全文获取类型
收费全文 | 937篇 |
免费 | 10篇 |
国内免费 | 15篇 |
专业分类
安全科学 | 59篇 |
废物处理 | 20篇 |
环保管理 | 131篇 |
综合类 | 140篇 |
基础理论 | 260篇 |
环境理论 | 1篇 |
污染及防治 | 227篇 |
评价与监测 | 82篇 |
社会与环境 | 34篇 |
灾害及防治 | 8篇 |
出版年
2023年 | 7篇 |
2022年 | 4篇 |
2021年 | 7篇 |
2020年 | 6篇 |
2019年 | 11篇 |
2018年 | 17篇 |
2017年 | 14篇 |
2016年 | 20篇 |
2015年 | 28篇 |
2014年 | 15篇 |
2013年 | 101篇 |
2012年 | 39篇 |
2011年 | 62篇 |
2010年 | 46篇 |
2009年 | 50篇 |
2008年 | 58篇 |
2007年 | 48篇 |
2006年 | 36篇 |
2005年 | 31篇 |
2004年 | 29篇 |
2003年 | 28篇 |
2002年 | 35篇 |
2001年 | 17篇 |
2000年 | 19篇 |
1999年 | 6篇 |
1998年 | 16篇 |
1997年 | 9篇 |
1996年 | 14篇 |
1995年 | 9篇 |
1994年 | 13篇 |
1993年 | 9篇 |
1992年 | 11篇 |
1991年 | 13篇 |
1990年 | 8篇 |
1989年 | 8篇 |
1988年 | 4篇 |
1987年 | 5篇 |
1986年 | 6篇 |
1985年 | 11篇 |
1984年 | 5篇 |
1982年 | 8篇 |
1981年 | 6篇 |
1978年 | 5篇 |
1977年 | 4篇 |
1976年 | 3篇 |
1975年 | 3篇 |
1971年 | 4篇 |
1969年 | 4篇 |
1960年 | 4篇 |
1956年 | 3篇 |
排序方式: 共有962条查询结果,搜索用时 31 毫秒
531.
Henne Paul D. Bigalke Moritz Büntgen Ulf Colombaroli Daniele Conedera Marco Feller Urs Frank David Fuhrer Jürg Grosjean Martin Heiri Oliver Luterbacher Jürg Mestrot Adrien Rigling Andreas Rössler Ole Rohr Christian Rutishauser This Schwikowski Margit Stampfli Andreas Szidat Sönke Theurillat Jean-Paul Weingartner Rolf Wilcke Wolfgang Tinner Willy 《Regional Environmental Change》2018,18(1):205-221
Regional Environmental Change - Planning for the future requires a detailed understanding of how climate change affects a wide range of systems at spatial scales that are relevant to humans.... 相似文献
532.
Elliott G. Duncan William A. Maher Rajani Jagtap Frank Krikowa Margaret M. Roper Cathryn A. O’Sullivan 《Environmental geochemistry and health》2017,39(4):955-966
This study investigated whether selenium species in wheat grains could be altered by exposure to different combinations of nitrogen (N) and sulphur (S) fertilisers in an agronomic biofortification experiment. Four Australian wheat cultivars (Mace, Janz, Emu Rock and Magenta) were grown in a glasshouse experiment and exposed to 3 mg Se kg?1 soil as selenate (SeVI). Plants were also exposed to 60 mg N kg?1 soil as urea and 20 mg S kg?1 soil as gypsum in a factorial design (N + S + Se; N + Se; S + Se; Se only). Plants were grown to maturity with grain analysed for total Se concentrations via ICP-MS and Se species determined via HPLC-ICP-MS. Grain Se concentrations ranged from 22 to 70 µg Se g?1 grain (dry mass). Selenomethionine (SeMet), Se-methylselenocystine (MeSeCys), selenohomolanthionine (SeHLan), plus a large concentration of uncharacterised Se species were found in the extracts from grains. SeMet was the major Se species identified accounting for between 9 and 24 µg Se g?1 grain. Exposure to different N and S fertiliser combinations altered the SeMet content of Mace, Janz and Emu Rock grain, but not that of Magenta. MeSeCys and SeHLan were found in far lower concentrations (<4 µg Se g?1 grain). A large component of the total grain Se was uncharacterisable (>30 % of total grain Se) in all samples. When N fertiliser was applied (with or without S), the proportion of uncharacterisable Se increased between 60 and 70 % of the total grain Se. The data presented here indicate that it is possible to alter the content of individual Se species in wheat grains via biofortification combined with manipulation of N and S fertiliser regimes. This has potential significance in alleviating or combating both Se deficiency and Se toxicity effects in humans. 相似文献
533.
Rigét F Vorkamp K Dietz R Rastogi SC 《Journal of environmental monitoring : JEM》2006,8(10):1000-1005
The concentrations of polybrominated diphenyl ethers (PBDEs) 17, 28, 47, 49, 66, 85, 99, 100, 153, 154, and 183 were determined in ringed seal blubber from central East Greenland collected in 1986, 1994, 1999 and during the period 2001 to 2004. The trend of PBDEs was compared with the trends of polychlorinated biphenyls (PCBs) 28, 31, 52, 101, 105, 118, 138, 153, 156, and 180 during the same period. The levels of sigmaPBDE in East Greenland ringed seals ranged from 21.8 ng g(-1) lipid weight (1w) in 1986 to 39.3 ng g(-1) lw in 2001 and are among the highest observed in ringed seal from the Arctic. The dominating congeners were BDE-47 (75.4%) and BDE-99 (9.7%). The concentrations of PBDEs and PCBs increased with the age of the seals, and therefore only young seals < or =4 years old) were included in the temporal trend analyses. No significant trend (p > 0.14) was observed in sigmaPBDE or the congeners BDE 28, 47 and, 99 during the period while sigmaPCB decreased significantly (p = 0.004) over the period from 1986 to 2004 with an estimated annual rate of 4.3%. 相似文献
534.
Whole tissue trace metal concentrations of ten metals in eight common coastal Australian polychaete species collected from uncontaminated locations were measured. The mean concentration range for each trace metal was: Mn: 2.6-13 microg g(-1); Co: 0.8-4.6 microg g(-1); Cu: 3.4-26 microg g(-1); Zn: 47-225 microg g(-1); As: 18-101 microg g(-1); Se: 2.2-20.4 microg g(-1); Ag: 0.03-2.5 microg g(-1); Cd: 0.07-17 microg g(-1); Hg: 0.08-0.88 microg g(-1) and Pb: 0.09-3.2 microg g(-1)dry mass. Principal components analysis of trace metal signatures revealed that the habitat, i.e. exposed coast sand or rock, estuarine sand or estuarine mud substrate in which a polychaete species was found, had a significant influence on the bioaccumulation of six trace metals (Mn, Cu, Zn, Ag, Cd and Pb). However, there is no clear relationship between trace metal concentrations in substrates and polychaetes. The results of the current study contribute to a reference dataset of polychaete species-specific natural background trace metal concentrations for use in determining the extent of trace metal contamination by urban and industrial sources. 相似文献
535.
536.
Sather ME Mathew J Nguyen N Lay J Golod G Vet R Cotie J Hertel T Aaboe E Callison R Adam J Keese D Freise J Hathcoat A Sakizzie B King M Lee C Oliva S San Miguel G Crow L Geasland F 《Journal of environmental monitoring : JEM》2008,10(11):1319-1325
Ambient ammonia monitoring using Ogawa passive samplers was conducted in the Four Corners area and eastern Oklahoma, USA during 2007. The resulting data will be useful in the multipollutant management of ozone, nitrogen oxides, and visibility (atmospheric regional haze) in the Four Corners area, an area with growing oil/gas production and increasing coal-based power plant construction. The passive monitoring data also add new ambient ammonia concentration information for the U.S. and will be useful to scientists involved in present and future visibility modeling exercises. Three week integrated passive ammonia samples were taken at five sites in the Four Corners area and two sites in eastern Oklahoma from December, 2006 through December, 2007 (January, 2008 for two sites). Results show significantly higher regional background ammonia concentrations in eastern Oklahoma (1.8 parts per billion (ppb) arithmetic mean) compared to the Four Corners area (0.2 ppb arithmetic mean). Annual mean ammonia concentrations for all Four Corners area sites for the 2007 study ranged from 0.2 ppb to 1.5 ppb. Peak ambient ammonia concentrations occurred in the spring and summer in both areas. The passive samplers deployed at the Stilwell, Oklahoma site compared favorably with other passive samplers and a continuous ammonia monitoring instrument. 相似文献
537.
Bashir W McGovern F O'Brien P Ryan M Burke L Paull B 《Journal of environmental monitoring : JEM》2008,10(6):730-738
A major Irish study, based upon more than 8000 samples collected over the measurement period of 22 years, for sulfur dioxide (SO2-S), sulfate (SO4-S) and nitrogen dioxide (NO2-N) concentrations (microg m(-3)) within air, and the ionic composition of precipitation samples based on sodium (Na+), potassium (K+), magnesium (Mg2+), calcium (Ca2+), chloride (Cl-), sulfate (SO4-S), non-sea salt sulfate (nssSO4-S), ammonium (NH4-N), and nitrate (NO3-N) weighted mean concentrations (mg l(-1)), has been completed. For the air samples, the sulfur dioxide and sulfate concentrations decreased over the sampling period (1980-2004) by 75% and 45%, respectively, whereas no significant trend was observed for nitrogen dioxide. The highest concentrations for sulfur dioxide, sulfate and nitrogen dioxide were associated with wind originating from the easterly and northeasterly directions i.e. those influenced by Irish and European sources. The lowest concentrations were associated with the westerly directions i.e. for air masses originating in the North Atlantic region. This was further verified with the use of backward (back) trajectory analysis, which allowed tracing the movement of air parcels using the European Centre for Medium range Weather Forecasting (ECMWF) ERA-40 re-analysis data. High non-sea salt sulfate levels were being associated with air masses originating from Europe (easterlies) with lower levels from the Atlantic (westerlies). With the precipitation data, analysis of the non-sea salt sulfate concentrations showed a decrease by 47% since the measurements commenced. 相似文献
538.
Levels and temporal trends of the hexachlorocyclohexane isomers alpha-, beta- and gamma-HCH were analysed in blubber of juvenile ringed seals from West Greenland (1994 to 2006) and juvenile and adult ringed seals from East Greenland (1986 to 2006). No significant differences in the concentration levels in the juvenile seals were found between East and West Greenland for any of the three isomers. alpha-HCH concentrations were not significantly different between juvenile and adult ringed seals from East Greenland, whereas beta- and gamma-HCH concentrations were significantly higher in adult ringed seals. alpha- and beta-HCH in Greenland ringed seals were approximately a factor two lower than in the Canadian Arctic, and alpha-HCH was a factor 2-3 higher than in ringed seals from an area east of Svalbard, Norway. Annual decreases in ringed seals from Greenland during the study periods were detected to be 9.1-11.7%, 1.4-3.9% and 6.0-6.4% for alpha-, beta- and gamma-HCH, respectively, being quite similar in both East and West Greenland. Similar levels and trends in East and West Greenland support the general understanding of the pathways of HCH isomers to and in the Arctic. 相似文献
539.
Agostini M de Vocht F van Tongeren M Cherrie JW Galea KS Kromhout H 《Journal of environmental monitoring : JEM》2010,12(5):1170-1178
The objective of this study was to compare measured concentrations of rubber process dust and rubber fume originating from different sources in the British rubber manufacturing industry. Almost 8000 exposure measurements were obtained from industry-based survey results collected by the British Rubber Manufacturers' Association (BRMA), and covering the years 1977 to 2002, and from a series of small surveys contained in the Health and Safety Executive's (HSE) National Exposure Database (HSE-NEDB) from 1980 to 2002. The analysis investigated temporal trends in the exposure concentrations and the underlying main factors responsible for these changes. Analyses were carried out using hierarchical linear mixed effects models. Average personal exposures to rubber process dust and rubber fumes were respectively a factor 2 and 4 higher for the HSE-NEDB data when compared to data originating from the industry (BRMA data). Personal exposure to rubber process dust decreased on average by 4.1% (95% CI 4.7-3.6) annually for the BRMA data and slightly less at 2.3% (95% CI 5.2-0.7%) per annum for the HSE-NEDB data. Personal exposure to rubber fume also showed a downward temporal trend of 2.9% (95% CI 3.6-2.3%) and 4.8% (95% CI 7.4-2.1%) annually for the BRMA and HSE-NEDB data, respectively. These trends differed considerably between departments. No major changes in the estimated temporal trends in exposure concentrations were observed after including the presence of local exhaust ventilation in the models for any department in the BRMA and HSE-NEDB datasets. Lack of information on the quality and status of the local exhaust ventilation is the most likely explanation for this. In conclusion, even though there were relatively similar downward time trends in both rubber process dust and fume concentrations in both datasets, the source of exposure data was an important determinant of average exposure concentrations present in the British rubber manufacturing industry. Lack of detailed auxiliary information on company size, reason for sampling, measurement strategy and other potentially important determinants of exposure prevented an explanation for the observed differences in exposure level. 相似文献
540.