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91.
Robert Schwarz 《Die Naturwissenschaften》1933,21(13):252-252
92.
Winfried Schwarz und André Leisewitz 《Umweltwissenschaften und Schadstoff-Forschung》1998,10(4):230-235
Zusammenfassung Die fluorierten Verbindungen Schwefelhexafluorid (SF6), perfluorierte Fluorkohlenwasserstoffe (CF4, C2F6) und wasserstoffhaltige Fluorkohlenwasserstoffe (H-FKW) z?hlen zu den atmosph?rischen Spurengasen mit extrem hohen Treibhauspotentialen.
Untersucht werden für Deutschland ihre realen Emissionen für 1990–1995, und Prognosen für die Jahre bis 2020 werden aufgestellt.
Diesen Prognosen zufolge vermindern sich die j?hrlichen Freisetzungen von CF4/C2F6 von 1990 bis 2000 von 335 t/34 t auf 100 t/10 t infolge Automatisierungsma?nahmen an der Hauptquelle (Aluminiumhütten). Die
Emissionen von SF6 bleiben dagegen bis 2020 im Schwankungsbereich zwischen 200 und 300 t j?hrlich. Hauptemittenten sind nicht elektrische Schaltanlagen,
da diese relativ dicht sind und über ein Entsorgungs-und Wiederaufarbeitungskonzept für gebrauchtes Gas verfügen, sondern
mit gro?em Abstand Autoreifen und Schallschutzscheiben. Bei den erst seit 1990 gezielt als FCKW-Nachfolger eingesetzten H-FKW
ist mit fortschreitender FCKW-Substitution in der station?ren und mobilen K?lte-und Klimatechnik, bei PU-Montageschaum und
Asthmasprays mit einer sprunghaften Zunahme der Emissionen bis auf über 9700 t/a ab dem Jahr 2007 zu rechnen, sofern sich
nicht halogenfreie Alternativen st?rker durchsetzen. Im Jahr 2020 werden bei Annahme dieser Trends die kumulierten Emissionen
der genannten fluorierten Verbindungen der Treibhauswirkung von 25 Mio. t CO2 entsprechen (GWP-Betrachtungszeitraum: 100 Jahre).
相似文献
93.
94.
Jud Harvey Jesus Gomez‐Velez Noah Schmadel Durelle Scott Elizabeth Boyer Richard Alexander Ken Eng Heather Golden Albert Kettner Chris Konrad Richard Moore Jim Pizzuto Greg Schwarz Chris Soulsby Jay Choi 《Journal of the American Water Resources Association》2019,55(2):369-381
Downstream flow in rivers is repeatedly delayed by hydrologic exchange with off‐channel storage zones where biogeochemical processing occurs. We present a dimensionless metric that quantifies river connectivity as the balance between downstream flow and the exchange of water with the bed, banks, and floodplains. The degree of connectivity directly influences downstream water quality — too little connectivity limits the amount of river water exchanged and leads to biogeochemically inactive water storage, while too much connectivity limits the contact time with sediments for reactions to proceed. Using a metric of reaction significance based on river connectivity, we provide evidence that intermediate levels of connectivity, rather than the highest or lowest levels, are the most efficient in removing nitrogen from Northeastern United States’ rivers. Intermediate connectivity balances the frequency, residence time, and contact volume with reactive sediments, which can maximize the reactive processing of dissolved contaminants and the protection of downstream water quality. Our simulations suggest denitrification dominantly occurs in riverbed hyporheic zones of streams and small rivers, whereas vertical turbulent mixing in contact with sediments dominates in mid‐size to large rivers. The metrics of connectivity and reaction significance presented here can facilitate scientifically based prioritizations of river management strategies to protect the values and functions of river corridors. 相似文献
95.
Scott W. Ator Ana Maria García Gregory E. Schwarz Joel D. Blomquist Andrew J. Sekellick 《Journal of the American Water Resources Association》2019,55(5):1149-1168
Understanding trends in stream chemistry is critical to watershed management, and often complicated by multiple contaminant sources and landscape conditions changing over varying time scales. We adapted spatially referenced regression (SPARROW) to infer causes of recent nutrient trends in Chesapeake Bay tributaries by relating observed fluxes during 1992, 2002, and 2012 to contemporary inputs and watershed conditions. The annual flow‐normalized nitrogen flux to the bay from its watershed declined by 14% to 127,000 Mg (metric tons) between 1992 and 2012, due primarily (more than 80% of the decline) to reduced point sources. The remainder of the decline was due to reduced atmospheric deposition (13%) and urban nonpoint sources. Agricultural inputs, which contribute most nitrogen to the bay, changed little, although trends in the average nitrogen yield (flux per unit area) from cropland and pasture to streams in some settings suggest possible effects of evolving nutrient applications or other land management practices. Point sources of phosphorus to local streams declined by half between 1992 and 2012, while nonpoint inputs were relatively unchanged. Annual phosphorus delivery to the bay increased by 9% to 9,570 Mg between 1992 and 2012, however, due mainly to reduced retention in the Susquehanna River at Conowingo Reservoir. 相似文献
96.
Kirsten Kinzer 《Journal of Environmental Planning and Management》2018,61(9):1594-1611
Although planning scholars often argue that public participation improves implementation outcomes, this relationship is rarely empirically tested. This study investigates how public engagement, during planning and after plan adoption, impacts on the speed of local government sustainability plan implementation. It includes a correlation analysis of quantized in-depth interviews with sustainability planners in 36 American cities. The study finds that individual characteristics of public engagement, both during planning and after plan adoption, had statistically significant relationships to implementation speed, but in some cases this relationship was negative. The correlations imply that sustainability planners can make strategic choices to improve implementation speed through public participation in plan creation and after plan adoption. Alternatively, planners also make choices during participatory planning that slow implementation, a problematic outcome when the ultimate goal of a planning process is on-the-ground change. 相似文献
97.
John W. Brakebill Scott W. Ator Gregory E. Schwarz 《Journal of the American Water Resources Association》2010,46(4):757-776
Brakebill, John W., Scott W. Ator, and Gregory E. Schwarz, 2010. Sources of Suspended-Sediment Flux in Streams of the Chesapeake Bay Watershed: A Regional Application of the SPARROW Model. Journal of the American Water Resources Association (JAWRA) 46(4): 757-776. DOI: 10.1111/j.1752-1688.2010.00450.x Abstract: We describe the sources and transport of fluvial suspended sediment in nontidal streams of the Chesapeake Bay watershed and vicinity. We applied SPAtially Referenced Regressions on Watershed attributes, which spatially correlates estimated mean annual flux of suspended sediment in nontidal streams with sources of suspended sediment and transport factors. According to our model, urban development generates on average the greatest amount of suspended sediment per unit area (3,928 Mg/km2/year), although agriculture is much more widespread and is the greatest overall source of suspended sediment (57 Mg/km2/year). Factors affecting sediment transport from uplands to streams include mean basin slope, reservoirs, physiography, and soil permeability. On average, 59% of upland suspended sediment generated is temporarily stored along large rivers draining the Coastal Plain or in reservoirs throughout the watershed. Applying erosion and sediment controls from agriculture and urban development in areas of the northern Piedmont close to the upper Bay, where the combined effects of watershed characteristics on sediment transport have the greatest influence may be most helpful in mitigating sedimentation in the bay and its tributaries. Stream restoration efforts addressing floodplain and bank stabilization and incision may be more effective in smaller, headwater streams outside of the Coastal Plain. 相似文献
98.
Filling and cleaning of pesticide sprayers presents a potential risk of pollution of soil and water. Three different solutions for handling sprayers have been suggested: Filling and cleaning in the field, filling and cleaning on hard surfaces with collection of the waste water, and filling and cleaning on a biobed, which is an excavation lined with clay and filled with a mixture of chopped straw, sphagnum and soil with turf on top, and with increased sorption capacity and microbial activity for degradation of the pesticides. In the present study the degradation and leaching of 21 pesticides (5 g of each) was followed in an established full-scale model biobed. Percolate was collected and analysed for pesticide residues, and the biobed material was sampled at three different depths and analysed by liquid chromatography double mass spectrometry (LC-MSMS). During the total study period of 563 days, no traces of 10 out of 21 applied pesticides were detected in the percolate (detection limits between 0.02 and 0.9 μg l−1) and three pesticides were only detected once and at concentrations below 2 μg l−1. During the first 198 days before second application, 14% of the applied herbicide bentazone was detected in the leachate with maximum and mean concentrations of 445 and 172 μg l−1, respectively. About 2% of the initial mecoprop and fluazifop dose was detected in the percolate, with mean concentrations of 23 μg l−1, while MCPA and dimethoate had mean concentrations of 3.5 and 4.7 μg l−1, respectively. Leachate concentrations for the remaining pesticides were generally below the detection limit (0.02–0.9 μg l−1, below 1% of applied). Sorption studies of five pesticides showed that compounds with a low Kd value appeared in the leachate. After 169 days, all pesticides in the biobed profile were degraded to a level below 50% of the calculated initial dose. Pesticides with Koc values above 100 were primarily found in the uppermost 10 cm and degraded slowest due to the low bioavailability. The 11 most degradable pesticides were all degraded such that less than 3% remained in the biobed after 169 days.
Following second pesticide application of the biobed, leachate was sampled 215 and 365 days after the treatment. This showed the same pesticides to be leached out and at concentrations comparable to those of the first treatment. The same pesticides as after the first treatment were retained in the biobed. 相似文献
99.
Root uptake of enteric pathogens and subsequent internalization has been a produce safety concern and is being investigated as a potential route of pre-harvest contamination. The objective of this study was to determine the ability of hepatitis A virus (HAV) and the human norovirus surrogate, murine norovirus (MNV), to internalize in spinach and green onions through root uptake in both soil and hydroponic systems. HAV or MNV was inoculated into soil matrices or into two hydroponic systems, floating and nutrient film technique systems. Viruses present within spinach and green onions were detected by RT-qPCR or infectivity assays after inactivating externally present viruses with Virkon®. HAV and MNV were not detected in green onion plants grown up to 20 days and HAV was detected in only 1 of 64 spinach plants grown in contaminated soil substrate systems up to 20 days. Compared to soil systems, a drastic difference in virus internalization was observed in hydroponic systems; HAV or pressure-treated HAV and MNV were internalized up to 4 log RT-qPCR units and internalized MNV was shown to remain infectious. Understanding the interactions of human enteric viruses on produce can aid in the elucidation of the mechanisms of attachment and internalization, and aid in understanding risks associated with contamination events. 相似文献
100.