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961.
Douglas A. Wolfe K. John Scott John R. Clayton Jr. John Lunz James R. Payne Timothy A. Thompson 《Chemistry and Ecology》1995,10(1):137-156
Standardized tests were applied to aromatic and polar fractions of sediment extracts to determine whether polar constituents or oxidative degradation products contributed significantly to the toxicity of sediments oiled by the Exxon Valdez spill. Intertidal sediment and pore-water samples were collected in September 1990 from two heavily oiled sites and an unoiled site in Prince William Sound (PWS). Methylene chloride extracts from these samples were fractionated by liquid chromatography into aliphatic, aromatic and polar fractions, and the aromatic and polar fractions were tested for toxicity using the MicrotoxR test, bivalve larval mortality and development (Mytilus); several measures of genotoxicity in Mytilus, including SOS ChromotestR, anaphase aberrations and sister chromatid exchange; and survival, anaphase aberrations and teratogenicity in coho salmon (Onchorhynchus kisutch). MicrotoxR and SOS ChromotestR protocols were applied in a screening mode to all samples, whereas other tests were applied only to selected fractions from two sites. Samples from Bay of Isles (oiled) were consistently more toxic (usually only 2 to 5-fold) than the Mooselips Bay (unoiled) samples, which gave very low responses in all tests. for both sites, however, responses to polar and aromatic fractions were about the same in most tests, suggesting that while the overall toxicity of the oil was low in these samples, at least part of that toxicity was derived from polar constituents. Compared to the parent hydrocarbons, polar oxidation products partition preferentially into pore-water and are more rapidly diluted and dispersed in the water column. These results suggest that polar oxidation products of petroleum hydrocarbons pose little risk to marine organisms, except possibly for infauna continuously exposed to pore-water in heavily oiled sediments. Independent surveys showed that sediment toxicity in PWS declined during 1989-1991 to near background levels, in accord with previous understanding of oil weathering and toxicity. 相似文献
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David C. Garen Gregory L. Johnson Clayton L. Hanson 《Journal of the American Water Resources Association》1994,30(3):481-491
ABSTRACT: A procedure using detrended kriging has been developed to calculate daily values of mean areal precipitation (MAP) for input to hydrologic models. The important features of this procedure that overcome weaknesses in existing MAP procedures are: (1) specific precipitation-elevation relationships are determined for each time period as opposed to using relationships based on climatological averages, (2) spatial variability is incorporated by estimating precipitation for each grid cell over a watershed, (3) the spatial correlation structure of precipitation is explicitly modeled, and (4) station weights for precipitation estimates are determined objectively and optimally. Detailed cross-validation testing of the procedure was done for the Reynolds Creek research watershed in southwestern Idaho. The procedure is suitable for use in operational streamflow forecasting. 相似文献
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