全文获取类型
收费全文 | 3243篇 |
免费 | 185篇 |
国内免费 | 844篇 |
专业分类
安全科学 | 259篇 |
废物处理 | 168篇 |
环保管理 | 286篇 |
综合类 | 1593篇 |
基础理论 | 581篇 |
环境理论 | 1篇 |
污染及防治 | 877篇 |
评价与监测 | 195篇 |
社会与环境 | 166篇 |
灾害及防治 | 146篇 |
出版年
2024年 | 6篇 |
2023年 | 41篇 |
2022年 | 118篇 |
2021年 | 140篇 |
2020年 | 124篇 |
2019年 | 103篇 |
2018年 | 115篇 |
2017年 | 157篇 |
2016年 | 117篇 |
2015年 | 146篇 |
2014年 | 171篇 |
2013年 | 256篇 |
2012年 | 245篇 |
2011年 | 232篇 |
2010年 | 198篇 |
2009年 | 201篇 |
2008年 | 196篇 |
2007年 | 241篇 |
2006年 | 174篇 |
2005年 | 124篇 |
2004年 | 135篇 |
2003年 | 124篇 |
2002年 | 114篇 |
2001年 | 113篇 |
2000年 | 107篇 |
1999年 | 88篇 |
1998年 | 75篇 |
1997年 | 71篇 |
1996年 | 50篇 |
1995年 | 44篇 |
1994年 | 30篇 |
1993年 | 32篇 |
1992年 | 34篇 |
1991年 | 13篇 |
1990年 | 17篇 |
1989年 | 23篇 |
1988年 | 16篇 |
1987年 | 9篇 |
1986年 | 7篇 |
1985年 | 5篇 |
1984年 | 5篇 |
1983年 | 6篇 |
1979年 | 7篇 |
1978年 | 4篇 |
1977年 | 4篇 |
1974年 | 3篇 |
1972年 | 3篇 |
1971年 | 3篇 |
1970年 | 4篇 |
1967年 | 4篇 |
排序方式: 共有4272条查询结果,搜索用时 31 毫秒
171.
172.
173.
Park SS Kim YJ Cho SY Kim SJ 《Journal of the Air & Waste Management Association (1995)》2007,57(4):434-443
Daily fine particulate matter (PM2.5) samples were collected at Gwangju, Korea, during the Aerosol Characterization Experiments (ACE)-Asia Project to determine the chemical properties of PM2.5 originating from local pollution and Asian dust (AD) storms. During the study period, two significant events occurred on April 10-13 and 24-25, 2001, and a minor event occurred on April 19, 2001. Based on air mass transport pathways identified by back-trajectory calculation, the PM2.5 dataset was classified into three types of aerosol populations: local pollution and two AD aerosol types. The two AD types were transported along different pathways. One originated from Gobi desert area in Mongolia, passing through Hunshandake desert in Northern Inner Mongolia, urban and polluted regions of China (AD1), and the other originated in sandy deserts located in the Northeast Inner Mongolia Plateau and then flowed southward through the Korean peninsula (AD2). During the AD2 event, a smoke plume that originated in North Korea was transported to our study site. Mass balance closures show that crustal materials were the most significant species during both AD events, contributing -48% to the PM2.5 mass; sulfate aerosols (19.1%) and organic matter (OM; 24.6%) were the second greatest contributors during the AD1 and AD2 periods, respectively, indicating that aerosol properties were dependent on the transport pathway. The sulfate concentration constituted only 6.4% (4.5 microg/m3) of the AD2 PM2.5 mass. OM was the major chemical species in the local pollution-dominated PM2.5 aerosols, accounting for 28.7% of the measured PM2.5 mass, followed by sulfate (21.4%), nitrate (15%), ammonium (12.8%), elemental carbon (8.9%), and crustal material (6.5%). Together with substantial enhancement of the crustal elements (Mg, Al, K, Ca, Sc, Ti, Mn, Fe, Sr, Zr, Ba, and Ce), higher concentrations of pollution elements (S, V, Ni, Zn, As, Cd, and Pb) were observed during AD1 and AD2 than during the local pollution period, indicating that, in addition to crustal material, the AD dust storms also had a significant influence on anthropogenic elements. 相似文献
174.
Biofiltration of waste gases is cost-effective and environment-friendly compared to the conventional techniques for treating large flow rates of gas streams with low concentrations of pollutants. Pulp and paper industry off-gases usually contain reduced sulfur compounds, such as hydrogen sulfide and a wide range of volatile organic compounds (VOCs), e.g., methanol. It is desirable to eliminate both of these groups of compounds. Since the co-treatment of inorganic sulfur compounds and VOCs in biotrickling filters is a relatively unexplored area, the simultaneous biotreatment of H2S and methanol as the model VOC was investigated. The results showed that, after adaptation, the elimination capacity of methanol could reach around 236 g m(-3) h(-1) with the simultaneous complete removal (100%) of 12 ppm H2S when the empty bed residence time is 24 s. The pH of the system was around 2. Methanol removal was hardly affected by the presence of hydrogen sulfide, despite the low pH. Conversely, the presence of the VOC in the waste gas reduced the efficiency of H2S biodegradation. The maximal methanol removal decreased somewhat when increasing the gas flow rate. This is the first report on the degradation of methanol at such low pH in a biotrickling filter and on the co-treatment of H2S and VOCs under such conditions. 相似文献
175.
Wen-Cheng Liu Jan-Tai Kuo Chih-Chieh Young Ming-Ching Wu 《Environmental Modeling and Assessment》2007,12(3):201-211
Numerical models are often used to evaluate the potential impact of human alternation of natural water bodies and to help
the design of the alternation to mitigate its impacts. In the past decade, three-dimensional hydrodynamic and reactive transport
modeling has matured from a research subject to a practical analysis technology. This paper presents a practical study in
which a three-dimensional hydrodynamic and water quality model [hydrodynamic eutrophication model (HEM-3D)] was applied to
determine the optimal location for treated wastewater discharged from marine outfall system in the Keelung harbor and the
adjacent coastal sea. First, model validation was conducted with respect to surface elevation, current, and water quality
variables measured in the Keelung harbor station and its coastal sea. The overall performance of the model was in qualitative
agreement with the available field data. The model was then used to evaluate several scenarios of the locations from marine
outfall system. Based on model simulation results, a location at the northeast of Ho-Ping Island was recommended for adoption
because the environmental impact is smaller than any other alternative.
相似文献
Wen-Cheng LiuEmail: |
176.
Composition and distribution of polycyclic aromatic hydrocarbons in the surface sediments from the Susquehanna River 总被引:6,自引:0,他引:6
Polycyclic aromatic hydrocarbon (PAH) concentrations in 34 surface sediments along the Susquehanna River were investigated in 2000. The total concentrations of PAHs in the surface sediments of Lake Clarke, Lake Aldred, the upper Conowingo Reservoir, and the lower Conowingo Reservoir were 3.3+/-1.5 microg g-1 (n=9), 1.6+/-1.3 microg g-1 (n=4), 9.8+/-5.5 microg g-1 (n=7), and 4.0+/-1.2 microg g-1 (n=14), respectively. These represent the first comprehensive measurement of PAHs in Susquehanna River surface sediments. Overall, total PAH concentrations were relatively lower in Lake Aldred, which is more shallow and sloped, and significantly higher in the upper Conowingo Reservoir. The sediment PAH levels were related to river flow rates, which are indirectly correlated with the particle size of the surface sediments. Total PAH levels in all the studied sites were below the effects range median (ERM) of 44.8 microg g-1 with 38% (13 of the 34 sampling sites) exceeding the effects range low (ERL) of 4.02 microg g-1. Principal component analysis indicated that variations in the PAH compound patterns of each reservoir decreased from upstream to downstream, indicating that the surface sediments were mixed along the Susquehanna River. The PAH patterns in the lower Conowingo Reservoir sediments were a combination of those upstream sources. Source analysis using isomer ratios as indicators suggested that PAHs in the Susquehanna River surface sediment are derived from the combustion of fossil fuels such as coal and gasoline with coal as the major source of contaminants. 相似文献
177.
Spectroscopic Distribution of Dissolved Organic Matter in a Dam Reservoir Impacted by Turbid Storm Runoff 总被引:1,自引:0,他引:1
Spectroscopic characteristics of dissolved organic matter (DOM) in a large dam reservoir were determined using ultraviolet
absorbance and fluorescence spectroscopy to investigate spatial distribution of DOM composition after turbid storm runoff.
Water samples were collected along a longitudinal axis of the reservoir at three to four depths after a severe storm runoff.
Vertical profiles of turbidity data showed that a turbid water layer was located at a middle depth of the entire reservoir.
The spectroscopic characteristics of DOM samples in the turbid water layer were similar to those of terrestrial DOM, as demonstrated
by the higher specific UV absorbance (SUVA) and the lower fluorescence emission intensity ratio (F
450/F
500) compared to other surrounding DOM samples in the reservoir. Synchronous fluorescence spectroscopy revealed that higher content
of humic-like DOM composition was contained in the turbid water. Fluorescence excitation–emission matrix (EEM) showed that
lower content of protein-like aromatic amino acids was present in the turbid water DOM. The highest protein-like fluorescence
was typically observed at a bottom layer of each sampling location. The bottom water DOM exhibited extremely high protein-like
florescence near the dam site. The particular observation was attributed to the low water temperature and the isolation of
the local bottom water due to the upper location of the withdrawal outlet near the dam. Our results suggest that the distribution
of DOM composition in a dam reservoir is strongly influenced by the outflow operation, such as selective withdrawal, as well
as terrestrial-origin DOM inputs from storm runoff. 相似文献
178.
Effect of amorphous silica and silica sand on removal of chromium(VI) by zero-valent iron 总被引:1,自引:0,他引:1
The effect of two surfaces (amorphous silica and silica sand) on the reduction of chromium(VI) by zero-valent iron (Fe(0)) was investigated using batch reactors. The amendment of both surfaces significantly increased the rate and extent of Cr(VI) removal. The rate enhancement by amended surfaces is presumed to result from scavenging of Fe(0)-Cr(VI) reaction products by the provided surfaces, which minimized surface deactivation of Fe(0). The rate enhancing effect was greater for silica compared to sand, and the difference is attributed to silica's higher surface area, greater affinity for reaction products and pH buffering effect. For a given mass of Fe(0), the reactivity and longevity of Fe(0) to treat Cr(VI) increased with increasing dose of silica. Elemental analyses of the reacted iron and silica revealed that chromium removed from the solution was associated with both surfaces, with its mass distribution being approximately 1:1 per mass of iron and silica. The overall result suggests reductive precipitation was a predominant Cr(VI) removal pathway, which involves initial reduction of Cr(VI) to Cr(III), followed by formation of Cr(III)/Fe(III) hydroxides precipitates. 相似文献
179.
180.
战略环境评价系统及工作程序 总被引:26,自引:0,他引:26
介绍了战略环境评价系统组成的五个要素 ,即评价者、评价对象、评价目的、评价标准和评价方法 ,分析了其相互关系及各要素与战略环境评价系统的关系 ,并提出了战略环境评价工作程序。 相似文献