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101.
Latawiec AE Swindell AL Reid BJ 《Environmental pollution (Barking, Essex : 1987)》2008,156(2):467-473
The evaluation of microbial availability of contaminants is of high importance for better reflecting the processes governing contaminant fate in soil and for establishing the risk associated with contaminated sites. A sub-critical water extraction technique was assessed for its potential to determine the microbially degradable fraction of [14C]phenanthrene-associated activity in two dissimilar soils at three different ageing times (14, 28 and 49 days). For the majority of determinations, no significant (p > 0.05) difference between sub-critical water-extracted 14C-activity at 160 °C and the fraction mineralized by catabolically active Pseudomonas sp. was observed. Collectively, the results suggested that the sub-critical water extraction technique was an appropriate technique for predicting the biodegradable fraction of phenanthrene-associated 14C-activity in dissimilar soils following increasing soil-contaminant contact time. 相似文献
102.
Hickman ZA Swindell AL Allan IJ Rhodes AH Hare R Semple KT Reid BJ 《Environmental pollution (Barking, Essex : 1987)》2008,156(3):1041-1045
This study sought to extend validation of a cyclodextrin based extraction method for the assessment of PAH-biodegradation potential to complex multi-contaminant matrices. To this end, four reference materials (RMs) were produced by blending, in different proportions, soils impacted with diesel, lubricating oil and spent oxide. These reference materials had modest ∑PAH (16 US EPA) concentrations that ranged from 5.6 ± 0.5 to 44.4 ± 4.5 mg kg−1. However, extractable petroleum hydrocarbon (EPH) concentrations were comparatively high (up to 2520 ± 204 mg kg−1). To complement these RMs, two further soils from a municipal gas plant (MGP) with highly elevated concentration of PAHs ranging from 877 ± 52 to 2620 ± 344 mg kg−1 were also tested. Results showed, regardless of matrix complexity, that PAH biodegradation within the four RM substrates, and two MGP soils correlated well with biodegradation predicted by hydroxypropyl-β-cyclodextrin (HPCD) extraction. 相似文献
103.
There is concern that elevated levels of selenium found in the source water of a newly formed wetland park in Las Vegas, Nevada,
may have detrimental effects on local wildlife. In this study, we collected and analyzed water samples monthly for a three
year period from the inflow and outflow of the system. We also gathered dominant aquatic plants and selected terrestrial plants
and analyzed the water and plant tissues (root, shoot, leaf and flower) for selenium by high resolution Inductively Coupled
Plasma Mass Spectrometer. Except for storm events and the introduction of an alternative low selenium content source water
during summer low-flow conditions, selenium in the water was relatively stable. The concentration in the outflow tended to
be slightly lower than the inflow. Concentrations of selenium in the dominant plant taxa in this wetlands were typical of
ecosystems in the western United States and varied by taxa, tissue type, localized conditions (e.g., contact with selenium-laden
water), and to a lesser extent, seasons. Selenium in the aquatic plant spiny naiad (Najas marina) was relatively high and may pose an ecological risk to wildlife during the late spring and summer. Additional work is underway
investigating aquatic food chain accumulations of selenium as well as mass balance of selenium in the system. 相似文献
104.
Estimating dissolved reactive phosphorus concentration in surface runoff water from major Ontario soils 总被引:1,自引:0,他引:1
Wang YT Zhang TQ Hu QC Tan CS O'Halloran IP Drury CF Reid DK Ma BL Ball-Coelho B Lauzon JD Reynolds WD Welacky T 《Journal of environmental quality》2010,39(5):1771-1781
Phosphorus (P) loss from agricultural land in surface runoff can contribute to eutrophication of surface water. This study was conducted to evaluate a range of environmental and agronomic soil P tests as indicators of potential soil surface runoff dissolved reactive P (DRP) losses from Ontario soils. The soil samples (0- to 20-cm depth) were collected from six soil series in Ontario, with 10 sites each to provide a wide range of soil test P (STP) values. Rainfall simulation studies were conducted following the USEPA National P Research Project protocol. The average DRP concentration (DRP30) in runoff water collected over 30 min after the start of runoff increased (p < 0.001) in either a linear or curvilinear manner with increases in levels of various STPs and estimates of degree of soil P saturation (DPS). Among the 16 measurements of STPs and DPSs assessed, DPS(M3) 2 (Mehlich-3 P/[Mehlich-3 Al + Fe]) (r2 = 0.90), DPS(M3)-3 (Mehlich-3 P/Mehlich-3 Al) (r2 = 0.89), and water-extractable P (WEP) (r2 = 0.89) had the strongest overall relationship with runoff DRP30 across all six soil series. The DPS(M3)-2 and DPS(M3)-3 were equally accurate in predicting runoff DRP30 loss. However, DPS(M3)-3 was preferred as its prediction of DRP30 was soil pH insensitive and simpler in analytical procedure, ifa DPS approach is adopted. 相似文献
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108.
Understanding antibiotic biodegradation is important to the appreciation of their fate and removal from the environment. In this research an Isotope Ratio Mass Spectrometry(IRMS)method was developed to evaluate the extent of biodegradation of the antibiotic,sulphanilamide, in contaminated groundwater. Results indicted an enrichment in δ~(13)C of8.44‰ from-26.56(at the contaminant source) to-18.12‰(300 m downfield of the source).These results confirm reductions in sulphanilamide concentrations(from 650 to 10 mg/L)across the contaminant plume to be attributable to biodegradation(56%) vs. other natural attenuation processes, such as dilution or dispersion(42%). To understand the controls on sulphanilamide degradation ex-situ microcosms assessed the influence of sulphanilamide concentration, redox conditions and an alternative carbon source. Results indicated, high levels of anaerobic capacity(~50% mineralisation) to degrade sulphanilamide under high(263 mg/L), moderate(10 mg/L) and low(0.02 mg/L) substrate concentrations. The addition of electron acceptors; nitrate and sulphate, did not significantly enhance the capacity of the groundwater to anaerobically biodegrade sulphanilamide. Interestingly, where alternative carbon sources were present, the addition of nitrate and sulphate inhibited sulphanilamide biodegradation. These results suggest, under in-situ conditions, when a preferential carbon source was available for biodegradation, sulphanilamide could be acting as a nitrogen and/or sulphur source. These findings are important as they highlight sulphanilamide being used as a carbon and a putative nitrogen and sulphur source, under prevailing iron reducing conditions. 相似文献
109.
Principal components analysis (PCA) is a multivariate statistical technique capable of discerning patterns in large environmental datasets. Although widely used, there is disparity in the literature with respect to data pre-treatment prior to PCA. This research examines the influence of commonly reported data pre-treatment methods on PCA outputs, and hence data interpretation, using a typical environmental dataset comprising sediment geochemical data from an estuary in SE England. This study demonstrated that applying the routinely used log (x + 1) transformation skewed the data and masked important trends. Removing outlying samples and correcting for the influence of grain size had the most significant effect on PCA outputs and data interpretation. Reducing the influence of grain size using granulometric normalisation meant that other factors affecting metal variability, including mineralogy, anthropogenic sources and distance along the salinity transect could be identified and interpreted more clearly. 相似文献
110.
Doug Beare Franz Hölker Georg H. Engelhard Eddie McKenzie David G. Reid 《Die Naturwissenschaften》2010,97(9):797-808
Marine protected areas (MPAs) are attaining increasing importance in the management of marine ecosystems. They are effective
for conservation in tropical and subtropical areas (mainly coral and rocky reefs), but it is debated whether they are useful
in the management of migratory fish stocks in open temperate regions. World War II created a large marine area within which
commercial fishing was prevented for 6 years. Here we analyse scientific trawl data for three important North Sea gadoids,
collected between 1928 and 1958. Using statistical models to summarise the data, we demonstrate the potential of MPAs for
expediting the recovery of over-exploited fisheries in open temperate regions. Our age-structured data and population models
suggest that wild fish stocks will respond rapidly and positively to reductions in harvesting rates and that the numbers of
older fish in a population will react before, and in much greater proportion, than their younger counterparts in a kind of
Mexican wave. Our analyses demonstrate both the overall increase in survival due to the lack of harvesting in the War and
the form of the age-dependent wave in numbers. We conclude that large closed areas can be very useful in the conservation
of migratory species from temperate areas and that older fish benefit fastest and in greater proportion. Importantly, any
rise in spawning stock biomass may also not immediately result in better recruitment, which can respond more slowly and hence
take longer to contribute to higher future harvestable biomass levels. 相似文献