全文获取类型
收费全文 | 381篇 |
免费 | 2篇 |
国内免费 | 1篇 |
专业分类
安全科学 | 2篇 |
废物处理 | 4篇 |
环保管理 | 9篇 |
综合类 | 202篇 |
基础理论 | 63篇 |
污染及防治 | 86篇 |
评价与监测 | 10篇 |
社会与环境 | 8篇 |
出版年
2021年 | 3篇 |
2018年 | 4篇 |
2016年 | 5篇 |
2014年 | 8篇 |
2013年 | 12篇 |
2012年 | 7篇 |
2011年 | 5篇 |
2010年 | 10篇 |
2009年 | 16篇 |
2008年 | 7篇 |
2007年 | 21篇 |
2006年 | 8篇 |
2005年 | 7篇 |
2004年 | 9篇 |
2003年 | 11篇 |
2002年 | 14篇 |
2001年 | 8篇 |
2000年 | 6篇 |
1999年 | 9篇 |
1998年 | 7篇 |
1997年 | 5篇 |
1995年 | 6篇 |
1994年 | 5篇 |
1993年 | 3篇 |
1992年 | 4篇 |
1983年 | 3篇 |
1981年 | 4篇 |
1978年 | 3篇 |
1967年 | 4篇 |
1966年 | 4篇 |
1965年 | 5篇 |
1964年 | 8篇 |
1963年 | 11篇 |
1962年 | 4篇 |
1961年 | 7篇 |
1960年 | 5篇 |
1959年 | 6篇 |
1958年 | 10篇 |
1957年 | 7篇 |
1956年 | 7篇 |
1955年 | 12篇 |
1954年 | 6篇 |
1952年 | 4篇 |
1951年 | 3篇 |
1950年 | 6篇 |
1947年 | 5篇 |
1943年 | 6篇 |
1939年 | 4篇 |
1928年 | 2篇 |
1924年 | 3篇 |
排序方式: 共有384条查询结果,搜索用时 46 毫秒
301.
Maren Olbrich Marion Wenig Karl-Heinz Häberle Rainer Matyssek Michael Leuchner Katja Schlink Gerhard Welzl Dieter Ernst Günther Bahnweg 《Environmental pollution (Barking, Essex : 1987)》2010,158(4):1043-1050
In 2006, a controlled infection study was performed in the ‘Kranzberger Forst’ to address the following questions: (1) Will massive artificial inoculation with Apiognomonia errabunda override the previously observed inhibitory effect of chronic ozone? (2) Can biochemical or molecular markers be detected to account for the action of ozone? To this end six adult beech trees were chosen, three ozone fumigated (2× ozone) and three control trees (ambient = 1× ozone). Spore-sprayed branches of sun and shade crown positions of each of the trees, and uninoculated control branches, were enclosed in 100-L plastic bags for one night to facilitate infection initiation. Samples were taken within a five-week period after inoculation. A. errabunda infestation levels quantified by real-time PCR increased in leaves that were not fumigated with additional ozone. Cell wall components and ACC (ethylene precursor 1-amino cyclopropane-1-carboxylic acid) increased upon ozone fumigation and may in part lead to the repression of fungal infection. 相似文献
302.
Robert Müller Daniel Müller Florian Schierhorn Gerhard Gerold Pablo Pacheco 《Regional Environmental Change》2012,12(3):445-459
Forests in lowland Bolivia suffer from severe deforestation caused by different types of agents and land use activities. We identify three major proximate causes of deforestation. The largest share of deforestation is attributable to the expansion of mechanized agriculture, followed by cattle ranching and small-scale agriculture. We utilize a spatially explicit multinomial logit model to analyze the determinants of each of these proximate causes of deforestation between 1992 and 2004. We substantiate the quantitative insights with a qualitative analysis of historical processes that have shaped land use patterns in the Bolivian lowlands to date. Our results suggest that the expansion of mechanized agriculture occurs mainly in response to good access to export markets, fertile soil, and intermediate rainfall conditions. Increases in small-scale agriculture are mainly associated with a humid climate, fertile soil, and proximity to local markets. Forest conversion into pastures for cattle ranching occurs mostly irrespective of environmental determinants and can mainly be explained by access to local markets. Land use restrictions, such as protected areas, seem to prevent the expansion of mechanized agriculture but have little impact on the expansion of small-scale agriculture and cattle ranching. The analysis of future deforestation trends reveals possible hotspots of future expansion for each proximate cause and specifically highlights the possible opening of new frontiers for deforestation due to mechanized agriculture. Whereas the quantitative analysis effectively elucidates the spatial patterns of recent agricultural expansion, the interpretation of long-term historic drivers reveals that the timing and quantity of forest conversion are often triggered by political interventions and historical legacies. 相似文献
303.
John H. Borden Ian M. Wilson Regine Gries Leslie J. Chong Harold D. Pierce Jr. Gerhard Gries 《Chemoecology》1998,8(2):69-75
Summary. Coupled gas chromatographic-electroantennographic detection (GC-EAD) analysis of the Porapak Q-captured volatiles from the
bark of trembling aspen, Populus tremuloides Michx., revealed four compounds that consistently elicited antennal responses by mountain pine beetles (MPBs), Dendroctonus ponderosae Hopkins. One of these, 1-hexanol, disrupted the capture of MPBs in multiple-funnel traps baited with the aggregation pheromones
trans-verbenol and exo-brevicomin and the host kairomone myrcene, a blend of semiochemicals that mediates the secondary attraction response in which
beetles mass attack and kill living pines. The other three EAD-active aspen bark volatiles, benzyl alcohol, benzaldehyde and
nonanal, were inactive alone, but in binary and ternary combinations contributed to a disruptive effect in an additive and
redundant manner when all four aspen bark volatiles were tested in all possible binary and ternary blends. The best ternary
blend and the quarternary blend achieved ≥ 80% disruption. The quarternary blend enhanced the disruptive effect of the antiaggregation
pheromone verbenone in traps, raising the disruptive effect to 98%, and also enhanced the inhibition of attack on attractant-baited
lodgepole pines. This is the first demonstration of specific compounds from the bark of angiosperm trees that disrupt the
secondary attraction response of sympatric coniferophagous bark beetles. The results support the hypothesis that such bark
beetles are adapted to recognize and avoid non-host angiosperm trees by responding to a broad spectrum of volatiles that can
act in various blends with equal effect.
Received 27 October 1997; accepted 20 February 1998. 相似文献
304.
A fixed-volume release of 1,2-DCE, tracked in space and time with a light transmission/image analysis system, provided a data set for the infiltration, redistribution, and immobilisation of a dense non-aqueous phase liquid (DNAPL) in a heterogeneous porous medium. The two-dimensional bench scale flow cell was packed with a spatially correlated, random heterogeneous distribution of six sand types. In order to provide the necessary modelling parameters, detailed constitutive relationships were measured at the local scale for the six sands. These experiments revealed that nonwetting phase (NWP) relative permeability-saturation (k(rN)-S(W)) relationships are strongly correlated to sand type. Trends in the best-fit k(rN)-S(W) parameters reflected a positive correlation between mean grain diameter and the maximum NWP relative permeability, k(rN)(max). Multiphase flow simulations of the bench scale experiment best reproduced the experimental observations, producing excellent matches in both time and space, when the measured, correlated local scale k(rN)-S(W) relationships were employed. 相似文献
305.
Lammel G Klöpffer W Semeena VS Schmidt E Leip A 《Environmental science and pollution research international》2007,14(3):153-165
Background, Aim and Scope Modelling of the fate of environmental chemicals can be done by relatively simple multi-media box models or using complex
atmospheric transport models. It was the aim of this work to compare the results obtained for both types of models using a
small set of non-ionic and non-polar or moderately polar organic chemicals, known to be distributed over long distances.
Materials and Methods Predictions of multimedia exposure models of different types, namely three multimedia mass-balance box models (MBMs), two
in the steady state and one in the non-steady state mode, and one non-steady state multicompartment chemistry-atmospheric
transport model (MCTM), are compared for the first time. The models used are SimpleBox, Chemrange, the MPI-MBM and the MPI-MCTM.
The target parameters addressed are compartmental distributions (i.e. mass fractions in the compartments), overall environmental
residence time (i.e. overall persistence and eventually including other final sinks, such as loss to the deep sea) and a measure
for the long-range transport potential. These are derived for atrazine, benz-[a]-pyrene, DDT, α and γ-hexachlorocyclohexane,
methyl parathion and various modes of substance entry into the model world.
Results and Discussion Compartmental distributions in steady state were compared. Steady state needed 2–10 years to be established in the MCTM. The
highest fraction of the substances in air is predicted by the MCTM. Accordingly, the other models predict longer substance
persistence in most cases. The results suggest that temperature affects the compartmental distribution more in the box models,
while it is only one among many climate factors acting in the transport model. The representation of final sinks in the models,
e.g. burial in the sediment, is key for model-based compartmental distribution and persistence predictions. There is a tendency
of MBMs to overestimate substance sinks in air and to underestimate atmospheric transport velocity as a consequence of the
neglection of the temporal and spatial variabilities of these parameters. Therefore, the long-range transport potential in
air derived from MCTM simulations exceeds the one from Chemrange in most cases and least for substances which undergo slow
degradation in air.
Conclusions and Perspectives MBMs should be improved such as to ascertain that the significance of the atmosphere for the multicompartmental cycling is
not systematically underestimated. Both types of models should be improved such as to cover degradation in air in the particle-bound
state and transport via ocean currents. A detailed understanding of the deviations observed in this work and elsewhere should
be gained and multimedia fate box models could then be ‘tuned in’ to match better the results of comprehensive multicompartmental
transport models.
ESS-Submission Editor: Prof. Dr. Michael Matthies (matthies@uos.de) 相似文献
306.
Cocoon-spinning larvae of the codling moth, Cydia pomonella L. (Lepidoptera: Olethreutidae) employ a pheromone that attracts or arrests conspecifics seeking pupation sites. Such intraspecific communication signals are important cues for illicit receivers such as parasitoids to exploit. We tested the hypothesis that the prepupal C. pomonella parasitoid Mastrus ridibundus Gravenhorst (Hymenoptera: Ichneumonidae) exploits the larval aggregation pheromone to locate host prepupae. In laboratory olfactometer experiments, female M. ridibundus were attracted to 3-day-old cocoons containing C. pomonella larvae or prepupae. Older cocoons containing C. pomonella pupae, or larvae and prepupae excised from cocoons, were not attractive. In gas chromatographic-electroantennographic detection (GC-EAD) analyses of bioactive Porapak Q extract of cocoon-derived airborne semiochemicals, ten compounds elicited responses from female M. ridibundus antennae. Comparative GC-mass spectrometry of authentic standards and cocoon-volatiles determined that these compounds were 3-carene, myrcene, heptanal, octanal, nonanal, decanal, (E)-2-octenal, (E)-2-nonenal, sulcatone, and geranylacetone. A synthetic 11-component blend consisting of these ten EAD-active compounds plus EAD-inactive (+)-limonene (the most abundant cocoon-derived volatile) was as effective as Porapak Q cocoon extract in attracting both female M. ridibundus and C. pomonella larvae seeking pupation sites. Only three components could be deleted from the 11-component blend without diminishing its attractiveness to M. ridibundus, which underlines the complexity of information received and processed during foraging for hosts. Mastrus ridibundus obviously eavesdrop on the pheromonal communication signals of C. pomonella larvae that reliably indicate host presence.
相似文献
Gerhard GriesEmail: |
307.
Gerhard Lagaly 《Die Naturwissenschaften》1981,68(2):82-88
Interactions of organic materials with solid surfaces can be successfully studied with inorganic layer crystals that take up organic compounds between the layers. The kind of information obtainable is illustrated by three selected examples. Investigations with long-chain compounds clarify the possible chain conformations in planar alkyl chain aggregates (mono- and bimolecular films). Studies with polyelectrolytes demonstrate the influence of the charge patterns on polymer adsorption and interactions with nucleotides present very specific adsorption phenomena. 相似文献
308.
309.
310.