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51.
Morgenstern P Versteegh AF de Korte GA Hoogerbrugge R Mooibroek D Bannink A Hogendoorn EA 《Journal of environmental monitoring : JEM》2003,5(6):885-890
An indicative survey has been carried out in The Netherlands investigating the presence of methyl tertiary butyl ether (MTBE) in drinking water and the corresponding sources. In total, 71 different sites used for the preparation of drinking water in The Netherlands were sampled in two successive seasons in 2001 involving the analysis of 156 samples. (ground water (n = 88), surface water (n = 17), bank filtrate water (n = 6) and drinking water (n = 45)). To combine high sample throughput with high selectivity and sensitivity, off-line purge and trap for sampling and gas chromatography mass spectrometry equipped with an automated thermal desorption sampler (TDS-GC-MS) was selected as the preferred analytical methodology. The developed procedure enabled the analysis of at least 40 samples per day and provided a limit of quantification of 2 ng l(-1). In the first period 63 samples of raw water were analyzed. Concentrations ranged between < 10 ng l(-1) and 420 ng l(-1) with a median concentration below 10 ng l(-1). The second period was focused at the re-sampling of positive locations (MTBE > 10 ng l(-1)) and a few additional drinking water utilities of which both the raw and drinking water of the utilities were analyzed. The median concentration of MTBE in the selected set of drinking water samples was 20 ng l(-1) (n = 45). At one location MTBE was found at a level of 2900 ng l(-1) caused by point source contamination of the ground water (11 900 ng l(-1)). Special attention has been paid to the quality of the results by analyzing all samples in duplicate and the analysis of control samples during each series of analyses. 相似文献
52.
Ponce de León CA DeNicola K Montes Bayón M Caruso JA 《Journal of environmental monitoring : JEM》2003,5(3):435-440
Different techniques have been employed in order to evaluate the most efficient procedure for the extraction of selenium from soil as required for speciation. Selenium contaminated sediments from Stewart Lake Wetland, California were used. A strong acid mineralization of the samples gives quantitative total selenium, which is then used to estimate recoveries for the milder extraction methods. The different extraction methodologies involve the sequential use of water, buffer (phosphate, pH 7) and either acid solution (e.g. HNO3 or HCl) or basic solutions (e.g. ammonium acetate, NaOH or TMAH). Pyrophosphate extraction was also evaluated and showed that selenium was not associated with humic acids. The extractants were subsequently analyzed by size exclusion chromatography (SEC) with UV (254 and 400 nm) and on-line ICP-MS detection; anion exchange chromatography, and ion-pair reversed phase chromatography with ICP-MS detection. For sequential extractions the extraction efficiencies showed that the basic extractions were more efficient than the acidic. The difference between the acidic and the basic extraction efficiency is carried to the sulfite extraction, suggesting that whatever is not extracted by the acid is subsequently extracted by the sulfite. The species identified with the different chromatographies were selenate, selenite, elemental selenium and some organic selenium. 相似文献
53.
指出水产品代谢物的排出及没有被水产品利用的残饵是造成渔业养殖中水环境污染的重要原因之一。针对渔业污染物的生成情况,提出了渔业污染物排放总量的3种核定方法:实测法、物料平衡法、经验系数法。 相似文献
54.
Assessing land use impacts on flood processes in complex terrain by using GIS and modeling approach 总被引:1,自引:0,他引:1
Y. B. Liu F. De Smedt L. Hoffmann L. Pfister 《Environmental Modeling and Assessment》2005,9(4):227-235
A distributed hydrologic modeling and GIS approach is applied for the assessment of land use impact in the Steinsel sub-basin, Alzette, Grand-Duchy of Luxembourg. The assessment focuses on the runoff contributions from different land use classes and the potential impact of land use changes on runoff generation. The results show that the direct runoff from urban areas is dominant for a flood event compared with runoff from other land use areas in this catchment, and tends to increase for small floods and for the dry season floods, whereas the interflow from forested, pasture and agricultural field areas contributes to the recession flow. Significant variations in flood volume, peak discharge, time to the peak, etc., are found from the model simulation based on the three hypothetical land use change scenarios. 相似文献
55.
Application of a checklist for quality assistance in environmental modelling to an energy model 总被引:2,自引:0,他引:2
James Risbey Jeroen van der Sluijs Penny Kloprogge Jerry Ravetz Silvio Funtowicz Serafin Corral Quintana 《Environmental Modeling and Assessment》2005,10(1):63-79
Large, complex energy models present considerable challenges to develop and test. Uncertainty assessments of such models provide only partial guidance on the quality of the results. We have developed a model quality assistance checklist to aid in this purpose. The model checklist provides diagnostic output in the form of a set of pitfalls for the model application. The checklist is applied here to an energy model for the problem of assessing energy use and greenhouse gas emissions. Use of the checklist suggests that results on this issue are contingent on a number of assumptions that are highly value-laden. When these assumptions are held fixed, the model is deemed capable of producing moderately robust results of relevance to climate policy over the longer term. Checklist responses also indicate that a number of details critical to policy choices or outcomes on this issue are not captured in the model, and model results should therefore be supplemented with alternative analyses. 相似文献
56.
Pacáková V Pockeviciute D Armalis S Stulík K Li J Veselý J 《Journal of environmental monitoring : JEM》2000,2(2):187-191
Experiments were carried out to monitor the equilibrium distribution of lead, cadmium and copper between an aqueous phase modelling natural water and a solid phase modelling natural sediment, under varying conditions. The aqueous phase was analysed using ETAAS and differential pulse anodic stripping voltammetry (DPASV), whereas XRD and FTIR were used to study the solid phase. Sorption isotherms at constant pH were measured. Conditional distribution constants were calculated as functions of the pH, the time of equilibration and the amount of solid material. The results obtained stress the need for standardization of the approaches to the study of water-sediment interactions in order to be able to evaluate and compare the extensive data from field measurements and to predict these interactions. 相似文献
57.
Sánchez López FJ Gil García MD Martínez Vidal JL Aguilera PA Garrido Frenich A 《Environmental monitoring and assessment》2004,93(1-3):17-29
Water quality assessment in the Aznalcollar area was attempted using multivariate methods based on heavy metal concentrations in red swamp crayfish (Procamburus clarkii). Trace levels of four heavy metals, copper (Cu), zinc (Zn), cadmium (Cd) and lead (Pb), were detected in crayfish from eleven different stations. Principal component analysis (PCA) highlighted a gradient of contamination between the sampling stations. Cluster analysis (CA) distinguished three groups of stations. Discriminant analysis also differentiated three groups. The group centroids of the first discriminant function were used to devise an index that varies according to the source of the crayfish. These standardized values are proposed for use as a water quality index. The ability of this index to successfully predict environmental quality was proved with random samples. 相似文献
58.
Gilberto C. Gallopín 《Environmental Modeling and Assessment》1996,1(3):101-117
Through a systems approach indicators are shown to have the nature of variables, adopting different values or states, while other associated terms allude to special meanings assigned to specific values of the indicators. Practical implications are discussed. The concept of situational indicators of sustainability is introduced, representing a non-numerical function of both “pressures” or “driving forces” and “state” variables. A cost-effective multi-tiered approach to situational indicators is proposed. The concept of situational indicators is shown to be a particular case of indicators of systems behavior. A general systems formulation of the problem of sustainability highlights the importance of indicators of systems behavior and the central role of models in their definition. 相似文献
59.
The modern theory of biological evolution: an expanded synthesis 总被引:12,自引:2,他引:12
In 1858, two naturalists, Charles Darwin and Alfred Russel Wallace, independently proposed natural selection as the basic mechanism responsible for the origin of new phenotypic variants and, ultimately, new species. A large body of evidence for this hypothesis was published in Darwins Origin of Species one year later, the appearance of which provoked other leading scientists like August Weismann to adopt and amplify Darwins perspective. Weismanns neo-Darwinian theory of evolution was further elaborated, most notably in a series of books by Theodosius Dobzhansky, Ernst Mayr, Julian Huxley and others. In this article we first summarize the history of life on Earth and provide recent evidence demonstrating that Darwins dilemma (the apparent missing Precambrian record of life) has been resolved. Next, the historical development and structure of the modern synthesis is described within the context of the following topics: paleobiology and rates of evolution, mass extinctions and species selection, macroevolution and punctuated equilibrium, sexual reproduction and recombination, sexual selection and altruism, endosymbiosis and eukaryotic cell evolution, evolutionary developmental biology, phenotypic plasticity, epigenetic inheritance and molecular evolution, experimental bacterial evolution, and computer simulations (in silico evolution of digital organisms). In addition, we discuss the expansion of the modern synthesis, embracing all branches of scientific disciplines. It is concluded that the basic tenets of the synthetic theory have survived, but in modified form. These sub-theories require continued elaboration, particularly in light of molecular biology, to answer open-ended questions concerning the mechanisms of evolution in all five kingdoms of life.Dedicated to Prof. Dr. Dr. hc mult. Ernst Mayr on the occasion of his 100th birthdayThis revised version was published online in March 2004, with corrections to the caption of Figure 6. 相似文献
60.
Nectar acquisition in the honeybee Apis mellifera is a partitioned task in which foragers gather nectar and bring it to the hive, where nest mates unload via trophallaxis
(i.e. mouth-to-mouth transfer) the collected food for further storage. Because forager mates exploit different feeding places
simultaneously, this study addresses the question of whether nectar unloading interactions between foragers and hive-bees
are established randomly, as it is commonly assumed. Two groups of foragers were trained to exploit a different scented food
source for 5 days. We recorded their trophallaxes with hive-mates, marking the latter ones according to the forager group
they were unloading. We found non-random probabilities for the occurrence of trophallaxes between experimental foragers and
hive-bees, instead, we found that trophallactic interactions were more likely to involve groups of individuals which had formerly
interacted orally. We propose that olfactory cues present in the transferred nectar promoted the observed bias, and we discuss
this bias in the context of the organization of nectar acquisition: a partitioned task carried out in a decentralized insect
society. 相似文献