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41.
Anne E. Huber David L. Kaplan Christopher Viney 《Journal of Polymers and the Environment》1994,2(3):195-199
Transmitted light measurements performed with a UV-visible spectrophotometer were used to characterize how starch affects the position of boundaries on the phase diagram for dilute aqueous solutions of levan (a branched polymer of fructose). Data were collected in the range 15 to 70°C; the minimum concentrations required for separation of a nematic phase and the minimum concentration required for a fully nematic solution were identified within this range. While hard interactions (repulsion between rod-like molecular segments) dictate the formation of a liquid crystalline phase at and above ambient temperature in the absence of starch, soft interactions become more significant as solutions are cooled toward ambient when starch is present. Small amounts of starch might be used as a filler to modify the mechanical properties (while retaining the process-related benefits) of levan films cast from liquid crystalline solution. 相似文献
42.
W. L. Miller J. A. Foran W. Huber J. M. Davidson H. A. Moye D. P. Spangler 《Journal of the American Water Resources Association》1989,25(1):79-86
ABSTRACT: Over 700 community drinking water supplies were sampled for the pesticide Temik (aldicarb and its oxidative metabolites aldicarb sulfoxide and aldicarb sulfone) in Florida. All community supply wells sampled for Temik were located in counties where Temik was reported to have been used and approximately one-half of the wells were located in counties where ground water was determined to be highly susceptible to contamination by Temik. Susceptibility was determined using ranking criteria that incorporated ground water recharge characteristics, water use, and Temik use patterns. Temik was not detected in any of the community supply wells sampled during the study. However, Temik was detected in shallow, private wells, as was the pesticide ethylene dibromide in counties with ground water characterized as highly susceptible to contamination. 相似文献
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R. W. Hill A. Leon Huber E. K. Israelsen J. P. Riley 《Journal of the American Water Resources Association》1972,8(5):909-921
ABSTRACT. As demands upon available water supplies increase, there is an accompanying increase in the need to assess the downstream consequences resulting from changes at specific locations within a hydrologic system. The problem is approached in this study by hybrid computer simulation of the hydrologic system. Modeling concepts are based upon the development of basic relationships which describe the various hydrologic processes. Within a system these relationships are linked by the continuity-of-mass principle. Spatial resolution is achieved by considering the modeled areas as a series of subbasins. The time increment adopted for the model is one month, so that time varying quantities are expressed in terms of mean monthly values. The model is general in nature and is applied to a particular hydrologic system through a programmed verification procedure whereby model coefficients are evaluated for the particular system. In this study the model is applied to the Bear River basin of western Wyoming, southern Idaho, and northern Utah. Comparisons between observed and computed outflow hydrographs show good agreement. The utility of the model is demonstrated by predicting the effects of various possible water resource management alternatives. The verified hybrid computer program can be digitized for application to the digital computer. 相似文献
46.
Manuela Baumgarten Christian Huber Patrick Büker Hans-Peter Dietrich Christian Heerdt Rainer Matyssek 《Environmental pollution (Barking, Essex : 1987)》2009,157(7):2091-2107
Exposure and flux-based indices of O3 risk were compared, at 19 forest locations across Bavaria in southern Germany from 2002 to 2005; leaf symptoms on mature beech trees found at these locations were also examined for O3 injury. O3 flux modelling was performed using continuously recorded O3 concentrations in combination with meteorological and soil moisture data collected from Level II forest sites. O3 measurements at nearby rural open-field sites proved appropriate as surrogates in cases where O3 data were lacking at forest sites (with altitude-dependent average differences of about 10% between O3 concentrations). Operational thresholds of biomass loss for both O3 indices were exceeded at the majority of the forest locations, suggesting similar risk under long-term average climate conditions. However, exposure-based indices estimated higher O3 risk during dry years as compared to the flux-based approach. In comparison, minor O3-like leaf injury symptoms were detected only at a few of the forest sites investigated. Relationships between flux-based risk thresholds and tree response need to be established for mature forest stands for validation of predicted growth reductions under the prevailing O3 regimes. 相似文献
47.
Long Term Effects of Acid Irrigation at the Höglwald on Seepage Water Chemistry and Nutrient Cycling
Wendelin Weis Roland Baier Christian Huber Axel Göttlein 《Water, Air, & Soil Pollution: Focus》2007,7(1-3):211-223
In order to test the hypothesis of aluminium toxicity induced by acid deposition, an experimental acid irrigation was carried out in a mature Norway spruce stand in Southern Germany (Höglwald). The experiment comprised three plots: no irrigation, irrigation (170 mm a?1), and acid irrigation with diluted sulphuric acid (pH of 2.6–2.8). During the seven years of acid irrigation (1984–1990) water containing 0.43 molc m?2 a?1 of protons and sulphate was added with a mean pH of 3.2 (throughfall?+?acid irrigation water) compared to 4.9 (throughfall) on both control plots. Most of the additional proton input was consumed in the organic layer and the upper mineral soil. Acid irrigation resulted in a long lasting elevation of sulphate concentrations in the seepage water. Together with sulphate both aluminium and appreciable amounts of base cations were leached from the main rooting zone. The ratio between base cations (Ca?+?Mg?+?K) and aluminium was 0.79 during acid irrigation and 0.92 on the control. Neither tree growth and nutrition nor the pool of exchangeable cations were affected significantly. We conclude that at this site protection mechanisms against aluminium toxicity exist and that additional base cation runoff can still be compensated without further reduction of the supply of exchangeable base cations in the upper mineral soil. 相似文献
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Rapid incorporation and short-term distribution of a nonylphenol isomer and the herbicide MCPA in soil-derived organo-clay complexes 总被引:1,自引:0,他引:1
Patrick Riefer Timm Klausmeyer Jan Schwarzbauer Andreas Sch?ffer Burkhard Schmidt Phillipe F. X. Corvini 《Environmental Chemistry Letters》2011,9(3):411-415
Organo-clay complexes in soil are a major sink for xenobiotics and, thus, often enhance their persistence dramatically. However,
the knowledge on environmental processes of non-extractable residue formation on a short time scale is very restricted. Therefore,
this study examined the distribution of 4-(3,5-dimethylhept-3-yl)phenol (NP) and 4-chloro-2-methylphenoxyacetic acid (MCPA)
in soil over a short time period of 48 h and in different soil sub-fractions. The overall proportion of organo-clay-associated
bound residues was not only abundant but also in the same range for both substances (MCPA: 8%; NP: 11% of applied 14C-radioactivity). However, a more detailed view revealed two different distribution patterns: a higher proportion of clay-associated
NP was accompanied by a lower content of bound residues, whereas a smaller fraction of clay-associated MCPA was characterized
by a higher proportion of non-extractable residues. Further on, a selective accumulation of bound residues among clay-associated
humic fractions was observed. NP residues were linked predominantly to humic acids, whereas MCPA residues tended to be incorporated
more into fulvic acids. It was evident that the overall distribution was influenced primarily by the physico-chemical properties
of the contaminants. This study demonstrates in detail a rapid initial incorporation accompanied by a specific distribution
into soil sub-fractions for selected xenobiotics in soil and points to a complex interaction of clay-associated organic matter
with low molecular weight compounds. 相似文献