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121.
Ramos Bruno Carneiro João Gabriel M. Nagamati Leandro Issamu Teixeira Antonio Carlos S. C. 《Environmental science and pollution research international》2021,28(19):24023-24033
Environmental Science and Pollution Research - Solar-driven photocatalysis is a promising water-cleaning and energy-producing technology that addresses some of the most urgent engineering problems... 相似文献
122.
Study of the distribution of the polychlorinated biphenyls in the milk fat globule by supercritical fluid extraction 总被引:1,自引:0,他引:1
The distribution of polychlorinated biphenyls (PCBs) in the milk fat globule has been studied by sequential extraction of four different lipidic fractions from powdered full-fat milk with supercritical carbon dioxide. Extractions were carried out in the dynamic mode in the pressure range 13.6-23.3 MPa at a temperature of 50 degrees C. The levels of PCBs and short-chain triglycerides (SCT), medium-chain triglycerides (MCT) and long-chain triglycerides (LCT), as well as the cholesterol in these four supercritical fluid extraction (SFE) fractions were determined. Extracts obtained at lower pressures were found to be enriched in PCBs, SCT, MCT and cholesterol, while the concentrations of all these analytes decreased for subsequent extractions. Satisfactory quadratic correlations were found between the PCB and SCT and MCT levels (r2 in the range 0.9-0.999), and between the PCB and cholesterol levels (r2 in the range 0.8-0.999, except for PCB 105) determined in the SFE fractions. These results suggested a similar distribution of the PCBs and the cholesterol in the milk fat globule. This conclusion was also supported by the comparison of the PCBs and the cholesterol chemical structures as well as by the total PCB levels determined by SFE to those obtained by using different extraction methods. The classical requirement for the analysis of this kind of lipophilic pollutants of an exhaustive extraction of the lipids of the matrix to ensure their quantitative recovery has been revised. 相似文献
123.
Ricardo M. Trigo Alexandre M. Ramos Paulo J. Nogueira Filipe D. Santos Ricardo Garcia-Herrera Célia Gouveia Fátima E. Santo 《Environmental Science & Policy》2009,12(7):844-854
This paper analyses the impact of the 2003 European heatwave on excessive human mortality in Portugal, a country that presents a relatively high level of exposure to heatwave events. A total of 2399 excessive deaths are estimated in continental Portugal, which implies an increase of 58% over the expected deaths. When these values are split by gender, it is seen that women increase (79%), was considerably higher than that recorded for men (41%). The increment of mortality due to this heatwave was detected for all the 18 districts of the country, but its magnitude was significantly higher in the inner districts close to the Spanish border. When we split by gender all districts reveal significant mortality increments for women, while the impact in men's excess deaths is not significant over 3 districts. Several temperature derived indices were used and evaluated in their capacity to explain, at the regional level, the excessive mortality (ratio between observed and expected deaths) by gender. It is shown that the best relationship is found for the total exceedance of extreme days, an index combining the length of the heatwave and its intensity. Both variables hold a linear relationship with r = 0.79 for women and a poorer adjustment (r = 0.50) for men. Additionally, availability of mortality data split by age also allowed obtaining detailed information on the structure of the population in risk, namely by showing that statistically significant increments are concentrated in the last three age classes (45–64, 65–74 and 75 or more). The use of air conditioning systems in some Portuguese hospitals had a major impact on the decrease (up to 40%) in excessive mortality values. A finer approach is relevant for prevention strategies, since it allows to identify better the target population of any preventive strategy regional and national authorities may be interested to implement. 相似文献
124.
Miren Pena-Abaurrea Liesbeth Weijs Lourdes Ramos Nicoletta Borghesi Simonetta Corsolini Hugo Neels Ronny Blust Adrian Covaci 《Chemosphere》2009,76(11):1477-1482
In the present study, bioaccumulation potential of two pyrethroid insecticides, bifenthrin and permethrin, was measured using a Lumbriculus variegatus sediment bioaccumulation test. Two sediments differing in their physical characteristics and two different aging periods were tested. Desorption rates measured by Tenax extraction suggested that pyrethroids were bioavailable to L. variegatus, however bioavailability varied among chemicals, sediments and aging time, and was greater for permethrin than bifenthrin. The relatively low biota-sediment accumulation factor (BSAF) values resulted from the extensive biotransformation of pyrethroids by L. variegatus. Biotransformation capacity of L. variegatus to permethrin was further studied with a water-only exposure, and the percentage parent compound dropped to 36.0% after 14 d. These results indicated sediment-associated pyrethroids were bioavailable to L. variegatus, however bioaccumulation was limited because L. variegatus was capable of biotransforming the pyrethroids. 相似文献
125.
Relationship between occupational social class and exposure to organochlorine pesticides during pregnancy 总被引:2,自引:0,他引:2
Freire C Amaya E Fernández MF González-Galarzo MC Ramos R Molina-Molina JM Arrebola JP Olea N 《Chemosphere》2011,83(6):831-838
Background
Little evidence is available on the influence of socioeconomic factors on exposure to persistent organic pollutants, especially during vulnerable periods such as pregnancy and early life.Objective
To investigate the relationship of maternal social class with placental concentrations of organochlorine pesticides (OCPs) and their combined estrogenic activity measured with a biomarker of exposure.Methods
Exposure to 16 OCPs (DDTs, endosulfans, and seven other compounds) and the total effective xenoestrogenic burden (TEXB) were analyzed in placentas from a mother-child cohort. OCP concentrations were quantified by gas chromatography and mass spectrometry, and TEXB was assessed with the E-Screen bioassay. Social class was classified according to maternal occupation. Multivariate regression analysis was conducted to examine variations in pesticide exposure and TEXB as a function of maternal social class in 257 subjects.Results
Placental p,p′-DDT concentrations were higher in social classes III and IV than in classes I-II (the most affluent); concentrations of the sum of DDTs were higher in class IV; and exposure to the sum of endosulfans was greater in class III. HCB concentrations were higher among women in class IV than in classes I-II and among manual (classes III-V) than non-manual workers. However, the trend across social classes was only statistically significant for HCB. Social class significantly explained 10% of the variability in concentrations of the sum of endosulfans.Conclusion
There is a need to explore whether more disadvantaged populations suffer higher levels of exposure to pesticides or other environmental chemicals and how different social processes contribute to this exposure. 相似文献126.
PCDD/Fs and dioxin-like PCBs in sediment and biota from the Mondego estuary (Portugal) 总被引:1,自引:0,他引:1
The concentrations of 17 polychlorinated dibenzo-p-dioxins and furans (PCDD/Fs), and 12 dioxin-like polychlorinated biphenyls (dl-PCBs) were measured in sediment and key species as an initial investigation on PCDD/Fs and dl-PCBs contamination in the Mondego estuary (Portugal). The results demonstrated that the values of the total PCDD/Fs (∑PCDD/Fs) concentrations were considerably lower than those of the sum of dl-PCBs (∑dl-PCBs) in all the studied samples. Regarding the contribution of individual congeners, OCDD was the predominant PCDD/F and the mono-ortho PCB 118 and PCB 105 were the dominant PCBs in the majority of the samples. Our results suggest that PCDD/Fs and PCBs behave quite differently along the aquatic food web: ∑PCDD/Fs concentrations were lower in higher trophic-level organisms with fish presenting a distinct PCDD/Fs congeners profile; on the contrary, the higher ∑dl-PCBs values were found in upper-level biota, although not exclusively, and quite similar dl-PCBs congener profiles were observed in nearly all the studied species. 相似文献
127.
Fruit-vegetable and fish wastes were evaluated as potential feedstuffs for growing-finishing pigs. Wastes were collected from shops in the city of Salamanca (Spain) and their nutritional composition, mineral content and digestibility were determined. The dry matter of the wastes under study was relatively low (12% for fruit-vegetable waste and 26% for fish waste), but they presented all of the nutrient requirements for swine diets. The fish waste contained 58% crude protein, 22% ash, 19% ether extract and 1% crude fibre, whereas the fruit-vegetable waste contained 65% nitrogen free extract, 13% crude fibre, 12% crude protein, 8% ash and 2% ether extract. Waste digestibility decreased with temperature, and hence temperatures over 65 degrees C for fruit-vegetable waste and 105 degrees C for fish waste should not be used in the treatment to reduce the moisture and to ensure the microbiology quality. Therefore, two diets were formulated using linear programming. The analysed waste was included in approximately 20% of one of the diets, while another diet was formulated without any type of waste. These data showed that this part of biodegradable municipal waste could be managed as alternative feedstuffs in swine diets, reducing the amount of biodegradable municipal waste going to landfills. 相似文献
128.
The wedge sole Dicologlossa cuneata (Moreau, 1881) is a coastal species that lives along the inner shelf waters of the Gulf of Cadiz down to a depth of 115 m.
Its fishery, the size composition of the exploited population, and its reproduction have been studied on the basis of data
acquired from commercial statistics from 1984 to 1994 and from sampling carried out during 1993 and 1994. The relative abundance
of the species and its geographic and bathymetric distribution have been examined by analysis of four trawl surveys carried
out from 1992 to 1994. D. cuneata is captured mainly by the trawl fleet, and to a lesser extent by gillnet gears. Wedge sole fishery has a marked seasonality.
Size-frequency distributions from commercial samples and from bottom-trawl surveys are very similar, ranging from 12 to 26 cm
total body length (TL). D. cuneata is a “repeat-spawner”. Peak spawning is from January to May. Females attain sexual maturity at 18 cm TL, while sexually mature
males have been observed at 15 cm TL. The flexibility of the spawning strategy of D. cuneata throughout its distribution range is discussed. The scarcity of small specimens in the monthly samples and sequential spawning
throughout the year prevented the estimation of growth parameters by means of length-frequency analysis. D. cuneata is present in greatest abundances in the sandy–muddy bottoms of the Guadalquivir River mouth at 15 to 30 m depth. Its optimum
habitat coincides with the principal commercial fishing grounds. The possibility of reproductive vertical migration is discussed,
but more precise data are needed before a viable hypothesis can be made.
Received: 1 July 1997 / Accepted: 27 November 1997 相似文献
129.
Araújo Leylia K. F. Albuquerque Allan A. Ramos Weslley C. O. Santos Alef T. Carvalho Sandra H. V. Soletti João I. Bispo Mozart D. 《Environment, Development and Sustainability》2021,23(8):11732-11750
Environment, Development and Sustainability - The activated biochar is a carbonaceous material obtained from thermal degradation of biomass with high adsorption potential. On the other hand, the... 相似文献
130.
Fátima Espírito Santo Alexandre M. Ramos M. Isabel P. de Lima Ricardo M. Trigo 《Regional Environmental Change》2014,14(5):1765-1788
This study aims mostly at understanding seasonal variations in the intensity, frequency and duration of extreme precipitation events in mainland Portugal. For this purpose, selected precipitation indices that mainly focus on extremes were calculated at the seasonal scale for daily data recorded in the period 1941–2007 at 57 meteorological stations scattered across the area. These indices were explored for trends at the local and regional levels. The results show that there are marked changes in precipitation indices at the seasonal scale. Trends in spring and autumn precipitation have opposite signals. In spring, statistically significant drying trends are found together with a reduction in extremes. In autumn, wetting trends are detected for all indices, although overall they are not significant at the 5 % level. In addition, the relationship between seasonal extreme precipitation indices and atmospheric large-scale modes of low-frequency variability is analysed by means of a seasonal correlation analysis. Four modes of low-frequency variability are explored. Results confirm that, over mainland Portugal, the North Atlantic Oscillation is one of the most important teleconnection patterns in any season and the mode of variability that has the greatest influence on precipitation extremes in the area, particularly in the winter and autumn. 相似文献