全文获取类型
收费全文 | 15953篇 |
免费 | 199篇 |
国内免费 | 134篇 |
专业分类
安全科学 | 451篇 |
废物处理 | 588篇 |
环保管理 | 2191篇 |
综合类 | 3088篇 |
基础理论 | 4005篇 |
环境理论 | 10篇 |
污染及防治 | 3916篇 |
评价与监测 | 972篇 |
社会与环境 | 940篇 |
灾害及防治 | 125篇 |
出版年
2022年 | 122篇 |
2021年 | 126篇 |
2020年 | 110篇 |
2019年 | 135篇 |
2018年 | 201篇 |
2017年 | 242篇 |
2016年 | 332篇 |
2015年 | 283篇 |
2014年 | 374篇 |
2013年 | 1338篇 |
2012年 | 476篇 |
2011年 | 633篇 |
2010年 | 508篇 |
2009年 | 572篇 |
2008年 | 635篇 |
2007年 | 664篇 |
2006年 | 625篇 |
2005年 | 503篇 |
2004年 | 488篇 |
2003年 | 498篇 |
2002年 | 434篇 |
2001年 | 543篇 |
2000年 | 424篇 |
1999年 | 243篇 |
1998年 | 199篇 |
1997年 | 191篇 |
1996年 | 208篇 |
1995年 | 216篇 |
1994年 | 208篇 |
1993年 | 205篇 |
1992年 | 215篇 |
1991年 | 203篇 |
1990年 | 204篇 |
1989年 | 175篇 |
1988年 | 152篇 |
1987年 | 132篇 |
1986年 | 157篇 |
1985年 | 158篇 |
1984年 | 160篇 |
1983年 | 162篇 |
1982年 | 156篇 |
1981年 | 162篇 |
1980年 | 151篇 |
1979年 | 145篇 |
1978年 | 108篇 |
1977年 | 121篇 |
1974年 | 109篇 |
1973年 | 91篇 |
1972年 | 107篇 |
1971年 | 88篇 |
排序方式: 共有10000条查询结果,搜索用时 15 毫秒
981.
U.S. National PM2.5 Chemical Speciation Monitoring Networks—CSN and IMPROVE: Description of networks
Paul A. Solomon Dennis Crumpler James B. Flanagan R.K.M. Jayanty Ed E. Rickman Charles E. McDade 《Journal of the Air & Waste Management Association (1995)》2014,64(12):1410-1438
The U.S. Environmental Protection Agency (EPA) initiated the national PM2.5 Chemical Speciation Monitoring Network (CSN) in 2000 to support evaluation of long-term trends and to better quantify the impact of sources on particulate matter (PM) concentrations in the size range below 2.5 μm aerodynamic diameter (PM2.5; fine particles). The network peaked at more than 260 sites in 2005. In response to the 1999 Regional Haze Rule and the need to better understand the regional transport of PM, EPA also augmented the long-existing Interagency Monitoring of Protected Visual Environments (IMPROVE) visibility monitoring network in 2000, adding nearly 100 additional IMPROVE sites in rural Class 1 Areas across the country. Both networks measure the major chemical components of PM2.5 using historically accepted filter-based methods. Components measured by both networks include major anions, carbonaceous material, and a series of trace elements. CSN also measures ammonium and other cations directly, whereas IMPROVE estimates ammonium assuming complete neutralization of the measured sulfate and nitrate. IMPROVE also measures chloride and nitrite. In general, the field and laboratory approaches used in the two networks are similar; however, there are numerous, often subtle differences in sampling and chemical analysis methods, shipping, and quality control practices. These could potentially affect merging the two data sets when used to understand better the impact of sources on PM concentrations and the regional nature and long-range transport of PM2.5. This paper describes, for the first time in the peer-reviewed literature, these networks as they have existed since 2000, outlines differences in field and laboratory approaches, provides a summary of the analytical parameters that address data uncertainty, and summarizes major network changes since the inception of CSN.
ImplicationsTwo long-term chemical speciation particle monitoring networks have operated simultaneously in the United States since 2001, when the EPA began regular operations of its PM2.5 Chemical Speciation Monitoring Network (IMPROVE began in 1988). These networks use similar field sampling and analytical methods, but there are numerous, often subtle differences in equipment and methodologies that can affect the results. This paper describes these networks since 2000 (inception of CSN) and their differences, and summarizes the analytical parameters that address data uncertainty, providing researchers and policymakers with background information they may need (e.g., for 2018 PM2.5 designation and State Implementation Plan process; McCarthy, 2013) to assess results from each network and decide how these data sets can be mutually employed for enhanced analyses. Changes in CSN and IMPROVE that have occurred over the years also are described. 相似文献
982.
Thomas M. Lewinsohn José Luiz Attayde Carlos Roberto Fonseca Gislene Ganade Leonardo Ré Jorge Johannes Kollmann Gerhard E. Overbeck Paulo Inácio Prado Valério D. Pillar Daniela Popp Pedro L. B. da Rocha Wesley Rodrigues Silva Annette Spiekermann Wolfgang W. Weisser 《Ambio》2015,44(2):154-162
Ecological science contributes to solving a broad range of environmental problems. However, lack of ecological literacy in practice often limits application of this knowledge. In this paper, we highlight a critical but often overlooked demand on ecological literacy: to enable professionals of various careers to apply scientific knowledge when faced with environmental problems. Current university courses on ecology often fail to persuade students that ecological science provides important tools for environmental problem solving. We propose problem-based learning to improve the understanding of ecological science and its usefulness for real-world environmental issues that professionals in careers as diverse as engineering, public health, architecture, social sciences, or management will address. Courses should set clear learning objectives for cognitive skills they expect students to acquire. Thus, professionals in different fields will be enabled to improve environmental decision-making processes and to participate effectively in multidisciplinary work groups charged with tackling environmental issues. 相似文献
983.
Drought is a significant natural hazard that slowly evolves over time. Because of its character, drought is difficult to monitor and impacts are often poorly documented. Agriculture is one of the most sensitive sectors that are prone to drought. The objective of this research is to assess the impacts of drought on soybean production and revenue in Kentucky. Soybeans are one of Kentucky’s most important commodities. In this study, impacts of 1930–1931, 1940–1942, 1952–1955, 1987–1988, 1999–2000, and 2007 droughts were considered. It was found that over the recent years, up to 56 % of the revenue from soybeans was lost due to drought. During the first half of the twentieth century, revenue loss reached up to 77 %. This research is valuable to the general public as well as planners and policy makers. Proper documentation of impacts of past droughts will help identify drought vulnerabilities and results in better risk management and mitigation. 相似文献
984.
Elizabeth Guthrie Nichols Rachel L. Cook James E. Landmeyer Brad Atkinson Donald R. Malone George Shaw Leilani Woods 《补救:环境净化治理成本、技术与工艺杂志》2014,24(2):29-46
A former bulk fuel terminal in North Carolina is a groundwater phytoremediation demonstration site where 3,250 hybrid poplars, willows, and pine trees were planted from 2006 to 2008 over approximately 579,000 L of residual gasoline, diesel, and jet fuel. Since 2011, the groundwater altitude is lower in the area with trees than outside the planted area. Soil‐gas analyses showed a 95 percent mass loss for total petroleum hydrocarbons (TPH) and a 99 percent mass loss for benzene, toluene, ethylbenzene, and xylenes (BTEX). BTEX and methyl tert‐butyl ether concentrations have decreased in groundwater. Interpolations of free‐phase, fuel product gauging data show reduced thicknesses across the site and pooling of fuel product where poplar biomass is greatest. Isolated clusters of tree mortalities have persisted in areas with high TPH and BTEX mass. Toxicity assays showed impaired water use for willows and poplars exposed to the site's fuel product, but Populus survival was higher than the willows or pines on‐site, even in a noncontaminated control area. All four Populus clones survived well at the site. © 2014 Wiley Periodicals, Inc.* 相似文献
985.
David G. Angeler Craig R. Allen Hannah E. Birgé Stina Drakare Brendan G. McKie Richard K. Johnson 《Ambio》2014,43(1):113-125
Freshwater ecosystems are important for global biodiversity and provide essential ecosystem services. There is consensus in the scientific literature that freshwater ecosystems are vulnerable to the impacts of environmental change, which may trigger irreversible regime shifts upon which biodiversity and ecosystem services may be lost. There are profound uncertainties regarding the management and assessment of the vulnerability of freshwater ecosystems to environmental change. Quantitative approaches are needed to reduce this uncertainty. We describe available statistical and modeling approaches along with case studies that demonstrate how resilience theory can be applied to aid decision-making in natural resources management. We highlight especially how long-term monitoring efforts combined with ecological theory can provide a novel nexus between ecological impact assessment and management, and the quantification of systemic vulnerability and thus the resilience of ecosystems to environmental change. 相似文献
986.
M. St. J. Warne G. E. Batley O. Braga J. C. Chapman D. R. Fox C. W. Hickey J. L. Stauber R. Van Dam 《Environmental science and pollution research international》2014,21(1):51-60
The Australian and New Zealand Guidelines for Fresh and Marine Water Quality are a key document in the Australian National Water Quality Management Strategy. These guidelines released in 2000 are currently being reviewed and updated. The revision is being co-ordinated by the Australian Department of Sustainability, Environment, Water, Population and Communities, while technical matters are dealt with by a series of Working Groups. The revision will be evolutionary in nature reflecting the latest scientific developments and a range of stakeholder desires. Key changes will be: increasing the types and sources of data that can be used; working collaboratively with industry to permit the use of commercial-in-confidence data; increasing the minimum data requirements; including a measure of the uncertainty of the trigger value; improving the software used to calculate trigger values; increasing the rigour of site-specific trigger values; improving the method for assessing the reliability of the trigger values; and providing guidance of measures of toxicity and toxicological endpoints that may, in the near future, be appropriate for trigger value derivation. These changes will markedly improve the number and quality of the trigger values that can be derived and will increase end-users’ ability to understand and implement the guidelines in a scientifically rigorous manner. 相似文献
987.
E. Amoozadeh M. Malek R. Rashidinejad S. Nabavi M. Karbassi R. Ghayoumi G. Ghorbanzadeh-Zafarani H. Salehi B. Sures 《Environmental science and pollution research international》2014,21(3):2386-2395
In the present study, cadmium and lead concentrations were compared in barnacles, ghost shrimps, polychaetes, bivalves, and sediment from ten different locations along the intertidal zone of the Persian Gulf and the Gulf of Oman. The results revealed significant differences in the heavy metal concentrations between the organisms with barnacles showing, by far, the highest metal concentrations. The bioaccumulation factor of Cd in different animals follows this pattern with barnacles?>?bivalves?>?polychaetes?>?ghost shrimps, while the pattern for Pb was barnacles?>?polychaetes?>?bivalves?>?ghost shrimps. In most of the stations, sediments showed the lowest lead and cadmium concentrations. Therefore, it is concluded that barnacles with Pb concentrations between 0.17 and 2,016.1 μg/g and Cd concentrations ranging from 0.4 to 147.1 μg/g are the best organisms to be employed in monitoring programs designed to assess pollution with bioavailable metals in the Persian Gulf and the Gulf of Oman. 相似文献
988.
M. Urbaniak E. Kiedrzyńska M. Zieliński W. Tołoczko M. Zalewski 《Environmental science and pollution research international》2014,21(6):4441-4452
Reservoirs situated along a river continuum are ecosystems where rates of transfer of suspended matter and associated micropollutants are reduced due to sedimentation, accumulation, and biological and physical transformation processes. Among the micropollutants, PCDDs and PCDFs are substances that are highly toxic and carcinogenic for humans and animals. They are emitted and dispersed in the environment throughout the whole catchment area and may accumulate in aquatic and terrestrial food chains, creating a risk for human health. A wealth of data exists indicating the increase in the concentrations of pollutants along a river continuum. A comparative analysis of total, individual, and TEQ PCDD/PCDF concentrations in large lowland, shallow reservoirs located in different catchments (“I”—industrial/urban/agricultural, “U”—urban/agricultural, and “A”—agricultural/rural) showed decreases of the TEQ concentrations in bottom sediments along a gradient from the middle sections to the dam walls. Moreover, penta-, hexa-, and heptachlorinated CDD/CDF congeners were reduced from 28.8 up to 93.6 % in all three types of reservoirs. A further analysis of water samples from the inlets and outlets of the “A” reservoir confirmed this tendency. 相似文献
989.
D. Medas P. Lattanzi F. Podda C. Meneghini A. Trapananti A. Sprocati M. A. Casu E. Musu G. De Giudici 《Environmental science and pollution research international》2014,21(11):6775-6782
An amorphous Zn biomineralization (“white mud”), occurring at Naracauli stream, Sardinia, in association with cyanobacteria Leptolyngbya frigida and diatoms, was investigated by electron microscopy and X-ray absorption spectroscopy. Preliminary diffraction analysis shows that the precipitate sampled on Naracauli stream bed is mainly amorphous, with some peaks ascribable to quartz and phyllosilicates, plus few minor unattributed peaks. Scanning electron microscopy analysis shows that the white mud, precipitated in association with a seasonal biofilm, is made of sheaths rich in Zn, Si, and O, plus filaments likely made of organic matter. Transmission electron microscopy analysis shows that the sheaths are made of smaller units having a size in the range between 100 and 200 nm. X-ray absorption near-edge structure and extended X-ray absorption fine structure data collected at the Zn K-edge indicate that the biomineral has a local structure similar to hemimorphite, a zinc sorosilicate. The differences of this biomineral with respect to the hydrozincite biomineralization documented about 3 km upstream in the same Naracauli stream may be related to either variations in the physicochemical parameters and/or different metabolic behavior of the involved biota. 相似文献
990.
J. Gasperi C. Sebastian V. Ruban M. Delamain S. Percot L. Wiest C. Mirande E. Caupos D. Demare M. Diallo Kessoo Kessoo M. Saad J. J. Schwartz P. Dubois C. Fratta H. Wolff R. Moilleron G. Chebbo C. Cren M. Millet S. Barraud M. C. Gromaire 《Environmental science and pollution research international》2014,21(8):5267-5281
This study aimed at: (a) providing information on the occurrence and concentration ranges in urban stormwater for a wide array of pollutants (n?=?77); (b) assessing whether despite the differences between various catchments (land use, climatic conditions, etc.), the trends in terms of contamination level are similar; and (c) analyzing the contribution of total atmospheric fallout (TAF) with respect to sources endogenous to this contamination. The studied contaminants include conventional stormwater contaminants (polycyclic aromatic hydrocarbons (PAHs), Zn, Cu, Pb, etc.), in addition to poorly or undocumented pollutants such as nonylphenol and octylphenol ethoxylates (NPnEO and OPnEO), bisphenol A (BPA), polybrominated diphenyl ethers (PBDEs), a wide variety of pesticides, and various metals of relevance (As, Ti, Sr, V). Sampling and analysis were performed using homogeneous methods on three urban catchments with different land use patterns located in three distinct French towns. For many of these pollutants, the results do not allow highlighting a significant difference in stormwater quality at the scale of the three urban catchments considered. Significant differences were, however, observed for several metals (As, Cr, Cu, Ni, Sr and Zn), PAHs, and PBDEs, though this assessment would need to be confirmed by further experiments. The pollutant distributions between dissolved and particulate phases were found to be similar across the three experimental sites, thus suggesting no site dependence. Lastly, the contributions of TAF to stormwater contamination for micropollutants were quite low. This finding held true not only for PAHs, as previously demonstrated in the literature, but also for a broader range of molecules such as BPA, NPnEO, OPnEO, and PBDEs, whose high local production is correlated with the leaching of urban surfaces, buildings, and vehicles. 相似文献