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41.
The typical method of cool-season grass-seed production in Mediterranean climates briefly exposes surface waters to potentially high concentrations of the herbicide diuron [3-(3,4-dichlorophenyl)-1,1-dimethyl urea] during the initial season of growth. To better understand the process, and the degree, of diuron transport from agricultural fields, two grass-seed fields in the Willamette Valley of Oregon were monitored for diuron loss in surface runoff and tile drainage during the first wet season after planting. Initial diuron concentrations in surface runoff were high (>1000 microg L(-1) in one field and >100 microg L(-1) in the other), though they decreased by two orders of magnitude by the end of the season. Concentrations in the tile drains were as much as 1000 times lower than in the surface runoff during the first few weeks of runoff events, and they remained lower than surface water concentrations throughout the season. Total losses in surface runoff were between 1.3 and 3% of the amount applied-much higher than losses via the tile drains. It is also shown by means of a simple first-order decay model that, when little information is available, it may be best to describe diuron depletion in runoff water as a function of cumulative rainfall during the wet season. 相似文献
42.
An input-output balance study for PCBs in humans 总被引:2,自引:0,他引:2
Polychlorinated biphenyl (PCB) input-output balance studies were performed on five male volunteers, aged between 24 and 30, for periods of 8-14 days in 1998. Dietary exposure was quantified by the duplicate meals method and varied between 220 and 460 ng of sigmaPCB (sum of 20 congeners) per day for each of the five individuals over the study period. Dietary intake was dominated by congeners 118, 138, 153 and 180. Average faecal outputs for the five volunteers were 50-290 ng of sigmaPCB (sum of 20 congeners) per day for each of the five individuals over the same period and was dominated by the same four congeners. Whilst the total PCB fluxes were therefore into the body (i.e., accumulation), important differences were noted for different individual congeners. PCBs 44, 47, 49, 52, 60, 66, 101, 105, 110, 118, 149, 151 and 183 all showed net absorption for all five volunteers. Some congeners showed a net absorption in some of the individuals but net excretion in others, as seen by other workers. These congeners (PCBs 138, 153, 180, 187 and 194) are all higher chlorinated congeners and lack meta-para-vicinal hydrogen atoms. There were differences in the net absorption/excretion between individuals, which appeared to be a function of body fat index (BFI). The volunteers with the lowest BFIs showed net excretion for the greatest number of congeners, whilst the individual with the highest BFI was a net absorber of all the congeners studied. The problems in determining and interpreting absorption efficiency values for use in quantitative exposure assessments are discussed. Various factors that influence net absorption of PCBs and other persistent organic pollutants are identified. These include compound properties (including susceptibility to metabolism), the individual's fat status and balance, exposure history and diet. 相似文献
43.
Scholz C. Jones T. G. West M. Ehbair A. M. S. Dunn C. Freeman C. 《Environmental science and pollution research international》2016,23(18):18192-18199
Environmental Science and Pollution Research - The objective of this study was to monitor a newly constructed wetland (CW) in north Wales, UK, to assess whether it contributes to an improvement in... 相似文献
44.
This paper presents an innovative, quantitative assessment of pollution avoidance attributable to environmental regulation enforced through integrated licensing, using Ireland's pharmaceutical-manufacturing sector as a case study. Emissions data reported by pharmaceutical installations were aggregated into a pollution trend using an Environmental Emissions Index (EEI) based on Lifecycle Assessment methodologies. Complete sectoral emissions data from 2001 to 2007 were extrapolated back to 1995, based on available data. Production volume data were used to derive a sectoral production index, and determine ‘no-improvement’ emission trends, whilst questionnaire responses from 20 industry representatives were used to quantify the contribution of integrated licensing to emission avoidance relative to these trends. Between 2001 and 2007, there was a 40% absolute reduction in direct pollution from 27 core installations, and 45% pollution avoidance relative to hypothetical ‘no-improvement’ pollution. It was estimated that environmental regulation avoided 20% of ‘no-improvement’ pollution, in addition to 25% avoidance under business-as-usual. For specific emissions, avoidance ranged from 14% and 30 kt a− 1 for CO2 to 88% and 598 t a− 1 for SOx. Between 1995 and 2007, there was a 59% absolute reduction in direct pollution, and 76% pollution avoidance. Pollution avoidance was dominated by reductions in emissions of VOCs, SOx and NOx to air, and emissions of heavy metals to water. Pollution avoidance of 35% was attributed to integrated licensing, ranging from between 8% and 2.9 t a− 1 for phosphorus emissions to water to 49% and 3143 t a− 1 for SOx emissions to air. Environmental regulation enforced through integrated licensing has been the major driver of substantial pollution avoidance achieved by Ireland's pharmaceutical sector — through emission limit values associated with Best Available Techniques, emissions monitoring and reporting requirements, and performance targets specified in environmental management plans. This compliant sector offers a positive, but not necessarily typical, case study of IPPC effectiveness. 相似文献
45.
J. R. Park M. J. Stabler P. J. Jones S. R. Mortimer J. R. Tiffin R. B. Tranter 《Environment, Development and Sustainability》2009,11(4):735-750
The issue of the sustainable development of rural economies in England has recently received considerable attention. This
is because many of the poorest areas in the country are rural, often of high environmental quality, but suffering from high
unemployment and a lack of services and facilities. The rapid decline in agricultural incomes and in-migration of affluent
urban workers since 1990 has exacerbated economic inequality in such areas. A number of factors have the potential to drive
rural development and this paper applies, and considers, the feasibility of a method from the USA for combining economic and
environmental variables in a regional growth model to examine the hypothesis that environmental quality is an important determinant
of sustainable rural development in England. The model output suggests that, although environmental quality does play a role
in sustainable rural development in England there are other, more important, factors driving development. These include business
and communications infra-structure, the degree and opportunities for commuting and underlying employment prospects. The robustness
and limitations of the method for combining economic and environmental variables is discussed in relation to the spatial interrelatedness
of Local Authority Districts in England, and conclusions are drawn about areas for refinement and improvement of the method.
相似文献
J. R. ParkEmail: |
46.
Chakra Chaemfa Jonathan L. Barber Kyoung-Sim Kim Tom Harner Kevin C. Jones 《Atmospheric environment (Oxford, England : 1994)》2009,43(25):3843-3849
Passive air samplers (PAS) can be used to monitor semi-volatile organic compounds in the atmosphere. Polyurethane foam (PUF) disks are a popular sampling medium because they have a high retention capacity for such compounds. This paper reports a highly time-resolved uptake study, to derive uptake rate data under field conditions, and investigate the effects of using different foam densities on the uptake rate. PUF disks were deployed alongside an active sampler, for periods of up to 12 weeks. The uptake rates were measured for a range of gas- and particle-bound persistent organic pollutants (polychlorinated biphenyls (PCBs) and polybrominated diphenyl ethers (PBDEs)), of different properties, to explore whether gas–particle partitioning affected uptake rate. Uptake rates for two different densities of foam (0.021 and 0.035 g cm?3) were not statistically significantly different from each other. Uptake rates of light PCBs averaged ~6.5 m3 day?1, somewhat higher than in previous studies; higher wind speeds and lower temperatures in this study are the likely reason for this difference. The study showed: i) the uptake rate of the compound with lowest KOA considered in this study (PCB-28/31) declined in the later weeks, indicating an approach to equilibrium; ii) uptake rates of lighter BDEs and heavier PCBs (compounds of intermediate KOA in this study) remain similar throughout the study period, indicating that they are not approaching equilibrium during the 12-week-study; iii) uptake rates were typically: ~8 m3 day?1 for PCB-52; ~9.5 m3 day?1 for PCB-95; ~11 m3 day?1 for BDE-28 and ~2 m3 day?1 BDE-99. The latter compound has an important particle-bound component and this lowers the sampling rate compared to predicted uptake rates for compounds which are in the gas phase only. It is shown that knowledge of gas–particle partitioning is needed to correct for this effect, and to improve predicted uptake rates. 相似文献
47.
Benjamin M. Jones Christopher D. Arp Kenneth M. Hinkel Richard A. Beck Joel A. Schmutz Barry Winston 《Environmental management》2009,43(6):1071-1084
Lakes are dominant landforms in the National Petroleum Reserve Alaska (NPRA) as well as important social and ecological resources.
Of recent importance is the management of these freshwater ecosystems because lakes deeper than maximum ice thickness provide
an important and often sole source of liquid water for aquatic biota, villages, and industry during winter. To better understand
seasonal and annual hydrodynamics in the context of lake morphometry, we analyzed lakes in two adjacent areas where winter
water use is expected to increase in the near future because of industrial expansion. Landsat Thematic Mapper and Enhanced
Thematic Mapper Plus imagery acquired between 1985 and 2007 were analyzed and compared with climate data to understand interannual
variability. Measured changes in lake area extent varied by 0.6% and were significantly correlated to total precipitation
in the preceding 12 months (p < 0.05). Using this relation, the modeled lake area extent from 1985 to 2007 showed no long-term trends. In addition, high-resolution
aerial photography, bathymetric surveys, water-level monitoring, and lake-ice thickness measurements and growth models were
used to better understand seasonal hydrodynamics, surface area-to-volume relations, winter water availability, and more permanent
changes related to geomorphic change. Together, these results describe how lakes vary seasonally and annually in two critical
areas of the NPRA and provide simple models to help better predict variation in lake-water supply. Our findings suggest that
both overestimation and underestimation of actual available winter water volume may occur regularly, and this understanding
may help better inform management strategies as future resource use expands in the NPRA. 相似文献
48.
Josephine A. Hagger Tamara S. Galloway Malcolm B. Jones 《Environmental pollution (Barking, Essex : 1987)》2009,157(7):2003-2010
A series of European Marine Sites has been designated as Special Areas of Conservation (SAC) in England. The aim of this study was to develop a practical methodology to assess the condition of SACs by applying a suite of biomarkers. Biomarkers were applied to the blue mussel Mytilus edulis and the shore crab Carcinus maenas from the Fal and Helford SAC (Cornwall). Individual biomarkers provided useful diagnostic information on the activity of certain classes of contaminants and an integrated Biomarker Response Index (BRI) was used to achieve a more holistic understanding of the condition of the SAC. The BRI indicated that the general health of both organisms was impacted in the upper part of the SAC (Fal Estuary) which correlated well with known chemical hotspots and sources of contamination. The BRI allows a pragmatic way to prioritise SAC sites that may require further investigative studies. 相似文献
49.
Kristina Cydzik Terri S. Hogue 《Journal of the American Water Resources Association》2009,45(3):702-714
Abstract: This paper investigates application of the Army Corps of Engineers’ Hydrologic Engineering Center Hydrologic Modeling System (HEC‐HMS) to a burned watershed in San Bernardino County, California. We evaluate the HEC‐HMS’ ability to simulate discharge in prefire and postfire conditions in a semi arid watershed and the necessary parameterizations for modeling hydrologic response during the immediate, and subsequent recovery, period after a wildfire. The model is applied to City Creek watershed, which was 90% burned during the Old Fire of October 2003. An optimal spatial resolution for the HEC‐HMS model was chosen based on an initial sensitivity analysis of subbasin configurations and related model performance. Five prefire storms were calibrated for the selected model resolution, defining a set of parameters that reasonably simulate prefire conditions. Six postfire storms, two from each of the following rainy (winter) seasons were then selected to simulate postfire response and evaluate relative changes in parameter values and model behavior. There were clear trends in the postfire parameters [initial abstractions (Ia), curve number (CN), and lag time] that reveal significant (and expected) changes in watershed behavior. CN returns to prefire (baseline) values by the end of Year 2, while Ia approaches baseline by the end of the third rainy season. However, lag time remains significantly lower than prefire values throughout the three‐year study period. Our results indicate that recovery of soil conditions and related runoff response is not entirely evidenced by the end of the study period (three rainy seasons postfire). Understanding the evolution of the land surface and related hydrologic properties during the highly dynamic postfire period, and accounting for these changes in model parameterizations, will allow for more accurate and reliable discharge simulations in both the immediate, and subsequent, rainy seasons following fire. 相似文献
50.
Stormwater runoff from the University of California, Davis/U.S. Department of Energy Laboratory for Energy‐Related Health Research (UCD/US DOE LEHR) Superfund site located on the University of California campus in Davis, California, has been found to contain over 500 ng/L of total recoverable mercury, which is about ten times the California Toxics Rule criterion. This stormwater runoff is discharged to Putah Creek, which is Clean Water Act Section 303(d) listed as impaired for excessive mercury bioaccumulation in edible fish. A discussion is presented on the potential impact of the mercury in stormwater runoff from LEHR leading to excessive bioaccumulation of mercury in Putah Creek fish. The mercury in the stormwater runoff is derived from former flooding of the soils near the creek, which contains mercury derived from abandoned upstream mercury mines located in the Coast Range Vaca Hills to the west of LEHR. The implications of this situation for implementing a Total Maximum Daily Load (TMDL) to control mercury in stormwater runoff to Putah Creek are presented. © 2009 Wiley Periodicals, Inc. 相似文献