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11.
Stloukal P Verney V Commereuc S Rychly J Matisova-Rychlá L Pis V Koutny M 《Chemosphere》2012,88(10):1214-1219
Three commercially available biodegradable polymers, two different aromatic-aliphatic copolyesters and polylactic acid, intended for the fabrication of agricultural mulching films, in addition to other applications, were subjected to a series of tests with the aim of studying the relationship between their photooxidation and biodegradation. Photooxidation resulted in the rearrangement of polymeric chains, in the case of both copolyesters the events led to polymeric chain crosslinking and the formation of insoluble polymeric gel. The tendency was significantly more pronounced for the copolyester with the higher content of the aromatic constituent. As regards polylactic acid photochemical reactions were not accompanied by crosslinking but instead provoked chain scissions. A biodegradation experiment showed that, despite marked structural changes, the extent of photooxidation was not the decisive factor, which significantly modified the rate of biodegradation in all three materials investigated. The specific surface area of the sample specimens was shown to be more important. 相似文献
12.
Ungtae Kim Jagath J. Kaluarachchi Vladimir U. Smakhtin 《Journal of the American Water Resources Association》2008,44(5):1231-1247
Abstract: This work develops a methodology to project the future precipitation in large river basins under limited data and climate change while preserving the historical temporal and spatial characteristics. The computationally simple and reliable conditional generation method (CGM) is presented and applied to generate reliable monthly precipitation data in the upper Blue Nile River Basin of Ethiopia where rain‐fed agriculture is prevalent. The results showed that the temporal analysis with the CGM performs better to reproduce the historical long‐term characteristics than other methods, and the spatial analysis with the CGM reproduced the historical spatial structure accurately. A 100‐year time series analysis using the outcomes of the six general circulation models showed that precipitation changes by the 2050s (2040 through 2069) can be ?7 to 28% with a mean increase of about 11%. The seasonal results showed increasing wet conditions in all seasons with changes of mean precipitation of 5, 47, and 6% for wet, dry, and mild seasons, respectively. 相似文献
13.
Luka Traven Vladimir Mićović Darija Vukić Lušić Tvrtko Smital 《Environmental monitoring and assessment》2013,185(11):9009-9018
The present study investigates the response of three hepatic biomarkers in adult sea bass (Dicentrarchus labrax, Linnaeus 1758) caged at a wastewater outlet of an oil refinery with fish caged at a pristine site used as controls. The biomarkers that were investigated were the hepatosomatic index (HSI), 7-ethoxyresorufin-O-deethylase (EROD) activity and glutathione-S-transferase (GST) activity. In addition, we have measured the levels of polycyclic aromatic hydrocarbons (PAHs) and selected heavy metals (lead, cadmium, mercury, copper and zinc) in sediment samples at the polluted site. Although the polluted site had high environmental levels of PAHs and heavy metals, there was no difference in hepatic EROD activity and HSI between fish caged at the polluted site and controls. On the other hand, GST activity was significantly lower in fish caged at the polluted site compared to controls. Our results point out that the studied biomarkers have limited use in environmental risk assessment studies, at least when caged adult sea bass is used as the sentinel species and complex toxicant mixtures are involved. 相似文献
14.
The effect of the Coriolis force on the oil spill spreading in the gravity-viscous regime is examined. A new shallow water model for the transport and spreading of oil slick of arbitrary shape is described in which the Coriolis force is included in the momentum equations and the oil–water friction is parameterized in a frame of the boundary layer theory including the Ekman friction. The numerical Lagrangian method based on smoothed particle dynamics is described. New similarity solutions of the model equations are obtained for unidirectional and axisymmetric spreading in gravity-viscous, gravity-turbulent and gravity-viscous-rotational regimes for instantaneous as well as continuous releases. The numerical simulation extends these results for the case of continuous release in the presence of currents. It was shown that Coriolis term in the momentum equation can be omitted if slick thickness is much less of the laminar Ekman layer thickness. However, the Ekman friction should be retained for slicks of any thickness for larger times. The Ekman friction results in the essential slowdown of the spreading as well as in the deflection of the oil spreading velocity at 45° from the direction of velocity in the non-rotation case. Numerical simulations of large-scale spills showed that after the 2?days the slick area with the Coriolis effect was approximately less than half of that without rotation. Therefore, the earth rotation can be also important in the oil weathering. 相似文献
15.
Bytnerowicz A Badea O Barbu I Fleischer P Fraczek W Gancz V Godzik B Grodzińska K Grodzki W Karnosky D Koren M Krywult M Krzan Z Longauer R Mankovska B Manning WJ McManus M Musselman RC Novotny J Popescu F Postelnicu D Prus-Głowacki W Skawiński P Skiba S Szaro R Tamas S Vasile C 《Environment international》2003,29(2-3):367-376
An international cooperative project on distribution of ozone in the Carpathian Mountains, Central Europe was conducted from 1997 to 1999. Results of that project indicated that in large parts of the Carpathian Mountains, concentrations of ozone were elevated and potentially phytotoxic to forest vegetation. That study led to the establishment of new long-term studies on ecological changes in forests and other ecosystems caused by air pollution in the Retezat Mountains, Southern Carpathians, Romania and in the Tatra Mountains, Western Carpathians on the Polish-Slovak border. Both of these important mountain ranges have the status of national parks and are Man & the Biosphere Reserves. In the Retezat Mountains, the primary research objective was to evaluate how air pollution may affect forest health and biodiversity. The main research objective in the Tatra Mountains was to evaluate responses of natural and managed Norway spruce forests to air pollution and other stresses. Ambient concentrations of ozone (O(3)), sulfur dioxide (SO(2)), nitrogen oxides (NO(x)) as well as forest health and biodiversity changes were monitored on densely distributed research sites. Initial monitoring of pollutants indicated low levels of O(3), SO(2), and NO(x) in the Retezat Mountains, while elevated levels of O(3) and high deposition of atmospheric sulfur (S) and nitrogen (N) have characterized the Tatra Mountains. In the Retezat Mountains, air pollution seems to have little effect on forest health; however, there was concern that over a long time, even low levels of pollution may affect biodiversity of this important ecosystem. In contrast, severe decline of Norway spruce has been observed in the Tatra Mountains. Although bark beetle seems to be the immediate cause of that decline, long-term elevated levels of atmospheric N and S depositions and elevated O(3) could predispose trees to insect attacks and other stresses. European and US scientists studied pollution deposition, soil and plant chemistry, O(3)-sensitive plant species, forest insects, and genetic changes in the Retezat and Tatra Mountains. Results of these investigations are presented in a GIS format to allow for a better understanding of the changes and the recommendations for effective management in these two areas. 相似文献
16.
Johan Tidblad Vladimir Kucera Farid Samie Surendra N. Das Chalothorn Bhamornsut Leong Chow Peng King Lung So Zhao Dawei Le Thi Hong Lien Hans Schollenberger Chozi V. Lungu David Simbi 《Water, Air, & Soil Pollution: Focus》2007,7(1-3):241-247
Many national exposure programmes have been performed in tropical and subtropical climates during the last 50 years. However,
ambitious programmes involving more than a few countries are scarce. In this paper a recently formed network of test sites
is described involving 12 test sites in Asia (India, Vietnam, Thailand, Malaysia and China including Hong Kong) and four test
sites in Africa (South Africa, Zambia and Zimbabwe). This effort is part of the 2001–2004 Swedish International Development
Agency (SIDA) funded Programme on Regional Air Pollution in Developing Countries (RAPIDC). Corrosion attack after one (2002–2003)
year of exposure (carbon steel, zinc, copper, limestone and paint coated steel) are presented together with environmental
data (SO2, NO2, HNO3, O3, particles, amount and pH of precipitation, temperature and relative humidity) for all the test sites. The obtained corrosion
values are substantially higher than expected for limestone, higher than expected for carbon steel and lower than expected
for zinc compared to values calculated using the best available dose–response functions. 相似文献
17.
18.
New data on the vapour pressures and aqueous solubility of 1,8-dichlorooctane and 1,8-dibromooctane are reported as a function of temperature between 20 °C and 80 °C and 1 °C and 40 °C, respectively. For the vapour pressures, a static method was used during the measurements which have an estimated uncertainty between 3% and 5%. The aqueous solubilities were determined using a dynamic saturation column method and the values are accurate to within ±10%. 1,8-Dichlorooctane is more volatile than 1,8-dibromooctane in the temperature range covered (psat varies from 3 to 250 Pa and from 0.53 to 62 Pa, respectively) and is also approximately three times more soluble in water (mole fraction solubilities at 25 °C of 5.95 × 10−7 and 1.92 × 10−7, respectively). A combination of the two sets of data allowed the calculation of the Henry’s law constants and the air water partition coefficients. A simple group contribution concept was used to rationalize the data obtained. 相似文献
19.
A new type of environmental numerical models, hybrid environmental numerical models (HEMs) based on combining deterministic modeling and machine learning components, is introduced and formulated. Conceptual and practical possibilities of developing HEM, as an optimal synergetic combination of the traditional deterministic/first principles modeling (like that used for solving PDEs on the sphere representing model dynamics of global climate models) and machine learning components (like accurate and fast neural network emulations of model physics or chemistry processes), are discussed. Examples of developed HEMs (hybrid climate models and a hybrid wind–wave ocean model) illustrate the feasibility and efficiency of the new approach for modeling extremely complex multidimensional systems. 相似文献
20.
Kondrashov VV Reshetin VP Regens JL Gunter JT 《Environmental science and pollution research international》2002,9(5):333-336
Urbanization typically involves a continuous increase in motor vehicle use, resulting in congestion known as traffic jams. Idling emissions due to traffic jams combine with the complex terrain created by buildings to concentrate atmospheric pollutants in localized areas. This research simulates emissions concentrations and distributions for a congested street in Minsk, Belarus. Ground-level (up to 50-meters above the street's surface) pollutant concentrations were calculated using STAR (version 3.10) with emission factors obtained from the U.S. Environmental Protection Agency, wind speed and direction, and building location and size. Relative emissions concentrations and distributions were simulated at 1-meter and 10-meters above street level. The findings demonstrate the importance of wind speed and direction, and building size and location on emissions concentrations and distributions, with the leeward sides of buildings retaining up to 99 percent of the emitted pollutants within 1-meter of street level, and up to 77 percent 10-meters above the street. 相似文献