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91.
The objectives of the present work were to study isotope ratios and the inventory of plutonium and uranium isotope compositions in sediments from Lake Obuchi, which is in the vicinity of several nuclear fuel facilities in Rokkasho, Japan. Pu and its isotopes were determined using sector-field ICP-MS and U and its isotopes were determined with ICP-QMS after separation and purification with a combination of ion-exchange and extraction chromatography. The observed (240)Pu/(239)Pu atom ratio (0.186 +/- 0.016) was similar to that of global fallout, indicating that the possible early tropospheric fallout Pu did not deliver Pu from the Pacific Proving Ground to areas above 40 degrees N. The previously reported higher Pu inventory in the deep water area of Lake Obuchi could be attributed to the lateral transportation of Pu deposited in the shallow area which resulted from the migration of deposited global fallout Pu from the land into the lake by river runoff and from the Pacific Ocean by tide movement and sea water scavenging, as well as from direct soil input by winds. The (235)U/(238)U atom ratios ranged from 0.00723 to 0.00732, indicating the natural origin of U in the sediments. The average (234)U/(238)U activity ratio of 1.11 in a sediment core indicated a significant sea water U contribution. No evidence was found for the release of U containing wastes from the nearby nuclear facilities. These results will serve as a reference baseline on the levels of Pu and U in the studied site so that any further contamination from the spent nuclear fuel reprocessing plants, the radioactive waste disposal and storage facilities, and the uranium enrichment plant can be identified, and the impact of future release can be rapidly assessed. 相似文献
92.
93.
Snappers (Lutjanidae) are one of the important fisheries resources in tropical and subtropical waters. However, there have
been few studies clarifying the ecology of newly settled juvenile snappers. The aims of the present study were to clarify
the seasonality and lunar periodicity of the larval settlement, and the microhabitat association of newly settled juveniles
for Lutjanus gibbus in an Okinawan coral reef. Fifteen coral patches were chosen and underwater visual surveys were conducted during a 2-year
period. The larval settlement of the species mainly occurred between May and October during the 2-year survey period. In terms
of lunar periodicity of the settlement, the newly settled juveniles were mainly found between the last quarter moon and new
moon during the main settlement season. Back calculations of settlement dates based on otolith microstructure showed that
most juveniles settled during the last quarter moon and new moon. Stepwise multiple regression analyses revealed that the
newly settled juveniles were mainly found on coral patches with a large number of holes on the top of the coral patch and
this tendency was mainly consistent during the study period. The volume of holes at the base of coral patches had also a positive
effect on the abundance of newly settled juveniles in some cases. The results of the present study suggest that larval settlement
has a strong seasonal and lunar periodicity, and newly settled juveniles select coral patches with available refuge spaces. 相似文献
94.
Morihiro Osada Ken Takamiya Kazutaka Manako Masato Noguchi Shin-ichi Sakai 《Journal of Material Cycles and Waste Management》2013,15(1):25-36
The service life of many buildings and houses built using asbestos-containing materials is coming to an end and their demolition will lead to a great deal of asbestos-containing waste (ACW). Conventionally, the disposal of such waste is conducted by isolation under controlled landfill procedures; however problems with this method exist, such as the risk at the time of re-utilization of landfill sites and the depletion of lands to be reclaimed. Melting treatment is a promising technology that could be used to solve these problems; a thermal process involving temperatures exceeding the melting points of asbestos, it transforms them into non-hazardous minerals. This technology may be applicable not only for friable ACW but also for nonfriable ACW. We performed a demonstration test of melting treatment of nonfriable ACW using a gasification and melting furnace of the shaft furnace type, which is a typical method for high temperature melting. Detailed observation using transmission electron microscopy as well as general analyses verified that the same level of asbestos remained in the slag obtained by high temperature melting as that of the background soil. In addition, the asbestos concentration in the exhaust gas and the dust from the facility were at sufficiently low levels, and it was thus verified that the asbestos concentration in the atmosphere in the vicinity of the facility during the melting treatment was comparable to that of Japan’s background level reported by the Ministry of the Environment in 2007. 相似文献
95.
Sonoko D. Kimura Yo Toma Zhijian Mu Hiroyuki Yamada Ryusuke Hatano 《Sustainability Science》2010,5(1):19-27
Relationships among global warming potential (GWP), farmland surplus nitrogen (FSN) and income for major land uses in the
Ikushunbetsu watershed were compared using the eco-balance method. An empirical model was created for carbon dioxide, methane
and nitrous oxide for both uplands and paddy rice using monitoring data from 22 fields. The greenhouse gas emissions were
converted into GWP, whereas yield and FSN were obtained from interviews with farmers and a literature survey. Land use distribution
was obtained by ground surveys in 2002, 2005 and 2007. The analysis showed that paddy rice and soybeans were characterized
by a high GWP, low FSN and high income, whereas onions and vegetables had a high FSN but low GWP and moderate income. Wheat
showed a negative GWP in some years, and abandoned areas always exhibited negative values. The total GWPs for the region were
14,184, 11,085 and 8,337 Mg CO2 year−1 for 2002, 2005 and 2007, respectively. The contribution of paddy rice to GWP was highest, ranging from 40 to 75%. To find
optimal land use combinations that provide higher incomes and lower GWPs and FSNs than at present, all possible land use combinations
were analyzed by changing the land use proportion from 0 to 100% at an interval of 10%. The number of land use combinations
meeting the requirements in the three investigated years was 205. Abandoned area, which had the smallest environmental load,
was included in every land use combination, indicating that land uses with low environmental impacts should be maintained
at a certain proportion to mitigate the environmental load accompanying land uses with high production. 相似文献
96.
Nakanishi T Zheng J Aono T Yamada M Kusakabe M 《Journal of environmental radioactivity》2011,102(8):774-779
Using a sector-field ICP-MS the vertical distributions of the 99Tc concentration and 99Tc/137Cs activity ratio were measured in the coastal waters off Aomori Prefecture, Japan, where a spent-nuclear-fuel reprocessing plant has begun test operation. The 99Tc concentrations in surface water ranged from 1.8 to 2.4 mBq/m3, no greater than the estimated background level. Relatively high 99Tc/137Cs activity ratios (10-12 × 10−4) would be caused by the inflow of the high-99Tc/137Cs water mass from the Japan Sea. There is no observable contamination from the reprocessing plant in the investigated area. The 99Tc concentration and the 99Tc/137Cs activity ratio in water column showed gradual decreases with depth. Our results implied that 99Tc behaves in a more conservative manner than 137Cs in marine environments. 相似文献
97.
Photodegradation of hexachlorobenzene and theoretical prediction of its degradation pathways using quantum chemical calculation 总被引:2,自引:0,他引:2
Experimentally determined photodegradation pathways of hexachlorobenzene (HCB), a chlorinated aromatic compound, in hexane, 2-propanol (IPA), and methanol were compared with those predicted by quantum chemical calculation based on density functional theory (DFT), and the adequacy of the prediction method was evaluated. The experimental main degradation pathways of HCB were virtually the same for the three solvents and also agreed with the predicted main degradation pathways. In the DFT method, the main degradation product was the dechlorinated benzene at the position where the C-Cl bond was predicted to have the lowest bond dissociation energy. This result suggested that the photodechlorination pathways of chlorinated aromatic compounds could be predicted by comparing the bond dissociation energies calculated with the DFT method. 相似文献
98.
Atsumi Miyake Arata Kimura Nobuyoshi Yamada 《Journal of Material Cycles and Waste Management》2008,10(2):124-128
An accidental explosion occurred in a waste storage tank at an incineration plant in Kawasaki, Japan, on May 11, 1997. The
accident was caused primarily by unintended mixing involving reactive chemicals, such as organic peroxides (POs) and acrylonitrile
(AN). The PO initiated polymerization of AN and the heat released during the polymerization led to a runaway reaction and
explosion. POs are widely used in the chemical industry and can be self-reactive and hazardous when mixed with other chemicals
such as acids and alkalis. The goal of this study was to obtain a better understanding of the mixing hazard of chemicals through
an evaluation of POs with other chemicals using conventional experimental techniques such as glass test-tube tests, Dewar
vessel tests, and differential scanning calorimetry (DSC). Seven types of POs were mixed with AN. Test results were classified
into four ranks based on the hazard criteria. In addition, di(2-ethylhexyl)-peroxydicarbonate/AN mixtures were investigated
in detail and the influences of the mixing ratio and the stirring rate were examined. 相似文献
99.
Using the number of segments of pleopod rami as a marker of instar number, the population structure (instar composition)
of the mesopelagic gammarid amphipod Cyphocaris challengeri was investigated by monthly samplings from May 1997 to April 1999 at a station off southwest Hokkaido, Japan. Laboratory-rearing
experiments were also conducted to establish the relationship between the number of segments of pleopod rami and instar number,
and to estimate the growth pattern of this gammarid based on the intermolt period and molt-increment data. Stratified sampling
in the field (0 to 200 and 200 to 400 m depth strata) showed this species occurred mainly at 200 to 400 m depth during the
day. Instar analysis indicated that C. challengeri has 12 instars in females and 11 instars in males. Based on observations of secondary sexual characters, Instars 1 to 6 were
designated juveniles (Instars 1 to 3 occurred in the marsupia of gravid females); in males, 7 to 9 were immature and 10 and
11 were mature, while in females 7 and 8 were immature and 9 to 12 were mature. Off southwest Hokkaido, Instar 4 (just released
from a female's marsupium) was found throughout the year, with a peak abundance occurring in April to July of each year. A
sequential development of Instar 4 to 9 (youngest adult instar) through the year was observed. Generation length (i.e. the
time required to grow from Instar 4 to 10) was estimated from a laboratory-obtained growth curve to be 216 to 584 d at the
in situ temperature range (2 to 5 °C), which is consistent with observations on field populations. Specimens older than Instar
9 were rare in the field and could not be used in laboratory-rearing experiments, so longevity could not be estimated. Eggs
were oval and measured 0.6 mm (large diameter). Brood size ranged from 20 to 65. Comparing the present results with those
of epipelagic hyperiid amphipods, the nearly identical growth rates together with the production of fewer but larger eggs
seen in C. challengeri appear to reflect to the typical life mode of deep-living pelagic crustaceans.
Received: 14 February 2000 / Accepted: 6 July 2000 相似文献
100.
Masaki Takaoka Nobuo Takeda Takeshi Fujiwara Masato Kurata Tetsuo Kimura 《Journal of the Air & Waste Management Association (1995)》2013,63(8):931-940
Abstract The control of Hg emissions from a municipal solid waste incinerator (MSWI) is very important, because more than 78% of municipal solid waste (MSW) is incinerated. The Hg content of coal used in utility boilers is relatively low in Japan. In this study, recent trends in the Hg content of MSW in Japan and activated carbon (AC) injection as a control technology of Hg emission from an MSWI are discussed. The effect of AC injection on Hg removal from flue gas in an MSWI was investigated by pilot-scale experiments using a bag filter (BF). The injection of AC increases the Hg reduction ratio by 20–30% compared with cases without AC injection. The Hg reduction ratio increases as the flue gas temperature decreases. The Hg reduction ratio is closely related to the inlet Hg concentration and was expressed with a Langmuir-type adsorption isotherm. 相似文献