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51.
Wenying Chen Yves-Michel Le Nindre Ruina Xu Delphine Allier Fei Teng Kim Domptail Xing Xiang Laura Guillon Jiyong Chen Lingyan Huang Rongshu Zeng 《International Journal of Greenhouse Gas Control》2010,4(2):341-350
A method, based on spatial analysis of the different criteria to be taken into consideration for building scenarios of CO2 capture and storage (CCS), has been developed and applied to real case studies in the Hebei province. Totally 88 point sources (42 from power sector, 9 from iron and steel, 18 from cement, 16 from ammonia, and 3 from oil refinery) are estimated and their total emission amounts to 231.7 MtCO2/year with power, iron and steel, cement, ammonia and oil refinery sharing 59.13%, 25.03%, 11.44%, 3.5%, and 0.91%, respectively. Storage opportunities can be found in Hebei province, characterised by a strong tectonic subsidence during the Tertiary, with several kilometres of accumulated clastic sediments. Carbon storage potential for 25 hydrocarbon fields selected from the Huabei complex is estimated as 215 MtCO2 with optimistic assumption that all recovered hydrocarbon could be replaced by an equivalent volume of CO2 at reservoir conditions. Storage potential for aquifers in the Miocene Guantao formation is estimated as 747 MtCO2 if closed aquifer assumed or 371 MtCO2 if open aquifer and single highly permeable horizon assumed. Due to poor knowledge on deep hydrogeology and to pressure increase in aquifer, injecting very high rates requested by the major CO2 sources (>10 MtCO2/year) is the main challenge, therefore piezometry and discharge must be carefully controlled. A source sink matching model using ArcGIS software is designed to find the least-cost pathway and to estimate transport route and cost accounting for the additional costs of pipeline construction due to landform and land use. Source sink matching results show that only 15–25% of the emissions estimated for the 88 sources can be sequestrated into the hydrocarbon fields and the aquifers if assuming sinks should be able to accommodate at least 15 years of the emissions of a given source. 相似文献
52.
Southern Chile encompasses one of the most extensive fjord regions of the world, the Patagonia, currently exposed to natural
and anthropogenic perturbations. These fjord ecosystems provide important services to humans, which have not been adequately
measured and valued. As a consequence, ecosystem services are commonly ignored in public policy design and in the evaluation
of development projects. Here we tackle questions that are highly relevant for the nation’s development, namely (1) understanding
fjord functioning, and (2) developing management strategies based on ecosystem services, in order to secure simultaneous and
adequate use of these ecosystems which area influenced by ecological (e.g., biogeochemical) and productive (e.g., aquaculture,
fisheries) processes. We also seek to strengthen the analysis of fjord ecosystem value from the economical (including coastal
zoning), socio-cultural, institutional, and governmental points of view. In addition, the investigation of current and future
effects of climate change on this large region offers a unique opportunity to understand the social and economic consequences
of a global phenomenon at local to regional scales. Biogeochemical and socio-economic models will be used to simulate future
scenarios under a gamut of management options. 相似文献
53.
Laura B. Brentner Sachiyo T. Mukherji Jerald L. Schnoor 《Environmental pollution (Barking, Essex : 1987)》2010,158(2):470-475
Phosphor imager autoradiography is a technique for rapid, sensitive analysis of the localization of xenobiotics in plant tissues. Use of this technique is relatively new to research in the field of plant science, and the potential for enhancing visualization and understanding of plant uptake and transport of xenobiotics remains largely untapped. Phosphor imager autoradiography is used to investigate the uptake and translocation of the explosives 1,3,5-trinitro-1,3,5-triazine (RDX) and 2,4,6-trinitrotoluene within Populus deltoides × nigra DN34 (poplar) and Panicum vigratum Alamo (switchgrass). In both plant types, TNT and/or TNT-metabolites remain predominantly in root tissues while RDX and/or RDX-metabolites are readily translocated to leaf tissues. Phosphor imager autoradiography is further investigated for use in semi-quantitative analysis of uptake of TNT by switchgrass. 相似文献
54.
Jianjun Niu Pat E. Rasmussen Amanda Wheeler Ron Williams Marc Chénier 《Atmospheric environment (Oxford, England : 1994)》2010,44(2):235-245
Factors and sources affecting measurement uncertainty associated with monitoring metals in airborne particulate matter (PM) were investigated as part of the Windsor, Ontario Exposure Assessment Study (WOEAS). The assessment was made using co-located duplicate samples and a comparison of two analytical approaches: ED-XRF and ICP-MS. Sampling variability was estimated using relative percent difference (RPD) of co-located duplicate samples. The comparison of ICP-MS and ED-XRF results yields very good correlations (R2 ≥ 0.7) for elements present at concentrations that pass both ICP-MS and ED-XRF detection limits (e.g. Fe, Mn, Zn, Pb and Cu). PM concentration ranges (median, sample number) of 24-h indoor PM10 and personal PM10 filters, and outdoor PM2.5 filters were determined to be 2.2–40.7 (11.0, n = 48) μg m?3, 8.0–48.3 (11.9, n = 48) μg m?3, and 17.1–42.3 (21.6, n = 18) μg m?3, respectively. The gravimetric analytical results reveal that the variations in PM mass measurements for same-day sampling are insignificant compared to temporal or spatial variations: 92%, 100% and 96% of indoor, outdoor and personal duplicate samples, respectively, pass the quality criteria (RPD ≤ 20%). Uncertainties associated with ED-XRF elemental measurements of S, Ca, Mn, Fe and Zn for 24-h filter samples are low: 78%–100% of the duplicate samples passed the quality criteria. In the case of 24-h filter samples using ICP-MS, more elements passed the quality criteria due to the lower detection limits. These were: Li, Na, K, Ca, Si, Al, V, Fe, Mn, Co, Cu, Mo, Ag, Zn, Pb, As, Mg, Sb, Sn, Sr, Th, Ti, Tl, and U. Low air concentrations of metals (near or below instrumental detection limits) and/or inadvertent introduction of metal contamination are the main causes for excluding elements based on the pass/fail criteria. Uncertainty associated with elemental measurements must be assessed on an element-by-element basis. 相似文献
55.
Ariela D'Angiola Laura E. Dawidowski Darío R. Gómez Mauricio Osses 《Atmospheric environment (Oxford, England : 1994)》2010,44(4):483-493
A new annual bottom–up emission inventory of criteria pollutants and greenhouse gases from on-road mobile sources was developed for 2006 for the metropolitan area of Buenos Aires, Argentina, within a four-year regional project aimed at providing tools for chemical weather forecast in South America. Under the scarcity of local emission factors, we collected data from measuring campaigns performed in Argentina, Brazil, Chile and Colombia and compiled a data set of regional emission factors representative of Latin American fleets and driving conditions. The estimated emissions were validated with respect to downscaled national estimates and the EDGAR global emission database. Our results highlight the role of older technologies accounting in average for almost 80% of the emissions of all species. The area exhibits higher specific emissions than developed countries, with figures two times higher for criteria pollutants. We analyzed the effect on emissions of replacing gasoline by compressed natural gas, occurring in Argentina since 1995. We identified (i) a relationship between number of vehicles and a compound socioeconomic indicator, and (ii) time-lags in vehicle technologies between developed and developing countries, which can be respectively applied for spatial disaggregation and the development of projections for other Latin American cities. The results may also be employed to complement global emission inventories and by local policy makers as an environmental management tool. 相似文献
56.
Marcelo Felix Alonso Karla Maria Longo Saulo R. Freitas Rafael Mello da Fonseca Virginie Marécal Michel Pirre Laura Gallardo Klenner 《Atmospheric environment (Oxford, England : 1994)》2010,44(39):5072-5083
This work describes the development of an urban vehicle emissions inventory for South America, based on the analysis and aggregation of available inventories for major cities, with emphasis on its application in regional atmospheric chemistry modeling. Due to the limited number of available local inventories, urban emissions were extrapolated based on the correlation between city vehicle density and mobile source emissions of carbon monoxide (CO) and nitrogen oxides (NOx). Emissions were geographically distributed using a methodology that delimits urban areas using high spatial resolution remote sensing products. This numerical algorithm enabled a more precise representation of urban centers. The derived regional inventory was evaluated by analyzing the performance of a chemical weather forecast model in relation to observations of CO, NOx and O3 in two different urban areas, São Paulo and Belo Horizonte. The gas mixing ratios simulated using the proposed regional inventory show good agreement with observations, consistently representing their hourly and daily variability. These results show that the integration of municipal inventories in a regional emissions map and their precise distribution in fine scale resolutions are important tools in regional atmospheric chemistry modeling. 相似文献
57.
58.
Climate change, drought risk and land capability for agriculture: implications for land use in Scotland 总被引:1,自引:0,他引:1
Iain Brown Laura Poggio Alessandro Gimona Marie Castellazzi 《Regional Environmental Change》2011,11(3):503-518
Land capability classification systems define and communicate biophysical limitations on land use, including climate, soils
and topography. They can therefore provide an accessible format for both scientists and decision-makers to share knowledge
on climate change impacts and adaptation. Underlying such classifications are complex interactions that require dynamic spatial
analysis, particularly between soil and climate. These relationships are investigated using a case study on drought risk for
agriculture in Scotland, which is currently considered less significant than wetness-related issues. The impact of drought
risk is assessed using an established empirical system for land capability linking indicator crops with water availability.
This procedure is facilitated by spatial interpolation of climate and soil profile data to provide soil moisture deficits
and plant available water on a regular 1-km grid. To evaluate potential impacts of future climate change, land capability
classes are estimated using both large-scale ensemble (multi-simulation) data from the HadRM3 regional climate model and local-scale
weather generator data (UKCP09) derived from multiple climate models. Results for the case study suggest that drought risk
is likely to have a much more significant influence on land use in the future. This could potentially act to restrict the
range of crops grown and hence reduce land capability in some areas unless strategic-level adaptation measures are developed
that also integrate land use systems and water resources with the wider environment. 相似文献
59.
60.
Ramos-Gómez J Coz A Viguri JR Luque A Martín-Díaz ML DelValls TÁ 《Environmental pollution (Barking, Essex : 1987)》2011,159(7):1914-1922
Biomarkers comprising activities of biotransformation enzymes (ethoxyresorufin-O-deethylase -EROD-, dibenzylfluorescein dealkylase -DBF-, glutathione S-transferase -GST), antioxidant enzymes (glutathione reductase -GR- and glutathione peroxidase -GPX), lipid peroxidation -LPO- and DNA strand breaks were analyzed in the clam Ruditapes philippinarum caged at Cádiz Bay, Santander Bay and Las Palmas de Gran Canaria (LPGC) Port (Spain). Sediments were characterized. Digestive gland was the most sensitive tissue to sediment contamination. In Cádiz Bay, changes in LPO regarding day 0 were related with metals. In LPGC Port, DBF, EROD, and GST activity responses suggested the presence of undetermined contaminants which might have led to DNA damage. In Santander Bay, PAHs were related with EROD activity, organic and metal contamination was found to be associated with GR and GST activities and DNA damage presented significant (p < 0.05) induction. R. philippinarum was sensitive to sediment contamination at biochemical level. Biomarkers allowed chemical exposure and sediment quality assessment. 相似文献