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691.
Inputs and distributions of synthetic musk fragrances in an estuarine and coastal environment; a case study 总被引:1,自引:0,他引:1
Nicola R. Sumner Carlos Guitart Gustavo Fuentes 《Environmental pollution (Barking, Essex : 1987)》2010,158(1):215-4648
Synthetic musks are ubiquitous contaminants in the environment. Compartmental distributions (dissolved, suspended particle associated and sedimentary) of the compounds throughout an axial estuarine transect and in coastal waters are reported. High concentrations of Galaxolide® (HHCB) and Tonalide® (AHTN) (987-2098 ng/L and 55-159 ng/L, respectively) were encountered in final effluent samples from sewage treatment plants (STPs) discharging into the Tamar and Plym Estuaries (UK), with lower concentrations of Celestolide® (ADBI) (4-13 ng/L), Phantolide® (AHMI) (6-9 ng/L), musk xylene (MX) (4-7 ng/L) and musk ketone (MK) (18-30 ng/L). Rapid dilution from the outfalls is demonstrated with resulting concentrations of HHCB spanning from 5 to 30 ng/L and those for AHTN from 3 to 15 ng/L. The other musks were generally not detected in the estuarine and coastal waters. The suspended particulate matter (SPM) and sedimentary profiles and compositions (HHCB:AHTN ratios) generally reflect the distribution in the water column with highest concentrations adjacent to sewage outfalls. 相似文献
692.
O.R.J. Anderson R.A. Phillips R.A.R. McGill S. Bearhop 《Environmental pollution (Barking, Essex : 1987)》2010,158(1):98-107
We investigated the concentrations of 22 essential and non-essential elements among a community of Procellariiformes (and their prey) to identify the extent to which trophic position and foraging range governed element accumulation. Stable isotope analysis (SIA) was used to characterise trophic (δ15N) and spatial patterns (δ13C) among species. Few consistent patterns were observed in element distributions among species and diet appeared to be highly influential in some instances. Arsenic levels in seabird red blood cells correlated with δ15N and δ13C, demonstrating the importance of trophic position and foraging range for arsenic distribution. Arsenic concentrations in prey varied significantly across taxa, and in the strength of association with δ15N values (trophic level). In most instances, element patterns in Procellariiformes showed the clearest separation among species, indicating that a combination of prey selection and other complex species-specific characteristics (e.g. moult patterns) were generally more important determining factors than trophic level per se. 相似文献
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Fredrik Wulff Christoph Humborg Hans Estrup Andersen Gitte Blicher-Mathiesen Mikołaj Czajkowski Katarina Elofsson Anders Fonnesbech-Wulff Berit Hasler Bongghi Hong Viesturs Jansons Carl-Magnus Mörth James C. R. Smart Erik Smedberg Per Stålnacke Dennis P. Swaney Hans Thodsen Adam Was Tomasz Żylicz 《Ambio》2014,43(1):11-25
The Baltic Sea Action Plan (BSAP) requires tools to simulate effects and costs of various nutrient abatement strategies. Hierarchically connected databases and models of the entire catchment have been created to allow decision makers to view scenarios via the decision support system NEST. Increased intensity in agriculture in transient countries would result in increased nutrient loads to the Baltic Sea, particularly from Poland, the Baltic States, and Russia. Nutrient retentions are high, which means that the nutrient reduction goals of 135 000 tons N and 15 000 tons P, as formulated in the BSAP from 2007, correspond to a reduction in nutrient loadings to watersheds by 675 000 tons N and 158 000 tons P. A cost-minimization model was used to allocate nutrient reductions to measures and countries where the costs for reducing loads are low. The minimum annual cost to meet BSAP basin targets is estimated to 4.7 billion €. 相似文献
695.
M. Amodio P. R. Dambruoso Gianluigi de Gennaro L. de Gennaro A. Demarinis Loiotile A. Marzocca F. Stasi L. Trizio M. Tutino 《Environmental science and pollution research international》2014,21(23):13186-13195
In order to assess indoor air quality (IAQ), two 1-week monitoring campaigns of volatile organic compounds (VOC) were performed in different areas of a multistorey shopping mall. High-spatial-resolution monitoring was conducted at 32 indoor sites located in two storehouses and in different departments of a supermarket. At the same time, VOC concentrations were monitored in the mall and parking lot area as well as outdoors. VOC were sampled at 48-h periods using diffusive samplers suitable for thermal desorption. The samples were then analyzed with gas chromatography–mass spectrometry (GC–MS). The data analysis and chromatic maps indicated that the two storehouses had the highest VOC concentrations consisting principally of terpenes. These higher TVOC concentrations could be a result of the low efficiency of the air exchange and intake systems, as well as the large quantity of articles stored in these small spaces. Instead, inside the supermarket, the food department was the most critical area for VOC concentrations. To identify potential emission sources in this department, a continuous VOC analyzer was used. The findings indicated that the highest total VOC concentrations were present during cleaning activities and that these activities were carried out frequently in the food department. The study highlights the importance of conducting both high-spatial-resolution monitoring and high-temporal-resolution monitoring. The former was able to identify critical issues in environments with a complex emission scenario while the latter was useful in interpreting the dynamics of each emission source. 相似文献
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Carolyn K. Huynh Signe R. Poquette W. Lindsay Whitlow 《Environmental science and pollution research international》2014,21(7):5211-5216
The present study sought to evaluate the behavioral responses of non-target organisms in order to determine whether phototactic responses of isopods to danger cues are altered as a function of exposure to the pyrethroid pesticides λ-cyhalothrin and bifenthrin. Experiments conducted on Gnorimosphaeroma oregonensis identified sublethal behavioral responses to pyrethroids, λ-cyhalothrin and bifenthrin at concentrations 0.15 ng/mL, 0.025 ng/mL, and 0.005 ng/mL. Experimental setup tested isopod phototactic responses across six treatments: control, pyrethroid, hemolymph, predator, hemolymph?+?pyrethroid, and predator?+?pyrethroid. Isopods exhibited no preference for phototactic responses in the control and pyrethroid treatments. When exposed to danger cues (hemolymph or predator), isopods exhibited significant negative phototaxis, as expected. When exposure to danger cues was combined with pyrethroids, isopods again exhibited no preference for phototactic response. Experiments indicate that pyrethroids diminish isopod’s negatively phototactic response to danger cues. 相似文献
700.
Major ionic compositions of fine particulate matter in an animal feeding operation facility and its vicinity 总被引:1,自引:0,他引:1
Qian-Feng Li Zifei Liu R.K.M. Jayanty Sanjay B. Shah Peter Bloomfield 《Journal of the Air & Waste Management Association (1995)》2014,64(11):1279-1287
Animal feeding operations (AFOs) produce particulate matter (PM) and gaseous pollutants. Investigation of the chemical composition of PM2.5 inside and in the local vicinity of AFOs can help to understand the impact of the AFO emissions on ambient secondary PM formation. This study was conducted on a commercial egg production farm in North Carolina. Samples of PM2.5 were collected from five stations, with one located in an egg production house and the other four located in the vicinity of the farm along four wind directions. The major ions of NH4+, Na+, K+, SO42?, Cl?, and NO3? were analyzed using ion chromatography (IC). In the house, the mostly abundant ions were SO42?, Cl?, and K+. At ambient stations, SO42?, and NH4+ were the two most abundant ions. In the house, NH4+, SO42?, and NO3? accounted for only 10% of the PM2.5 mass; at ambient locations, NH4+, SO42?, and NO3? accounted for 36–41% of the PM2.5 mass. In the house, NH4+ had small seasonal variations indicating that gas-phase NH3 was not the only major force driving its gas–particle partitioning. At the ambient stations, NH4+ had the highest concentrations in summer. In the house, K+, Na+, and Cl? were highly correlated with each other. In ambient locations, SO42? and NH4+ had a strong correlation, whereas in the house, SO42? and NH4+ had a very weak correlation. Ambient temperature and solar radiation were positively correlated with NH4+ and SO42?. This study suggests that secondary PM formation inside the animal house was not an important source of PM2.5. In the vicinity, NH3 emissions had greater impact on PM2.5 formation.
ImplicationsThe chemical composition of PM2.5 inside and in the local vicinity of AFOs showed the impact of the AFO emissions on ambient secondary PM2.5 formation, and the fate and transport of air pollutants associated with AFOs. The results may help to manage in-house animal facility air quality, and to develop regional air quality control strategies and policies, especially in animal agriculture-concentrated areas. 相似文献