全文获取类型
收费全文 | 12461篇 |
免费 | 139篇 |
国内免费 | 98篇 |
专业分类
安全科学 | 365篇 |
废物处理 | 459篇 |
环保管理 | 1775篇 |
综合类 | 2198篇 |
基础理论 | 3329篇 |
环境理论 | 7篇 |
污染及防治 | 3071篇 |
评价与监测 | 764篇 |
社会与环境 | 637篇 |
灾害及防治 | 93篇 |
出版年
2023年 | 66篇 |
2022年 | 117篇 |
2021年 | 110篇 |
2020年 | 99篇 |
2019年 | 108篇 |
2018年 | 184篇 |
2017年 | 172篇 |
2016年 | 243篇 |
2015年 | 216篇 |
2014年 | 296篇 |
2013年 | 922篇 |
2012年 | 393篇 |
2011年 | 538篇 |
2010年 | 443篇 |
2009年 | 506篇 |
2008年 | 554篇 |
2007年 | 551篇 |
2006年 | 476篇 |
2005年 | 438篇 |
2004年 | 370篇 |
2003年 | 385篇 |
2002年 | 368篇 |
2001年 | 481篇 |
2000年 | 351篇 |
1999年 | 217篇 |
1998年 | 140篇 |
1997年 | 167篇 |
1996年 | 165篇 |
1995年 | 197篇 |
1994年 | 197篇 |
1993年 | 163篇 |
1992年 | 135篇 |
1991年 | 170篇 |
1990年 | 167篇 |
1989年 | 162篇 |
1988年 | 116篇 |
1987年 | 117篇 |
1986年 | 119篇 |
1985年 | 91篇 |
1984年 | 109篇 |
1983年 | 114篇 |
1982年 | 120篇 |
1981年 | 108篇 |
1980年 | 97篇 |
1979年 | 114篇 |
1978年 | 73篇 |
1977年 | 77篇 |
1975年 | 76篇 |
1973年 | 72篇 |
1967年 | 66篇 |
排序方式: 共有10000条查询结果,搜索用时 406 毫秒
431.
Washing aggregate sludge from a gravel pit, sewage sludge from a wastewater treatment plant (WWTP) and a clay-rich sediment have been physically, chemically and mineralogically characterized. They were mixed, milled and formed into pellets, pre-heated for 5 min and sintered in a rotary kiln at 1150 °C, 1175 °C, 1200 °C and 1225 °C for 10 and 15 min at each temperature. The effects of the raw material characteristics, heating temperatures and dwell times on the loss on ignition (LOI), bloating index (BI), bulk density (ρb), apparent and dry particle densities (ρa, ρd), voids (H), water absorption (WA24h) and compressive strength (S) were determined. All the mixtures presented a bloating potential taking into consideration the gases released at high temperatures. The products obtained were lightweight aggregates (LWAs) in accordance with Standard UNE-EN-13055-1 (ρb ≤ 1.20 g/cm3 or particle density ≤ 2.00 g/cm3). LWAs manufactured with 50% washing aggregate sludge and 50% clay-rich sediment were expanded LWAs (BI > 0) and showed the lowest apparent particle density, the lowest water absorption and the highest compressive strength. It was possible to establish three groups of LWAs on the basis of their properties in comparison to Arlita G3, F3 and F5, commercially available lightweight aggregates manufactured in Spain. Our LWAs may have the same or similar applications as these commercial products, such as horticulture, prefabricated lightweight structures and building structures. 相似文献
432.
Warmer, drier summers brought by climate change increase the potential risk of wildfires on the moorland of the Peak District of northern England. Fires are costly to fight, damage the ecosystem, harm water catchments, cause erosion scars and disrupt transport. Fires release carbon dioxide to the atmosphere. Accurate forecasts of the timing of fires help deployment of fire fighting resources. 相似文献
433.
Kerry A. Brown J. Carter Ingram Dan F. B. Flynn Rova Razafindrazaka Vololoniaina Jeannoda 《Environmental management》2009,44(1):136-148
Despite their prevalence in both developed and developing countries, there have been surprisingly few field assessments of
the ecological effectiveness of protected areas. This study aimed to assess the effectiveness of a key protected area in eastern
Madagascar, Ranomafana National Park (RNP). We established paired 100 × 4-m vegetation transects (400 m2) within RNP and in remnant forests in the park’s peripheral zone. In each 400-m2 plot, all woody stems >1.5 cm in diameter at breast height were measured and identified to species. All species were also
identified as native or non-native. We identified utilitarian species within all transects and they were sorted into use category.
We calculated plot-level taxonomic biodiversity and functional diversity of utilitarian species; the latter was calculated
by clustering the multivariate distances between species based on their utilitarian traits, and all metrics were tested using
paired t-tests. Our results showed that there was significantly higher biodiversity inside RNP than in remnant forests and this pattern
was consistent across all diversity metrics examined. Forests not located within the park’s boundary had significantly higher
non-native species than within RNP. There was no statistically significant difference in functional diversity of utilitarian
species inside RNP vs. remnant forests; however, the overall trend was toward higher diversity inside park boundaries. These
findings suggested that RNP has been effective at maintaining taxonomic diversity relative to surrounding unprotected areas
and restricting the spread of non-native plants. The results also suggested that low functional redundancy of forests outside
of RNP might be of concern, because residents in surrounding villages may have few other substitutes for the services provided
by species that are of critical importance to their livelihoods. This study highlights the challenges of trying to reconcile
biodiversity conservation with human use of natural resources in economically poor, remote areas. 相似文献
434.
A. Tieber H. Lettner P. Bossew A. Hubmer B. Sattler W. Hofmann 《Journal of environmental radioactivity》2009
Cryoconites are airborne sediments which accumulate on the surface of glaciers. In samples of cryoconites a temperate Austrian glacier high activity concentrations of anthropogenic radionuclides were found, which stem from global and Chernobyl fallouts. Radionuclides identified were 137Cs, 134Cs, 238Pu, 239+240Pu, 90Sr, 241Am, 60Co, 154Eu, 207Bi, and 125Sb. 相似文献
435.
A compilation has been undertaken of data which can be used to derive animal product transfer coefficients for radionuclides, including an extensive review of Russian language information. The resultant database has been used to provide recommended transfer coefficient values for a range of radionuclides to (i) cow, sheep and goat milk, (ii) meat (muscle) of cattle, sheep, goats, pigs and poultry and (iii) eggs. The values are used in a new IAEA handbook on transfer parameters which replaces that referred to as ‘TRS 364’. The paper outlines the approaches and procedures used to identify and collate data, and assumptions used. There are notable differences between the TRS 364 ‘expected’ values and the recommended values in the revised Handbook from the new database. Of the recommended values, three milk values are at least an order of magnitude higher than the TRS 364 values (Cr, Pu (cow) Pu (sheep)) and one milk value is lower (Ni (cow)). For meat, four values (Am, Cd, Sb (beef) I (pork)) are at least an order of magnitude higher than the TRS 364 values and eight values are at least an order of magnitude lower (Ru, Pu (beef), Ru, Sr, Zn (sheep), Ru, Sr (pork), Mn (poultry)). Many data gaps remain. 相似文献
436.
Comparison of manufactured and black carbon nanoparticle concentrations in aquatic sediments 总被引:1,自引:0,他引:1
Koelmans AA Nowack B Wiesner MR 《Environmental pollution (Barking, Essex : 1987)》2009,157(4):1110-1116
In this paper, we show that concentrations of manufactured carbon-based nanoparticles (MCNPs) in aquatic sediments will be negligible compared to levels of black carbon nanoparticles (BCNPs). This is concluded from model calculations accounting for MCNP sedimentation fluxes, removal rates due to aggregation or degradation, and MCNP burial in deeper sediment layers. The resultant steady state MCNP levels are compared with BCNP levels calculated from soot levels in sediments and weight fractions of nanosized fractions of these soot particles. MCNP/BCNP ratios range from 10−7 to 10−4 (w:w). This suggests that the often acclaimed effect of MCNPs on organic pollutant binding and bioavailability will likely be below the level of detection if natural BCNPs are present, even if binding to MCNP is one to two orders of magnitude stronger than to BCNPs. Furthermore, exposure and toxic effects of MCNPs in sediments and soils will be negligible compared to that of BCNPs. 相似文献
437.
Sarah B. Gewurtz Nilima Gandhi Guttorm N. Christensen Anita Evenset Dennis Gregor Miriam L. Diamond 《Environmental science and pollution research international》2009,16(2):176-190
Background, aim, and scope
Lake Ellasjøen, located in the Norwegian high arctic, contains the highest concentrations of polychlorinated biphenyls (PCBs) ever recorded in fish and sediment from high arctic lakes, and concentrations are more than 10 times greater than in nearby Lake Øyangen. These elevated concentrations in Ellasjøen have been previously attributed, in part, to contaminant loadings from seabirds that use Ellasjøen, but not Øyangen, as a resting area. However, other factors, such as food web structure, organism growth rate, weight, lipid content, lake morphology, and nutrient inputs from the seabird guano, also differ between the two systems. The aim of this study is to evaluate the relative influence of these factors as explanatory variables for the higher PCB fish concentrations in Ellasjøen compared with Øyangen, using both a food web model and empirical data.Methods
The model is based on previously developed models but parameterized for Lakes Ellasjøen and Øyangen using measured data wherever possible. The model was applied to five representative PCB congeners (PCB 105, 118, 138, 153, and 180) using measured sediment and water concentrations as input data and evaluated with previously collected food web data.Results
Modeled concentrations are within a factor of two of measured concentrations in 60% and 40% of the cases in Lakes Ellasjøen and Øyangen, respectively, and within a factor of 10 in 100% of the cases in both lakes. In many cases, this is comparable to the variability associated with the data as well as the efficacy of the predictions of other food web model applications.Discussion
We next used the model to quantify the relative importance of five major differences between Ellasjøen and Øyangen by replacing variables representing each of these factors in the Ellasjøen model with those from Øyangen, in separate simulations. The model predicts that the elevated PCB concentrations in Ellasjøen water and sediment account for 49%–58% of differences in modeled fish PCB concentrations between lakes. These elevated sediment and, to a lesser extent, water concentrations in Ellasjøen are due to PCB loadings from seabird guano. However, sediment–water fugacity ratios of PCBs are consistently greater in Ellasjøen compared with Øyangen, which suggests that internal lake processes also contribute to differences in sediment and water concentrations. We hypothesize that the nutrients associated with guano influence sediment–water fugacity ratios of PCBs by increasing the stock of pelagic algae. As both these algae and the guano settle, their organic carbon content is degraded faster than PCBs, which causes an extra magnification step in Ellasjøen before these detrital particles are consumed by benthic organisms, which are in turn consumed by fish. The model predicts that the remaining ~50% of the differences in PCB concentrations observed between the fish of these lakes are due to other subtle differences in their food web structures.Conclusions
In conclusion, based on the results of a food web model, we found that the most dominant factors influencing the higher PCB fish concentrations in Lake Ellasjøen compared with Øyangen are the higher sediment and water concentrations in Ellasjøen, caused by seabird guano. Together, sediment and water are predicted to account for 49%–58% of differences in fish concentrations between lakes. Although seabird guano provides a source of nutrients to the lake, in addition to contaminants, empirical data and indirect model results suggest that nutrients are not leading to decreased bioaccumulation, in contrast to what has been observed in temperate, pelagic food webs.Recommendations and perspectives
The results of this study emphasize the importance of considering even small differences in food web structure when comparing bioaccumulation in two lakes; although the food web structures of Ellasjøen and Øyangen differ only slightly, the model predicts that these differences account for most of the remaining ~50% of the differences in PCB fish concentrations between the two lakes. This study further demonstrates the utility of food web models as we were able to predict and tease apart the influence of various factors responsible for the elevated concentrations in the fish from Lake Ellasjøen, which would have been difficult using the field data alone. 相似文献438.
439.
440.
Identifying natural and anthropogenic sources of metals in urban and rural soils using GIS-based data,PCA, and spatial interpolation 总被引:2,自引:0,他引:2
Harley T. Davis C. Marjorie Aelion Suzanne McDermott Andrew B. Lawson 《Environmental pollution (Barking, Essex : 1987)》2009,157(8-9):2378-2385
Determining sources of neurotoxic metals in rural and urban soils is important for mitigating human exposure. Surface soil from four areas with significant clusters of mental retardation and developmental delay (MR/DD) in children, and one control site were analyzed for nine metals and characterized by soil type, climate, ecological region, land use and industrial facilities using readily available GIS-based data. Kriging, principal component analysis (PCA) and cluster analysis (CA) were used to identify commonalities of metal distribution. Three MR/DD areas (one rural and two urban) had similar soil types and significantly higher soil metal concentrations. PCA and CA results suggested that Ba, Be and Mn were consistently from natural sources; Pb and Hg from anthropogenic sources; and As, Cr, Cu, and Ni from both sources. Arsenic had low commonality estimates, was highly associated with a third PCA factor, and had a complex distribution, complicating mitigation strategies to minimize concentrations and exposures. 相似文献