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51.
After the prohibition of organochlorine-pesticide use in Brazil for controlling insect vector diseases, Mato Grosso State gathered the exceeding DDT and stored it irregularly in an open air area that belongs to the National Health Foundation, causing soil contamination. This study aimed to evaluate the contamination level and dissipation of p,p'-DDT and p,p'-DDE in this area. For that, surface soil samples were collected on 19 September 2000, 15 December 2000, 4 April 2001 and soil samples 30-40 cm; 60-70 cm and 90-100 cm deep were taken from five points in the studied area on 17 July 2001. The contaminants were determined by a small scale method which consists on extraction and clean-up steps combined into one step by transferring soil samples mixed with neutral alumina to a chromatographic column prepacked with neutral alumina and elution with hexane:dichloromethane (7:3 v:v). The eluate was concentrated and the analytes were quantified by gas chromatography with an electron-capture detector. p,p'-DDT at surface soil ranged from 3,800 to 7,300 mg kg(-1). 30-40 cm deep soil sample concentrations varied from 0.036 to 440 mg kg(-1) while 90-100 cm deep samples varied from 0.069 to 180 mg kg(-1). Volatilization is probably the main dissipation process. The p,p'-DDT is moving slowly downward in the soil profile, however, the levels of this contaminant are high enough to present risk to underground waters. 相似文献
52.
Araújo CV Cohin-de-Pinho SJ da S Santos J Delgado F Santana LC Chastinet CB da Silva EM 《Chemosphere》2006,65(4):599-603
The suitability and viability of acute in situ bioassays were investigated in the biomonitoring program of an acidic lake contaminated with sulphur residues. Responses of organisms observed in laboratory and in situ bioassays were also assessed to determine whether or not they were similar and comparable, regarding accuracy and precision. Newborn Poecilia reticulata were employed as test organisms and exposed to the same water samples under in situ and laboratory conditions. Mortality/immobility was the endpoint assessed and dead/immobile organisms were counted at various time intervals during exposure. The mean calculated LT50 values and 95% confidence intervals were 1.61 (1.36-1.87) h in the laboratory bioassays and 0.72 (0.55-0.89) h in the in situ bioassays. Statistical comparison of these values revealed a significant difference (p<0.05). In situ bioassays were more accurate than those carried out in the laboratory, demonstrating higher sensitivity and better reproduction of what occurs in nature, while laboratory bioassays were more precise. 相似文献
53.
Comprehensive understanding of (222)Rn exhalation from phosphogypsum-bearing building material and its accumulation in indoor air is likely to rely on numerical simulation, particularly if transient effects, three-dimensional domains and convection are to be included and investigated. Yet, experimental data and analytical results are helpful (if not crucial) as far as validation is concerned. Having in mind computational code simplicity and in the light of a recent experimental and theoretical report on (222)Rn release from phosphogypsum boards for housing panels, this paper presents and discusses an alternative testing set-up and the corresponding boundary conditions, namely one side of the panel bounded by impermeable wall. Although this is a new facility to be tested, the resultant steady-state one-dimensional diffusion-dominant analytical solution is shown to match the counterpart deduced in the aforementioned previous report, despite it relaxes the constraint of symmetry about the phosphogypsum board centerline, which is inferred in that prior experimental scenario. In addition, numerical results are conducted for a diffusion-dominant two-dimensional time-varying test case concerning (222)Rn accumulation in a closed chamber having an exhaling phosphogypsum board tightly placed at one wall. 相似文献
54.
234U and 230Th determination by FIA-ICP-MS and application to uranium-series disequilibrium in marine samples 总被引:1,自引:0,他引:1
Godoy ML Godoy JM Kowsmann R Dos Santos GM Petinatti da Cruz R 《Journal of environmental radioactivity》2006,88(2):109-117
A 234U and 230Th determination method based on an extraction chromatographic separation on a flow injection system coupled to a quadruple ICP-MS was developed. Two-milliliter UTEVA (Eichrom Co.) cartridges were applied as separation tool and 236U and 229Th as spikes. Loading and washing steps were carried out in 3 M HNO3 solution and 0.05 M ammonium oxalate applied to elute both uranium and thorium. The method was applied initially to the IAEA-327 soil reference sample and NIST SRM 4357 ocean sediment reference material, with the obtained 234U and 230Th concentrations in agreement with the reference levels. Samples from a deep-sea sediment core (2450 m water depth) were analyzed and based on 230Th/234U dating, a mean sedimentation rate of 3.3 cm ky(-1) was calculated. Samples from two sediment layers were also dated by 14C-AMS and the observed ages agree with the 230Th/234U results. 相似文献
55.
Gabriel N. de O. Teixeira Arthur M. S. da Cruz Gisella R. L. Samanamud Alexandre B. França Luzia L. R. Naves Diego Melo 《Journal of environmental science and health. Part. B》2020,55(1):19-29
AbstractThe main objective of this study is the degradation of a synthetic solution of atrazine by a modified vermiculite catalyzed ozonation, in a rotating packed bed (RPB) reactor. A 0.5?L RPB reactor was used to perform the experiments, using a Central Composite Design (CCD) response surface to construct the quadratic model based on the factors: pH, catalyst concentration and reactor rotation frequency. The response variable was the removal of the organic load measured in terms of Chemical Oxygen Demand (COD). After the complete quadratic model was constructed through the response surface, the COD degradation process had an optimal removal of 41% under the following conditions: pH 8.0, rotation of 1150?rpm and catalyst concentration 0.66?g L?1. 相似文献
56.
Biodegradation of anthracene and different PAHs by a yellow laccase from Leucoagaricus gongylophorus
Ike Priscila Tomie Leme Birolli Willian Garcia dos Santos Danilo Martins Porto André Luiz Meleiro Souza Dulce Helena Ferreira 《Environmental science and pollution research international》2019,26(9):8675-8684
Environmental Science and Pollution Research - Laccases produced by Leucoagaricus gongylophorus act in lignocellulose degradation and detoxification processes. Therefore, the use of L.... 相似文献
57.
Hani R. El Bizri Thaís Q. Morcatty João Valsecchi Pedro Mayor Jéssica E. S. Ribeiro Carlos F. A. Vasconcelos Neto Jéssica S. Oliveira Keilla M. Furtado Urânia C. Ferreira Carlos F. S. Miranda Ciclene H. Silva Valdinei L. Lopes Gerson P. Lopes Caio C. F. Florindo Romerson C. Chagas Vincent Nijman Julia E. Fa 《Conservation biology》2020,34(2):438-448
The switch from hunting wild meat for home consumption to supplying more lucrative city markets in Amazonia can adversely affect some game species. Despite this, information on the amounts of wild meat eaten in Amazonian cities is still limited. We estimated wild meat consumption rates in 5 cities in the State of Amazonas in Brazil through 1046 door-to-door household interviews conducted from 2004 to 2012. With these data, we modeled the relationship between wild meat use and a selection of socioeconomic indices. We then scaled up our model to determine the amounts of wild meat likely to be consumed annually in the 62 urban centers in central Amazonia. A total of 80.3% of all interviewees reported consuming wild meat during an average of 29.3 (CI 11.6) days per year. Most wild meat was reported as bought in local markets (80.1%) or hunted by a family member (14.9%). Twenty-one taxa were cited as consumed, mostly mammals (71.6%), followed by reptiles (23.2%) and then birds (5.2%). The declared frequency of wild meat consumption was positively correlated with the proportion of rural population as well as with the per capita gross domestic product of the municipality (administrative divisions) where the cities were seated. We estimated that as much as 10,691 t of wild meat might be consumed annually in the 62 urban centers within central Amazonia, the equivalent of 6.49 kg per person per year. In monetary terms, this amounts to US$21.72 per person per year or US$35.1 million overall, the latter figure is comparable to fish and timber production in the region. Given this magnitude of wild meat trade in central Amazonia, it is fundamental to integrate this activity into the formal economy and actively develop policies that allow the trade of more resilient taxa and restrict trade in species sensitive to hunting. 相似文献
58.
59.
Verônica da Fonsêca-Genevois Paul J. Somerfield Maria Helena Baeta Neves Ricardo Coutinho Tom Moens 《Marine Biology》2006,148(5):1039-1050
An experiment was undertaken at Farol Island, Brazil, to examine colonization of bare aluminium surfaces by microbes and meiofauna.
It was hypothesized that a primary source of meiofaunal colonists was sediment resuspended during upwelling events, two of
which occurred during the experiment. Microbial biofilms formed on the experimental substrata within 1 day, and continued
to develop throughout the experimental period. Among meiofaunal groups copepods also appeared on the first day, and nematodes
on the second. Meiofaunal community structure developed in three main phases: an initial phase of 2 days, characterized by
low abundances of copepods; a second phase during the first upwelling period characterized by higher abundances of copepods
and also by turbellarians; and a third phase from day 13 onwards characterized by relatively stable abundances of a range
of taxa including copepods, cirripedes, nematodes and ostracods. Nematode assemblages also developed in three phases, but
with different timings coinciding with upwelling events: an initial phase, from the beginning of the experiment to day 9,
characterized by few species and low (or no) abundances; a second phase following the first upwelling characterized by moderate
abundances of Chromadorina, Chromadorella, Daptonema and Euchromadora sp. 3; a third phase following the second upwelling period (from day 26 onwards) in which Daptonema disappeared and the assemblage was characterized by moderate to high abundances of Euchromadora (species 1 and 2) and Chromadorella. Although shifts in nematode assemblage structure coincided with upwelling events no evidence was found for sediments being
the primary source of colonizers on the aluminium substrata, in contrast to our hypothesis. 相似文献
60.