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Distribution,sources, and ecological risk assessment of SVOCs in surface sediments from Guan River Estuary,China 总被引:1,自引:0,他引:1
Xinran He Xiaojuan Song Yong Pang Yiping Li Binlin Chen Zhihua Feng 《Environmental monitoring and assessment》2014,186(7):4001-4012
The contamination of semi-volatile organic compounds (SVOCs) in the surface sediments of the Guan River Estuary, China was fully investigated. Total concentrations of 56 species of SVOCs ranged from 132 to 274 ng/g with an average of 186 ng/g (dry weight). Polycyclic aromatic hydrocarbon (PAH) concentrations were positively correlated with clay content and negatively correlated with sediment grain size. Source identification indicated that PAHs originated mainly from pyrolytic sources. However, intense ship traffic in the estuary may provide sources of petrogenic PAHs. Organochlorine pesticides (OCPs) mainly originated from direct input of dichlorodiphenyltrichloroethanes (DDTs) during some industrial processes. The SVOC concentrations were also compared with International Sediments Quality Guidelines and Sediments Quality Criteria, and the results indicated that negative biological impacts may originate from high concentrations of FLO, p,p′-DDE, and total DDTs. 相似文献
225.
Molecular detection of three gastroenteritis viruses in urban surface waters in Beijing and correlation with levels of fecal indicator bacteria 总被引:1,自引:0,他引:1
To assess the presence of three gastroenteritis viruses responsible for human acute gastroenteritis in surface water, a 1-year study was carried out in the city of Beijing, China. A total of 108 urban surface water samples were collected from nine collection sites which were defined with a global positioning system in rivers or lakes from September 2006 to August 2007. The water samples were subjected to virus concentration using an HA electronegative filter, followed by polymerase chain reaction (PCR) for rotavirus (RV) astrovirus (AV), and norovirus (NV). It showed that the number of viruses detected in water samples from different sites was variable, totaling 63 virus strains, with rotavirus (48.1%) verified as the most prevalent detected, followed by astrovirus (AV, 5.6%), and norovirus (NV, 4.6%). RV was also quantified by real-time PCR and the concentration of RV ranged from 0 to 18.27 genome copies·L(-1). And the distributions of RV in surface water were abundant in cold weather (from September to February) while less prevailing in warm weather (from March to August). The high detection rate of RV we encountered in this study provided convincing evidence that RV circulated at a certain frequency in the Beijing population. There was no statistically significant correlation between RV levels and both fecal coliform (R (2)?=?0.02) and Enterococcus faecalis (R (2)?=?0.02) densities. Our study suggests prolonged virus persistence in aquatic environments and emphasizes the enteric virus group as the most reliable for environmental monitoring. 相似文献
226.
Metal contents (Al, Ca, Cd, Cr, Cu, Fe, Hg, Mg, Mn, Ni, Pb, Ti, and Zn) have been measured in 30 surface soils on Fildes Peninsula, King George Island, Antarctica, yielding values (in milligrams kilogram(-1)) of 41.57-80.65 (Zn), 2.76-60.52 (Pb), 0.04-0.34 (Cd), 7.18-25.03 (Ni), 43,255-70,534 (Fe), 449-1,401 (Mn), 17.10-64.90 (Cr), 1,440-25,684 (Mg), 10,941-49,354 (Ca), 51.10-176.50 (Cu), 4,388-12,707 (Ti), 28,038-83,849 (Al), and for Hg (in nanograms gram(-1)) 0.01-0.06. Relative cumulative frequency analysis was used to determine the baseline values for the 13 metals. Compared with adjacent areas in Antarctica, Mg and Ni are significantly lower, but Cu is significantly higher than that of McMurdo Station. Enrichment factor analysis and the geo-accumulation index method were applied in order to determine the extent of anthropogenic contamination, and both show that Pb, Cd, and Hg have been significantly increased by human activities. Principal component analysis was used to identify the sources of metals in these soil samples. 相似文献
227.
液相色谱-质谱法测定土壤中四溴双酚A和六溴环十二烷 总被引:1,自引:1,他引:0
文章建立了液相色谱-串联四级杆质谱仪同时测定土壤中四溴双酚A及3种六溴环十二烷同分异构体的分析方法。土壤样品经快速溶剂仪萃取,全自动凝胶净化系统净化后,使用液相色谱-串联四级杆质谱仪,负离子电喷雾多反应监测模式监测,内标法定量分析。结果表明,土壤中四溴双酚A、α-六溴环十二烷、β-六溴环十二烷和γ-六溴环十二烷的检出限为0.1~1.2 pg/g,加标回收率为81.8%~113%,相对标准偏差小于10%。该方法分析时间短,灵敏度高,操作简单,对电子固废拆解场地中的179个土壤样品进行分析,取得满意结果。 相似文献
228.
Sónia R. Q. Serra Ana Raquel Calapez Amaia Pérez-Bilbao Maria João Feio 《Environmental monitoring and assessment》2015,187(1):1-13
Bioassessment tools should distinguish between the effects of anthropogenic degradation in communities and natural temporal changes. The present study tests the influence of natural seasonal variability on macroinvertebrate stream communities assessed by a predictive model (PORTRIV) and a multimetric index (IPtI) calibrated for spring. The scores of PORTRIV decreased significantly between spring and autumn, and between spring and winter (ca. 37 to 53 %, respectively), while those of IPtI did not change significantly between seasons. For non-reference samples, the results of the predictive model also indicate no significant differences. A correction factor (CF) was calculated to adjust the existing differences in the model assessments between seasons, based on the percentage of variation of reference site scores from spring to autumn and winter. After the application of the CF to the OE50 scores of spring reference samples, the differences were no longer significant. Independent reference validation sites confirmed this tendency. This method has the advantage of avoiding large efforts required for the construction of databases from other seasons and the development of new models to allow the assessment of streams in seasons other than spring. Further tests with models developed in regions with more marked seasonal changes should be done to confirm its wider applicability. 相似文献
229.
As facile “environmental media”, the outdoor dust may reflect the changes of contaminants in environment more promptly. In
the present study, selected organochlorine contaminants (OCs) include hexachlorocyclohexanes (HCHs), dichlorodiphenyltrichloroethanes
(DDTs), hexachlorobenzene (HCB), and pentachlorobenzene (PeCB) were detected in 20 outdoor dust samples collected from Xinxiang
City. The concentrations of ΣHCHs, ΣDDTs, HCB, and PeCB in dust were in the range of 0.18–5.05 ng/g dry weight, 0.44–13.50 ng/g
dry weight, 0.13–51.61 ng/g dry weight and ND-0.74 ng/g dry weight, respectively. Long-range transport, historical use, and
recent impact of impure pesticides might be the main sources of OCs in the outdoor dust. The results of this study indicated
that impure pesticide application maybe an important source of DDTs and HCB in the environment. 相似文献
230.
The chemical forms and ecological risk of As were characterized in the sediment of the Daliao River System (DRS), which has
been affected by long-term intensive industrial, urban, and agricultural activities. Twenty-seven samples of surface sediment
were collected and analyzed for total As content and that of its chemical forms. The results indicated that the average total
As content in the sediment was 9.83 mg kg − 1 but that the levels ranged from 1.57 to 83.09 mg kg − 1. At the sites near cities, mining sites, and the estuary of the DRS, it is likely that adverse effects on aquatic organisms
occur, due to As levels in the sediment that are often higher than the threshold effect level and occasionally higher than
the probable effect level. A selectively sequential extraction indicated that the majority of As in the sediment was bound
to Fe oxides (62.1%), with moderate proportions of residual As (19.8%), specifically adsorbed As (17.9%), and a low proportion
of non-specifically adsorbed As (1.1%). In addition, the content of Fe in the sediment was positively and significantly correlated
with the contents of amorphous and crystalline Fe oxide-bound As, confirming the crucial role of Fe oxides in immobilizing
high amounts of As in superficial environments. The average molar ratio of As to Fe was 1.18 × 10 − 4 in the surface sediment of the DRS, similar to that of natural Fe oxides, but much lower than that of synthesized Schwertmannite.
Therefore, the release of As under reduced and low pH conditions can cause serious problems for water resources and for living
organisms. 相似文献