974 by comparing median values for similar sampling locations and periods. A total of 17 river reaches were identified for which two agencies reported NO3 concentrations during similar periods. Nonparametric comparison of median values and analysis of covariance with discharge as a covariant produced similar results. Nitrate concentrations reported by the U.S. Geological Survey (USGS) from 1967 to 1971 were not statistically (P > 0.05) different from values reported by the Illinois State Water Survey (ISWS) for two of three river reaches. Additionally, NO3 concentrations reported by USGS from 1972 to 1974 were not statistically different than concentrations reported by the Illinois Environmental Protection Agency (IEPA) for four of five river reaches. From 1969 to 1971, NO3 concentrations reported by the Illinois Department of Public Heath and the Illinois Environmental Protection Agency (IDPH/IEPA) were less than one‐fourth the magnitude of values reported by ISWS. The median NO3 concentrations measured by the Central Illinois Public Service (CIPS) were significantly greater than those measured by USGS and IDPH/IEPA in the three comparable sampling locations. The use of NO3 concentrations measured by CIPS and IDPH/IEPA prior to 1972 is not recommended. 相似文献
110.
Lance S. Evans George R. Hendrey Keith H. Thompson 《Journal of the Air & Waste Management Association (1995)》2013,63(11):1107-1116
Published results of four field experiments testing effects of acidic precipitation in field-grown soybeans have led to contradictory conclusions. This paper examines the experimental procedures and protocols of the four experiments which could have contributed to differences in both the reported crop yields and the interpretations or conclusions drawn from the experiments. The most important difference among the experiments is in their statistical designs. Two of the field layouts used only one plot per treatment, providing replication only for plants, rows or sectors within plots, but not among plots. By using real data from a highly replicated experiment it is shown that with such deficient statistical designs treatment effects cannot be separated from other microenvironmental variables peculiar to a specific plot location. The other two experiments were highly replicated. They were designed to detect differences of approximately 10% among treatment means. Type 1 error, a, was predetermined, and replication was sufficient to keep type 2 error low. This design was made possible because a preliminary experiment was available to estimate the expected components of variance. Despite differences in the procedures and protocols among the four experiments, it is primarily the quality of the experimental design which has determined their validity and relative utility for crop loss assessment. 相似文献