全文获取类型
收费全文 | 624篇 |
免费 | 8篇 |
国内免费 | 2篇 |
专业分类
安全科学 | 22篇 |
废物处理 | 18篇 |
环保管理 | 85篇 |
综合类 | 92篇 |
基础理论 | 135篇 |
环境理论 | 2篇 |
污染及防治 | 190篇 |
评价与监测 | 39篇 |
社会与环境 | 45篇 |
灾害及防治 | 6篇 |
出版年
2023年 | 2篇 |
2022年 | 8篇 |
2021年 | 13篇 |
2020年 | 4篇 |
2019年 | 8篇 |
2018年 | 21篇 |
2017年 | 17篇 |
2016年 | 18篇 |
2015年 | 27篇 |
2014年 | 28篇 |
2013年 | 47篇 |
2012年 | 26篇 |
2011年 | 36篇 |
2010年 | 43篇 |
2009年 | 38篇 |
2008年 | 30篇 |
2007年 | 36篇 |
2006年 | 31篇 |
2005年 | 20篇 |
2004年 | 28篇 |
2003年 | 21篇 |
2002年 | 26篇 |
2001年 | 10篇 |
2000年 | 16篇 |
1999年 | 16篇 |
1998年 | 6篇 |
1997年 | 7篇 |
1996年 | 4篇 |
1995年 | 7篇 |
1994年 | 9篇 |
1993年 | 3篇 |
1991年 | 2篇 |
1989年 | 2篇 |
1984年 | 2篇 |
1980年 | 3篇 |
1976年 | 1篇 |
1972年 | 1篇 |
1971年 | 1篇 |
1966年 | 1篇 |
1965年 | 1篇 |
1964年 | 1篇 |
1963年 | 1篇 |
1962年 | 1篇 |
1961年 | 1篇 |
1958年 | 1篇 |
1955年 | 1篇 |
1949年 | 1篇 |
1948年 | 1篇 |
1937年 | 1篇 |
1920年 | 1篇 |
排序方式: 共有634条查询结果,搜索用时 141 毫秒
511.
The composition of chlorinated hydrocarbon DNAPLs (dense non-aqueous phase liquids) from field sites can be substantially different than the material originally purchased for use as a solvent. Waste management practices at the U.S. Department of Energy's (DOE) Savannah River Site (SRS) included co-disposal of a wide range of organic and inorganic wastes. In 1991, a clear, orange-colored DNAPL was found in two wells near the SRS M-area settling basin. Waste effluent from the fuel and target fabrication facilities that were discharged to this settling basin included acids, caustics, metals and chlorinated solvents. The characterization of the SRS DNAPL suggests that numerous constituents partitioned into the DNAPL during its use as a solvent, co-disposal and ultimate migration through the subsurface. Trace constituents in the DNAPL include metals, from processing operations or co-disposal practices and subsurface minerals, high molecular weight hydrocarbons and alkyl esters, and acids. This complex mixture results in DNAPL-water interfacial properties that are substantially different than would be expected from a simple mixture of PCE and TCE. Under conditions when there is a high DNAPL to water volume ratio, a semi-rigid film accumulates on water droplets suspended in the DNAPL. It is concluded that the array of precipitated metal species comprising this film contributes to the interfacial tension that is over an order of magnitude lower than expected for a "clean" PCE/TCE mixture. 相似文献
512.
Meinelt T Schreckenbach K Pietrock M Heidrich S Steinberg CE 《Environmental science and pollution research international》2008,15(1):17-22
GOALS, SCOPE AND BACKGROUND: Changing environmental conditions and handling stress are well known to cause chronic or acute stress situations in fish with subsequent infections. These requires a therapy by means of antibiotics and chemicals. In contrast to the huge number of pathogens, only a few substances are permitted for application as therapeutics in German aquaculture. Hence, there emerges an urgent need for highly effective and residueless alternatives. MAIN FEATURES: The prophylactic stimulation and training of the defense system of fish by alternative approaches becomes increasingly necessary. One approach is the application of dissolved humic substances (HS) of natural or artificial origin. For example, there exist several reports on the positive effect of HS to fishes. These effects shall be considered in detail. Furthermore, the impact of HS on the constitution of parasites and pathogens will be displayed. The reports on this issue are diverse, if not inconsistent. We try to shed some light on these discrepancies. The last aspect covered by this review is the outdated paradigm that calcium ions act as antidotes. In the presence of HS, even the opposite effect may occur. APPROACH: To overcome old paradigms on HS and their potential interactions with fish and fish parasites, we reviewed recent international literature, as well as 'grey' literature. We also include results from own former and ongoing studies. RESULTS AND DISCUSSION: HS are able to increase the physiological condition of the individuals and to reduce adverse physiological and histological consequences caused by stress; the mechanism behind remains obscure. HS detoxify heavy metals and organic pollutants. Damages caused by several fish pathogens, such as bacteria and parasites, can be repaired more quickly in the presence of HS. Some parasites--mainly fungi--appear to be directly affected by HS. Comparing the fungicidal effects of HS from various sources, evidence is increasing that the aliphatic moiety may be the effective structures. However, further research is necessary to relate more physiological and anti-pathogenic effects to the chemical characteristics of HS. CONCLUSIONS: HS are not real alternatives to strong traditional therapeutics. However, they show different advantages in repairing secondary, stress induced damages in fish. The ecophysiological relevance of HS in either aquatic systems or aquaculture is getting conspicuously. PERSPECTIVES: The lack of therapeutic and antiparasitic substances in aquaculture requires new strategies and ways of thinking. The search for alternatives to the 'traditional' chemical therapeutics calls for the intensive research. Inevitably, this search will lead to an intensive contemplation on HS as 'health promoting substances' and/or even therapeutics. Basic research is needed to detect the functional groups of the HS responsible for the effects observed. Health promoting effects of first investigations made in vitro to affect pathogens via application of HS and several field studies with HS raises hopes for a broader utilisation of HS to reduce stress consequences in fish and fish pathogens residuelessly. 相似文献
513.
Stefan Banzhaf Marko Filipovic Jeffrey Lewis Charlotte J. Sparrenbom Roland Barthel 《Ambio》2017,46(3):335-346
Perfluoroalkyl and polyfluoroalkyl substances (PFASs) are found in aquatic systems, flora, and fauna worldwide. These potentially harmful compounds are also frequently detected in Sweden and have already resulted in severe problems for public drinking water supply, i.e., some wells had to be closed due to high PFAS concentrations both in raw water and produced drinking water. Knowledge on PFAS occurrence in Sweden is still quite low, although monitoring is currently ongoing. This work describes potential sources for PFASs to enter the drinking water supply in Sweden and compares different occurrences of PFASs in raw and drinking water in the country. Moreover, the monitoring history, the legal situation, and remediation actions taken are presented. Finally, future challenges and the way forward in Sweden are discussed. 相似文献
514.
Samuelsson Göran S Raymond Caroline Agrenius Stefan Schaanning Morten Cornelissen Gerard Gunnarsson Jonas S 《Environmental science and pollution research international》2017,24(16):14218-14233
Environmental Science and Pollution Research - A field experiment with thin-layer capping was conducted in the Grenland fjords, Norway, for remediation in situ of mercury and dioxin-contaminated... 相似文献
515.
The gooseneck barnacle fishery in Asturias (N. Spain) has undergone three important changes: (1) the early implementation of a co-management system based on Territorial User Rights for Fishing, (2) a change in management measures (due to a decrease in landings), and (3) an economic crisis. This has allowed us to analyze the systems’ sustainability in time through examining five critical variables: landings, effort, catch per unit effort (CPUE), mean market prices, and annual revenue. Additionally, we used focus groups and questionnaires to determine the response of the system to these three changes. Co-management has succeeded in maintaining or increasing CPUE throughout all management areas and produced stable mean market prices. This was achieved through flexible management policies and adaptive strategies adopted by the fishers, such as increased selectivity and diversification. The analysis of this fishery provides important lessons regarding the need to understand the evolutionary dynamics of co-management and the importance of embracing adaptive capacity.
Electronic supplementary material
The online version of this article (doi:10.1007/s13280-015-0687-z) contains supplementary material, which is available to authorized users. 相似文献516.
Winfried Schröder Stefan Nickel Simon Schönrock Michaela Meyer Werner Wosniok Harry Harmens Marina V. Frontasyeva Renate Alber Julia Aleksiayenak Lambe Barandovski Alejo Carballeira Helena Danielsson Ludwig de Temmermann Barbara Godzik Zvonka Jeran Gunilla Pihl Karlsson Pranvera Lazo Sebastien Leblond Antti-Jussi Lindroos Siiri Liiv Sigurður H. Magnússon Blanka Mankovska Javier Martínez-Abaigar Juha Piispanen Jarmo Poikolainen Ion V. Popescu Flora Qarri Jesus Miguel Santamaria Mitja Skudnik Zdravko Špirić Trajce Stafilov Eiliv Steinnes Claudia Stihi Lotti Thöni Hilde Thelle Uggerud Harald G. Zechmeister 《Environmental science and pollution research international》2016,23(11):10457-10476
For analysing element input into ecosystems and associated risks due to atmospheric deposition, element concentrations in moss provide complementary and time-integrated data at high spatial resolution every 5 years since 1990. The paper reviews (1) minimum sample sizes needed for reliable, statistical estimation of mean values at four different spatial scales (European and national level as well as landscape-specific level covering Europe and single countries); (2) trends of heavy metal (HM) and nitrogen (N) concentrations in moss in Europe (1990–2010); (3) correlations between concentrations of HM in moss and soil specimens collected across Norway (1990–2010); and (4) canopy drip-induced site-specific variation of N concentration in moss sampled in seven European countries (1990–2013). While the minimum sample sizes on the European and national level were achieved without exception, for some ecological land classes and elements, the coverage with sampling sites should be improved. The decline in emission and subsequent atmospheric deposition of HM across Europe has resulted in decreasing HM concentrations in moss between 1990 and 2010. In contrast, hardly any changes were observed for N in moss between 2005, when N was included into the survey for the first time, and 2010. In Norway, both, the moss and the soil survey data sets, were correlated, indicating a decrease of HM concentrations in moss and soil. At the site level, the average N deposition inside of forests was almost three times higher than the average N deposition outside of forests. 相似文献
517.
Martyn N. Futter Salar Valinia Stefan Löfgren Stephan J. Köhler Jens Fölster 《Ambio》2014,43(1):77-90
Long-term (1987–2012) water quality monitoring in 36 acid-sensitive Swedish lakes shows slow recovery from historic acidification. Overall, strong acid anion concentrations declined, primarily as a result of declines in sulfate. Chloride is now the dominant anion in many acid-sensitive lakes. Base cation concentrations have declined less rapidly than strong acid anion concentrations, leading to an increase in charge balance acid neutralizing capacity. In many lakes, modeled organic acidity is now approximately equal to inorganic acidity. The observed trends in water chemistry suggest lakes may not return to reference conditions. Despite declines in acid deposition, many of these lakes are still acidified. Base cation concentrations continue to decline and alkalinity shows only small increases. A changing climate may further delay recovery by increasing dissolved organic carbon concentrations and sea-salt episodes. More intensive forest harvesting may also hamper recovery by reducing the supply of soil base cations. 相似文献
518.
Bert Allard Mattias Bäckström Stefan Karlsson Anja Grawunder 《Environmental science and pollution research international》2014,21(11):6930-6938
A former open pit where black shale (alum shale) was excavated during 1942–1965 has been water filled since 1966. The water chemistry was dominated by calcium and sulphate and had a pH of 3.2–3.4 until 1997–1998, when pH was gradually increasing. This was due to the intrusion of leachates from alkaline cement waste deposited close to the lake. A stable pH of around 7.5 was obtained after 6–7 years. The chemistry of the pit lake has changed due to the neutralisation. Concentrations of some dissolved metals, notably zinc and nickel, have gone down, as a result of adsorption/co-precipitation on solid phases (most likely iron and aluminium hydroxides), while other metals, notably uranium and molybdenum, are present at elevated levels. Uranium concentration is reaching a minimum of around pH 6.5 and is increasing at higher pH, which may indicate a formation of neutral and anionic uranyl carbonate species at high pH (and total carbonate levels around 1 mM). Weathering of the water-exposed shale is still in progress. 相似文献
519.
Stefan Bouzarovski Sergio Tirado Herrero Saska Petrova Diana Ürge-Vorsatz 《Local Environment》2016,21(9):1151-1170
This paper focuses on the embeddedness of energy poverty – understood as the inability to secure a socially and materially necessitated level of energy services in the home – in the socio-technical legacies inherited from past development trajectories, as well as broader economic and institutional landscapes. Using Hungary as an example, we explore the recent expansion of energy poverty across different demographic and income groups. While much of the mainstream literature focuses on cases where energy poverty affects distinct social groups and issues, our analyses examine the systemic implications of a form of deprivation that involves a much wider range of social and spatial strata. We develop a framework that highlights the different ways in which inadequate access to energy services has resulted in the emergence of new political reconfigurations among a variety of actors, while prompting the articulation of household strategies with far-reaching structural consequences. 相似文献
520.
Dinesh Bhatt Shreedhar Maskey Mukand S. Babel Stefan Uhlenbrook Krishna C. Prasad 《Regional Environmental Change》2014,14(4):1291-1301
Understanding crop responses to climate is essential to cope with anticipated changes in temperature and precipitation. We investigated the climate–crop yield relationship and the impact of historical climate on yields of rice, maize and wheat in the Koshi basin of Nepal. The results show significant impact of growing season temperature and precipitation on crop production in the region. Rice, maize and wheat cultivated at altitudes below 1,100, 1,350 and 1,700 m amsl (above mean sea level), respectively, suffer from stress due to higher temperatures particularly during flowering and yield formation stages. Responses of crop yields to a unitary increment in growing season mean temperature vary from ?6 to 16 %, ?4 to 11 % and ?12 to 3 % for rice, maize and wheat, respectively, depending on the location and elevation in the basin. In most parts of the basin, we observe warming trends in growing season mean temperatures of rice, maize and wheat over the last few decades with clear evidence of negative impacts on yields. However, at some high-elevation areas, positive impacts of warming are also observed on rice and maize yields. If the observed trends in temperature continue in future, the impact is likely to be mostly negative on crop production in the basin. However, crop production may gain from the warming at relatively higher altitudes provided other conditions, e.g., water availability, soil fertility, are favorable. 相似文献