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111.
Occurrence of halogenated disinfection by-products (DBPs) (trihalomethanes –THMs– and haloacetic acids –HAAs–) in the waters
of two utilities in Quebec City (Canada) was investigated using two approaches: experimental chlorination studies and full-scale
sampling within distribution systems. Experimental studies were designed to reproduce treatment plant and distribution system
conditions (chlorine dose, water temperature, pH and water residence time). Differences in halogenated DBPs in the two distribution
systems under study were significant and comparable to those observed in experimental laboratory studies. For the waters of
both utilities, chlorination studies better reproduced the occurrence of halogenated DBPs in points of the distribution system
located near the treatment plant (low residence time of water) than in other points. Multivariate regression models for THMs,
HAAs and their species were developed using the data from experimental studies in order to predict halogenated DBP levels
measured in the distribution system. Models were all statistically significant, but showed low ability to predict full-scale
halogenated DBPs, particularly in points located at distribution system extremities. Specifically, experimental chlorination-based
models are not able to simulate the decrease of HAA levels. Results of this research suggest that the use of experimental
data to predict halogenated DBP levels in full-scale distribution systems – for operational, regulatory and epidemiological
purposes – must be done with caution. 相似文献
112.
The clearing of forests to obtain land for pasture and agriculture and the replacement of autochthonous species by other faster-growing varieties of trees for timber have both led to the loss of vast areas of forest worldwide. At present, many developed countries are attempting to reverse these effects, establishing policies for the restoration of older woodland systems. Reforestation is a complex matter, planned and carried out by experts who need objective information regarding the type of forest that can be sustained in each area. This information is obtained by drawing up feasibility models constructed using statistical methods that make use of the information provided by morphological and environmental variables (height, gradient, rainfall, etc.) that partially condition the presence or absence of a specific kind of forestation in an area. The aim of this work is to construct a set of feasibility models for woodland located in the basin of the River Liébana (NW Spain), to serve as a support tool for the experts entrusted with carrying out the reforestation project. The techniques used are multilayer perceptron neural networks and support vector machines. Their results will be compared to the results obtained by traditional techniques (such as discriminant analysis and logistic regression) by measuring the degree of fit between each model and the existing distribution of woodlands. The interpretation and problems of the feasibility models are commented on in the Discussion section. 相似文献
113.
Lucía Emilia Iglesias Carlos Saumell Federica Sagüés Juan Manuel Sallovitz Adrián Luis Lifschitz 《Journal of environmental science and health. Part. B》2018,53(1):42-48
The aim of this work was to evaluate the fate of ivermectin (IVM) at two concentrations in cattle feces and its movement to the nearby soil and plants. Feces were spiked with IVM at two levels: 3000 ng g?1 (high group, HG) and 300 ng g?1 (low group, LG). Artificial dung pats were prepared and deposited in an experimental field area. Feces and underlying soil were sampled up to 60 days post-deposition (dpd). As an additional analysis, grasses growing around the pats were sampled at 30 and 60 dpd. Ivermectin concentrations in all matrices were determined by HPLC. Mean IVM fecal concentrations were in the range between 3901.9 ng g?1 and 2419.2 ng g?1 (high group) and 375.3 ng g?1 and 177.49 ng g?1 (low group). Mean times for 50% and 90% dissipation were 88.23 and 293.03 days (HG) and 39.1 and 129.9 days (LG). Soil concentrations ranged from 26.1 ng g?1 to 71.1 ng g?1 (HG) and 3.4 to 5.9 ng g?1 (LG); in plants, concentrations were between 71.4 and 380.8 ng g?1 and 5.40 and 51.8 ng g?1 in HG and LG, respectively. These results confirm that IVM moves from feces to the underlying soil as well as to nearby plants. The potential risk of detrimental effects on soil organisms and the impact on herbivorous animals should be further evaluated. 相似文献
114.
Ariane Maciel Neiva Marco Aurelio Sperança Vinicius Câmara Costa Manuel Antonio Chagas Jacinto Edenir Rodrigues Pereira-Filho 《Environmental monitoring and assessment》2018,190(10):618
The tanning industry is one of the largest environmental polluters due to high generation waste in all production processes, but the tanning is particularly worrisome due to the use of significant amounts of chromium. Cr is an element potentially toxic to both health and the environment, depending on the concentration and the oxidation state. Cr(VI) can come in contact with human skin when using leather goods, which can cause allergies and dermatitis, besides being carcinogenic. Considering that approximately 90% of the world production of leather is performed with Cr salts, the determination of this element in leather is necessary to avoid exposure to the risks that the element can provide. The main goal of this study was the development of an alternative analytical method for the determination of Cr in leathers (ovine and bovine leather tanned with Cr and vegetable tannin) using wavelength dispersive X-ray fluorescence (WDXRF) for direct solid analysis. Besides performing analysis of the chemical composition and determination of Al, As, Ba, Ca, Cd, Cr, Cu, Fe, Mg, Ni, Pb, Sb, Sr, Ti, and Zn in leather by inductively coupled plasma optical emission spectrometry (ICP OES). Principal component analysis (PCA) was also used in the evaluation of the WDXRF and ICP OES data sets. WDXRF calibration models for Cr presented satisfactory figures of merit and the analysis of the leathers revealed an alarming concentration of total Cr in the samples reaching 21,353 mg kg?1. 相似文献
115.
Gredilla Ainara Fdez-Ortiz de Vallejuelo Silvia Gomez-Nubla Leticia Carrero Jose Antonio de Leão Felipe B. Madariaga Juan Manuel Silva Luis F. O. 《Environmental science and pollution research international》2017,24(31):24333-24345
Environmental Science and Pollution Research - In city playgrounds, there is a potential risk of harming children’s health by contamination coming from anthropogenic activities. With the aim... 相似文献
116.
This paper analyses the relationship between nitrous oxide (N2O) emissions, economic growth, agricultural land used and exports in Germany. We use time‐series data between 1970 and 2012 and the Autoregressive Distributed Lag (ARDL) methodology to test for cointegration in the long run. Results show that there is a quadratic long run relationship between N2O emissions and economic growth, confirming the existence of an Environmental Kuznets Curve (EKC) for Germany. Agricultural land area affects N2O emissions positively, whereas exports affect emissions negatively. The turning point is $27,880, which is within the sample and implies that Germany is in the decreasing part of the curve of environmental degradation. The paper shows that, contrary to testing the EKC in less developed countries, mitigation of N2O emissions does not negatively affect growth in Germany. As such, it is feasible to undertake any conservative policy in order to reduce emissions without major consequences on economic sectors. 相似文献
117.
Joyotee Smith Manuel Winograd Gilberto Gallopin Douglas Pachico 《Environmental Modeling and Assessment》1998,3(1-2):31-46
While many government policies stimulating deforestation have been reversed, private sector lobbies for uncontrolled logging and soybean export corridors threaten the Amazon. Under a favorable scenario (macroeconomic stabilization, controlled logging and road building, sustainable technologies, global environmental markets) reconversion of natural habitat could be 30% lower than under unfavorable policies and technologies, without sacrificing production. 相似文献
118.
Buanuam J Tiptanasup K Shiowatana J Miró M Harald Hansen E 《Journal of environmental monitoring : JEM》2006,8(12):1248-1254
A continuous-flow system comprising a novel, custom-built extraction module and hyphenated with inductively coupled plasma-mass spectrometric (ICP-MS) detection is proposed for assessing metal mobilities and geochemical associations in soil compartments as based on using the three step BCR (now the Measurements and Testing Programme of the European Commission) sequential extraction scheme. Employing a peristaltic pump as liquid driver, alternate directional flows of the extractants are used to overcome compression of the solid particles within the extraction unit to ensure a steady partitioning flow rate and thus to maintain constant operationally defined extraction conditions. The proposed flow set-up is proven to allow for trouble-free handling of soil samples up to 1 g and flow rates < or =10 mL min(-1). The miniaturized extraction system was coupled to ICP-MS through a flow injection interface in order to discretely introduce appropriate extract volumes to the detector at a given time and with a given dilution factor. The proposed hyphenated method demonstrates excellent performance for on-line monitoring of major and trace elements (Ca, Mn, Fe, Ni, Pb, Zn and Cd) released when applying the various extracting reagents as addressed in the BCR scheme, that is, 0.11 M CH(3)COOH, 0.1 NH(2)OH.HCl and 30% H(2)O(2), even when a well recognized matrix-sensitive detector, such as ICP-MS, is used. As a result of the enhanced temporal resolution of the ongoing extraction, insights into the breaking down of phases and into the kinetics of the metal release are obtained. With the simultaneous multielement detection capability of ICP-MS, the dynamic fractionation system presents itself as an efficient front-end for evaluation of actual elemental association by interelement comparison of metals leached concurrently during the extraction time. Thus, the intimate elemental association between Cd and Zn in contaminated soils could be assessed. 相似文献
119.
Thermodynamic analysis of the energy recovery from the aerobic bioconversion of solid urban waste organic fraction 总被引:1,自引:0,他引:1
Waste management is of the utmost importance for many countries and especially for highly developed ones due to its implications on society. In particular, proper treatment before disposal of the solid urban waste organic fraction is one of the main issues that is addressed in waste management. In fact, the organic fraction is particularly reactive and if disposed in sanitary landfills without previous adequate treatment, a large amount of dangerous and polluting gaseous, liquid and solid substances can be produced. Some waste treatment processes can also present an opportunity to produce other by-products like energy, recycled materials and other products with both economic and environmental benefits. In this paper, the aerobic treatment of the organic fraction of solid urban waste, performed in a biocell plant with the possibility of recovering heat for civil or industrial needs, was examined from the thermodynamic point of view. A theoretical model was proposed both for the biological process of the organic fraction, as well as for the heat recovery system. The most significant results are represented and discussed. 相似文献
120.
Awareness of groundwater protection has increased substantially in recent decades. In the Province of Quebec, Canada, the Groundwater Catchment Regulation (GWCR) was promulgated in 2002 to protect water quality in public wells. The goal of the present study was to document groundwater protection in the context of emerging regulations and identify factors explaining the propensity of municipalities applying protection strategies. Two types of information were used in this study: data from a questionnaire-based survey conducted among 665 municipalities in the Province of Quebec and complementary information gathered from various sources. Data from the survey revealed that fewer than half of the municipalities have been able to comply with the GWCR, mainly because of financial limitations. Also, close to half of the municipalities have either identified or are expecting land use conflicts to arise between protection areas required by the GWCR and other land usage, with agriculture being the main conflicting activity. Multivariate logistic regression models served to identify factors explaining the likelihood of municipalities to take groundwater protection measures. Those factors were municipality revenue, history of water contamination in distribution systems, land use near wellheads, location of municipalities within a provincial priority watershed and the importance of groundwater use in a region. Results of the study may prove helpful for government authorities in better understanding the groundwater protection issue and in implementing strategies that improve the ability of municipalities to protect groundwater. 相似文献