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排序方式: 共有80条查询结果,搜索用时 15 毫秒
31.
James G. Edinger Morris H. McCutchan Paul R. Miller Bill C. Ryan Mark J. Schroeder Joseph V. Behar 《Journal of the Air & Waste Management Association (1995)》2013,63(11):882-886
On June 18, 19, and 20, 1970, two aircraft, a rawinsonde, two pibal stations, and four ground stations provided simultaneous samples of total oxidant, temperature, and winds up to 8000 ft in an area extending from Santa Monica, Calif., east to Redlands and north across the San Bernardino Mountains. It was shown that photochemical oxidant formed in the marine layer is vented up the slopes and over the crest of the San Bernardino Mountains during the day. Layers of high oxidant concentrations were detected above the inversion base, suggesting that some pollution is vented up the slopes and subsequently advected back to the south. The diurnal changes in the temperature inversion also contribute to the high concentration found above the inversion base. These processes result in multi-layers of pollution. The study suggests that oxidant air pollution is transported up to 80 mi to forested mountains, where severe damage to conifer species has been documented. 相似文献
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Mohamed Edali Raphael Idem Ahmed Aboudheir 《International Journal of Greenhouse Gas Control》2010,4(2):143-151
The kinetics of the reaction between carbon dioxide (CO2) and mixed solutions of methyldiethanolamine (MDEA) and piperazine (PZ) was investigated experimentally in a laminar jet apparatus. The experimental kinetic data were obtained under no interfacial turbulence and over a temperature range from 313 to 333 K, MDEA/PZ wt% concentration ratios of 27/3, 24/6 and 21/9, and CO2 loadings from 0.0095 to 0.33 mol CO2/mol amine. In addition, a new absorption-rate/kinetics model for the kinetics of the mixed of solvents was developed, which takes into account the coupling between chemical equilibrium, mass transfer, and all possible chemical reactions involved in the CO2 reaction with MDEA/PZ solvent. The partial differential equations of this model were solved by the finite element numerical method (FEM) based on COMSOL software. The obtained experimental kinetics data were used to obtain the kinetic parameters of CO2 absorption into MDEA/PZ solutions. The reaction-rate constant obtained for PZ blended with MDEA was kPZ = 2.572 × 1012 exp(?5211/T). The 2D model for the blended amines MDEA/PZ has revealed the concentration profiles of all the species in both the radial and axial directions of the laminar jet which has enabled a better understanding of the correct sequence in which the reaction steps involved in the reactive absorption of CO2 in aqueous mixed MDEA/PZ solution occur. It also revealed that PZ may be depleted by the time the solvent blend of MDEA/PZ with a loading greater than 0.015 mol/mol amine is exposed to CO2 from the top of the laminar jet absorber. 相似文献
33.
Teerawat Sanpasertparnich Raphael Idem Irene Bolea David deMontigny Paitoon Tontiwachwuthikul 《International Journal of Greenhouse Gas Control》2010,4(3):499-510
Post-combustion CO2 capture and storage (CCS) presents a promising strategy to capture, compress, transport and store CO2 from a high volume–low pressure flue gas stream emitted from a fossil fuel-fired power plant. This work undertakes the simulation of CO2 capture and compression integration into an 800 MWe supercritical coal-fired power plant using chemical process simulators. The focus is not only on the simulation of full load of flue gas stream into the CO2 capture and compression, but also, on the impact of a partial load. The result reveals that the energy penalty of a low capture efficiency, for example, at 50% capture efficiency with 10% flue gas load is higher than for 90% flue gas load at the equivalent capture efficiency by about 440 kWhe/tonne CO2. The study also addresses the effect of CO2 capture performance by different coal ranks. It is found that lignite pulverized coal (PC)-fired power plant has a higher energy requirement than subbituminous and bituminous PC-fired power plants by 40.1 and 98.6 MWe, respectively. In addition to the investigation of energy requirement, other significant parameters including energy penalty, plant efficiency, amine flow rate and extracted steam flow rate, are also presented. The study reveals that operating at partial load, for example at half load with 90% CO2 capture efficiency, as compared with full load, reduces the energy penalty, plant efficiency drop, amine flow rate and extracted steam flow rate by 9.9%, 24.4%, 50.0% and 49.9%, respectively. In addition, the effect of steam extracted from different locations from a series of steam turbine with the objective to achieve the lowest possible energy penalty is evaluated. The simulation shows that a low extracted steam pressure from a series of steam turbines, for example at 300 kPa, minimizes the energy penalty by up to 25.3%. 相似文献
34.
Raphael A. Lavoie Louise Champoux David R.S. Lean 《Environmental pollution (Barking, Essex : 1987)》2010,158(6):2189-2199
Concentrations of organochlorines (OCs), brominated flame retardants (BFRs) and mercury (Hg) were measured in eggs of six seabird species breeding in the Gulf of St. Lawrence, Canada. Stable nitrogen (δ15N) and carbon (δ13C) isotopes were used as ecological tracers to measure trophic level and connectivity with benthos, respectively. Concentrations, patterns as well as ecological tracers varied significantly between species. The sum of polychlorinated biphenyls (ΣPCBs) was the most important group measured in all seabird species based on concentration followed generally by the sum of chlorinated pesticides (ΣCPs), the sum of brominated flame retardants (ΣBFRs) and finally total Hg (THg). ΣPCBs, ΣCPs and ΣBFRs increased with trophic level, whereas THg did not. Only ΣBFRs increased with a higher connectivity with the benthos. Seabird species resident to the Great Lakes-St. Lawrence ecosystem showed higher Hg and BFR levels than migratory species. Molt patterns were used to explain variations of contaminant levels. 相似文献
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Joseph S. Wroblewski Trevor J. Bell Alison I. Copeland Evan N. Edinger Charles Yu Feng James D. Saxby David C. Schneider Jason M. Simms 《Journal of Cleaner Production》2009,17(3):424-430
Iceland scallop (Chlamys islandica) stocks in the North Atlantic are usually pulse harvested, resulting in boom and bust local landings. We describe an adaptive management strategy for a sustainable harvest of Iceland scallops in Gilbert Bay, a Marine Protected Area (MPA) of coastal Labrador. The current management plan for the MPA closes pristine scallop habitat, a practice that under favourable ocean conditions may lead to local reseeding. The community-based co-management structure for the MPA utilizes the local ecological knowledge of fishermen. Scallop harvesters are participating in research on the present state of the resource. Currently scallops are smaller near the mouth of the bay where fishing effort has been concentrated historically. The cooperation of fishers in enforcing area closures and in monitoring the scallop harvest may lead to a sustainable scallop fishery. 相似文献
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