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151.
Vintró LL McMahon CA Mitchell PI Josefsson D Holm E Roos P 《Journal of environmental radioactivity》2002,60(1-2):73-89
New data on the levels and long-range transport of plutonium in the Arctic Ocean, recorded in the course of two expeditions to this zone in 1994 and 1996, are discussed in this paper. Specifically, approximately 100 plutonium measurements in surface and sub-surface water sampled at 58 separate stations throughout the Kara, Laptev and East Siberian Seas, as well as along latitudinal transects across the Lomonosov Ridge, are reported and interpreted in terms of the circulation pathways responsible for the transport of this element from the North Atlantic to the Arctic Shelf and into the Arctic interior. In addition, the behaviour of plutonium in its transit through the vast Arctic shelf seas to open waters under extreme environmental conditions is discussed in terms of the partitioning of plutonium between filtered (<0.45 microm) seawater and suspended particulate, and its association with colloidal matter. Finally, limited evidence of the presence of a colloidal plutonium component in Arctic waters subject to direct riverine input is adduced. 相似文献
152.
Herbel MJ Johnson TM Tanji KK Gao S Bullen TD 《Journal of environmental quality》2002,31(4):1146-1156
Selenium stable isotope ratios are known to shift in predictable ways during various microbial, chemical, and biological processes, and can be used to better understand Se cycling in contaminated environments. In this study we used Se stable isotopes to discern the mechanisms controlling the transformation of oxidized, aqueous forms of Se to reduced, insoluble forms in sediments of Se-affected environments. We measured 80Se/76Se in surface waters, shallow ground waters, evaporites, digested plants and sediments, and sequential extracts from several sites where agricultural drainage water is processed in the San Joaquin Valley of California. Selenium isotope analyses of samples obtained from the Tulare Lake Drainage District flow-through wetland reveal small isotopic contrasts (mean difference 0.7%) between surface water and reduced Se species in the underlying sediments. Selenium in aquatic macrophytes was very similar isotopically to the NaOH and Na2SO3 sediment extracts designed to recover soluble organic Se and Se(0), respectively. For the integrated on-farm drainage management sites, evaporite salts were slightly (approximately 0.6%) enriched in the heavier isotope relative to the inferred parent waters, whereas surface soils were slightly (approximately 1.4%) depleted. Bacterial or chemical reduction of Se(VI) or Se(IV) may be occurring at these sites, but the small isotopic contrasts suggest that other, less isotopically fractionating mechanisms are responsible for accumulation of reduced forms in the sediments. These findings provide evidence that Se assimilation by plants and algae followed by deposition and mineralization is the dominant transformation pathway responsible for accumulation of reduced forms of Se in the wetland sediments. 相似文献
153.
Forecasting environmental equity: air quality responses to road user charging in Leeds, UK 总被引:2,自引:0,他引:2
Mitchell G 《Journal of environmental management》2005,77(3):212-226
Sustainable development requires that the goals of economic development, environmental protection and social justice are considered collectively when formulating development strategies. In the context of planning sustainable transport systems, trade-offs between the economy and the environment, and between the economy and social justice have received considerable attention. In contrast, much less attention has been paid to environmental equity, the trade-off between environmental and social justice goals, a significant omission given the growing attention to environmental justice by policy makers in the EU and elsewhere. In many countries, considerable effort has been made to develop clean transport systems by using, for example, technical, economic and planning instruments. However, little effort has been made to understand the distributive and environmental justice implications of these measures. This paper investigates the relationship between urban air quality (as NO2) and social deprivation for the city of Leeds, UK. Through application of a series of linked dynamic models of traffic simulation and assignment, vehicle emission, and pollutant dispersion, the environmental equity implications of a series of urban transport strategies, including road user cordon and distance-based charging, road network development, and emission control are assessed. Results indicate a significant degree of environmental inequity exists in Leeds. Analysis of the transport strategies indicates that this inequity will be reduced through natural fleet renewal, and, perhaps contrary to expectations, road user charging is also capable of promoting environmental equity. The environmental equity response is, however, sensitive to road pricing scheme design. 相似文献
154.
Nitrogen biogeochemistry in the Adirondack Mountains of New York: hardwood ecosystems and associated surface waters 总被引:5,自引:0,他引:5
Mitchell MJ Driscoll CT Inamdar S McGee GG Mbila MO Raynal DJ 《Environmental pollution (Barking, Essex : 1987)》2003,123(3):355-364
Studies on the nitrogen (N) biogeochemistry in Adirondack northern hardwood ecosystems were summarized. Specific focus was placed on results at the Huntington Forest (HFS), Pancake-Hall Creek (PHC), Woods Lake (WL), Ampersand (AMO), Catlin Lake (CLO) and Hennessy Mountain (HM). Nitrogen deposition generally decreased from west to east in the Adirondacks, and there have been no marked temporal changes in N deposition from 1978 through 1998. Second-growth western sites (WL, PHC) had higher soil solution NO(3-) concentrations and fluxes than the HFS site in the central Adirondacks. Of the two old-growth sites (AMO and CLO), AMO had substantially higher NO(3-) concentrations due to the relative dominance of sugar maple that produced litter with high N mineralization and nitrification rates. The importance of vegetation in affecting N losses was also shown for N-fixing alders in wetlands. The Adirondack Manipulation and Modeling Project (AMMP) included separate experimental N additions of (NH4)2SO4 at WL, PHC and HFS and HNO3 at WL and HFS. Patterns of N loss varied with site and form of N addition and most of the N input was retained. For 16 lake/watersheds no consistent changes in NO(3-) concentrations were found from 1982 to 1997. Simulations suggested that marked NO(3-) loss will only be manifested over extended periods. Studies at the Arbutus Watershed provided information on the role of biogeochemical and hydrological factors in affecting the spatial and temporal patterns of NO(3-) concentrations. The heterogeneous topography in the Adirondacks has generated diverse landscape features and patterns of connectivity that are especially important in regulating the temporal and spatial patterns of NO(3-) concentrations in surface waters. 相似文献
155.
Nuclear and nonnuclear industrial and research activities have been conducted on the Hanford reservation since 1943. Materials originating from these activities may enter the surrounding environment through releases of airborne and liquid effluents and solid wastes. Concern about the environmental effects of these releases has evolved over the past four decades into a comprehensive onsite and offsite monitoring program. Today, environmental monitoring to assess potential impacts of released materials includes field sampling and chemical and physical analyses of air, ground and surface water, fish and wildlife, soil, vegetation, and foodstuffs. This paper reviews the history of Hanford operations and summarizes the current environmental monitoring program and its major findings. Mathematical models based on monitoring data show that radiation doses to people living near the Hanford site are well below existing regulatory standards. Only trace amounts of radionuclides from Hanford have been detected in the offsite environment. 相似文献
156.
157.
Mitchell R. Peters Steven R. Abt Chester C. Watson Craig Fischenich John M. Nestler 《Journal of the American Water Resources Association》1995,31(4):745-752
ABSTRACT: The Riverine Community Habitat Assessment and Restoration Concept (RCHARC) was developed to integrate habitat enhancement into the stream restoration process. RCHARC assumes that aquatic habitat quality is closely related to hydraulic diversity based upon a “comparison standard” reach approach to stream restoration. A Beta test was performed by applying the RCHARC process to Rapid Creek in Rapid City, South Dakota. Standard and restored stream reaches were selected and data were collected. A comparison of field data and velocity-depth distributions indicated that the restored stream closely replicated the standard reach. The RCHARC methodology has the potential to assess habitat quality for planned comparison reaches and indicate the level of success resulting from restoration. 相似文献
158.
Donald A. Mitchell 《Environment international》1981,6(1-6)
A free-jet scrubber is an innovative gas cleaner in which the primary liquid/gas contacting takes place in the turbulent mixing zone emanating from a jet nozzle. The first such devices, powered by supersonic steam or air ejectors, were exceptionally effective cleaners but were criticized as being high-energy users. A great reduction in the energy consumption of free-jet scrubbers has been accomplished in the last four years, a feat which may seem in contradiction to the “contacting power rule.” An explanation of what is happening in these devices must take into account the effectiveness with which energy and water are utilized. thereby leading one to a somewhat circular definition of “effective contacting power.” The theoretical implication of this analysis is primarily to remind us that there are many paths between two states and some are more energy efficient than others. The practical value is that such analysis generates information which aids in choosing between several design options, a direct benefit of the various free-jet configurations. 相似文献
159.
Ones and Viswesvaran (1996) have argued for the use of broad bandwidth, rather than narrow bandwidth, personality predictors in personnel selection research when overall job performance is the criterion of interest. We take the opposite position in this article—that homogeneous measures of unidimensional personality traits are always to be preferred as predictors of work (and other) criteria. We maintain that the use of multiple unidimensional predictors provides important advantages over the use of multidimensional aggregates of those predictors. These advantages pertain to both (a) empirical accuracy in predicting job performance, and (b) psychological meaningfulness in explaining work behavior. Our conclusions are supported by Ones and Viswesvaran's own data. Copyright © 1999 John Wiley & Sons, Ltd. 相似文献
160.