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571.
Sorption and desorption of sulfadiazine in soil and soil-manure systems 总被引:10,自引:0,他引:10
Sulfadiazine is a widely used veterinary medicine that has high potential to enter the environment, especially the soil compartment by the application of manure on agricultural land and grass land or by the deposition of dung pats on pasture. Once it reaches the soil environments, it may enter into surface and ground water. Therefore, sorption-desorption behavior of sulfadiazine was studied under laboratory conditions in five different soils varying in their physicochemical properties. A batch equilibration technique was used with initial aqueous solution concentration of sulfadiazine at 5, 0.5, 0.05, and 0.005 microg mL(-1). Sorption-desorption data in soils with and without manure were well fitted with Freundlich model in log form (r(2), 0.99). A sorption-desorption hysteresis effect was apparent in all soils. A significant amount of sulfadiazine was found tightly bound to the soil particles and did not desorb after the desorption process. Moreover, presence of manure enhanced hysteresis effect. Hysteresis coefficient (H) value from soils in absence of manure (0.9-1.0) increased to the soils in presence of manure (0.9-1.8). Soils in the absence of manure showed low level of K(D Sorp.) values ranging from 0.1 to 24.3, suggesting low level sorption of sulfadiazine with appreciable risk of run-off and leaching, and in turn, surface and ground water contamination. However, presence of manure increased the sorption tendency of sulfadiazine significantly (K(D Sorp.), 6.9-40.2). K(D) values pertaining to desorption cycle increased from 1.2-90.4 to 10.4-167.3 in absence and presence of manure, respectively. 相似文献
572.
The degradation of bitertanol by ozone treatment is investigated. Solutions of bitertanol (8.4 μg mL?1) were prepared either by dissolution of the standard or by dilution of Gaucho Blé seed loading solution and then ozonated under different conditions. Evolution of the concentrations of bitertanol and its ozonation by-products in both solutions was monitored by HPLC–UV as a function of the treatment time for a concentration of 100 g m?3 of ozone in the inlet gas. Bitertanol degradation was found to follow a pseudo-first order reaction in both cases. However, the rate of the reaction in diluted seed loading solution was much lower (0.19 vs. 0.27 min?1 in standard solution) and was close to the reaction rate observed in the presence of a radical scavenger, tert-butanol (0.11 min?1). Thus, it may be suggested that additives present in the seed loading solution may play the role of radical scavengers. Study of ozone concentration in the inlet gas (from 25 to 100 g m?3) showed that ozone degradation is also a first-order reaction with respect to ozone. Four ozonation by-products were highlighted, collected and identified by HPLC coupled with an ion trap mass spectrometer using positive electrospray ionization mode. A degradation pathway of bitertanol was finally proposed. 相似文献
573.
Crini Grégorio Cosentino Cesare Bradu Corina Fourmentin Marc Torri Giangiacomo Ruzimuradov Olim Alaton Idil Arslan Tomei Maria Concetta Derco Ján Barhoumi Mondher Prosen Helena Malinović Borislav N. Vrabeľ Martin Huq Mohammad Mahmudul Soltan Jafar Lichtfouse Eric Morin-Crini Nadia 《Environmental Chemistry Letters》2022,20(4):2597-2628
Environmental Chemistry Letters - Alkylphenols and alkylphenol polyethoxylates are emerging hazardous contaminants due in particular to their endocrine-disrupting properties. These compounds... 相似文献
574.
Morin-Crini Nadia Lichtfouse Eric Fourmentin Marc Ribeiro Ana Rita Lado Noutsopoulos Constantinos Mapelli Francesca Fenyvesi Éva Vieira Melissa Gurgel Adeodato Picos-Corrales Lorenzo A. Moreno-Piraján Juan Carlos Giraldo Liliana Sohajda Tamás Huq Mohammad Mahmudul Soltan Jafar Torri Giangiacomo Magureanu Monica Bradu Corina Crini Grégorio 《Environmental Chemistry Letters》2022,20(2):1333-1375
Environmental Chemistry Letters - The rise of emerging contaminants in waters challenges the scientific community and water treatment stakeholders to design remediation techniques that are simple,... 相似文献