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811.
Yu Shi Zhanbin Huang Xiujie Liu Suheryani Imran Licheng Peng Rongji Dai Yulin Deng 《Environmental science and pollution research international》2016,23(7):6168-6178
Heavy metal pollution is a severe environmental problem. Remediation of contaminated soils can be accomplished using environmental materials that are low cost and environmentally friendly. We evaluated the individual and combination effects of humic acid (HA), super absorbent polymer (SAP), zeolite (ZE), and fly ash composites (FC) on immobilization of lead (Pb) and cadmium (Cd) in contaminated soils. We also investigated long-term practical approaches for remediation of heavy metal pollution in soil. The biochemical and morphological properties of maize (Zea mays L.) were selected as biomarkers to assess the effects of environmental materials on heavy metal immobilization. The results showed that addition of test materials to soil effectively reduced heavy metal accumulation in maize foliage, improving chlorophyll levels, plant growth, and antioxidant enzyme activity. The test materials reduced heavy metal injury to maize throughout the growth period. A synergistic effect from combinations of different materials on immobilization of Pb and Cd was determined based on the reduction of morphological and biochemical injuries to maize. The combination of zeolite and humic acid was especially effective. Treatment with a combination of HA?+?SAP?+?ZE?+?FC was superior for remediation of soils contaminated with high levels of Pb and Cd. 相似文献
812.
The biogas upgrading by membrane separation process using a highly efficient CO2-selective polyvinylamine/polyvinylalcohol (PVAm/PVA) blend membrane was investigated by experimental study and simulation with respect to process design, operation optimization and economic evaluation. This blend membrane takes advantages of the unique CO2 facilitated transport from PVAm and the robust mechanical properties from PVA, exhibits both high CO2/CH4 separation efficiency and very good stability. CO2 transports through the water swollen membrane matrix in the form of bicarbonate. CO2/CH4 selectivity up to 40 and CO2 permeance up to 0.55 m3(STP)/m2 h bar at 2 bar were documented in lab with synthesized biogas (35% CO2 and 65% CH4). Membrane performances at varying feed pressures were recorded and used as the simulation basis in this work. The process simulation of an on-farm scale biogas upgrading plant (1000 Nm3/h) was conducted. Processes with four different membrane module configurations with or without recycle were evaluated technically and economically, and the 2-stage in cascade with recycle configuration was proven optimal among the four processes. The sensitivity of the process to various operation parameters was analyzed and the operation conditions were optimized. 相似文献
813.
Contaminant transport in soils is complicated and involves some physical and chemical nonequilibrium processes. In this research, the soil column displacement experiments of Cl− and atrazine under different flow velocities were carried out. The data sets of Cl− transport in sandy loam fitted to the convection dispersion equation (CDE) and the two-region model (TRM) indicated that the effects of physical nonequilibrium process produced by immobile water on the breakthrough curves (BTCs) of Cl− and atrazine transport through the repacking soil columns were negligible. The two-site model (TSM) and the continuous time random walk (CTRW) were also used to fit atrazine transport behavior at the flow rate of 19.86 cm h−1. The CTRW convincingly captured the full evolution of atrazine BTC in the soil column, especially for the part of long tailing. However, the TSM failed to characterize the tailing of atrazine BTC in the soil column. The calculated fraction of equilibrium sorption sites, F, ranging from 0.78 to 0.80 for all flow rates suggested the contribution of nonequilibrium sorption sites to the asymmetry of atrazine BTCs. Furthermore, the data sets for the flow rates of 6.68 cm h−1 and 32.81 cm h−1 were predicted by the TSM and the CTRW. As to the flow rate of 6.68 cm h−1, the CTRW predicted the entire BTC of atrazine transport better than the TSM did. For the flow rate of 32.81 cm h−1, the CTRW characterized the late part of the tail better, while the TSM failed to predict the tailings of atrazine BTC. 相似文献
814.
长江水系河流与水库中鲤鱼的元素含量特征 总被引:6,自引:3,他引:3
针对长江三峡水库蓄水后引起水库汞活化效应对生态与环境的影响问题,系统地分析了长江水系水库与河流鲤鱼肌肉的As,Cd,Cu,Fe,Hg,Mn,Pb,Se,Na,Mg等元素含量的分布特征。并以丹江口水库-汉江,陈村水库-青戈江为例,用多元分析证明水库与河流的鲤肌肉中As,Se,Hg,Cd等元素含量存在显著差异,同时指出水库汞活化效应引起的鱼体汞含量增加是该元素的一种生物地球化学现象,并利用同一水系水库 相似文献
815.
Xiaoxiao Zhang Xiang Ding Dilinuer Talifu Xinming Wang Abulikemu Abulizi Mailikezhati Maihemuti Suwubinuer Rekefu 《环境科学学报(英文版)》2021,33(2):279-286
Atmospheric visibility can directly reflect the air quality. In this study, we measured water-soluble ions (WSIs), organic and element carbon (OC and EC) in PM2.5 from September 2017 to August 2018 in Urumqi, NW China. The results show that SO42?, NO3? and NH4+ were the major WSIs, together accounting for 7.32%–84.12% of PM2.5 mass. Total carbon (TC=OC+EC) accounted for 12.12% of PM2.5 mass on average. And OC/EC > 2 indicated the formation of secondary organic carbon (SOC). The levels of SO42?, NO3? and NH4+ in low visibility days were much higher than those in high visibility days. Relative humidity (RH) played a key role in affecting visibility. The extinction coefficient (bext) that estimated via Koschmieder formula with visibility was the highest in winter (1441.05 ± 739.95 Mm?1), and the lowest in summer (128.58 ± 58.00 Mm?1). The bext that estimated via IMPROVE formula with PM2.5 chemical component was mainly contributed by (NH4)2SO4 and NH4NO3. The bext values calculated by both approaches presented a good correlation with each other (R2 = 0.87). Multiple linear regression (MLR) method was further employed to reconstruct the empirical regression model of visibility as a function of PM2.5 chemical components, NO2 and RH. The results of source apportionment by Positive Matrix Factorization (PMF) model showed that residential coal combustion and vehicle emissions were the major sources of bext. 相似文献
816.
介绍了大港油田大气颗粒物和多环芳烃的污染现状,并对大港油田地区大气特征构成及大气颗粒物中多环芳烃的污染特征作了初步分析,得出大港油田地区大气颗粒物中多环芳烃污染类型为燃油型,并据此提出了防治多环芳烃污染的相应对策。 相似文献
817.
818.
微波技术在废物处理中的应用 总被引:2,自引:0,他引:2
综述了微波在废物处理中的应用,主要介绍了微波加热的机理及特点,微波在处理放射性废物、废旧电路板、污泥、医疗垃圾、废轮胎中的应用,展望了微波技术在废物处理中的应用前景。 相似文献
819.
Xuliang Zhuang Yuesi Wang Hong He Jianguo Liu Xinming Wang Tingyu Zhu Maofa Ge Ju Zhou Guiqian Tang Jinzhu Ma 《环境科学学报(英文版)》2014,26(1):2-12
The present article provides an overview of the chemical and physical features of haze in China, focusing on the relationship between haze and atmospheric fine particles, and the formation mechanism of haze. It also summarizes several of control technologies and strategies to mitigate the occurrence of haze. The development of instruments and the analysis of measurements of ambient particles and precursor concentrations have provided important information about haze formation. Indeed, the use of new instruments has greatly facilitated current haze research in China. Examples of insightful results include the relationship between fine particles and haze, the chemical compositions and sources of particles, the impacts of the aging process on haze formation, and the application of technologies that control the formation of haze. Based on these results, two relevant issues need to be addressed: understanding the relationship between haze and fine particles and understanding how to control PM2.5. 相似文献
820.