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101.
Sodium-rich montmorillonite was modified with iron in order to introduce active centers for hydrogen sulfide adsorption. In the first modification, interlayer sodium cations were exchanged with iron. In another modification, iron oxocations were introduced to the clay surface. The most elaborated modification was based on doping of iron within the interlayer space of aluminum-pillared clay. The modified clay samples were tested as hydrogen sulfide adsorbents. Iron-doped samples showed a significant improvement in the capacity for H2S removal, despite of a noticeable decrease in microporosity compared to the initial pillared clay. The smallest capacity was obtained for the clay modified with iron oxocations. Variations in adsorption capacity are likely due to differences in the chemistry of iron species, degree of their dispersion on the surface, and accessibility of small pores for H2S molecule. The results suggest that on the surface of iron-modified clay hydrogen sulfide reacts with Fe(+3) forming sulfides or it is catalytically oxidized to SO2 on iron (hydro)oxides. Subsequent oxidation may lead to sulfate formation. 相似文献
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Female mate choice in the Pied Flycatcher Ficedula hypoleuca 总被引:2,自引:0,他引:2
Rauno V. Alatalo Arne Lundberg Karin Ståhlbrandt 《Behavioral ecology and sociobiology》1984,14(4):253-261
Summary We have examined male and territorial factors which might influence female mate choice in the Pied Flycatcher (Ficedula hypoleuca). Mating success of males was largely determined by the order of arrival on the breeding grounds. Females actively selected those males that had been longest in the area. This is likely to be due to territorial cues, early males having the best territories. About 15% of the males become polygynous, and these are the males that arrived earliest.Male age was relatively unimportant for breeding success, but because old males tend to arrive earlier than yearlings, most polygynous males were old. On average, old males are somewhat darker than young males, but male colour also varies within males of the same age. Polygynous and monogamous males did not differ significantly in colour, and female breeding success was not correlated with the colour of their mates. We show theoretically that it does not pay for females to select young males to avoid polygyny unless polygyny frequency or the number of reliable monogamous males almost double. Hence our hypothesis of polygyny-by-deceit in the Pied Flycatcher remains realistic. Because of male polyterritoriality, females are unaware of the males' status when mating. 相似文献
105.
Karin Mathes 《Environmental Sciences Europe》1997,9(1):17-23
Extrapolation is one of the most severe problems in ecotoxicological risk assessment. The protection of the environment requires the prediction of exposure to the ecosystem as well as the resulting changes in structural and functional properties. Three types of extrapolation models for effect assessment are discussed: ratio tests, empirical statistical models and the computer simulation of mathematical models. It has been demonstrated that the extrapolations used to regulate the release of chemicals into the environment are not supported scientifically. Aside from unrealistic or invalidated assumptions, problems are seen to result from the irreducible uncertainties inherent in the prediction of such ecological effects. Keeping precautionary principles in mind, some consequences concerning the decision-making processes in pre or post-marketing regulation as well as the legal aspects of such processes are introduced. 相似文献
106.
Per Stålnacke Anders Grimvall Karin Sundblad Anders Wilander 《Environmental monitoring and assessment》1999,59(1):47-72
Concern about nitrogen loads in marine environments has drawn attention to the existence and possible causes of long-term trends in nitrogen transport in rivers. The present study was based on data from the Swedish environmental monitoring programme for surface water quality; the continuity of these data is internationally unique. A recently developed semiparametric method was employed to study the development of relationships between runoff and river transport of nitrogen since 1971; the observed relationships were then used to produce time series of flow-normalised transports for 66 sites in 39 river basins. Subsequent statistical analyses of flow-normalised data revealed only few significant downward trends (p 0.05) during the time period 1971–1994, and the most pronounced of these downward trends were caused by reduced point emissions of nitrogen. The number of significant upward trends was substantially larger (15 for total-N and 18 for NO3-N). Closer examination of obtained results revealed the following: (i) the most pronounced upward trends were present downstream of lakes, and (ii) observed increases in nitrogen transport coincided in time and space with reduced point emissions of phosphorus or organic matter. This indicated that changes in the retention of nitrogen in lakes were responsible for the upward nitrogen trends. The hypothesis that nitrogen saturation of forest soils has caused a general increase in the riverine export of nitrogen from forested catchments in Sweden was not confirmed. Neither did the results indicate that improved agricultural practices have reduced the export of nitrogen from agricultural catchments. 相似文献
107.
Tisca Juliana F. dos Santos Karin Pessati Tomás B. Zacchi Flávia L. Soares Fabíola S. Oliveira Vanessa A. Bebianno Maria J. A. F. Bainy Afonso C. D. Razzera Guilherme 《Environmental science and pollution research international》2021,28(22):27823-27824
Environmental Science and Pollution Research - A Correction to this paper has been published: https://doi.org/10.1007/s11356-021-13135-x 相似文献
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109.
Examining Source-Receptor Relationships for Mercury in Scandinavia Modelled and Empirical Evidence 总被引:1,自引:0,他引:1
Munthe John Kindbom Karin Kruger Olaf Petersen Gerhard Pacyna Jozef Iverfeldt Åke 《Water, Air, & Soil Pollution: Focus》2001,1(3-4):299-310
The atmosphere remains the major source of mercuryin Swedish ecosystems. Since the late eighties,atmospheric emissions of mercury have drasticallydecreased in Europe. Wet deposition of mercury hasdecreased over the last decade but still exhibitsa clear south-to-north gradient, greatlyinfluenced by source areas in northern and centralEurope. The decreases in emissions can beattributed to both direct measures to close knownpoint sources and a declining economy and energyconsumption in many East European countries.Further reductions of mercury emissions willrequire that other source categories such asindirect emissions from mercury-containingproducts and crematories are be considered. 相似文献
110.
Remediation of recalcitrant compounds at sites with high concentrations of volatile organic compounds (VOCs) or nonaqueous‐phase liquids (NAPLs) can present significant technical and financial (long‐term) risk for stakeholders. Until recently, however, sustainability has not been included as a significant factor to be considered in the feasibility and risk evaluation for remediation technologies. The authors present a framework for which sustainability can be incorporated into the remediation selection criteria focusing specifically on off‐gas treatment selection for soil vapor extraction (SVE) remediation technology. SVE is generally considered an old and standard approach to in situ remediation of soils at a contaminated site. The focus on off‐gas treatment technology selection in this article allows for more in‐depth analysis of the feasibility evaluation process and how sustainable practices might influence the process. SVE is more commonly employed for recovery of VOCs from soils than other technologies and generally employs granular activated carbon (GAC), catalytic, or thermal oxidation, or an emerging alternative technology known as cryogenic‐compression and condensation combined with regenerative adsorption (C3–Technology). Of particular challenge to the off‐gas treatment selection process is the potential variety of chemical constituents and concentrations changing over time. Guidance is available regarding selection of off‐gas treatment technology (Air Force Center for Environmental Excellence, 1996; U.S. Environmental Protection Agency, 2006). However, there are common shortcomings of off‐gas treatment technology guidance and applications; practitioners have rarely considered sustainability and environmental impact of off‐gas treatment technology selection. This evaluation includes consideration of environmental sustainability in the selection of off‐gas treatment technologies and a region‐specific (Los Angeles, California) cost per pound and time of remediation comparisons between GAC, thermal oxidation, and C3–Technology. © 2008 Wiley Periodicals, Inc. 相似文献