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881.
Soil vapor extraction (SVE) is commonly used to remediate nonaqueous phase liquids (NAPLs) from the vadose zone. This paper aims to determine the effect of grain size heterogeneity on the removal of NAPL in porous media during SVE. Magnetic resonance imaging (MRI) was used to observe and quantify the amount and location of NAPL in flow-through columns filled with silica gel grains. MRI is unique because it is nondestructive, allowing three-dimensional images to be taken of the phases as a function of space and time. Columns were packed with silica gel in three ways: coarse grains (250-550 microm) only, fine grains (32-63 microm) only, and a core of fine grains surrounded by a shell of coarse grains. Columns saturated with water were drained under a constant suction head, contaminated with decane, and then drained to different decane saturations. Each column was then continuously purged with water-saturated nitrogen gas and images were taken intermittently. Results showed that at residual saturation, a sharp volatilization front moved through the columns filled with either coarse-grain or fine-grain silica gel. In the heterogeneous columns, the volatilization front in the core lagged just behind the shell because gas flow was greater through the shell and decane in the core diffused outward to the shell. When decane saturation in the core was above residual saturation, decane volatilization occurred near the inlet, the relative decane saturation throughout the core dropped uniformly, and decane in the core flowed in the liquid phase to the shell to replenish volatilized decane. These results indicate that NAPL trapped in low-permeability zones can flow to replenish areas where NAPL is lost due to SVE. However, when residual NAPL saturation is reached, NAPL flow no longer occurs and diffusion limits removal from low-permeability zones. 相似文献
882.
Hawes AK Solomon S Portmann RW Daniel JS Langford AO Miller HL Eubank CS Goldan P Wiedinmyer C Atlas E Hansel A Wisthaler A 《Journal of environmental monitoring : JEM》2003,5(6):977-983
Measuring hydrocarbons from aircraft represents one way to infer biogenic emissions at the surface. The focus of this paper is to show that complementary remote sensing information can be provided by optical measurements of a vegetation index, which is readily measured with high temporal coverage using reflectance data. We examine the similarities between the vegetation index and in situ measurements of the chemicals isoprene, methacrolein, and alpha-pinene to estimate whether the temporal behavior of the in situ measurements of these chemicals could be better understood by the addition of the vegetation index. Data were compared for flights conducted around Houston in August and September 2000. The three independent sets of chemical measurements examined correspond reasonably well with the vegetation index curves for the majority of flight days. While low values of the vegetation index always correspond to low values of the in situ chemical measurements, high values of the index correspond to both high and low values of the chemical measurements. In this sense it represents an upper limit when compared with in situ data (assuming the calibration constant is adequately chosen). This result suggests that while the vegetation index cannot represent a purely predictive quantity for the in situ measurements, it represents a complementary measurement that can be useful in understanding comparisons of various in situ observations, particularly when these observations occur with relatively low temporal frequency. In situ isoprene measurements and the vegetation index were also compared to an isoprene emission inventory to provide additional insight on broad issues relating to the use of vegetation indices in emission database development. 相似文献
883.
Fox A Harley W Feigley C Salzberg D Sebastian A Larsson L 《Journal of environmental monitoring : JEM》2003,5(2):246-252
Our group previously demonstrated that carbon dioxide (CO2) levels in heavily occupied schools correlate with the levels of airborne bacterial markers. Since CO2 is derived from the room occupants, it was hypothesized that in schools, bacterial markers may be primarily increased in indoor air because of the presence of children; directly from skin microflora or indirectly, by stirring up dust from carpets and other sources. The purpose of this project was to test the hypothesis. Muramic acid (Mur) is found in almost all bacteria whereas 3-hydroxy fatty acids (3-OH FAs) are found only in Gram-negative bacteria. Thus Mur and 3-OH FA serve as markers to assess bacterial levels in indoor air (pmol m(-3)). In our previous school studies, airborne dust was collected only from occupied rooms. However, in the present study, additional dust samples were collected from the same rooms each weekend when unoccupied. Samples were also collected from outside air. The levels of dust, Mur and C10:0, C12:0, C14:0, and C16:0 3-OH FAs were each much higher (range 5-50 fold) in occupied rooms than in unoccupied school rooms. Levels in outdoor air were much lower than that of indoor air from occupied classrooms and higher than the levels in the same rooms when unoccupied. The mean CO2 concentrations were around 420 parts per million (ppm) in unoccupied rooms and outside air; and they ranged from 1017 to 1736 ppm in occupied rooms, regularly exceeding 800-1000 ppm, which are the maximum levels indicative of adequate indoor ventilation. This indicates that the children were responsible for the increased levels of bacterial markers. However, the concentration of Mur in dust was also 6 fold higher in occupied rooms (115.5 versus 18.2 pmole mg(-1)). This further suggests that airborne dust present in occupied and unoccupied rooms is quite distinct. In conclusion in unoccupied rooms, the dust was of environmental origin but the children were the primary source in occupied rooms. 相似文献
884.
Maria T. Morandi Thomas H. Stock Charles F. Contant 《Environmental monitoring and assessment》1988,10(2):105-122
Personal monitoring (PM) for respirable suspended particulate matter (RSP) of thirty subjects was performed as part of an air pollution health effects study conducted in Houston, Texas. Parallel RSP measurements were performed in the study subjects' homes and two fixed site monitoring stations. The participants' daytime activities were independently recorded by study techicians. These data were used to characterize RSP concentrations in each microenvironment visited by the participants. Four estimates of daytime exposure to RSP were calculated based on two different microenvironmental models, and home and fixed site mean daytime RSP concentrations. These estimates were compared to mean daytime personal exposure from PM. Hourly estimates of exposure were calculated from a microenvironmental model and mean hourly home RSP concentrations and compared to hourly PM data. The results of the study indicate that, as in the case of NO2, it is important to characterize indoor microenvironmental RSP concentrations according to location, sources, and concurrent activities, both qualitatively and quantitatively. Stratification of concentrations according to sources present and self-reported activity can lead to misclassification of exposures. For RSP and, probably, other pollutants with indoor sources and with short exposure integration times, adequate measures of exposure can only be obtained with very detailed and complex microenvironmental models or comprehensive personal monitoring. 相似文献
885.
Gerard A. Nyssen Eric T. Miller Todd F. Glass Charles R. Quinn II Julie Underwood David J. Wilson 《Environmental monitoring and assessment》1987,9(1):1-11
Solubilities of several hydrophobic organic substances (paradichlorobenzene, endrin, naphthalene, and dibutyl phthalate) in aqueous solutions containing up to 0.10 mole fraction of common alcohols and ketones, were measured by gas chromatography. The solubilities are significantly increased by the alcohols and ketones. The results are interpreted in terms of the association of n molecules of alcohol or ketone with each hydrophobic organic molecule. Values of n and the equilibrium constant for this association are reported for each hydrophobic organic-alcohol and organic-ketone combination. The implications of these results for the disposal of toxic wastes by landfilling is discussed. 相似文献
886.
Heinz Gary H. Erdman Thomas C. Haseltine Susan D. Stafford Charles 《Environmental monitoring and assessment》1985,5(3):223-236
Residues of organochlorine pesticides, polychlorinated biphenyls (PCBs), polybrominated biphenyls (PBBs), polychlorinated styrenes (PCSs), and mercury were measured in the eggs of 10 species of colonial waterbirds nesting in areas around Green Bay or Lake Michigan from 1975 to 1980. Residues also were measured in the carcasses and brains of black-crowned night-herons (Nycticorax nycticorax). The highest residues were of PCBs, DDE, mercury, and dieldrin; for some species, levels of these chemicals possibly were high enough to have caused reproductive effects. Other organochlorine pesticides were found at low levels. Only trace amounts of PCSs and PBBs were found. Eggs of herring gulls (Larus argentatus) collected in 1977 from an island in Lake Michigan contained an average of 100 ppm PCBs and 33 ppm DDE; this was the most-contaminated species. Cattle egrets (Bubulcus ibis), the only bird that is not a fish eater, contained only small quantities of DDE and mercury. 相似文献
887.
888.
Stephanie A. Snyder Robert G. Haight Charles S. ReVelle 《Environmental Modeling and Assessment》2004,9(3):179-187
Conservation planners are called upon to make choices and trade-offs about the preservation of natural areas for the protection of species in the face of development pressures. We addressed the problem of selecting sites for protection over time with the objective of maximizing species representation, with uncertainty about future site development, and with periodic constraints on the number of sites that can be selected. We developed a 0–1, linear optimization model with 2 periods to select the sites that maximize expected species coverage subject to budget constraints. The model is based on the idea that development uncertainty can be characterized by a set of scenarios, each of which is a possible second-period development outcome for the set of sites. We also suggest that our 2-period model can be used in a sequential fashion that is consistent with adaptive planning. Results are presented for the Fox River watershed in Chicago. 相似文献
889.
Stephanie A. Snyder Robert G. Haight Charles S. ReVelle 《Environmental Modeling and Assessment》2005,9(3):179-187
Conservation planners are called upon to make choices and trade-offs about the preservation of natural areas for the protection of species in the face of development pressures. We addressed the problem of selecting sites for protection over time with the objective of maximizing species representation, with uncertainty about future site development, and with periodic constraints on the number of sites that can be selected. We developed a 0–1, linear optimization model with 2 periods to select the sites that maximize expected species coverage subject to budget constraints. The model is based on the idea that development uncertainty can be characterized by a set of scenarios, each of which is a possible second-period development outcome for the set of sites. We also suggest that our 2-period model can be used in a sequential fashion that is consistent with adaptive planning. Results are presented for the Fox River watershed in Chicago. 相似文献
890.
Scott?A.?MalcolmaEmail author Charles?ReVelle 《Environmental Modeling and Assessment》2005,10(4):341-348
Models for designing habitat reserve networks have focused on minimizing the number of sites necessary to cover each species
one or more times. A solution to this problem is usually one from among a large number of alternative optimal configurations
of sites. This paper develops an iterative method for building reserve networks that produces an optimal solution to the species
set covering problem (SSCP) and also maximizes the number of species covered two or more times, three or more times, and so
on, conditional on the solution to the previous iteration. We refer to this as representational success. Thus, a pareto optimal species set covering is achieved that is preferable to an arbitrary optimal solution to the SSCP. 相似文献