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Guofeng Shen Wei Wang Yifeng Yang Chen Zhu Yujia Min Miao Xue Junnan Ding Wei Li Bin Wang Huizhong Shen Rong Wang Xilong Wang Shu Tao 《Atmospheric environment (Oxford, England : 1994)》2010,44(39):5237-5243
Coal consumption is one important contributor to energy production, and is regarded as one of the most important sources of air pollutants that have considerable impacts on human health and climate change. Emissions of polycyclic aromatic hydrocarbons (PAHs) from coal combustion were studied in a typical stove. Emission factors (EFs) of 16 EPA priority PAHs from tested coals ranged from 6.25 ± 1.16 mg kg?1 (anthracite) to 253 ± 170 mg kg?1 (bituminous), with NAP and PHE dominated in gaseous and particulate phases, respectively. Size distributions of particulate phase PAHs from tested coals showed that they were mostly associated with particulate matter (PM) with size either between 0.7 and 2.1 μm or less than 0.4 μm (PM0.4). In the latter category, not only were more PAHs present in PM0.4, but also contained higher fractions of high molecular weight PAHs. Generally, there were more than 89% of total particulate phase PAHs associated with PM2.5. Gas-particle partitioning of freshly emitted PAHs from residential coal combustions were thought to be mainly controlled by absorption rather than adsorption, which is similar to those from other sources. Besides, the influence of fuel properties and combustion conditions was further investigated by using stepwise regression analysis, which indicated that almost 57 ± 10% of total variations in PAH EFs can be accounted for by moisture and volatile matter content of coal in residential combustion. 相似文献
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农业化学品投入状况及其对环境的影响 总被引:9,自引:0,他引:9
蔡荣 《中国人口.资源与环境》2010,20(3)
农业生产中,农业化学品的大量使用产生了明显的负外部性影响,尤其是农业的面源污染问题随化肥、农药投入的增加而不断加剧。通过统计分析方法,对农业化学品投入数量及区域分布特征、农业化学品投入存在的问题及其所造成的面源污染问题进行分析。结果表明:化肥和农药总投入不断增加,其中河南、山东、江苏、安徽、湖北和湖南6省投入总额接近全国的一半;农业化学品使用存在过量投入、投入结构失衡和施肥施药技术落后等问题;农业化学投入品的过量使用造成的环境污染问题正不断加剧,农业面源污染排放对污染总量的贡献率不断上升。最后提出了相关政策建议,包括加强农业面源污染控制的政策框架和配套制度建设、推广成熟的化肥农药施用技术和加强农业环保教育。 相似文献
86.
Afforestation of agricultural lands has been one of the major land use changes in China in recent decades. To better understand
the effect of such land use change on soil quality, we investigated selected soil physical, chemical and microbial properties
(0–15 cm depth) in marginal agricultural land and a chronosequence of poplar (Populus
euramericana cv. ‘N3016’) plantations (5-, 10-, 15- and 20-years old) in a semi-arid area of Northeast China. Soil bulk density significantly
declined after conversion of agricultural lands to poplar plantations. Soil total organic carbon (TOC) and nitrogen (TN) concentrations,
microbial biomass C (MBC) and potential N mineralization rate (PNM) decreased initially following afforestation of agricultural
lands, and then increased with stand development. However, soil metabolic quotient (qCO2) exhibited a reverse trend. In addition, soil particulate organic matter C (POM-C) and N (POM-N) concentrations showed no
significant changes in the first 10 years following afforestation, and then increased with stand age. These findings demonstrated
that soil quality declined initially following afforestation of agricultural lands in semi-arid regions, and then recovered
with stand development. Following 15 years of afforestation, many soil quality parameters recovered to the values found in
agricultural land. We propose that change in soil quality with stand age should be considered in determining optimum rotation
length of plantations and best management practices for afforestation programs. 相似文献
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Limei Chen Guodong Ding Yu Gao Pei Wang Rong Shi Hong Huang Ying Tian 《Environmental science and pollution research international》2014,21(9):6170-6175
Manganese (Mn) is an essential mineral nutrient in mammals. The physiological role of Mn in animal models is well documented, but little is known about the adverse effects of Mn deficiency or overexposure in humans, including pregnancy outcomes such as birth weight. We examined the relationship of the maternal and cord blood Mn levels with birth weight in a cohort of 172 mother–infant pairs born in Shanghai, China. Non-linear spline and quadratic regression models were used to test the hypothesis of an inverted U-shaped association between the Mn levels and birth weight. The median (range) levels of Mn in the maternal and cord blood were 5.38 (2.34–30.37) μg/dL and 7.66 (2.57–34.23) μg/dL, respectively. An inverted U-shaped relationship was observed between maternal Mn and birth weight after adjusting for potential confounders. The birth weight increased with Mn levels up to 4.18 μg/dL, and a slight reduction in weight was observed at higher levels. The cord blood Mn levels were not found to be associated with birth weight. Both lower and higher Mn exposures are associated with lower birth weight, which may influence important developmental parameters; the association of higher Mn levels with lower weight was weak and imprecise. 相似文献
89.
用静态吸附法考察粉末活性炭对水中三烯丙基异氰脲酸酯(CAIC)的吸附行为,采用单因素分析法对活性炭吸附化工废水中TAIC的工艺条件进行研究。实验结果表明,在TAIC模拟废水中,其TAIC初始浓度为800 mg/L,pH为7,在温度为298 K、转速为150 r/min的条件下,当活性炭的投加量达到4.4 g/L,吸附反应时间为50 min时,TAIC的去除效率最高为96.17%;对于实际废水,其TAIC初始浓度为1 500 mg/L,溶液pH为3,在温度为298 K、转速为150 r/min的条件下,当活性炭投加量达到10 g/L,吸附反应时间为2 h时,TAIC的去除效率最高为46.8%。这也是由于实际废水组分复杂,其他有机物存在一定的吸附竞争机制。 相似文献
90.
雅砻江流域湿地景观格局变化分析 总被引:1,自引:0,他引:1
应用ArcGIS软件,对雅砻江流域湿地1986和2000年遥感数据进行解译、矢量化处理,用Apack软件进行湿地景观格局指数计算,研究了近15 a雅砻江流域景观空间格局特征及其变化。结果表明:(1)近15 a雅砻江流域湿地景观面积减少,减少量为49404 hm2,占2000年湿地总面积的0506%;(2)两个时期内湿地斑块密度保持不变,湿地景观的聚集度都很高,均在099以上,湿地景观集中分布,破碎化水平低;(3)雅砻江流域湿地景观的多样性指数水平和均匀度水平较低,而且两指数在两个个时期内没有发生太大的变化,且各类湿地景观比例差异相对较大,沼泽湿地景观控制的程度较高;(4)雅砻江流域的5类湿地景观分布质心基本上未发生变化,但总体格局分布质心向南偏移001°,再向西偏移023°,整体上向西南方向偏移了2532 km 相似文献