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71.
This review summarises and evaluates the present knowledge on the behaviour, the biological effects and the routes of uptake of silver nanoparticles (Ag NPs) to organisms, with considerations on the nanoparticle physicochemistry in the ecotoxicity testing systems used. Different types of Ag NP syntheses, characterisation techniques and predicted current and future concentrations in the environment are also outlined. Rapid progress in this area has been made over the last few years, but there is still a critical lack of understanding of the need for characterisation and synthesis in environmental and ecotoxicological studies. Concentration and form of nanomaterials in the environment are difficult to quantify and methodological progress is needed, although sophisticated exposure models show that predicted environmental concentrations (PECs) for Ag NPs in different environmental compartments are at the range of ng L(-1) to mg kg(-1). The ecotoxicological literature shows that concentrations of Ag NPs below the current and future PECs, as low as just a few ng L(-1), can affect prokaryotes, invertebrates and fish indicating a significant potential, though poorly characterised, risk to the environment. Mechanisms of toxicity are still poorly understood although it seems clear that in some cases nanoscale specific properties may cause biouptake and toxicity over and above that caused by the dissolved Ag ion. This review concludes with a set of recommendations for the advancement of understanding of the role of nanoscale silver in environmental and ecotoxicological research. 相似文献
72.
In March 2011, the Interstate Technology & Regulatory Council (ITRC) Contaminated Sediments Team published a web‐based Technical and Regulatory Guidance on the concepts, processes, and uses of bioavailability in a risk decision‐making framework at a contaminated sediment site. Bioavailability processes, as defined by the National Research Council (NRC; 2003), are the “individual physical, chemical, and biological interactions that determine the exposure of plants and animals to chemicals associated with soils and sediments.” Bioavailability assessment tools aid in the assessment of human and ecological exposure and development of site‐specific remedial objectives. The guidance provides information on the processes that may affect contaminant bioavailability within sediments to understand exposure within ecological and human receptors; supports the development of conceptual site models (CSMs); and describes available tools (biological, chemical, and physical) and models that are used to measure and characterize the fate and transport and potential bioavailability of contaminants. Case studies, referenced throughout the document, demonstrate the practical application of bioavailability measures. The guidance will describe the proper application of traditional and emerging sediment remediation technologies to support the selection of a remedy that is protective of human health and the environment. © 2013 Wiley Periodicals, Inc. 相似文献
73.
GIS and the Analytic Hierarchy Process for Regional Landfill Site Selection in Transitional Countries: A Case Study From Serbia 总被引:1,自引:0,他引:1
Zelenović Vasiljević T Srdjević Z Bajčetić R Vojinović Miloradov M 《Environmental management》2012,49(2):445-458
The Serbian National Waste Management Strategy for the Period 2010–2019, harmonized with the European Union Directives, mandates
new and very strict requirements for landfill sites. To enable analysis of a number of required qualitative and quantitative
factors for landfill site selection, the traditional method of site selection must be replaced with a new approach. The combination
of GIS and the Analytic Hierarchy Process (AHP) was selected to solve this complex problem. The Srem region in northern Serbia,
being one of the most environmentally sensitive areas, was chosen as a case study. Seventeen factors selected as criteria/sub-criteria
were recognized as most important, divided into geo-natural, environmental, social and techno-economic factors, and were evaluated
by experts from different fields using an AHP extension in Arc GIS. Weighted spatial layers were combined into a landfill
suitability map which was then overlapped with four restriction maps, resulting in a final suitability map. According to the results, 82.65% of the territory of Srem is unsuitable for regional landfill siting. The most suitable
areas cover 9.14%, suitable areas 5.24%, while areas with low and very low suitability cover 2.21 and 0.76% of the territory,
respectively. Based on these findings, five sites close to two large urban agglomerations were suggested as possible locations
for a regional landfill site in Srem. However, the final decision will require further field investigation, a public acceptance
survey, and consideration of ownership status and price of the land. 相似文献
74.
Quantitative threat analysis for management of an imperiled species: Chinook salmon (Oncorhynchus tshawytscha). 总被引:1,自引:0,他引:1
Jonathan M Hoekstra Krista K Bartz Mary H Ruckelshaus Jennifer M Moslemi Tamara K Harms 《Ecological applications》2007,17(7):2061-2073
Chinook salmon (Oncorhynchus tshawytscha) have declined dramatically across the Pacific Northwest because of multiple human impacts colloquially characterized as the four "H's": habitat degradation, harvest, hydroelectric and other dams, and hatchery production. We use this conceptual framework to quantify the relative importance of major threats to the current status of 201 Chinook populations. Current status is characterized by two demographic indices: population density and trend. We employ path analytic models and information theoretic methods for multi-model inference. Our results indicate that dams most strongly affect variation in population density, while harvest and hatchery production most strongly affect variation in population trend. Comparable results arise when the sample size of the analysis is reduced to 22 Chinook populations within a smaller region typical of the scale at which salmon recovery planning is conducted. Results from these threat analyses suggest that recovery strategies targeting specific demographic indices, and those considering natural and human-mediated interdependencies of major threats, are most likely to succeed. 相似文献
75.
In November 2002, the Prestige oil tanker was wrecked in front of Galician coast (NW of Spain), spilling near 63,000 tons of heavy oil until February 2003. Contamination produced was very extensive (70% of Galician beaches were reached by the oil) but heterogeneous, alternating intensely affected zones with neighbour locations where the repercussion was minimal. The objective of this study was to monitor sea environment contamination caused by Prestige oil spill during an 11-month period (August 2003-June 2004, nine samplings) in two locations of Galician coast with different geographical properties (Lira and Ancoradoiro beaches), by means of chemical determination of total polycyclic aromatic hydrocarbons (TPAH) in seawater, and using as exposure biomarker TPAH content in mussel (Mytilus galloprovincialis) tissues, and as effect biomarker DNA damage in mussel gills, evaluated by the comet assay. In addition, recovery ability of the mussels was determined after a 7-day stay in the laboratory. TPAH contents in seawater were very high in the earliest samplings, but then they maintained below 200 ng L(-)(1), similar to reference seawater. However, TPAH levels in mussel tissues were more variable: they increased again from January 2004, probably due to the adverse meteorological conditions that turned over the sea bottom and dispersed the oil accumulated in sediments. In most samplings, these levels decreased during the recovery stage. DNA damage in oil-exposed mussels was significantly higher than in reference mussels, both before and after the recovery phase, but they did not differ to one another. Comet tail length was slightly reduced during the recovery stage, indicative of a certain DNA repair in exposed mussels. This study showed up the importance of monitoring sea contamination events during an extended time, not only in evaluating the presence of the contaminants in the environment but also in determining their bioaccumulation and their effect on the exposed organisms. 相似文献
76.
Five centuries of mining and processing of mercury ore in the Idrija area have resulted in widespread contamination of different environmental compartments. Environmental impacts on a regional and local scale, caused by atmospheric emissions from the Idrija ore roasting plant, were established in the investigations of mercury spatial distribution in soil and attic dust in 160 km(2) area. Very high values were determined in the Idrijca River valley, and they decrease exponentially with the distance from Idrija. Mercury concentrations in attic dust are higher than in surrounding soils and the attic dust/soil ratio changes with distance. Measurements of mercury in the air confirmed widespread dispersion of mercury and showed highly elevated mercury concentrations around roasting plant and mine ventilation shaft. Beside, systematic monitoring of mercury contents in the stream sediments has demonstrated that huge amounts of mercury are stored in areas where ancient overbank sediments were deposited, and there was no decrease in mercury concentration in active sediments during the last 15 years. Recently, interesting and extremely polluted locations of historical small-scale roasting sites in the Idrija surroundings were discovered. Ongoing geochemical study aims to determine the extreme pollution and significance of these sites for wider contamination of soils and aquatic systems. Presented studies have shown that Hg mining in Idrija caused intense pollution of local and regional environment including the aquatic systems in the Gulf of Trieste, which is seen as the final sink of a major part of the Hg stored in soils and river sediments in the Idrija area. 相似文献
77.
Neural stem cell-based in vitro bioassay for the assessment of neurotoxic potential of water samples
Muhammad Irfan Masoo Natalie Tamara Hauke Muhammad Jawad Nasim Muhammad Sarfraz Mahrukh Naseem Karl Herbert Schäfer 《环境科学学报(英文版)》2021,33(3):72-86
Intensive agriculture activities, industrialization and growing numbers of wastewater treatment plants along river banks collectively contribute to the elevated levels of neurotoxic pollutants in natural water reservoirs across Europe. We established an in vitro bioassay based upon neural stem cells isolated from the subventricular zone of the postnatal mouse to evaluate the neurotoxic potential of raw wastewater, treated sewage effluent, groundwater and drinking water. The toxic potential of water samples was evaluated employing viability, proliferation, differentiation and migration assays. We found that raw wastewater could reduce the viability and proliferation of neural stem cells, and decreased the neuronal and astrocyte differentiation, neuronal neurite growth, astrocyte growth and cell migration. Treated sewage water also showed inhibitory effects on cell proliferation and migration. Our results indicated that relatively high concentrations of nitrogenous substances, pesticides, mercuric compounds, bisphenol-A, and phthalates, along with some other pollutants in raw wastewater and treated sewage water, might be the reason for the neuroinhibitory effects of these water samples. Our model successfully predicted the neurotoxicity of water samples collected from different sources and also revealed that the incomplete removal of contaminants from wastewater can be problematic for the developing nervous system. The presented data also provides strong evidence that more effective treatments should be used to minimize the contamination of water before release into major water bodies which may be considered as water reservoirs for human usage in the future. 相似文献
78.
Chiara Gambardella Tina Mesarič Tamara Milivojević Kristina Sepčić Lorenzo Gallus Serena Carbone Sara Ferrando Marco Faimali 《Environmental monitoring and assessment》2014,186(7):4249-4259
The aim was to investigate the toxicity of selected metal oxide nanoparticles (MO-NPs) on the brine shrimp Artemia salina, by evaluating mortality and behavioural and biochemical responses. Larvae were exposed to tin(IV) oxide (stannic oxide (SnO2)), cerium(IV) oxide (CeO2) and iron(II, III) oxide (Fe3O4) NPs for 48 h in seawater, with MO-NP suspensions from 0.01 to 1.0 mg/mL. Mortality and behavioural responses (swimming speed alteration) and enzymatic activities of cholinesterase, glutathione-S-transferase and catalase were evaluated. Although the MO-NPs did not induce any mortality of the larvae, they caused changes in behavioural and biochemical responses. Swimming speed significantly decreased in larvae exposed to CeO2 NPs. Cholinesterase and glutathione-S-transferase activities were significantly inhibited in larvae exposed to SnO2 NPs, whereas cholinesterase activity significantly increased after CeO2 NP and Fe3O4 NP exposure. Catalase activity significantly increased in larvae exposed to Fe3O4 NPs. In conclusion, swimming alteration and cholinesterase activity represent valid endpoints for MO-NP exposure, while glutathione-S-transferase and catalase activities appear to be NP-specific. 相似文献
79.
Karen Van de Vel Clemens Mensink Koen De Ridder Felix Deutsch Joachim Maes Jo Vliegen Artash Aloyan Alexander Yermakov Vardan Arutyunyan Tamara Khodzher Bas Mijling 《Environmental monitoring and assessment》2010,165(1-4):665-674
In this paper, we assess the status of the air quality in the Lake Baikal region which is strongly influenced by the presence of anthropogenic pollution sources. We combined the local data, with global databases, remote sensing imagery and modelling tools. This approach allows to inventorise the air-polluting sources and to quantify the air-quality concentration levels in the Lake Baikal region to a reasonable level, despite the fact that local data are scarcely available. In the simulations, we focus on the month of July 2003, as for this period, validation data are available for a number of ground-based measurement stations within the Lake Baikal region. 相似文献
80.
Ryunosuke Kikuchi Tamara T. Gorbacheva 《Environmental science and pollution research international》2009,16(4):431-438
Background, aim, and scope The Arctic holds large stores of minerals, and extracted materials are provided to the world’s economy; in this sense, the
Arctic issue associated with mining is not local but global. In a part of the Arctic region (the Kola Peninsula, 66–70° N
and 28–41° E), metal levels are generally elevated in the lake sediment. There is a question as to what results in elevated
metal levels—a natural process (naturally abundant minerals) or an anthropogenic process (mining and metallurgy). In terms
of solving this question, Staroe lake located on the Kola Peninsula was researched as a case study.
Materials and methods The following parameters were determined in relation with Staroe lake: (1) the current quality of the lake’s water—each 1,000-ml
sample was collected at a surface point and a deep point (near the bottom layer), and the collected samples were directly
analyzed after filtration; (2) atmospheric bulk deposition—bulk deposition was collected using a set of three rainwater samplers
near the lake. In addition, bulk deposition was collected in a background site (250 km to the southwest of the smelter complex)
as a reference; and (3) sediment profile (plus principal component analysis)—lake-bottom sediment was collected by an open-gravimetric
column sampler equipped with an automatic diaphragm. After collection, the sample columns were cut at a 1-cm interval for
analysis. Eigenvalues and variances by factor were calculated from the correlation coefficients.
Results The obtained data show that (1) naturally poor elements (Cu, Ni, Si, and SO4
2−) dominantly influence the lake’s water quality; (2) they are transported from the anthropogenic sources to the study lake
through the atmospheric pathway; (3) mainly the contents of Cu, Ni, Sr, and Ca have influenced the sediment quality since
the 1950s, corresponding to the industrial movement; and (4) Cu, Ni, and Sr originate from an anthropogenic source (smelter),
and Ca originates from both natural and anthropogenic sources.
Discussion As compared with the Russian standard (San Pin 2.1.980–00), the contents of NO3
− (50.3 ± 0.1 mg l−1) and particulates (2.3 ± 0.2 mg l−1) exceeded the standard levels (0.7 mg l−1 NO3
− and 45 mg l−1 particulates); Staroe lake may be slightly contaminated. However, the contamination factor (comparison with the background
data) implies that Staroe lake is considerably contaminated. There is a strong possibility that fine overburden detritus (<0.1 mm
diameter) may be transported from an open pit to the study lake by natural forces such as wind. Although it is difficult to
suppose that one factor dominantly affects the sediment quality, it follows from a factor analysis that factors 1 and 2 account
for about 70% of the total variance: Factor 1 is the most dominant, and factor 2 is the second most dominant in the variability
of sediment quality. It is considered that Cu, Sr, and Ni in factor 1 originate from anthropogenic sources because they are
poor in sediment rocks.
Conclusions The field survey conducted in Staroe lake can give the following answers to the key objectives: (1) The present water quality
is affected by Cu, Ni, Si, and SO4
2− in light of the contamination factor, and these elements originate from anthropogenic sources (the smelter and the open pit)
and are transported to the lake through the atmospheric pathway; (2) the sediment profile and statistic analysis show that
the lake quality has been influenced by deposition of metals since the 1950s; and (3) Cu, Ni, Sr, and Ca have influenced the
sediment quality in light of the most dominant factor—Cu, Ni, and Sr originate from an anthropogenic source, whereas Ca comes
from both natural and anthropogenic sources.
Recommendations and perspectives The presented lake survey shows that the dispersion of human-related pollutants via the atmospheric pathway takes place in
the Arctic region. If the current pollution continues without countermeasures, the high-latitude environment may lose its
original characteristics; hence, this subject is important when considering how to implement a wide range of environmental
protection measures in the Arctic. 相似文献