全文获取类型
收费全文 | 1361篇 |
免费 | 13篇 |
国内免费 | 7篇 |
专业分类
安全科学 | 38篇 |
废物处理 | 67篇 |
环保管理 | 136篇 |
综合类 | 138篇 |
基础理论 | 265篇 |
环境理论 | 3篇 |
污染及防治 | 502篇 |
评价与监测 | 130篇 |
社会与环境 | 97篇 |
灾害及防治 | 5篇 |
出版年
2023年 | 14篇 |
2022年 | 35篇 |
2021年 | 37篇 |
2020年 | 16篇 |
2019年 | 23篇 |
2018年 | 14篇 |
2017年 | 27篇 |
2016年 | 52篇 |
2015年 | 53篇 |
2014年 | 82篇 |
2013年 | 149篇 |
2012年 | 99篇 |
2011年 | 97篇 |
2010年 | 64篇 |
2009年 | 67篇 |
2008年 | 88篇 |
2007年 | 69篇 |
2006年 | 80篇 |
2005年 | 49篇 |
2004年 | 44篇 |
2003年 | 38篇 |
2002年 | 53篇 |
2001年 | 25篇 |
2000年 | 8篇 |
1999年 | 11篇 |
1998年 | 9篇 |
1997年 | 10篇 |
1996年 | 11篇 |
1995年 | 10篇 |
1994年 | 10篇 |
1993年 | 6篇 |
1992年 | 3篇 |
1991年 | 4篇 |
1990年 | 5篇 |
1989年 | 2篇 |
1986年 | 2篇 |
1983年 | 2篇 |
1982年 | 2篇 |
1981年 | 1篇 |
1977年 | 2篇 |
1976年 | 1篇 |
1975年 | 1篇 |
1973年 | 1篇 |
1966年 | 1篇 |
1965年 | 1篇 |
1964年 | 1篇 |
1958年 | 1篇 |
1956年 | 1篇 |
排序方式: 共有1381条查询结果,搜索用时 312 毫秒
51.
Romário J. da Silv Lizeth Carolina Mojica-Sánchez Filipe D.S. Gorz Graciela C. Pedro Bruna G. Maciel Gabriela P. Ratkovski Hérica D. da Roch Kamila T.O. do Nascimento Juan C. Medina-Llamas Alicia E. Chávez-Guajardo José J. Alcaraz-Espinoz Celso P. de Melo 《环境科学学报(英文版)》2021,33(2):62-73
We report the preparation of poly(3,4-ethylene dioxythiophene) (PEDOT)-modified polyvinylidene fluoride electrospun fibers and their use as a novel adsorbent material for the removal of the anionic dye Methyl Orange (MO) from aqueous media. This novel adsorbent material can be used to selectively remove MO on a wide pH range (3.0–10.0), with a maximum capacity of 143.8 mg/g at pH 3.0. When used in a recirculating filtration system, the maximum absorption capacity was reached in a shorter time (20 min) than that observed for batch mode experiments (360 min). Based on the analyses of the kinetics and adsorption isotherm data, one can conclude that the predominant mechanism of interaction between the membrane and the dissolved dye molecules is electrostatic. Besides, considering the estimated values for the Gibbs energy, and entropy and enthalpy changes, it was established that the adsorption process is spontaneous and occurs in an endothermic manner. The good mechanical and environmental stability of these membranes allowed their use in at least 20 consecutive adsorption/desorption cycles, without significant loss of their characteristics. We suggest that the physical-chemical characteristics of PEDOT make these hybrid mats a promising adsorbent material for use in water remediation protocols and effluent treatment systems. 相似文献
52.
Santos Luciane Cavalcante da Silva Anamália Ferreira dos Santos Lins Pollyanna Vanessa da Silva Duarte José Leandro Ide Alessandra Honjo Meili Lucas 《Environmental science and pollution research international》2020,27(6):5890-5900
Environmental Science and Pollution Research - Mg-Fe layered double hydroxide intercalated with chloride (Mg-Fe-Cl LDH) was synthetized, characterized, and evaluated as adsorbent to remove nitrate... 相似文献
53.
de Castro Lima José Augusto Monteiro Labanowski Jérôme Bastos Marília Camotti Zanella Renato Prestes Osmar Damian de Vargas Jocelina Paranhos Rosa Mondamert Leslie Granado Eugenie Tiecher Tales Zafar Mohsin Troian Alexandre Le Guet Thibaut dos Santos Danilo Rheinheimer 《Environmental science and pollution research international》2020,27(10):10581-10598
Environmental Science and Pollution Research - The total cultivated area in Brazil reached to 62 million ha in 2018, with the predominance of genetically modified soybean and corn (36 and 17... 相似文献
54.
Pompermaier Aline Kirsten Karina Soares Suelen Mendonça Fortuna Milena Kalichak Fabiana Idalencio Renan Koakoski Gessi Barreto Rodrigo Egydio Barcellos Leonardo José Gil 《Environmental science and pollution research international》2020,27(31):38559-38567
Environmental Science and Pollution Research - Due to human activities, there is an increasing presence of agrochemicals residues in water bodies, which could be attributed to an increased use of... 相似文献
55.
San Vicente Bay is a coastal shallow embayment in Central Chile with multiple uses, one of which is receiving wastewater from
industrial fisheries, steel mill effluents, and domestic sewage. A simulation model was developed and applied to dissolved
oxygen consumption by organic residues released into this embayment. Three compartments were established as function of: depth,
circulation and outfall location. The model compartments had different volumes, and their oxygen saturation value was used
as baseline. The parameters: (a) BOD5 of the industrial and urban effluents, (b) oxygen demand by organic sediments, (c) respiration, (d) photosynthesis and (e)
re-aeration were included in the model. Iteration results of the model showed severe alterations in Compartment 1, with a
decrease of 65% in the oxygen below saturation. Compartment 2 showed a small decline (10%) and compartment 3 did not show
apparent changes in oxygen values. Measures recommended for remediation were to decrease the BOD5 loading by 30% in the affected sector. Iteration of the model for 200 h following recommendations derived from the preceding
results produced an increase in saturation of 60% (5 ml O2 L−1), which suggested an improvement of the environmental conditions. 相似文献
56.
Maysa Venturoso Gongora Buckeridge Serra Paula Rezende Camargo José Eduardo Zaia Maria Georgina Marques Tonello 《International journal of occupational safety and ergonomics》2018,24(1):62-67
Background. The effect of physical exercise in the workplace (PEW) on health promotion of workers is contradictory. Objective. To evaluate the effects of the PEW in musculoskeletal disorders (MSDs), perception of stress and quality of life in workers. Methods. The participants were divided into two groups: control group (n?=?46) including non-participant workers of the PEW program, and PEW group (n?=?50) including workers who regularly participate in the exercise program. All workers answered the Nordic general questionnaire, the perceived stress scale and the quality-of-life questionnaire. Results. The PEW group reported a lower prevalence of MSDs for the trunk in the last 7 days and 12 months (p?=?0.021 and p?=?0.001, respectively), and for the upper limbs in the last 12 months (p?=?0.001) compared with the control group. The results for the perception of stress and quality of life showed no significant differences between the groups. Conclusion. PEW is a potential method to reduce MSDs in workers, but it was not efficient in reducing stress levels or improving the quality of life of the workers. 相似文献
57.
André Berton Michelle F. Brugnera 《Journal of environmental science and health. Part. B》2018,53(4):237-245
In this study, the quality of surface water in the headwaters of São Lourenço River in Mato Grosso, Brazil, was evaluated in relation to contamination by pesticides. For this purpose, samples were collected between December 2015 and June 2016 by grab sampling and by passive sampling using an integrative polar organic compound sampler installed in the field during four 14-day cycles between March and June 2016. The analyses were performed by gas chromatography (CG/MS) and by liquid chromatography (UPLC-MS/MS). The results showed the detection of two pesticides (atrazine and pyraclostrobin) of the five analyzed by passive sampling and eight active principles among the 20 analyzed (malathion, diuron, carbofuran, carbendazim, trifluralin, imidacloprid, metolachlor, and acetamiprid) by grab sampling. The detection of 10 pesticides, even almost a decade after the beginning of a recovery process of the ciliary forest, confirms the headwaters' vulnerability to these contaminants and passive sampling proved to be an important tool in capturing small concentrations of pesticides constituting an interesting complement to grab sampling. 相似文献
58.
Aziz Azri Galal Elmanfe René Olier Mireille Privat 《Atmospheric environment (Oxford, England : 1994)》2010,44(39):5211-5217
From a literature-based assessment of the current knowledge about both the toxic or salutary properties of copper, this study focused on the determination, at 25 °C, of the interfacial properties of CuCl2, either alone or in mixture with carbofuran used, here, as a model of organics and/or pesticide. The interfaces under study were: i) the air/solution interface and ii) the silica/solution interface. The former is considered as a path for volatilization, whereas the latter permits a modelling of physical adsorption upon solids, which is the first and unavoidable step in any adsorption process. One should note that it can also mimic adsorption on some sandy soils. Coadsorption was clearly identified as implicated in an enhancement of the surface content of both solutes at both interfaces. However, at the two interfaces under study, the way the surface became structured led to opposite adsorption mechanisms for the organic compounds and the salt. A rough theory about ionic adsorption is also proposed. 相似文献
59.
Kärrman Anna Domingo José L. Llebaria Xavier Nadal Martí Bigas Esther van Bavel Bert Lindström Gunilla 《Environmental science and pollution research international》2010,17(3):750-758
Background, aim and scope
Perfluorinated compounds (PFCs) are global environmental pollutants that bioaccumulate in wildlife and humans. Laboratory experiments have revealed toxic effects such as delayed development, humoral suppression, and hepatotoxicity. Although numerous human blood levels have been reported, little is known about distribution in the human body. Knowledge about PFC distribution and accumulation in the human body is crucial to understanding uptake and subsequent effects as well as to conduct risk assessments. The present study reports PFC levels in human liver and breast milk from a general population living in Catalonia, Spain. Liver and milk levels are compared to previously reported levels in blood from the same geographic area as well as to other existing reports on human liver and milk levels in other countries. 相似文献60.
Alexandre Joly Audrey Smargiassi Tom Kosatsky Michel Fournier Ewa Dabek-Zlotorzynska Valbona Celo David Mathieu René Servranckx Réal D'amours Alain Malo Jeffrey Brook 《Atmospheric environment (Oxford, England : 1994)》2010,44(34):4325-4329
Little is known about the level and content of exposure to fine particles (PM2.5) among persons who attend fireworks displays and those who live nearby. An evaluation of the levels of PM2.5 and their elemental content was carried out during the nine launches of the 2007 Montréal International Fireworks Competition. For each event, a prediction of the location of the firework plume was obtained from the Canadian Meteorological Centre (CMC) of the Meteorological Service of Canada. PM2.5 was measured continuously with a photometer (Sidepak?, TSI) within the predicted plume location (“predicted sites”), and integrated samples were collected using portable personal samplers. An additional sampler was located on a nearby roof (“fixed site”). The elemental composition of the collected PM2.5 samples from the “predicted sites” was determined using both a non-destructive energy dispersive ED-XRF method and an ICP-MS method with a near-total microwave-assisted acid digestion. The elemental composition of the “fixed site” samples was determined by the ICP-MS with the near-total digestion method. The highest PM2.5 levels reached nearly 10 000 μg m?3, roughly 1000 times background levels. Elements such as K, Cl, Al, Mg and Ti were markedly higher in plume-exposed filters. This study shows that 1) persons in the plume and in close proximity to the launch site may be exposed to extremely high levels of PM2.5 for the duration of the display and, 2) that the plume contains specific elements for which little is known of their acute cardio-respiratory toxicity. 相似文献