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排序方式: 共有98条查询结果,搜索用时 46 毫秒
71.
Polycyclic aromatic hydrocarbons and their hydroxylated metabolites in fish bile and sediments from coastal waters of Colombia 总被引:3,自引:0,他引:3
Johnson-Restrepo B Olivero-Verbel J Lu S Guette-Fernández J Baldiris-Avila R O'Byrne-Hoyos I Aldous KM Addink R Kannan K 《Environmental pollution (Barking, Essex : 1987)》2008,151(3):452-459
Sediments and fish bile collected from the Atlantic coastal waters of Colombia were analyzed for 16 parent polycyclic aromatic hydrocarbons (PAHs), and 23 hydroxylated PAHs (OH-PAHs), respectively. Sediments contained overall mean SigmaPAH concentrations of 2090, 234 and 170 ng/g, dry wt, for Cartagena Bay, Caimanera Marsh, and Totumo Marsh, respectively. The mean concentration of the summed OH-PAHs in fish bile was 1250, 180 and 64.1 ng/g bile wt for Cartagena Bay, Caimanera Marsh, and Totumo Marsh, respectively. The results suggest that Cartagena Bay is heavily polluted by PAHs, and that exposure to high concentrations of PAHs together with other factors could contribute to the decreased health of fish living in this ecosystem. This is one of the first studies to describe the analysis of 23 individual OH-PAHs in fish bile, using authentic standards. 相似文献
72.
Pere Ariza-Montobbio Katharine N. Farrell Gonzalo Gamboa Jesus Ramos-Martin 《Environment, Development and Sustainability》2014,16(4):925-956
Abandoning fossil fuels and increasingly relying on low-density, land-intensive renewable energy will increase demand for land, affecting current global and regional rural–urban relationships. Over the past two decades, rural–urban relationships all over the world have witnessed unprecedented changes that have rendered their boundaries blurred and have lead to the emergence of “new ruralities.” In this paper, we analyze the current profiles of electricity generation and consumption in relation to sociodemographic variables related to the use of time and land across the territory of Catalonia, Spain. Through a clustering procedure based on multivariate statistical analysis, we found that electricity consumption is related to functional specialization in the roles undertaken by different types of municipalities in the urban system. Municipality types have distinctive metabolic profiles in different sectors depending on their industrial, services or residential role. Villages’ metabolism is influenced by urban sprawl and industrial specialization, reflecting current “new ruralities.” Segregation between work activity and residence increases both overall electricity consumption and its rate (per hour) and density (per hectare) of dissipation. A sustainable spatial organization of societal activities without the use of fossil fuels or nuclear energy would require huge structural and sociodemographic changes to reduce energy demand and adapt it to regionally available renewable energy. 相似文献
73.
Laize Queiroz Alves Raildo Mota de Jesus Alex-Alan Furtado de Almeida Vânia Lima Souza Pedro Antônio Oliveira Mangabeira 《Environmental science and pollution research international》2014,21(10):6558-6570
Lead (Pb) has been highlighted as a major pollutant of both terrestrial and aquatic ecosystems, causing negative impacts to these environments. The concentration of Pb in plants has increased in recent decades, mainly due to anthropogenic activities. This study has as a hypothesis that the species Oxycaryum cubense (Poep. & Kunth) Palla, abundant in aquatic environments, has the potential to be used a phytoremediator. The plants were grown in a hydroponic system with Pb in increasing concentrations (0, 4, 8, 16 and 32 mg l?1) for 15 days. Inductively coupled mass spectrometer (ICP OES) was used to determine the concentration of mineral nutrients and lead. Optical and transmission electron microscopy were used for the analysis of cellular damage induced by lead in roots and leaves. Ultrastructural alterations were observed as disorganization of thylakoids in the chloroplast and disruption of mitochondrial membranes in cells of leaf tissues of plants subjected to increasing Pb concentrations. There was accumulation of Pb, especially in the root system, affecting the absorption and translocation of some mineral nutrients analysed. In roots, there was reduction in the thickness of the epidermis in plants treated with Pb. This species was shown to be tolerant to the Pb concentrations evaluated, compartmentalizing and accumulating Pb mainly in roots. Due to these results, it may be considered a species with phytoremediation capacity for Pb, with potential rizofiltration of this metallic element in contaminated watersheds. 相似文献
74.
Carlos Ayora Manuel A. Caraballo Francisco Macias Tobias S. Rötting Jesús Carrera Jose-Miguel Nieto 《Environmental science and pollution research international》2013,20(11):7837-7853
The Iberian Pyrite Belt (IPB), SW Spain and Portugal, contains about 100 abandoned mine wastes and galleries that release acid mine drainages (AMD) to the Tinto and Odiel rivers. In situ passive remediation technologies are especially suitable to remediate the drainages of these orphan sites. However, traditional remediation systems, designed for coal mines, have been demonstrated inefficient to treat the IPB mine waters. Due to their high acidity and metal loads, large amount of solids precipitate and fast clogging of porosity or passivation (coating) of the reactive grains occurs. To overcome these problems, the dispersed alkaline substrate (DAS) a mixture of fine-grained limestone sand and a coarse inert matrix (e.g., wood shavings) was developed. The small grains provide a large reactive surface and dissolve almost completely before the growing layer of precipitates passivates the substrate. The high porosity retards clogging. However, calcite dissolution only raises pH to values around 6.5, at which the hydroxides of trivalent metals (Al and Fe) precipitate, but it is not high enough to remove divalent metals. Caustic magnesia (MgO) buffers the solution pH between 8.5 and 10. A DAS system replacing limestone with caustic magnesia has been tested to be very efficient to remove divalent metals (Zn, Cd, Mn, Cu, Co, Ni, and Pb) from the water previously treated with calcite. 相似文献
75.
Investigating the potential of functionalized MCM-41 on adsorption of Remazol Red dye 总被引:1,自引:0,他引:1
Danilo Oliveira Santos Maria de Lourdes Nascimento Santos José Arnaldo Santana Costa Roberta Anjos de Jesus Sandro Navickiene Eliana Midori Sussuchi Maria Eliane de Mesquita 《Environmental science and pollution research international》2013,20(7):5028-5035
The modification of MCM-41 was performed with 3-aminopropropyltrimethoxysilane. The structural order and textural properties of the synthesized materials were studied by X-ray diffraction, Fourier transform infrared spectroscopy, thermogravimetry/differential thermogravimetry, nitrogen adsorption, and desorption analysis. The adsorption capacity of NH2-MCM-41 was studied with Remazol Red dye. The following parameters were studied in the adsorption process: pH, temperature, adsorbent dosage, and initial concentration. The desorption process was studied in different concentrations of NaOH solutions. The Freundlich isotherm model was found to be fit with the equilibrium isotherm data. Kinetics of adsorption follows the modified Avrami rate equation. The maximum adsorption capacity was estimated to be 45.9 mg?g?1, with removal of the dye of 99.1 %. The NH2-MCM-41 material exhibited high desorption capacity with 98.1 %. 相似文献
76.
S.A. Bea C. Ayora J. Carrera M.W. Saaltink B. Dold 《Journal of contaminant hydrology》2010,111(1-4):65-82
Water-soluble efflorescent salts often form on tailings in hyperarid climates. Their high solubility together with the high risk of human exposure to heavy metals such as Cu, Ni, Zn, etc., makes this occurrence a serious environmental problem.Understanding their formation (genesis) is therefore key to designing prevention and remediation strategies.A significant amount of these efflorescences has been described on the coastal area of Chañaral (Chile). There, highly soluble salts such as halite (NaCl) and eriochalcite (CuCl2·2H2O) form on 4 km2 of marine shore tailings. Natural occurrence of eriochalcite is rare: its formation requires extreme environmental and geochemical conditions such as high evaporation rate and low relative air humidity, and continuous Cl and Cu supply from groundwater, etc. Its formation was examined by means of reactive transport modeling.A scenario is proposed involving sea water and subsequently a mixture of sea water/freshwater in the groundwater composition in the formation of these efflorescences. The strong competition from other halides (i.e. halite and silvite (KCl)) for the Cl may inhibit the precipitation of eriochalcite. Therefore, the Cl/Na ratio trend > 1 is a key parameter in its formation. Cation-exchange between Na+ and other major ions such as K+, Ca2+, Mg2+ and Cu2+ in the clay fraction of tailings is proposed to account for realistic Cl/Na ratios.With regard to preventing the formation of eriochalcite, a capillary barrier on the tailings surface is proposed as a suitable alternative. Its efficiency as a barrier is also tested by means of reactive transport models. 相似文献
77.
Orellana FA Alegre JM Cordero Pérez JC Martín Redondo MP Delgado Huertas A Fernández Sampedro MT Menor-Salván C Ruiz-Bermejo M López-Vera F Rodríguez-Losada JA Martinez-Frias J 《Journal of environmental monitoring : JEM》2008,10(4):570-574
Certain local atmospheric anomalies, such as the formation of unusually large ice conglomerations (megacryometeors), have been proposed to be a potential natural hazard for people and aviation, as well as geoindicators for fingerprinting larger-scale atmospheric environmental changes. On March 13th 2007, at approximately 10:15 am, an ice chunk weighing about 10 kg fell from the clear-sky and crashed through the roof (around 15 m) of an industrial storage house in Mejorada del Campo, a town located 20 km east from Madrid. The megacryometeor monitoring follow-up and the original investigation presented here includes, for the first time, both logistic and scientific collaboration between the Laboratory of the Environment, Criminalistic Service (SECRIM, the Spanish "Guardia Civil") and academic and scientific institutions (universities and the Spanish National Research Council). We propose that the management procedure of the incident, along with the detailed scientific research and combination of analytical methodologies in different laboratories, can serve as a protocol model for other similar events. 相似文献
78.
Ikebe Otomo Juliana Araujo de Jesus Tatiane Gomes Coelho Lúcia Helena Rebelo Monteiro Lucilena Hunter Colin Helwig Karin Roberts Joanne Pahl Ole 《Environmental science and pollution research international》2021,28(32):43747-43762
Environmental Science and Pollution Research - The growth of two species of macrophytes (Lemna minor and Salvinia auriculata) under the effect of a mixture of amoxicillin, caffeine, carbamazepine,... 相似文献
79.
Gabriel Pereira Saulo R. Freitas Elisabete Caria Moraes Nelson Jesus Ferreira Yosio Edemir Shimabukuro Vadlamudi Brahmananda Rao Karla M. Longo 《Atmospheric environment (Oxford, England : 1994)》2009,43(40):6388-6397
Contemporary human activities such as tropical deforestation, land clearing for agriculture, pest control and grassland management lead to biomass burning, which in turn leads to land-cover changes. However, biomass burning emissions are not correctly measured and the methods to assess these emissions form a part of current research area. The traditional methods for estimating aerosols and trace gases released into the atmosphere generally use emission factors associated with fuel loading and moisture characteristics and other parameters that are hard to estimate in near real-time applications. In this paper, fire radiative power (FRP) products were extracted from Moderate Resolution Imaging Spectroradiometer (MODIS) and from the Geostationary Operational Environmental Satellites (GOES) fire products and new South America generic biomes FRE-based smoke aerosol emission coefficients were derived and applied in 2002 South America fire season. The inventory estimated by MODIS and GOES FRP measurements were included in Coupled Aerosol-Tracer Transport model coupled to the Brazilian developments on the Regional Atmospheric Modeling System (CATT-BRAMS) and evaluated with ground truth collected in Large Scale Biosphere–Atmosphere Smoke, Aerosols, Clouds, rainfall, and Climate (SMOCC) and Radiation, Cloud, and Climate Interactions (RaCCI). Although the linear regression showed that GOES FRP overestimates MODIS FRP observations, the use of a common external parameter such as MODIS aerosol optical depth product could minimize the difference between sensors. The relationship between the PM2.5μm (Particulate Matter with diameter less than 2.5 μm) and CO (Carbon Monoxide) model shows a good agreement with SMOCC/RaCCI data in the general pattern of temporal evolution. The results showed high correlations, with values between 0.80 and 0.95 (significant at 0.5 level by student t test), for the CATT-BRAMS simulations with PM2.5μm and CO. 相似文献
80.
Winfried Schröder Stefan Nickel Simon Schönrock Michaela Meyer Werner Wosniok Harry Harmens Marina V. Frontasyeva Renate Alber Julia Aleksiayenak Lambe Barandovski Alejo Carballeira Helena Danielsson Ludwig de Temmermann Barbara Godzik Zvonka Jeran Gunilla Pihl Karlsson Pranvera Lazo Sebastien Leblond Antti-Jussi Lindroos Siiri Liiv Sigurður H. Magnússon Blanka Mankovska Javier Martínez-Abaigar Juha Piispanen Jarmo Poikolainen Ion V. Popescu Flora Qarri Jesus Miguel Santamaria Mitja Skudnik Zdravko Špirić Trajce Stafilov Eiliv Steinnes Claudia Stihi Lotti Thöni Hilde Thelle Uggerud Harald G. Zechmeister 《Environmental science and pollution research international》2016,23(11):10457-10476
For analysing element input into ecosystems and associated risks due to atmospheric deposition, element concentrations in moss provide complementary and time-integrated data at high spatial resolution every 5 years since 1990. The paper reviews (1) minimum sample sizes needed for reliable, statistical estimation of mean values at four different spatial scales (European and national level as well as landscape-specific level covering Europe and single countries); (2) trends of heavy metal (HM) and nitrogen (N) concentrations in moss in Europe (1990–2010); (3) correlations between concentrations of HM in moss and soil specimens collected across Norway (1990–2010); and (4) canopy drip-induced site-specific variation of N concentration in moss sampled in seven European countries (1990–2013). While the minimum sample sizes on the European and national level were achieved without exception, for some ecological land classes and elements, the coverage with sampling sites should be improved. The decline in emission and subsequent atmospheric deposition of HM across Europe has resulted in decreasing HM concentrations in moss between 1990 and 2010. In contrast, hardly any changes were observed for N in moss between 2005, when N was included into the survey for the first time, and 2010. In Norway, both, the moss and the soil survey data sets, were correlated, indicating a decrease of HM concentrations in moss and soil. At the site level, the average N deposition inside of forests was almost three times higher than the average N deposition outside of forests. 相似文献