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251.
Aaron I. Packman Andrea Marion Mattia Zaramella Cheng Chen Jean-François Gaillard Denis T. Keane 《Water, Air, & Soil Pollution: Focus》2006,6(5-6):433-442
Hyporheic exchange is known to provide an important control on nutrient and contaminant fluxes across the stream-subsurface
interface. Similar processes also mediate interfacial transport in other permeable sediments. Recent research has focused
on understanding the mechanics of these exchange processes and improving estimation of exchange rates in natural systems.
While the structure of sediment beds obviously influences pore water flow rates and patterns, little is known about the interplay
of typical sedimentary structures, hyporheic exchange, and other transport processes in fluvial/alluvial sediments. Here we
discuss several processes that contribute to local-scale sediment heterogeneity and present results that illustrate the interaction
of overlying flow conditions, the development of sediment structure, pore water transport, and stream-subsurface exchange.
Layered structures are shown to develop at several scales within sediment beds. Surface sampling is used to analyze the development
of an armor layer in a sand-and-gravel bed, while innovative synchrotron-based X-ray microtomography is used to observe patterns
of grain sorting within sand bedforms. We show that layered bed structures involving coarsening of the bed surface increase
interfacial solute flux but produce an effective anisotropy that favors horizontal pore water transport while limiting vertical
penetration. 相似文献
252.
T. D. Blackall M. R. Theobald C. Milford K. J. Hargreaves E. Nemitz L. J. Wilson J. Bull P. J. Bacon K. C. Hamer S. Wanless M. A. Sutton 《Water, Air, & Soil Pollution: Focus》2004,4(6):279-285
Ammonia emissions from two contrasting seabird colonies in Scotland were measured, based on the determination of atmospheric concentrations downwind of the colonies. Atmospheric concentrations of ammonia (NH3) across the downwind plume were compared with the inverse application of a Gaussian dispersion model (ID) to calculate the modelled NH3 emission that would generate the measured cross-wind-integrated plume concentration. In parallel, a tracer gas (sulphur hexafluoride, SF6) was released from the colonies with air samples taken to allow determination of SF6 concentrations. On the basis of the known emission rate of SF6, the magnitude of ammonia emissions was estimated by the cross-wind-integrated tracer ratio (TR) of NH3/SF6 concentrations. Coupled with data on annual bird attendance, the measurements indicate annual emissions from the Isle of May and the Bass Rock of 18 and 132 tonnes NH3-N year–1, respectively. The measured NH3 emissions were compared with estimates of seabird nitrogen excretion to estimate the proportion of excreted N that is volatilised as NH3 (FNr). The emission estimates of the two methods compared favourably, giving 4 and 6 kg NH3-N h–1 (FNr = 15%) for the Isle of May for the ID and TR methods, respectively, and 21 and 25 kg NH3-N h–1 (FNr = 50%) for the Bass Rock for the ID and TR methods, respectively. The results provide the first measurement-based estimates to allow regional up scaling of ammonia emissions from seabirds. 相似文献
253.
Impact of Land Use on Soluble Organic Nitrogen in Soil 总被引:5,自引:0,他引:5
Victoria B. Willett James J. Green Andrew J. Macdonald John A. Baddeley Georg Cadisch Steven M. J. Francis Keith W. T. Goulding Gary Saunders Elizabeth A. Stockdale Christine A. Watson David L. Jones 《Water, Air, & Soil Pollution: Focus》2004,4(6):53-60
Although it has been hypothesized that soluble organic nitrogen (SON) plays a central role in regulating productivity in some terrestrial ecosystems, the factors controlling the size of the SON pool in soil remain poorly understood. Therefore our principal aim in this work was to assess the impact of seven different land use systems (rough and managed grassland, deciduous and coniferous woodland, heathland, wetland and tilled land) on the size of the SON and inorganic N (NO
3
–
, NH
4
+
) pools in the surface soil layer (0–15 cm). After extraction with deionised water, we found that in most cases the size of the water extractable organic N (WEON) pool was similar in size to the inorganic N pool. In contrast, the KCl extractable organic N (KClEON) pool constituted the dominant form of soluble N in soils under all land uses, perhaps indicating that significant amounts were held on the soil exchange phase. In contrast to inorganic N, which varied significantly with land use, the size of the KClEON and WEON pool was similar for all land uses with the exception of KClEON in tilled land, where significantly lower amounts were observed. We conclude that SON constitutes an important soil N pool in a broad range of land uses, and that its role in microbial N assimilation, plant nutrition and ecosystem responses to atmospheric N deposition warrants further attention.
SAFRD, University of Newcastle, Newcastle-upon-Tyne, NE1 7RU, U.K. 相似文献
254.
Steven N. Chillrud Richard F. Bopp James M. Ross Damon A. Chaky Sidney Hemming Edward L. Shuster H. James Simpson Frank Estabrooks 《Water, Air, & Soil Pollution: Focus》2004,4(2-3):469-482
Radionuclide, radiogenic lead isotope and trace metal analyses on fine-grained sediment cores collected along 160 km of the upper and tidal Hudson River were used to examine temporal trends of contaminant loadings and to develop radiogenic lead isotopes both as a stratigraphic tool and as tracers for resolving decadal particle transport fluxes. Very large inputs of Cd, Sb, Pb, and Cr are evident in the sediment record, potentially from a single manufacturing facility. The total range in radiogenic lead isotope ratios observed in well-dated cores collected about 24 km downstream of the plant is large (e.g., maximum difference in 206Pb/207Pb is 10%), characterized by four major shifts occurring in the 1950s, 1960s, 1970s and 1980s. The upper Hudson signals in Cd and radiogenic lead isotopes were still evident in sediments collected 160 km downstream in the tidal Hudson. The large magnitude and abrupt shifts in radiogenic lead isotope ratios as a function of depth provide sensitive temporal constraints that complement information derived from radionuclide analyses to significantly improve the precision of dating assignments. Application of a simple dilution model to data from paired cores suggests much larger sediment inputs in one section of the river than previously reported, suggesting particle influxes to the Hudson have been underestimated. 相似文献
255.
A solution containing 35SO4 2- and 3H2O was applied to four plots (5 × 5 m) in a boreal coniferous forest in the Laflamme Lake watershed, Québec, under two contrasting conditions: in summer (plots 1 and 2), and on the snowpack before snowmelt (plots 3 and 4). The transit of both these tracers in the soil solution was then followed through a network of soil lysimeters located at different depths. Four months after the summer application, 3H2O had infiltrated the whole soil profile at plot 1, while 35SO4 2- was only observed in the LFH and Bhf horizons. A 35SO4 2- budget calculated from mid-August to November indicated that 89 and 10.6% of the added 35SO4 2- was retained within the LFH and the Bhf layers, respectively. Fifteen months later, the added 35SO4 2- was distributed in the following proportions within the soil horizons: LFH (73.7%), Bhf (11.8%) and Bf (12.8%), for a total retention rate of 98.3%. The superficial penetration of 3H2O at plot 2 was indicative of a major lateral water movement that prevented the calculation of a 35SO4 2- budget. This situation also was observed at plot 4 during snowmelt. At plot 3, 3H2O moved freely through the soil profile and a significant fraction of the added 35SO4 2- reached the B horizons, where it was presumably adsorbed on aluminum (Al) and ferric (Fe) oxides. The 35SO4 2- budget for plot 3 from March to November indicated that 87% of the added 35SO4 2- was retained within the soil profile, with most being retained in the B horizons (LFH = 33.1%, Bhf = 33.1%, Bf = 20.8%). The contrasting retention patterns of 35SO4 2- within the soil profile following the summer addition and snowmelt likely was caused by the contrastingsoil temperatures and soil solution residence times within the differentsoil layers. The persistence of 35SO4 2- in the soil solution of the entire profile long after the initial tracer infiltration, and the relative temporal stability of specific activity of SO4 2-, point to the establishment of an isotopic equilibrium between the added 35SO4 and the active S-containing reservoirs within a given soil horizon. Overall, the results clearly illustrate the very strong potential for 35SO4 2- retention and recycling in forest soils. 相似文献
256.
Miskewitz R. J. Hires R. I. Su T. L. Korfiatis G. P. Sidhoum M. 《Water, Air, & Soil Pollution: Focus》2004,4(4-5):45-54
A 50 ha known contaminated site in Bayonne, New Jersey, U.S.A. is permitted to receive up to 3 × 106 m3 of sediment dredged from navigation channels in the New York/New Jersey Harbor. Much of the sediment is expected to contain low to moderate concentrations of industrial and agricultural chemicals, including Polychlorinated Biphenyls (PCBs). The dredged material brought to the site is stabilized with cement and then placed as a capping and grading layer. The flux of PCBs from drying stabilized dredged material has been estimated from measurements of PCB air concentrations at two heights above the ground along with micrometeorological observations. A statistically significant gradient in PCB concentrations has been consistently measured in the first 3 m above the ground. Observed PCB fluxes were highest over freshly placed stabilized dredged sediment and decreased as it cured. The highest flux observed in this study was 7214 ng/m2/h, but during subsequent sampling intervals at the same site, the flux estimates decreased by an order of magnitude over a 5-day interval. 相似文献
257.
Ali M Alhemood Ashraf M Genaidy Richard Shell Michael Gunn Christin Shoaf 《International journal of occupational safety and ergonomics》2004,10(4):303-318
In this study, a survey instrument was developed to measure safety climate. A review of the scientific literature as well as consultation with an expert panel was used to determine the survey's dimensions. Next, the survey was administered, first as a pilot study (n = 15) and then as a full scale study (n = 229), to employees of the City of Cincinnati Department of Public Works. The psychometric integrity of the survey was assessed according to validity, reliability and utility criteria. Results are presented and discussed. 相似文献
258.
This study addresses the behaviors of project managers under various conditions of cognitive and affective trust, and the implications for obtaining client loyalty. Theoretical foundations were drawn from interpersonal and interorganizational trust literature. A test of the proposed theoretical framework was conducted in a field setting utilizing a matched design of both project managers and their clients. The results show that reliable project performance positively impacted client loyalty intentions and service‐oriented OCBs positively impacted client secondary retention. An interaction showed that in low cognitive trust situations the project manager behavior of reliable project performance facilitated the obtainment of client loyalty intentions. Implications for research and practice are discussed. Copyright © 2004 John Wiley & Sons, Ltd. 相似文献
259.
260.
Forest resources play a key role and provide many basic needs to communities in developing economies. To assess the patterns of vegetation cover change, as a corollary of resource utilization, satellite imagery, ground truth data, and image processing techniques can be useful. This article is concerned with identifying change in major vegetation types in East Timor between 1989 and 1999, using Landsat Thematic Mapper data. The results highlight a significant level of deforestation and decline in foliage cover. All major vegetation cover types declined from 1989 to 1999, and there was a sizeable increase in degraded woodlands. This decline has had considerable impact on the livelihoods of rural and urban communities. Causes for these changes include: economic exploitation of abundant resources; and implications of transmigration policies implemented during Indonesian rule, resulting in increased competition for land and woodland resources. As the new nation of Timor‐Leste establishes itself, it must consider its current stock and distribution of natural capital to ensure that development efforts are geared towards sustainable outcomes. Without the knowledge of historical patterns of resource consumption, development efforts may, unwittingly, lead to continuing decline in forest resources. 相似文献