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841.
Water polluted with arsenic presents a challenge for remediation. A combination of phyto- and electro-remediation was attempted in this study. Four tanks were setup in order to assess the arsenic removal ability of the two methods separately and in combination. Lemna minor was chosen for As remediation and collected from a ditch in Utrecht, The Netherlands. The tanks were filled with surface water without any pre-cleaning, therefore containing various elements including metals as Mn (2.9 mg L(-1)), Cu (0.05 mg L(-1)), Fe (1.39 mg L(-1)), and Ba (0.13 mg L(-1)). This water was then spiked with As and allocated to a feed container, guaranteeing a continuous flow of 0.12 mL s(-1) to each tank. Two experiments were performed: Exp. 1 with 3 consecutive stages with rising applied voltage and Exp. 2, with a constant voltage over a period of 6 d. Measurements of pH and temperature were taken every working day, as well as water samples from outlets of all tanks including feed container for control. From the present study, there was no evidence that As had been taken up by the plants, but a strong depletion of As was observed in the tanks where current was applied. Preliminary results clearly showed that applying voltage to the electrodes caused 90% removal of As from the spiked surface water. 相似文献
842.
Toxicity, dioxin-like activities, and endocrine effects of DDT metabolites—DDA, DDMU, DDMS, and DDCN
Wetterauer B Ricking M Otte JC Hallare AV Rastall A Erdinger L Schwarzbauer J Braunbeck T Hollert H 《Environmental science and pollution research international》2012,19(2):403-415
Background, aim, and scope
2,2-bis(chlorophenyl)-1,1,1-trichloroethane (DDT) metabolites, other than those routinely measured [i.e., 2,2-bis(chlorophenyl)-1,1-dichloroethylene (DDE) and 2,2-bis(chlorophenyl)-1,1-dichloroethane (DDD)], have recently been detected in elevated concentrations not only in the surface water of Teltow Canal, Berlin, but also in sediment samples from Elbe tributaries (e.g., Mulde and Havel/Spree). This was paralleled by recent reports that multiple other metabolites could emerge from the degradation of parent DDT by naturally occurring organisms or by interaction with some heavy metals. Nevertheless, only very few data on the biological activities of these metabolites are available to date. The objective of this communication is to evaluate, for the first time, the cytotoxicity, dioxin-like activity, and estrogenicity of the least-studied DDT metabolites. 相似文献843.
Jan E. Vermaat Estra Estradivari Leontine E. Becking 《Regional Environmental Change》2012,12(3):437-444
Using the drivers–pressures–state–impact–responses (DPSIR) analytical framework, local stakeholder respondents and experts were interviewed to construct and prioritize a causality network that links ecosystem state of the coastal waters of Berau (East Kalimantan, Indonesia) with societal drivers of change. Particularly on the perceived top priority drivers and pressures, consensus among respondents was considerable. The constructed network was found to be consistent with literature findings from elsewhere in SE Asia. This causality network was then confronted with a local articulation of the SRES scenarios (IPCCs Special Report on Emissions Scenarios: A1, A2, B1, B2), and four plausible trajectories of future change were deduced over a period of 20?years, until 2030. Our scenario articulations differed greatly in the projected immigration influx into the region, in local economic growth and in institutional strength of governance. Under business-as-usual conditions, it is foreseen that fisheries will continue to overexploit the resource, and inland and mangrove deforestation, as well as sediment and sewage loading of the coastal waters, will increase, leading to declines in coral and seagrass extent and depleted fisheries. Scenarios with continued immigration (~A1, A2) will probably aggravate this pattern, whereas those with reduced immigration (~B1, B2) would appear to lead to considerable improvements in the state of the coastal waters of Berau. 相似文献
844.
Critical review of actually available chemical compounds for prevention and management of cyanobacterial blooms 总被引:3,自引:0,他引:3
Cyanobacteria proliferation is among the most threatening consequences of freshwater pollution. Health risks from human and other-organism exposure to cyanobacteria have led to an effort to find practical methods for cyanobacterial water-bloom reduction. Hence, methods and techniques have been developed in order to reduce the amount of phosphorus or to decrease the abundance of nuisance phytoplankton species directly in the water bodies (in-lake measures). Although these “acute” methods do not solve the problem of catchment area eutrophication, they are cheaper, easier to manage, and for some areas they are the only way to protect human and environmental health against massive cyanobacterial proliferation. This review summarizes the extent of knowledge and published data about the management using metals (Al, Fe, Cu, Ag, Ca), photosensitizers (hydrogen peroxide, phthalocyanines, TiO2), herbicides and chemicals derived from natural compounds as fast and efficient removal agents of cyanobacteria. This review concludes that some compounds, when non-persistent and ecotoxicologically acceptable may help to manage cyanobacterial blooms in an efficient way compared to previous methods (e.g. copper sulfate). 相似文献
845.
Bonten LT Groenenberg JE Meesenburg H de Vries W 《Environmental pollution (Barking, Essex : 1987)》2011,159(10):2831-2839
Various dynamic soil chemistry models have been developed to gain insight into impacts of atmospheric deposition of sulphur, nitrogen and other elements on soil and soil solution chemistry. Sorption parameters for anions and cations are generally calibrated for each site, which hampers extrapolation in space and time. On the other hand, recently developed surface complexation models (SCMs) have been successful in predicting ion sorption for static systems using generic parameter sets. This study reports the inclusion of an assemblage of these SCMs in the dynamic soil chemistry model SMARTml and applies this model to a spruce forest site in Solling Germany. Parameters for SCMs were taken from generic datasets and not calibrated. Nevertheless, modelling results for major elements matched observations well. Further, trace metals were included in the model, also using the existing framework of SCMs. The model predicted sorption for most trace elements well. 相似文献
846.
Monitoring plastic ingestion by the northern fulmar Fulmarus glacialis in the North Sea 总被引:1,自引:0,他引:1
van Franeker JA Blaize C Danielsen J Fairclough K Gollan J Guse N Hansen PL Heubeck M Jensen JK Le Guillou G Olsen B Olsen KO Pedersen J Stienen EW Turner DM 《Environmental pollution (Barking, Essex : 1987)》2011,159(10):2609-2615
The abundance of plastics in stomachs of northern fulmars from the North Sea is used in the OSPAR Ecological Quality Objective (EcoQO) for marine litter. The preliminary EcoQO defines acceptable ecological quality as the situation where no more than 10% of fulmars exceed a critical level of 0.1 g of plastic in the stomach. During 2003-2007, 95% of 1295 fulmars sampled in the North Sea had plastic in the stomach (on average 35 pieces weighing 0.31 g) and the critical level of 0.1 g of plastic was exceeded by 58% of birds, with regional variations ranging from 48 to 78%. Long term data for the Netherlands since the 1980s show a decrease of industrial, but an increase of user plastics, with shipping and fisheries as the main sources. The EcoQO is now also used as an indicator for Good Environmental Status in the European Marine Strategy Framework Directive. 相似文献
847.
Petersen IL Tomasi G Sørensen H Boll ES Hansen HC Christensen JH 《Environmental pollution (Barking, Essex : 1987)》2011,159(10):3071-3077
Metabolic profiling in plants can be used to differentiate between treatments and to search for biomarkers for exposure. A methodology for processing Ultra-High-Performance Liquid Chromatography-Diode-Array-Detection data is devised. This methodology includes a scheme for selecting informative wavelengths, baseline removal, retention time alignment, selection of relevant retention times, and principal component analysis (PCA). Plant crude extracts from rapeseed seedling exposed to sublethal concentrations of glyphosate are used as a study case. Through this approach, plants exposed to concentrations down to 5 μM could be distinguished from the controls. The compounds responsible for this differentiation were partially identified and were different from those specific for high exposure samples, which suggests that two different responses to glyphosate are elicited in rapeseed depending on the level of exposure. The PCA loadings indicate that a combination of other metabolites could be more sensitive than the response of shikimate to detect glyphosate exposure. 相似文献
848.
The maximum specific growth rates of both ammonium oxidizing bacteria (AOB) and nitrite oxidizing bacteria (NOB) were investigated under varying aerobic solids retention time (SRTa) and in the presence/absence of anoxic (alternating) conditions. Two bench SBRs, reactor R1 and R2, were run in parallel for 150 d. Reactor R1 was operated in aerobic conditions while R2 operated in alternating anoxic/aerobic conditions. The feed (synthetic wastewater), temperature, hydraulic retention time and mixing were identical in both reactors. The SRTa in both reactors was, sequentially, set at four values: 5, 4, 3 and 2 d.Kinetic tests with the biomasses from both reactors were carried out to estimate the maximum specific growth rates (μmax) at each tested SRTa and decay rates, in both aerobic and anoxic conditions. The kinetic parameters of nitrifier were estimated through the calibration of a two step nitrification-denitrification activated sludge model.The results point to a slightly higher μmax,AOB and μmax,NOB in alternating conditions, while both μmax,AOB and μmax,NOB were shown not to vary in the tested range of SRTa (from 2 to 5 d) at 20 °C. They were relatively high when compared to literature data: 1.05 d−1 < μmax,AOB < 1.4 d−1 and 0.91 d−1 < μmax,NOB < 1.31 d−1. The decay coefficients of both AOB and NOB were much higher in aerobic (from 0.22 d−1 to 0.28 d−1) than in anoxic (0.04 d−1 to 0.16 d−1) conditions both in R1 and R2, which explained the higher nitrification rates observed in the alternating reactor. 相似文献
849.
Brems A Baeyens J Vandecasteele C Dewil R 《Journal of the Air & Waste Management Association (1995)》2011,61(7):721-731
Polyethylene terephthalate (PET) is a widely used thermoplastic. PET residues represent on average 7.6 wt% of the different polymer wastes in Europe. Pyrolysis of these wastes is attracting increasing interest, and PET is a potential candidate for this thermal process. The paper measures and discusses the kinetics of the pyrolysis reaction in terms of the reaction rate constants as determined by dynamic thermogravimetric analysis, with special emphasis on the required heating rate to obtain relevant results. The product yields and compositions are also determined. Gaseous products represent 16-18 wt%. The amounts of condensables and carbonaceous residue are a function of the operating mode, with slow pyrolysis producing up to 24 wt% of carbonaceous residue. Major condensable components are benzoic acid, monovinyl terephthalate, divinyl terephthalate, vinyl benzoate, and benzene. The present paper complements previous literature findings by (1) the study of the influence of the heating rate on the reaction kinetics in dynamic pyrolysis tests, (2) the isothermal investigation in a fluidized bed reactor to pyrolyze PET, and (3) the assessment of upgrading and recovery of the products. The paper concludes with a proposed reactor recommendation for PET pyrolysis, in either the bubbling or circulating fluidized bed operating mode. 相似文献
850.
Status and prospects of pay-as-you-throw in Europe - a review of pilot research and implementation studies 总被引:1,自引:0,他引:1
Reichenbach J 《Waste management (New York, N.Y.)》2008,28(12):2809-2814
Over the past 20 years, significant advances have been made in developing efficient schemes to charge households for their actual waste generation. Viable fee models and technical solutions which are applicable to different environments and provide waste generators with individual incentives for waste diversion efforts have increased the recognition of pay-as-you-throw (PAYT) as an effective instrument for recycling-oriented waste management and financing. On this basis, PAYT has become a practical reality in an increasing number of countries in Europe. Even countries with traditional reservations for direct charging have started to make consideration of PAYT in the revision of their national policy programmes. A situational analysis performed at the European level showed that detailed insights regarding the concrete reactions, red flags and wider benefits inherent to such scheme may still have to be further dispersed in order to overcome the caveats on PAYT and eventually adopt the approach on a larger scale. Claims that the results of PAYT applications are only local in meaning can be disproved as many of the developments bear universal character and can be verified even for larger territories using such schemes in different ways. Including results from an international research co-operation and comparative studies conducted in Germany, this article examines the state-of-the-art of PAYT and shades light onto some of the generally observed implications of its implementation. In conclusion, an outlook on the further potentials and propagation of this scheme is given. 相似文献